SearcharxivSearch

arXiv subjects

Yongxin Zeng

Publications and source records attributed to Yongxin Zeng.

16 recordsLinked to original sources

Emergent Trion Resonance Driven by Lattice Reconstruction in a Moiré Superlattice

We investigate how many-electron excited states emerge in twisted MoSe2 homobilayers when the lattice reconstructions evolve. Notably, we identify a new trion resonance that arises in the transition regime of lattice reconstruction, where gradual changes in atomic alignment between the layers occur. Magnetic field-dependent measurements, supported by first-principles calculations, indicate that the exciton forms at the K valley while the doped hole resides in the Gamma valley. First-principles calculations further indicate that two nearly degenerate exciton resonances can arise, localized at different sites within the moiré supercell. We propose that the new trion resonance is a "charge-transfer" trion, in which the electron-hole pair is spatially separated from the doped hole. The emergence of these complex excited states stems from the distinct moiré potentials acting on holes and excitons, resulting in their different spatial distribution within the superlattice.

cond-mat.mes-hall

Topological excitonic insulators in electron bilayers modulated by twisted hBN

Equilibrium interlayer exciton condensation is common in bilayer quantum Hall systems and is characterized by spontaneous phase coherence between isolated layers. It has been predicted that similar physics can occur in the absence of a magnetic field in some two-dimensional semiconductor bilayers. In this work we consider the case of two transition metal dichalcogenide (TMD) monolayers separated by a twisted hexagonal boron nitride (hBN) bilayer or multilayer. The hBN layers suppress tunneling between the TMD layers so that phase coherence is spontaneous when it is present. When twisted, the hBN layers also form a ferroelectric moiré pattern that applies opposite triangular-lattice modulation potentials to the two TMD layers. We show via mean-field theory that at total hole filling per moiré unit cell $ν=1$, this geometry can favor a chiral p-wave exciton condensate state in which the quantum anomalous Hall effect coexists with counter-flow superfluidity. We present a mean-field phase diagram for TMD hole bilayers modulated by twisted hBN, discuss the conditions needed for the realization of the p-wave condensate state, and propose experiments that could confirm its presence.

cond-mat.mes-hall

Superfluid stiffness bounds in time-reversal symmetric superconductors

Quantum geometry has been shown to make an important contribution to the superfluid stiffness of superconductors, especially for flat-band systems such as moiré materials. In this work we use mean-field theory to derive an expression for the superfluid stiffness of time-reversal symmetric superconductors at zero temperature by computing the energy of the mean-field ground state as a function of pairing momentum. We show that the quantum geometric contribution to superfluid stiffness is a consequence of broken Galilean invariance in the interaction Hamiltonian, arising from momentum-dependent form factors related to the momentum dependence of Bloch states. The effects of broken Galilean invariance are not fully parametrized by the quantum metric considered in previous work. We obtain general lower and upper bounds that apply to both continuum and lattice models and present numerical calculations of the precise value in several important cases. The superfluid stiffness of superconductivity in a Landau level saturates the lower bound and the superfluid stiffness of the other cases we consider is close to the general lower bound we derive. In multilayer rhombohedral graphene the geometric contribution is shown not to be the dominant contribution to the superfluid stiffness, despite the flat band behavior in the vicinity of the Fermi level. Finally, assuming contact interaction and uniform pairing, we show that the superfluid stiffness is proportional to the ``minimal quantum metric" introduced in previous work. We provide a continuum version of the minimal quantum metric and explain its physical origin.

cond-mat.supr-con

Berry Phase Dynamics of Sliding Electron Crystals

Systems such as Wigner crystals and incommensurate charge density waves that spontaneously break a continuous translation symmetry have unusual transport properties arising from their ability to slide coherently in space. Recent experimental and theoretical studies suggest that spontaneous translation symmetry breaking in some two-dimensional materials with nontrivial quantum geometry (e.g., rhombohedral pentalayer graphene) leads to a topologically nontrivial electron crystal state called the anomalous Hall crystal and characterized by a vanishing linear-response dc longitudinal conductivity and a non-vanishing Hall conductivity. In this work we present a theoretical investigation of the sliding dynamics of this new type of electron crystal, taking into account the system's nontrivial quantum geometry. We find that when accelerated by an external electric field, the crystal acquires a transverse anomalous velocity that stems from not only the Berry curvature of the parent band but also the Galilean non-invariance of the crystal state (i.e., crystal states with different momenta are not related by simple momentum boosts). We further show that acceleration of the crystal modifies its internal current from the static crystal value that is determined by the Chern number of the crystal state. The net Hall conductance including contributions from center-of-mass motion and internal current is in general not quantized. As an experimentally relevant example, we present numerical results in rhombohedral pentalayer graphene and discuss possible experimental implications.

cond-mat.mes-hall

Keldysh field theory of dynamical exciton condensation transitions in nonequilibrium electron-hole bilayers

Recent experiments have realized steady-state electrical injection of interlayer excitons in electron-hole bilayers subject to a large bias voltage. In the ideal case in which interlayer tunneling is negligibly weak, the system is in quasi-equilibrium with a reduced effective band gap. Interlayer tunneling introduces a current and drives the system out of equilibrium. In this work we derive a nonequilibrium field theory description of interlayer excitons in biased electron-hole bilayers. In the large bias limit, we find that p-wave interlayer tunneling reduces the effective band gap and increases the effective temperature for intervalley excitons. We discuss possible experimental implications for InAs/GaSb quantum wells and transition metal dichalcogenide bilayers.

cond-mat.mes-hall

Sublattice structure and topology in spontaneously crystallized electronic states

The prediction and realization of the quantum anomalous Hall effect are often intimately connected to honeycomb lattices in which the sublattice degree of freedom plays a central role in the nontrivial topology. Two-dimensional Wigner crystals, on the other hand, form triangular lattices without sublattice degrees of freedom, resulting in a topologically trivial state. In this Letter, we discuss the possibility of spontaneously formed honeycomb-lattice crystals that exhibit the quantum anomalous Hall effect. Starting from a single-band system with nontrivial quantum geometry, we derive the mean-field energy functional of a class of crystal states and express it as a model of sublattice pseudospins in momentum space. We find that nontrivial quantum geometry leads to extra terms in the pseudospin model that break an effective `time-reversal symmetry' and favor a topologically nontrivial pseudospin texture. When the effects of these extra terms dominate over the ferromagnetic exchange coupling between pseudospins, the anomalous Hall crystal state becomes energetically favorable over the trivial Wigner crystal state.

cond-mat.str-el

Gate-tunable topological phases in superlattice modulated bilayer graphene

Superlattice potential modulation can produce flat minibands in Bernal-stacked bilayer graphene. In this work we study how band topology and interaction-induced symmetry-broken phases in this system are controlled by tuning the displacement field and the shape and strength of the superlattice potential. We use an analytic perturbative analysis to demonstrate that topological flat bands are favored by a honeycomb-lattice-shaped potential, and numerics to show that the robustness of topological bands depends on both the displacement field strength and the periodicity of the superlattice potential. At integer fillings of the topological flat bands, the strength of the displacement field and the superlattice potential tune phase transitions between quantum anomalous Hall insulator, trivial insulator, and metallic states. We present mean-field phase diagrams in a gate voltage parameter space at filling factor $ν=1$, and discuss the prospects of realizing quantum anomalous Hall insulators and fractional Chern insulators when the superlattice potential modulation is produced by dielectric patterning or adjacent moiré materials.

cond-mat.mes-hall

Electrical Control of Two-Dimensional Electron-Hole Fluids in the Quantum Hall Regime

We study the influence of quantizing perpendicular magnetic fields on the ground state of a bilayer with electron and hole fluids separated by an opaque tunnel barrier. In the absence of a field, the ground state at low carrier densities is a condensate of s-wave excitons that has spontaneous interlayer phase coherence. We find that a series of phase transitions emerge at strong perpendicular fields between condensed states and incompressible incoherent states with full electron and hole Landau levels. When the electron and hole densities are unequal, condensation can occur in higher angular momentum electron-hole pair states and, at weak fields, break rotational symmetry. We explain how this physics is expressed in dual-gate phase diagrams, and predict transport and capacitively-probed thermodynamic signatures that distinguish different states.

cond-mat.mes-hall

Weak localization as a probe of intervalley coherence in graphene multilayers

Spontaneous intervalley coherence is suspected in several different graphene multilayer systems, but is difficult to confirm because of a paucity of convenient experimental signatures. Here we suggest that magneto-conductance features associated with quantum corrections to Drude conductivity can serve as a smoking gun for intervalley coherence that does not break time-reversal symmetry. In this class of ordered multilayer quantum transport corrections can produce weak localization or weak antilocalization, depending on whether the valley order belongs to the orthogonal or symplectic symmetry class. Our analysis motivates low-temperature weak-field magnetoresistance measurements in graphene multilayers in which time-reversal invariant intervalley coherent order is conjectured.

cond-mat.mes-hall

Thermodynamic behavior of correlated electron-hole fluids in van der Waals heterostructures

Coupled two-dimensional electron-hole bilayers provide a unique platform to study strongly correlated Bose-Fermi mixtures in condensed matter. Electrons and holes in spatially separated layers can bind to form interlayer excitons, composite Bosons expected to support high-temperature exciton superfluids. The interlayer excitons can also interact strongly with excess charge carriers when electron and hole densities are unequal. Here, we use optical spectroscopy to quantitatively probe the local thermodynamic properties of strongly correlated electron-hole fluids in MoSe2/hBN/WSe2 heterostructures. We observe a discontinuity in the electron and hole chemical potentials at matched electron and hole densities, a definitive signature of an excitonic insulator ground state. The excitonic insulator is stable up to a Mott density of ~$0.8\times {10}^{12} \mathrm{cm}^{-2}$ and has a thermal ionization temperature of ~70 K. The density dependence of the electron, hole, and exciton chemical potentials reveals strong correlation effects across the phase diagram. Compared with a non-interacting uniform charge distribution, the correlation effects lead to significant attractive exciton-exciton and exciton-charge interactions in the electron-hole fluid. Our work highlights the unique quantum behavior that can emerge in strongly correlated electron-hole systems.

cond-mat.str-el

The strong modulation limit of excitons and trions in moiré materials

The optical properties of weakly-doped two-dimensional materials are dominated by strong exciton and trion absorption and luminescence features. In this article we examine the influence of moiré patterns in semiconductor heterobilayers on exciton and trion states in the limit of strong moiré modulation potentials, commenting on similarities and differences compared to the case of excitons and trions in semiconductor quantum dots. We discuss strategies for using optical properties as quantitative probes of moiré materials, and the prospects for exploiting moiré materials to design unique light emitters.

cond-mat.mes-hall

Layer Pseudospin Magnetism in Transition-Metal-Dichalcogenide Double-Moirés

Spontaneous order of layer pseudospins in two-dimensional bilayers is common in quantum Hall systems, where it is responsible for hysteretic responses to gate fields in states with Ising order, and giant drag voltages in states with XY (spontaneous inter-layer phase coherence) order. In this article we predict that layer pseudospin order will also occur in double-moiré strongly correlated two-dimensional electron systems. We comment on similarities and differences in the competition between the two types of order in quantum Hall and double-moiré systems, and relate our findings to previous work on Falicov-Kimball models of electronic ferroelectrics.

cond-mat.str-el

In-plane magnetic field induced density wave states near quantum spin Hall phase transitions

We study the influence of an in-plane magnetic field and Coulomb interactions on the physics of quantum spin Hall insulators, like those in InAs/GaSb and HgTe/CdTe quantum wells. Using a Hartree-Fock mean-field theory approximation, we calculate phase diagrams as functions of the band gap, band hybridization, and magnetic field strength. We show that when the band hybridization is weak, the system is unstable against the formation of density wave states. As the strength of the in-plane magnetic field increases, the density-wave region of the phase diagram expands and distinct density-wave states appear. We discuss possible experimental implications of our results.

cond-mat.mes-hall

Strongly correlated excitonic insulator in atomic double layers

Excitonic insulators (EI) arise from the formation of bound electron-hole pairs (excitons) in semiconductors and provide a solid-state platform for quantum many-boson physics. Strong exciton-exciton repulsion is expected to stabilize condensed superfluid and crystalline phases by suppressing both density and phase fluctuations. Although spectroscopic signatures of EIs have been reported, conclusive evidence for strongly correlated EI states has remained elusive. Here, we demonstrate a strongly correlated spatially indirect two-dimensional (2D) EI ground state formed in transition metal dichalcogenide (TMD) semiconductor double layers. An equilibrium interlayer exciton fluid is formed when the bias voltage applied between the two electrically isolated TMD layers, is tuned to a range that populates bound electron-hole pairs, but not free electrons or holes. Capacitance measurements show that the fluid is exciton-compressible but charge-incompressible - direct thermodynamic evidence of the EI. The fluid is also strongly correlated with a dimensionless exciton coupling constant exceeding 10. We further construct an exciton phase diagram that reveals both the Mott transition and interaction-stabilized quasi-condensation. Our experiment paves the path for realizing the exotic quantum phases of excitons, as well as multi-terminal exciton circuitry for applications.

cond-mat.mtrl-sci

Electrically Controlled Two-Dimensional Electron-Hole Fluids

We study the electronic properties of dual-gated electron-hole bilayers in which the two layers are separated by a perfectly opaque tunnel barrier. Combining an electrostatic and thermodynamic analysis with mean-field theory estimates of interacting system chemical potentials, we explain the dependence of the electron and hole densities on the two gate voltages. Because chemical potential jumps occur for both electrons and holes at neutrality, there is a finite area in gate voltage parameter space over which electron and hole densities are equal. In that regime the electron-hole pair density depends only on the sum of the two gate voltages. We are able to explain a recent experimental study of electrically controlled bilayers by allowing for interlayer tunneling and using a non-equilibrium steady-state transport picture.

cond-mat.mes-hall

The Quantum Anomalous Hall Majorana Platform

We show that quasi-one-dimensional (1D) quantum wires can be written onto the surface of magnetic topological insulator (MTI) thin films by gate arrays. When the MTI is in a quantum anomalous Hall (QAH) state, MTI$/$superconductor quantum wires have especially broad stability regions for both topological and non-topological states, facilitating creation and manipulation of Majorana particles on the MTI surface.

cond-mat.mes-hall