arXiv subjects

Yongyuan Chu

Publications and source records attributed to Yongyuan Chu.

7 recordsLinked to original sources

arXiv2026

High-speed mid-infrared single-photon upconversion spectrometer

Sensitive and fast mid-infrared (MIR) spectroscopy is highly attractive in a variety of applications including astronomical observation, pharmaceutical synthesis, and environmental monitoring. However, the performance of conventional MIR spectrometers has long been hindered by the limited sensitivity of narrow-bandgap detectors and/or the deficient brightness of broadband light sources. Here, we devise and implement an ultra-sensitive and broadband MIR upconversion spectrometer, which integrates a supercontinuum source covering 1.5-4.2 $μ$m based on a silicon nitride nanophotonic waveguide. High-efficiency and low-noise nonlinear frequency upconversion is realized based on coincidence pulsed pumping with spectro-temporal optimization, which enables to leverage silicon detectors for facilitating MIR single-photon spectroscopy at 0.2 photons/nm/pulse. Furthermore, the upconversion-based array spectrometer is manifested with high-speed spectral acquisition rates beyond 200 kHz, which is about ten-fold faster than the state-of-the-art scan rates for FTIR-based spectrometers at a comparable spectral resolution. The achieved features of broadband spectral coverage, single-photon sensitivity, and sub-MHz refreshing rate might open up new possibilities in infrared transient spectral measurements in combustion analysis, high-throughput sorting and reaction tracking, among others.

physics.optics↗

arXiv2026

Single-photon time-stretch infrared spectroscopy

Sensitive mid-infrared (MIR) spectroscopy is highly demanded in various fields ranging from industrial inspection, biomedical diagnosis to astronomical observation. However, the detection sensitivity of conventional MIR spectrometers has been severely limited by excessive noises for existing infrared sensors, which hinders widespread use in photon-scarce scenarios. Here, we devise and implement a broadband MIR single-photon time-stretch spectrometer based on high-fidelity spectral upconversion and time-correlated coincidence counting. Specifically, a nanophotonic supercontinuum illumination covering 2.4-4.2 $μ$m is nonlinearly converted to the near-infrared band, where low-loss single-mode fiber and high-performance silicon detector can be leveraged to facilitate dispersive operation and sensitive detection, respectively. The arrival time for the dispersed upconversion photons is precisely registered with a low-timing-jitter photon counter, which enables us to obtain a high spectral resolution about 0.5 cm$^{-1}$ under a low-light-level illumination down to 0.14 photons/nm/pulse. In comparison to previous MIR upconversion spectrometers, the presented time-stretch architecture favors single-pixel simplicity and high-throughput acquisition for the single-photon spectral measurement. The achieved MIR spectroscopic features of broadband spectral coverage, sub-wavenumber resolution, single-photon sensitivity, and room-temperature operation would stimulate immediate applications in material and life sciences.

physics.optics↗

arXiv2026

Mid-Infrared Single-Photon Compressive Spectroscopy

Sensitive mid-infrared (MIR) spectroscopy plays an indispensable role in various photon-starved conditions. However, the detection sensitivity of conventional MIR spectrometers is severely limited by excessive noises of the involved infrared sensors, especially for multi-pixel arrays in parallel spectral acquisition. Here, we devise and implement an ultra-sensitive MIR single-pixel spectrometer, which relies on high-fidelity spectral upconversion and wavelength-encoding compressive measurement. Specifically, a MIR nanophotonic supercontinuum from 3.1 to 3.9 $μ$m is nonlinearly converted to the near-infrared band via synchronous chirped-pulse pumping, which facilitates both the precise spectral mapping and sensitive upconversion detection. The upconverted signal is then spatially dispersed onto a programmable digital micromirror device, before being registered by a single-element silicon detector. Consequently, the spectral information can be deciphered from the correlation between encoded patterns and recorded measurements, which results in a spectral resolution of 0.5 cm$^{-1}$ under an illumination flux down to 0.01 photons/nm/pulse. Moreover, we demonstrate faithful reconstructions at sub-Nyquist sampling rates by using the compressive sensing algorithm, which leads to a 95\% reduction in data acquisition time. The presented single-pixel computational spectrometer features wavelength multiplexing, high throughput, and efficient sampling, which thus paves a new way for sensitive and fast spectroscopic analysis at the single-photon level.

physics.optics↗

arXiv2026

1-GHz VIS-to-MIR frequency combs enabled by CMOS-compatible nanophotonic waveguides

A fully stabilized frequency comb is essential for precision metrology and coherent optical synthesis. However, fully-stabilized frequency combs generally require separate stages for supercontinuum generation (SCG) and self-referencing, largely limiting their compactness. Here, enabled by the low-threshold multi-octave supercontinuum generation and concurrent third-harmonic generation in low-loss silicon nitride waveguides, we present a novel approach to a self-referenced frequency comb source at 1 GHz repetition rate spanning from the full visible (VIS) to the mid-infrared (MIR). Our coherent comb is seeded by an all-polarization-maintaining ultrafast fiber laser at 1556 nm, with a pulse duration of 73 fs at 1 GHz repetition rate. With an injected energy of merely 110 pJ, the pulses propagate through dispersion-engineered Si3N4 waveguides, generating supercontinuum spanning over three octaves from 350-3280 nm i.e. 0.76 PHz of coherent bandwidth. Moreover, the on-chip third harmonic generation provides a carrier envelope offset beat note via f-3f with a signal-to-noise ratio of 43 dB. Fueled by the evolving photonic integration providing possibilities of on-chip filtering and photo-detectors, this approach for single-chip self-referencing of high-repetition-rate frequency combs paves the way for ultrabroadband comb sources with unprecedented compactness and field-readiness.

physics.optics↗

arXiv2025

Laser transfer and retrieval via nanophotonic supercontinuum process

The nature of optical metrology is to perform efficient transfer and precise retrieval for lasers and optical signals, which is beneficial for a variety of applications ranging from optical clocking, spectroscopy, to telecommunications and quantum optics. While efforts have been made to promote the detection accuracy of optical frequencies, retrieval on optical waveforms remains on the autocorrelation scheme with limited performances. Here, we demonstrate a novel scheme for optical metrology, particularly on direct retrieval of optical waveform in terms of the field amplitude profile. The scheme is based on massive four-wave-mixings underlying a nanophotonic supercontinuum process, which enables arbitrary transfer of an additive laser to modulational sidebands of the broadened continuum. Detection of the transferred signals is then flexible to be within the whole span of the supercontinuum from visible to the mid-infrared range. We demonstrate such a transfer scheme for both CW lasers and pulsed lasers. For the latter, the temporal amplitude profile of the optical wave can be retrieved, which reveals high-order dynamics of solitary pulses including the self-steepening, self-compression, and the soliton splitting, and shows a remarkable square-fold increase of signal-to-noise ratio in the power spectrum. Our results may contribute to advance optical metrology particularly towards chip scale optical waveform detection, and more fundamentally, they reveal insights of massive ultrafast nonlinear interactions underlying the soliton-based supercontinuum process.

physics.optics↗

arXiv2025

2.7-octave supercontinuum generation spanning from ultraviolet to near-infrared in thin-film lithium niobate waveguides

Supercontinuum generation (SCG) with spectral coverage across the full visible and ultraviolet (UV) ranges is crucial for optical clocks, quantum computing and sensing. However, achieving such SCG in nanophotonic platforms is challenging due to the difficulties in spectrum broadening. Here, Such ultrabroad-bandwidth SCG was demonstrated in thin-film lithium niobate (TFLN) nanophotonic waveguides by dispersion management, without periodic poling for spectral broadening. Anomalous-dispersion waveguides were designed in the telecom band, simultaneously enabling dispersive wave emergence, modal-matched second harmonic generation, and third harmonic generation for spectrum broadening. Moreover, MgO was intentionally doped to mitigate the photorefractive effect of lithium niobate, which frequently results in un-sustained spectrum broadening and in turn limits the accessible SCG coverage. By leveraging photolithography assisted chemo-mechanical etching, low-loss MgO doped TFLN nanophotonic waveguides were fabricated. As a result, thanks to the utilization of the strong second-order and third-order nonlinear processes, gap-free 2.7-octave SCG spanning from 330 nm to 2250 nm was observed by pumping the waveguide with a 1550-nm femtosecond pulsed laser with 0.687 nJ, agreeing well with numerical simulation. This spectral coverage represents the state of the art in TFLN platforms without fine microdomains, and even close to the record in sophisticated chirped periodically poled TFLN waveguides.

physics.optics↗

arXiv2022

Optical microcombs in whispering gallery mode crystalline resonators with dispersive intermode interactions

Soliton microcombs have shown great potential in a variety of applications ranging from chip scale frequency metrology to optical communications and photonic data center, in which light coupling among cavity transverse modes, termed as intermode interactions, are long-existing and usually give rise to localized impacts on the soliton state. Of particular interest are whispering gallery mode based crystalline resonators, which with dense mode families, potentially feature interactions of all kind. While effects of narrow-band interactions such as spectral power spikes have been well recognized in crystalline resonators, that of broadband interactions remains unexplored. Here, we demonstrate microcombs with broadband and dispersive intermode interactions, in home-developed magnesium fluoride microresonators with an intrinsic $\mathbf{Q}$-factor approaching 10 billion.In addition to conventional soliton comb generation in the single mode pumping scheme, comb states with broadband spectral tailoring effect have been observed, via an intermode pumping scheme.Remarkably, footprints of both constructive and destructive interference on the comb spectrum have been observed, which as confirmed by simulations, are connected to the dispersive effects of the coupled mode family.Our results not only contribute to the understanding of dissipative soliton dynamics in multi-mode or coupled resonator systems, but also extend the access to stable soliton combs in crystalline microresonators where mode control and dispersion engineering are usually challenging.

physics.optics↗