arXiv subjects

Yoshiyuki Fukumoto

Publications and source records attributed to Yoshiyuki Fukumoto.

At least 19 recordsLinked to original sources

arXiv2024

Six magnetization plateau phases in a spin-1/2 distorted kagome antiferromagnet: application to $\rm{Y}_3\rm{Cu}_9(\rm{OH})_{19}\rm{Cl}_8$

A recently discovered kagome antiferromagnet $\rm{Y}_3\rm{Cu}_9(\rm{OH})_{19}\rm{Cl}_8$ has attracted significant interest due to its unique kagome lattice structure and magnetic properties. The kagome lattice has three types of exchange interactions: one hexagonal coupling and two different triangular couplings. Previous studies have shown that its ground state is significantly different from that predicted for the undistorted kagome lattice, forming a coplanar spin state with a commensurate magnetic wave vector ${\mathbf Q}=(1/3,1/3)$. Two separate studies have proposed distinct sets of exchange interaction parameters for this compound. In this study, we investigate the ground state of the spin-1/2 Heisenberg kagome model with three types of nearest-neighbor exchange interactions under a magnetic field by exact diagonalization using the Lanczos method. We reveal that clear magnetization plateaus at $M/M_{\rm sat}$=1/3, 5/9, and 7/9 are present under both parameter sets, which are identified as magnon crystal states based on their spin structures. Our findings suggest that these plateaus could potentially be experimentally confirmed with magnetization measurements on $\rm{Y}_3\rm{Cu}_9(\rm{OH})_{19}\rm{Cl}_8$ under a magnetic field of approximately 300 T, achievable with state-of-the-art magnetic field generators. In order to get a deeper understanding of magnetism of $\rm{Y}_3\rm{Cu}_9(\rm{OH})_{19}\rm{Cl}_8$, we perform additional calculations by varying these interactions. Consequently, we discover additional plateau phases at $M/M_{\rm sat}$=1/3, 5/9, and 7/9, each distinctly different from the magnon crystal states.

cond-mat.str-el↗

arXiv2023

A Series Expansion Study for Large Negative Quantum Renormalization of Magnon Spectra in the $S=1/2$ Kagome-Lattice Heisenberg Antiferromagnet Cs$_{2}$Cu$_{3}$SnF$_{12}$

The series expansion method is used to study magnon spectra of the kagome system with nearest-neighbor exchange interaction $J$ and out-of-plane Dzyaloshinskii-Moriya (DM) interaction $D^{\parallel}$, which is a minimal model for Cs$_{2}$Cu$_{3}$SnF$_{12}$. Compared to the magnon spectra by the linear spin wave (LSW) theory, we find that dispersions at high energy part suffer downward deformation, which is similar to the triangle lattice case, in addition to the reduction of the energy scale of about 40\% as pointed out in a neutron-scattering study by Ono {\it et al.} Using a reliable estimation $J=20.7$ meV in a previous study on the magnetic susceptibility of Cs$_{2}$Cu$_{3}$SnF$_{12}$, we use $D^{\parallel}$ as the fitting parameter to reproduce the experimental magnon spectra and obtain $D^{\parallel}=0.12J$. We also report that a roton-like minimum occurs at the M point and a maximum at points somewhat away from the $Γ$ point. Compression of the LSW magnon band is commonly seen in the kagome and triangular-lattice systems, which may be viewed as being pushed from above by the spinon continuum.

cond-mat.str-el↗

arXiv2022

Effects of bond-randomness and Dzyaloshinskii-Moriya interactions on the specific heat at low temperatures of a spherical kagomé cluster in {W$_{72}$V$_{30}$}

For the spin-1/2 spherical kagomé cluster, as well as for the 2D kagomé lattice, many low-energy singlet excitations have been expected to exist in the energy region below the spin gap, which has been actually confirmed by Kihara $et \ al.$ in their specific heat measurements up to 10K in {W$_{72}$V$_{30}$}, for which the exchange interaction was estimated as $J=115$K. However, the experimental result of the specific heat can not be reproduced by the theoretical result in the Heisenberg model. Although the theoretical result has a peak around 2 K, the experimental one does not. To elucidate this difference, we incorporate Dzyaloshinskii-Moriya (DM) interactions and bond-randomness into the model Hamiltonian for {W$_{72}$V$_{30}$} and calculate density of states, entropy, and specific heat at low temperatures by using the Lanczos method. We find that DM interactions do not significantly affect the energy distribution of about ten singlet states above the ground state, which are involved in the peak structure of the specific heat around 2K, while even 10% bond-randomness disperses this distribution to collapse the 2K peak. Kihara $et \ al.$ also reported experimental specific heats under magnetic fields up to 15T $(=0.17J)$, and found that the specific heats show almost no magnetic-field dependence, which strongly suggests that the bond randomness is much stronger than the magnetic fields. For example, our calculated specific heats with 50% randomness reproduce the experimental ones up to about 5K.

cond-mat.str-el↗

arXiv2022

Structures of magnetic excitations in the spin-1/2 kagome-lattice antiferromagnets Cs$_2$Cu$_3$SnF$_{12}$ and Rb$_2$Cu$_3$SnF$_{12}$

We show the structures of magnetic excitations in spin-1/2 kagome-lattice antiferromagnets Cs$_2$Cu$_3$SnF$_{12}$ and Rb$_2$Cu$_3$SnF$_{12}$ investigated by inelastic neutron scattering in wide energy and momentum ranges. For Cs$_2$Cu$_3$SnF$_{12}$, four single-magnon excitation modes were observed. Low-energy three modes are assigned to be transverse modes and the high-energy fourth mode is suggested to be an amplitude mode. It was found that the broad excitation continuum without a marked structure spreads in a wide energy range from $0.15J$ to approximately $2.5J$ in contrast to the clearly structured excitation continuum observed in the spin-1/2 triangular-lattice Heisenberg antiferromagnet. These findings strongly suggest spinon excitations as elementary excitations in Cs$_2$Cu$_3$SnF$_{12}$. In Rb$_2$Cu$_3$SnF$_{12}$, singlet-triplet excitations from the pinwheel VBS state and their ghost modes caused by the enlargement of the chemical unit cell were clearly confirmed. It was found that the excitation continuum is structured in the low-energy region approximately below $J_{\mathrm{avg}}$ and the almost structureless high-energy excitation continuum extends to approximately $2.6J_{\mathrm{avg}}$. The characteristics of the high-energy excitation continuum are common to both Cs$_2$Cu$_3$SnF$_{12}$ and Rb$_2$Cu$_3$SnF$_{12}$, irrespective of their ground states. The experimental results strongly suggest that the spin liquid component remains in the ground state as quantum fluctuations in Cs$_2$Cu$_3$SnF$_{12}$ and Rb$_2$Cu$_3$SnF$_{12}$.

cond-mat.str-el↗

arXiv2020

Quantum dimer model containing Rokhsar-Kivelson point expressed by spin-1/2 Heisenberg antiferromagnets

We obtain a quantum dimer model (QDM) containing a Rokhsar-Kivelson (RK) point expressed by spin-1/2 Heisenberg antiferromagnets on a diamond-like decorated square lattice. This lattice has macroscopically degenerated nonmagnetic ground states, which are equivalent to the Hilbert space of a square-lattice QDM. Then, a square-lattice QDM containing the RK point as a second-order effective Hamiltonian is obtained by introducing further neighbor couplings as perturbation. Our model can provide a new method for the experimental realization of a resonating valence bond state in the QDM.

cond-mat.stat-mech↗

arXiv2019

$d_{x^2-y^2}$-wave density wave and $d_{x^2-y^2}$-wave superconducting gap on the extended Hubbard model on a square lattice

The extended Hubbard model with a nearest-neighbor Coulomb repulsion on the square lattice is studied to obtain insight into the phase diagram of cuprate high $T_c$ superconductors (HTS). To pursue the hidden-order scenario proposed in [S. Chakravarty et al., Phys. Rev. B 63, 094503 (2001)], we derive an effective Hamiltonian by using the canonical transformation and develop a mean-field theory. The calculated phase diagrams are qualitatively consistent with the experimental phase diagrams of HTS, and we thus conclude that the pseudogap can be interpreted as the order parameter of the $d_{x^2-y^2}$-wave density wave (DDW) state, and the $d_{x^2-y^2}$-wave superconducting (DSC) rises based on the DDW order. Furthermore, the analytical representation of the density of states is obtained and, near the optimal doping of the DSC, the van Hove singular point of the density of states is located at the Fermi level.

cond-mat.supr-con↗

arXiv2018

Typical Purification Reproducing the Time Evolution of an Open Quantum System

It is known that an arbitrary quantum state can always be expressed in a pure state by preparing an appropriate ancilla system, which is called purification. The purification can always be performed when considering only a quantity not dependent on the quantum state of the ancilla system. Otherwise, the possibility of purification cannot be elucidated. In this study, we focus on the cases where a quantum system S and the ancilla system interact with each other, and investigate whether purification, which correctly reproduces the time evolution of the system S, is possible. Accordingly, when the ancilla system is a macrosystem, it can be shown that this purification is possible for a specific initial state.

cond-mat.stat-mech↗

arXiv2018

Novel constructive method for the quantum dimer model in spin-1/2 Heisenberg antiferromagnets with frustration on a diamond-like-decorated square lattice

We study spin-1/2 Heisenberg antiferromagnets on a diamond-like-decorated square lattice. The diamond-like-decorated square lattice is a lattice in which the bonds in a square lattice are replaced with diamond units. The diamond unit has two types of antiferromagnetic exchange interactions, and the ratio $λ$ of the diagonal bond strength to that of the other four edges controls the frustration strength. For $0.974<λ<2$, the present system has a nontrivial macroscopic degeneracy, which is called the macroscopically degenerated tetramer-dimer (MDTD) states. The MDTD states are identical to the Hilbert space of the Rokhsar-Kivelson (RK) quantum dimer model (QDM). By introducing further neighbor couplings in the MDTD states, we calculate the second-order effective Hamiltonian, which is exactly the same as the square-lattice QDM with a finite hopping amplitude $t$ and dimer-dimer interaction $v$. Furthermore, we calculate $v/|t|$ as a function of the ratio $λ$ in the Heisenberg model and examine which phases of the square-lattice QDM appear in our obtained states. Our obtained QDM has a region where $λ$ exhibits a finite hopping amplitude ($|t|>0$) and repulsive interaction between dimers ($v>0$). This suggests the possibility of realizing the resonating valence bond (RVB) state because the RVB state is obtained at $v=|t|$, which is known as the RK point.

cond-mat.stat-mech↗

arXiv2018

Impact of Dzyaloshinsky-Moriya Interactions and Tilts of the g Tensors on the Magnetization Process of a Spherical Kagome Cluster in {W72V30}

In order to clarify why the experimental magnetization curve of the spherical kagome cluster in {W72V30} at 0.5 K shows no sign of staircase behavior up to 50 T, we study the effects of Dzyaloshinsky-Moriya (DM) interactions and tilts of the g tensors, both of which lead to the breaking of the total-S z conservation, by using the exact diagonalization method. It is found that the D vector component parallel to the radiation direction of the polyhedron cancels out the staircase in a low magnetic field region efficiently. The tilts of the g tensors are inherent to systems defined on the poly- hedrons and lead to induced magnetic fields varying site by site. This induced magnetic field affects the magnetization only at high magnetic fields. We also discuss two existing experimental results on the basis of our calculated results.

cond-mat.str-el↗

arXiv2017

Emergence of a Dimer-Dimer Interaction in the Low-Energy Effective Quantum-Dimer Model of a Diamond-Like-Decorated Square-Lattice Heisenberg Antiferromagnets with Further Neighbor Couplings

We study spin-1/2 Heisenberg antiferromagnets on a diamond-like-decorated square lattice perturbed by two kinds of further neighbor couplings. In our previous study [J. Phys. Soc. Jpn. 85, 094002 (2016)], the second-order effective Hamiltonian for the Heisenberg model perturbed by a further neighbor coupling was found to be a square-lattice quantum-dimer model with a finite hopping amplitude, t>0, and no dimer-dimer interaction, v=0. In this study, we introduce another kind of further neighbor coupling and show that it leads to an attractive interaction between dimers, which suggests the stabilization of the columnar phase of the square-lattice quantum-dimer model. The calculated v/t is presented as a function of the ratio of the two exchange parameters in the Heisenberg model.

cond-mat.stat-mech↗

arXiv2017

Notes on Ground-State Properties of Mixed Spin-1 and Spin-1=2 Lieb-Lattice Heisenberg Antiferromagnets

Quantum Monte Carlo (QMC) simulations are performed to study ground-state properties of a mixed spin-1 and spin-1/2 Lieb-lattice Heisenberg antiferromagnet, in order to get further insight beyond the modified spin-wave (MSW) study reported in [J. Phys. Soc. Jpn. 86, 014002 (2017)]. It is confirmed that the MSW results are in good agreement with the QMC results. In particular, the scaling relation found in the MSW study, which argues that sublattice spin reductions are inversely proportional to the sublattice sizes, is observed in our QMC simulation. We present a rigorous proof for spontaneous sublattice magnetizations induced by an infinitesimal uniform magnetic field. The calculation process in the MSW theory is reexamined to clarify the mathematical structure behind the scaling relation for sublattice long-range orders.

cond-mat.stat-mech↗

arXiv2016

Exact Solutions on the Ground States of Ising Models in Magnetic Fields with Frustration on a Diamond Hierarchical Lattice

Magnetization processes of Ising models with frustration on diamond hierarchical lattices, which contain vertices with high coordination numbers, are exactly obtained at zero temperature. In antiferromagnetic systems, the magnetization cannot saturate under finite magnetic fields owing to the competition between the antiferromagnetic and Zeeman interactions and the intrinsic long-range nature of hierarchical lattices. For the zero-field classical spin-liquid phase found in [Kobayashi et al., J. Phys. Soc. Jpn. 78, 074004 (2009)], an infinitely small applied magnetic field can induce an infinitely small magnetization, despite Ising models that have discrete energy levels. By examining the structure of the partition function, we obtain the ground state spin-configurations and clarify the mechanism of the "gapless like behavior".

cond-mat.stat-mech↗

arXiv2016

Infinitely Multiple Steps in Magnetization of Ferro- and Antiferromagnetic Ising Models with Frustration on a Diamond Hierarchical Lattice

Magnetizations of ferro- and antiferromagnetic Ising models with frustration on diamond hierarchical lattices are exactly obtained at zero temperature. For the zero-field classical spin-liquid phase found in [Kobayashi {\it et al}, J. Phys. Soc. Jpn. 78, 074004 (2009) ], for which frustrating interactions play an important role, an infinitely small applied magnetic field can induce an infinitely small magnetization, despite classical Ising models that have discrete energy levels. In antiferromagnetic systems, the magnetization cannot saturate under finite magnetic fields owing to the competition between the unfrustrating antiferromagnetic interaction and the Zeeman interaction and an intrinsic long-range nature of hierarchical lattices.

cond-mat.stat-mech↗

arXiv2016

Ground States of Spin-1/2 Heisenberg Antiferromagnets with Frustration on a Diamond-Like Decorated Square Lattice

We study the ground-state phase diagram of a Heisenberg model with spin $S=\frac{1}{2}$ on a diamond-like decorated square lattice. A diamond unit has two types of antiferromagnetic exchange interactions, and the ratio $λ$ between the length of the diagonal bond and that of the other four edges determines the strength of frustration. It has been pointed out [J. Phys. Soc. Jpn {\bf85}, 033705 (2016)] that the so-called tetramer-dimer states, which are expected to be stabilized in an intermediate region of $λ_{\rm c}<λ<2$, are identical to the square-lattice dimer covering states, which ignited renewed interest in high-dimensional diamond-like decorated lattices. In order to determine the phase boundary $λ_{\rm c}$, we employ the modified spin wave method to estimate the energy of the ferrimagnetic state and obtain $λ_{\rm c}=0.974$. Our obtained magnetizations for spin-$\frac{1}{2}$ sites and for spin-1 sites are $m=0.398$ and $\tilde{m}=0.949$, and spin reductions are 20 \% and 5\%, respectively. This indicates that spin fluctuation is much smaller than that of the $S=\frac{1}{2}$ square-lattice antiferromagnet: thus, we can consider that our obtained ground-state energy is highly accurate. Further, our numerical diagonalization study suggests that other cluster states do not appear in the ground-state phase diagram.

cond-mat.stat-mech↗

arXiv2016

Exact Realization of a Quantum-Dimer Model in Heisenberg Antiferromagnets on a Diamond-Like Decorated Lattice

We study Heisenberg antiferromagnets on a diamond-like decorated square lattice perturbed by further neighbor couplings. The second-order effective Hamiltonian is calculated and the resultant Hamiltonian is found to be a square-lattice quantum-dimer model with a finite hopping amplitude and no repulsion, which suggests the stabilization of the plaquette phase. Our recipe for constructing quantum-dimer models can be adopted for other lattices and provides a route for the experimental realization of quantum-dimer models.

cond-mat.stat-mech↗

arXiv2007

Superconductivity in the Three-Fold Charge-Ordered Metal of the Triangular-Lattice Extended Hubbard Model

The quarter-filling extended Hubbard model on the triangular lattice is studied to explore pairing instability in the three-fold charge-ordered (CO) metal. We derive a second-order strong-coupling effective Hamiltonian of doped carriers into the three-fold CO insulator at electron density of $n=2/3$, and then study the $f$- and $d_{xy}$-wave superconductivities down to $n=1/2$ by using the BCS mean-field approximation. It is found that the triplet $f$-wave pairing is more stable than the $d_{xy}$-wave one. We also point out that this coexisting state of the charge ordering and superconductivity is possible to have critical temperature $T_c \sim 0.01 t$.

cond-mat.supr-con↗

arXiv2007

An exact calculation of the transverse susceptibility for an antiferromagnetic Ising $Δ$ chain

We study the transverse susceptibility of the fully frustrated antiferromagnetic Ising $Δ$-chain, extending Minami's transfer-matrix method for the transverse susceptibility of general-type Ising linear-chains [JPSJ 67,1998,2255]. For transverse fields $Γ_1$ on tip spin sites and $Γ_2$ on bottom spin sites, we calculate zero-field transverse-susceptibilities $χ_{tip}^x=\lim_{Γ_1,Γ_2 -> 0}M_{tip}^x/Γ_1$ and $χ_{bottom}^x=\lim_{Γ_1,Γ_2 -> 0}M^x_{bottom}/Γ_2$, where $M_{tip (bottom)}^x$ denotes the magnetization for tip (bottom) spin sites. Both the transverse susceptibilities follow Curie's law at low temperatures. We also calculate $χ_{bottom}^x(Γ_1>0)$, transverse susceptibility of the bottom spin chain under finite tip-spin transverse-fields, to understand the Curie type behavior in the zero-field susceptibility. Using the second-order perturbation theory, we discuss the $Γ_1$ dependence of $χ_{bottom}^x(Γ_1)$ at zero temperature.

cond-mat.stat-mech↗

arXiv2007

Thermodynamic Properties of the Heisenberg Antiferromagnet on a Railroad-Trestle Lattice with Asymmetric Leg Interactions

Using an approximation method for eigenvalue distribution functions, we study the temperature dependence of specific heat of the antiferromagnetic Heisenberg model on the asymmetric railroad-trestle lattice. This model contains both the sawtooth-lattice and Majumdar-Ghosh models as special cases. Making extrapolations to the thermodynamic limit using finite size data up to 28 spins, it is found that specific heat of the Majumdar-Ghosh model has a two-peak structure in its temperature dependence and those of systems near the sawtooth-lattice point have a three-peak structure.

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