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Youngdo Kim

Publications and source records attributed to Youngdo Kim.

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Superconductivity in Isolated Single Copper Oxygen Plane

One of the central questions in cuprate superconductivity is if superconductivity can exist in an isolated single CuO$_2$ plane without any interlayer coupling. There have been numerous experimental efforts to answer this question, but it still has not been clearly resolved. Here we present a heterostructure system with an isolated half-unit-cell La$_{2-x}$Sr$_x$CuO$_4$ which has a single CuO$_2$ plane. Using in-situ angle-resolved photoemission spectroscopy, we measured the electronic and gap structures of a single CuO$_2$ plane. We observed a \textit{d}-wave-like gap which closes somewhat above the bulk T$_c$. Moreover, almost identical gap properties are seen for both single CuO$_2$ plane and bulk. These observations lead us to the conclusion that the d-wave superconductivity of cuprates also exists in a single CuO$_2$ plane. Our results demonstrate that cuprate superconductivity is essentially a two-dimensional phenomenon and provide a platform to study cuprate superconductivity in a purely two-dimensional system.

cond-mat.supr-con

Single-shot reconstruction of three-dimensional morphology of biological cells in digital holographic microscopy using a physics-driven neural network

Recent advances in deep learning-based image reconstruction techniques have led to significant progress in phase retrieval using digital in-line holographic microscopy (DIHM). However, existing deep learning-based phase retrieval methods have technical limitations in generalization performance and three-dimensional (3D) morphology reconstruction from a single-shot hologram of biological cells. In this study, we propose a novel deep learning model, named MorpHoloNet, for single-shot reconstruction of 3D morphology by integrating physics-driven and coordinate-based neural networks. By simulating the optical diffraction of coherent light through a 3D phase shift distribution, the proposed MorpHoloNet is optimized by minimizing the loss between the simulated and input holograms on the sensor plane. Compared to existing DIHM methods that face challenges with twin image and phase retrieval problems, MorpHoloNet enables direct reconstruction of 3D complex light field and 3D morphology of a test sample from its single-shot hologram without requiring multiple phase-shifted holograms or angle scanning. The performance of the proposed MorpHoloNet is validated by reconstructing 3D morphologies and refractive index distributions from synthetic holograms of ellipsoids and experimental holograms of biological cells. The proposed deep learning model is utilized to reconstruct spatiotemporal variations in 3D translational and rotational behaviors and morphological deformations of biological cells from consecutive single-shot holograms captured using DIHM. MorpHoloNet would pave the way for advancing label-free, real-time 3D imaging and dynamic analysis of biological cells under various cellular microenvironments in biomedical and engineering fields.

cs.CV

Tuning orbital-selective phase transitions in a two-dimensional Hund's correlated system

Hund's rule coupling ($\textit{J}$) has attracted much attention recently for its role in the description of the novel quantum phases of multi orbital materials. Depending on the orbital occupancy, $\textit{J}$ can lead to various intriguing phases. However, experimental confirmation of the orbital occupancy dependency has been difficult as controlling the orbital degrees of freedom normally accompanies chemical inhomogeneities. Here, we demonstrate a method to investigate the role of orbital occupancy in $\textit{J}$ related phenomena without inducing inhomogeneities. By growing SrRuO$_3$ monolayers on various substrates with symmetry-preserving interlayers, we gradually tune the crystal field splitting and thus the orbital degeneracy of the Ru $\textit{t$_2$$_g$}$ orbitals. It effectively varies the orbital occupancies of two-dimensional (2D) ruthenates. Via in-situ angle-resolved photoemission spectroscopy, we observe a progressive metal-insulator transition (MIT). It is found that the MIT occurs with orbital differentiation: concurrent opening of a band insulating gap in the $\textit{d$_x$$_y$}$ band and a Mott gap in the $\textit{d$_x$$_z$$_/$$_y$$_z$}$ bands. Our study provides an effective experimental method for investigation of orbital-selective phenomena in multi-orbital materials.

cond-mat.str-el

Heteroepitaxial control of Fermi liquid, Hund metal, and Mott insulator phases in the single-atomic-layer limit

Interfaces between dissimilar correlated oxides can offer devices with versatile functionalities. In that respect, manipulating and measuring novel physical properties of oxide heterointerfaces are highly desired. Yet, despite extensive studies, obtaining direct information on their momentum-resolved electronic structure remains a great challenge. This is because most correlated interfacial phenomena appear within a few atomic layers from the interface, thus limiting the application of available experimental probes. Here, we utilize atomic-scale epitaxy and photoemission spectroscopy to demonstrate the interface control of correlated electronic phases in atomic-scale ruthenate--titanate heterostructures. While bulk SrRuO$_3$ is a ferromagnetic metal, the heterointerfaces exclusively realize three distinct correlated phases in the single-atomic-layer limit. Our theory reveals that atomic-scale structural proximity effects lead to the emergence of Fermi liquid, Hund metal, and Mott insulator phases in the quantum-confined SrRuO$_3$. These results highlight the extensive interfacial tunability of electronic phases, hitherto hidden in the atomically thin correlated heterostructure.

cond-mat.str-el

Observation of spin-dependent dual ferromagnetism in perovskite ruthenates

We performed in-situ angle-resolved photoemission spectroscopy (ARPES) and spin-resolved ARPES (SARPES) experiments to investigate the relationship between electronic band structures and ferromagnetism in SrRuO$_3$ (SRO) thin films. Our high-quality ARPES and SARPES results show clear spin-lifted band structures. The spin polarization is strongly dependent on momentum around the Fermi level, whereas it becomes less dependent at high-binding energies. This experimental observation matches our dynamical mean-field theory (DMFT) results very well. As temperature increases from low to the Curie temperature, spin-splitting gap decreases and band dispersions become incoherent. Based on the ARPES study and theoretical calculation results, we found that SRO possesses spin-dependent electron correlations in which majority and minority spins are localized and itinerant, respectively. Our finding explains how ferromagnetism and electronic structure are connected, which has been under debate for decades in SRO.

cond-mat.str-el

Observation of metallic electronic structure in a single-atomic-layer oxide

Correlated electrons in transition metal oxides (TMOs) exhibit a variety of emergent phases. When TMOs are confined to a single-atomic-layer thickness, experiments so far have shown that they usually lose diverse properties and become insulators. In an attempt to extend the range of electronic phases of the single-atomic-layer oxide, we search for a metallic phase in a monolayer-thick epitaxial SrRuO$_3$ film. Combining atomic-scale epitaxy and angle-resolved photoemission measurements, we show that the monolayer SrRuO$_3$ is a strongly correlated metal. Systematic investigation reveals that the interplay between dimensionality and electronic correlation makes the monolayer SrRuO$_3$ an incoherent metal with orbital-selective correlation. Furthermore, the unique electronic phase of the monolayer SrRuO$_3$ is found to be highly tunable, as charge modulation demonstrates an incoherent-to-coherent crossover of the two-dimensional metal. Our work emphasizes the potentially rich phases of single-atomic-layer oxides and provides a guide to the manipulation of their two-dimensional correlated electron systems.

cond-mat.str-el

Capping and gate control of anomalous Hall effect and hump structure in ultra-thin SrRuO$_3$ films

Ferromagnetism and exotic topological structures in SrRuO$_3$ (SRO) induce sign-changing anomalous Hall effect (AHE). Recently, hump structures have been reported in the Hall resistivity of SRO thin films, especially in the ultra-thin regime. We investigate the AHE and hump structure in the Hall resistivity of SRO ultra-thin films with an SrTiO$_3$ (STO) capping layer and ionic liquid gating. STO capping results in sign changes in the AHE and modulation of the hump structure. In particular, the hump structure in the Hall resistivity is strongly modulated and even vanishes in STO-capped 4 unit cell (uc) films. In addition, the conductivity of STO-capped SRO ultra-thin films is greatly enhanced with restored ferromagnetism. We also performed ionic liquid gating to modulate the electric field at SRO/STO interface. Drastic changes in the AHE and hump structure are observed with different gate voltages. Our study shows that the hump structure as well as the AHE can be controlled by tuning inversion symmetry and the electric field at the interface.

cond-mat.mtrl-sci

Map equation for link community

Community structure exists in many real-world networks and has been reported being related to several functional properties of the networks. The conventional approach was partitioning nodes into communities, while some recent studies start partitioning links instead of nodes to find overlapping communities of nodes efficiently. We extended the map equation method, which was originally developed for node communities, to find link communities in networks. This method is tested on various kinds of networks and compared with the metadata of the networks, and the results show that our method can identify the overlapping role of nodes effectively. The advantage of this method is that the node community scheme and link community scheme can be compared quantitatively by measuring the unknown information left in the networks besides the community structure. It can be used to decide quantitatively whether or not the link community scheme should be used instead of the node community scheme. Furthermore, this method can be easily extended to the directed and weighted networks since it is based on the random walk.

physics.soc-ph

LinkRank: Finding communities in directed networks

To identify communities in directed networks, we propose a generalized form of modularity in directed networks by introducing a new quantity LinkRank, which can be considered as the PageRank of links. This generalization is consistent with the original modularity in undirected networks and the modularity optimization methods developed for undirected networks can be directly applied to directed networks by optimizing our new modularity. Also, a model network, which can be used as a benchmark network in further community studies, is proposed to verify our method. Our method is supposed to find communities effectively in citation- or reference-based directed networks.

physics.soc-ph