arXiv subjects

Younjung Jo

Publications and source records attributed to Younjung Jo.

12 recordsLinked to original sources

arXiv2026

Interfacial chirality-induced magnetic-field-free switching with high energy efficiency in all-vdW heterostructures

Chirality, a central concept across many scientific disciplines, continues to inspire the discovery of novel physical phenomena. In condensed matter physics, structural chirality - defined by the absence of mirror plane symmetries - has primarily been explored in bulk materials. However, new chiral phenomena can emerge uniquely at the interface, distinct from their bulk counterparts, when a chiral material forms a heterostructure. Here, we demonstrate that all van-der-Waals (vdW) heterostructure composed of the chiral Co1/3TaS2 and the achiral vdW ferromagnet Fe3GeTe2 exhibits two distinct and unconventional spin-orbit torques originating from the interfacial chirality. These torques enable magnetic-field-free switching of perpendicular magnetization with ultralow current density ~ 10^6 A/cm^2 and minimal power dissipation < 10^15 W/m^3. Moreover, by replacing Fe3GeTe2 with a similar vdW ferromagnet, Fe3GaTe2, but of higher Curie temperature, we achieved the magnetic-field-free switching at room temperature in the Fe3GaTe2/Co1/3TaS2 vdW heterostructure. Our findings establish interfacial chirality as a powerful new handle for spintronic control, opening a new pathway to explore chirality-induced phenomena beyond the bulk symmetry constraints - and paving the way toward highly efficient, low-power spintronic devices based on all-vdW heterostructures.

cond-mat.mtrl-sci↗

arXiv2026

Coherent canted ferrimagnetism and higher-order anisotropy in the nodal-line magnetic semiconductor Mn3Si2Te6

The interplay between magnetic order and electronic topology in van der Waals materials enables extreme responses to external stimuli. The nodal-line semiconductor Mn3Si2Te6 exemplifies this, exhibiting colossal angular magnetoresistance (CAMR) where resistivity changes by orders of magnitude upon rotating the magnetic field. While this phenomenon implies a profound coupling between spin orientation and charge transport, the microscopic magnetic potentials driving spin orientations remain elusive. Here, we combine thermodynamic torque magnetometry and electron spin resonance spectroscopy to reconstruct the magnetic anisotropy energy that controls magnetization rotation in Mn3Si2Te6. We show that low-temperature ground state is a coherent canted ferrimagnet stabilized by competing second- (K1) and fourth-order (K2) magnetic anisotropy. Crucially, torque requires a substantial symmetry-allowed sixth-order term (K3), which provides near-plane stiffness and sustains canting at high fields. Using the resulting anisotropy parameters, we compute the non-linear relation between field angle θ_H and magnetization angle θ_M and reparameterize CAMR in terms of θ_M, providing a concrete magnetic basis for how sharp angular transport features can emerge near the in-plane configuration.

cond-mat.str-el↗

arXiv2025

Current-driven collective control of helical spin texture in van der Waals antiferromagnet

Electrical control of quantum magnetic states is essential in spintronic science. Initial studies on the ferromagnetic state control were extended to collinear antiferromagnets and, more recently, noncollinear antiferromagnets. However, electrical control mechanisms of such exotic magnetic states remain poorly understood. Here, we report the first experimental and theoretical example of the current control of helical antiferromagnets, arising from the competition between collinear antiferromagnetic exchange and interlayer Dzyaloshinskii-Moriya interaction in new van-der-Waals (vdW) material Ni1/3NbS2. Due to the intrinsic broken inversion symmetry, an in-plane current generates spin-orbit torque that, in turn, interacts directly with the helical antiferromagnetic order. Our theoretical analyses indicate that a weak ferromagnetic order coexists due to the Dzyaloshinskii-Moriya interaction, mediating the spin-orbit torque to collectively rotate the helical antiferromagnetic order. Our Ni1/3NbS2 nanodevice experiments produce current-dependent resistance change consistent with the theoretical prediction. This work widens our understanding of the electrical control of helical antiferromagnets and promotes vdW quantum magnets as interesting material platforms for electrical control.

cond-mat.mtrl-sci↗

arXiv2022

Kondo interaction in FeTe and its potential role in the magnetic order

Finding d-electron heavy fermion (HF) states has been an important topic as the diversity in d-electron materials can lead to many exotic Kondo effect-related phenomena or new states of matter such as correlation-driven topological Kondo insulator or cooperation between long-range magnetism and Kondo lattice behavior. Yet, obtaining direct spectroscopic evidence for a d-electron HF system has been elusive to date. Here, we report the observation of Kondo lattice behavior in an antiferromagnetic metal, FeTe, via angle-resolved photoemission spectroscopy (ARPES) and transport properties measurements. The Kondo lattice behavior is represented by the emergence of a sharp quasiparticle at low temperatures. The transport property measurements confirm the low-temperature Fermi liquid behavior and reveal successive coherent-incoherent crossover upon increasing temperature. We interpret the Kondo lattice behavior as a result of hybridization between localized Fe 3dxy and itinerant Te 5pz orbitals. Our interpretation is further evidenced by Fano-type tunneling spectra which accompany a hybridization gap. Our observations strongly suggest unusual cooperation between Kondo lattice behavior and long-range magnetic order.

cond-mat.str-el↗

arXiv2021

Orbit topology analysed from $π$ phase shift of magnetic quantum oscillations in three-dimensional Dirac semimetal

With the emergence of Dirac fermion physics in the field of condensed matter, magnetic quantum oscillations (MQOs) have been used to discern the topology of orbits in Dirac materials. However, many previous researchers have relied on the single-orbit Lifshiftz-Kosevich formula, which overlooks the significant effect of degenerate orbits on MQOs. Since the single-orbit LK formula is valid for massless Dirac semimetals with small cyclotron masses, it is imperative to generalize the method applicable to a wide range of Dirac semimetals, whether massless or massive. This report demonstrates how spin-degenerate orbits affect the phases in MQOs of three-dimensional massive Dirac semimetal, NbSb$_2$. With varying the direction of the magnetic field, an abrupt $π$ phase shift is observed due to the interference between the spin-degenerate orbits. We investigate the effect of cyclotron mass on the $π$ phase shift and verify its close relation to the phase from the Zeeman coupling. We find that the $π$ phase shift occurs when the cyclotron mass is 1/2 of the electron mass, indicating the effective spin gyromagnetic ratio is $g_s$ = 2. Our approach is not only useful for analysing MQOs of massless Dirac semimetals with a small cyclotron mass, but also can be used for MQOs in massive Dirac materials with degenerate orbits, especially in topological materials with a sufficiently large cyclotron mass. Furthermore, this method provides a useful way to estimate the precise $g_s$ value of the material.

cond-mat.mes-hall↗

arXiv2021

Complete mapping of magnetic anisotropy for prototype Ising van der Waals FePS$_3$

Several Ising-type magnetic van der Waals (vdW) materials exhibit stable magnetic ground states. Despite these clear experimental demonstrations, a complete theoretical and microscopic understanding of their magnetic anisotropy is still lacking. In particular, the validity limit of identifying their one-dimensional (1-D) Ising nature has remained uninvestigated in a quantitative way. Here we performed the complete mapping of magnetic anisotropy for a prototypical Ising vdW magnet FePS$_3$ for the first time. Combining torque magnetometry measurements with their magnetostatic model analysis and the relativistic density functional total energy calculations, we successfully constructed the three-dimensional (3-D) mappings of the magnetic anisotropy in terms of magnetic torque and energy. The results not only quantitatively confirm that the easy axis is perpendicular to the $ab$ plane, but also reveal the anisotropies within the $ab$, $ac$, and $bc$ planes. Our approach can be applied to the detailed quantitative study of magnetism in vdW materials.

cond-mat.mtrl-sci↗

arXiv2019

Magnetic and electrical anisotropy with correlation and orbital effects in dimerized honeycomb ruthenate Li$_2$RuO$_3$

Li2RuO3 undergoes a structural transition at a relatively high temperature of 550 K with a distinct dimerization of Ru-Ru bonds on the otherwise isotropic honeycomb lattice. It exhibits a unique herringbone dimerization pattern with a largest ever reported value of the bond shrinkage of about ~ 0.5 Å. Despite extensive studies, both theoretical and experimental, however, its origin and its effect on physical properties still remain to be understood. In this work, using high quality single crystals we investigated the anisotropy of resistivity ($ρ$) and magnetic susceptibility ($χ$) to find a very clear anisotropy: $ρ$$_c*$ > $ρ$$_b$ > $ρ$$_a$ and $χ$$_b$ > $χ$$_a$ > $χ$$_c*$. For possible theoretical interpretations, we carried out density functional calculations to conclude that these anisotropic behavior is due to the correlation effects combined with the unique orbital structure and the dimerization of Ru 4d bands.

cond-mat.str-el↗

arXiv2018

Antiferromagnet-based spintronic functionality by controlling isospin domains in a layered perovskite iridate

The novel electronic state of the canted antiferromagnetic (AFM) insulator, strontium iridate (Sr2IrO4) has been well described by the spin-orbit-entangled isospin Jeff = 1/2, but the role of isospin in transport phenomena remains poorly understood. In this study, antiferromagnet-based spintronic functionality is demonstrated by combining unique characteristics of the isospin state in Sr2IrO4. Based on magnetic and transport measurements, large and highly anisotropic magnetoresistance (AMR) is obtained by manipulating the antiferromagnetic isospin domains. First-principles calculations suggest that electrons whose isospin directions are strongly coupled to in-plane net magnetic moment encounter the isospin mismatch when moving across antiferromagnetic domain boundaries, which generates a high resistance state. By rotating a magnetic field that aligns in-plane net moments and removes domain boundaries, the macroscopically-ordered isospins govern dynamic transport through the system, which leads to the extremely angle-sensitive AMR. As with this work that establishes a link between isospins and magnetotransport in strongly spin-orbit-coupled AFM Sr2IrO4, the peculiar AMR effect provides a beneficial foundation for fundamental and applied research on AFM spintronics.

cond-mat.str-el↗

arXiv2016

Broken-Symmetry Quantum Hall States in Twisted Bilayer Graphene

Twisted bilayer graphene offers a unique bilayer two-dimensional-electron system where the layer separation is only in sub-nanometer scale. Unlike Bernal-stacked bilayer, the layer degree of freedom is disentangled from spin and valley, providing eight-fold degeneracy in the low energy states. We have investigated broken-symmetry quantum Hall (QH) states and their transitions due to the interplay of the relative strength of valley, spin and layer polarizations in twisted bilayer graphene. The energy gaps of the broken-symmetry QH states show an electron-hole asymmetric behaviour, and their dependence on the induced displacement field are opposite between even and odd filling factor states. These results strongly suggest that the QH states with broken valley and spin symmetries for individual layer become hybridized via interlayer tunnelling, and the hierarchy of the QH states is sensitive to both magnetic field and displacement field due to charge imbalance between layers.

cond-mat.mes-hall↗

arXiv2016

NMR Evidences for the coupling between conduction electrons and molecular degrees of freedom in the exotic member of the Bechgaard salt, (TMTSF)2FSO3

We performed Se and F-NMR measurements on single crystals of (TMTSF)2FSO3 to characterize the electronic structures of different phases in the Temperature-Pressure phase diagram, determined by precise transport measurements [Jo et al., Phys. Rev. B67, 014516 (2003)]. We claim that such varieties of electronic states in the refined phase diagram are caused by strong couplings of the conduction electrons with FSO3 anions, especially with the permanent electric dipoles on the anions. We suggest that as temperature decreases, the FSO3 anions form orientational ordering through two steps; first only the tetrahedrons form an orientational order leaving the orientations of the electronic dipoles in random (transition I); then the dipoles form a perfect orientational order at a lower temperature (transition II). In the intermediate temperature range between transitions I and II, we found an appreciable enhancement of homogeneous and inhomogeneous widths of 77Se-NMR spectrum. From the analysis of the angular dependence of the linewidth, we attributed these anomalies to the intramolecular charge disproportionation or imbalance and its slow dynamics caused by the coupling with the permanent electric dipole of anion. Results of 19F-NMR relaxation and lineshape measurements support this picture very well. Electronic structures at higher pressures up to 1.25 GPa are discussed on the basis of the results of the 77Se and 19F-NMR measurements.

cond-mat.str-el↗

arXiv2013

Surface electronic structure of the topological Kondo insulator candidate correlated electron system SmB6

The Kondo insulator SmB6 has long been known to exhibit low temperature transport anomalies whose origin is of great interest. Here we uniquely access the surface electronic structure of the anomalous transport regime by combining state-of-the-art laser- and synchrotron-based angle-resolved photoemission techniques. We observe clear in-gap states (up to 4 meV), whose temperature dependence is contingent upon the Kondo gap formation. In addition, our observed in-gap Fermi surface oddness tied with the Kramers' points topology, their coexistence with the two-dimensional transport anomaly in the Kondo hybridization regime, as well as their robustness against thermal recycling, taken together, collectively provide by-far the strongest evidence for protected surface metallicity with a Fermi surface whose topology is consistent with the theoretically predicted topological surface Fermi surface (TSS). Our observations of systematic surface electronic structure provide the fundamental electronic parameters for the anomalous Kondo ground state of the correlated electron material SmB6.

cond-mat.str-el↗

arXiv2011

Evidence that the upper critical field of Nb3Sn is independent of whether it is cubic or tetragonal

Although 2011 marks the 50th anniversary of Nb3Sn as the first high field superconductor, real understanding of its upper critical field behavior μ0Hc2 is incomplete. Here we show surprising μ0Hc2 data on highly homogeneous bulk samples examined both by small-current, transport and by volumetric-averaging specific heat and the reversible magnetization techniques, which exhibit identical upper critical field μ0Hc2(0.3 K) ~ 29{\pm} 0.2 T with or without undergoing the cubic to tetragonal transition, a result in strong contrast to widely used multiple-source data compilations that show a strong depression of μ0Hc2(0K) from 29 T to 21.4 T in the tetragonal state.

cond-mat.supr-con↗