arXiv subjects

Yu Tao

Publications and source records attributed to Yu Tao.

At least 19 recordsLinked to original sources

arXiv2026

Amorphous and Nanocrystalline Topological Semimetal YPtBi/W/CoFeB Heterostructures for BEOL-Compatible Spin-Orbit Torque Devices

Spin-orbit torque (SOT) devices require spin-source materials that combine efficient charge-to-spin conversion with back-end-of-line (BEOL) thermal compatibility. Here, we show that YPtBi/W/CoFeB heterostructures deposited directly on Si/SiOx remain predominantly amorphous or weakly nanocrystalline from room temperature to 400 {\deg}C while preserving a large effective damping-like SOT response. Anomalous Hall and harmonic Hall measurements, together with X-ray diffraction, cross-sectional transmission electron microscopy, X-ray reflectivity, and electron energy-loss spectroscopy, show that the response does not correlate with bulk crystallization of YPtBi. Instead, the interfacial analysis indicates that the strongest trend of the spin Hall angle is associated with the chemistry of the upper YPtBi/W boundary: the effective SOT response tracks the integrated W concentration at that YPtBi surface. Meanwhile, a two-spin source analysis shows that the Pt-W-rich interlayer provides only a small positive correction, insufficient to explain the large negative effective spin Hall angle by itself. The dominant control variable is therefore inferred to be the incorporation of W into the upper YPtBi interface, which plausibly modifies the local electronic structure of YPtBi and amplifies the stack-level response. These results provide a more physically constrained interpretation of the stack behavior and identify a BEOL-compatible route to disordered topological spin-source layers for scaled SOT memory and compute-in-memory hardware.

cond-mat.mtrl-sci↗

arXiv2026

Noise-resilient nanophotonic gyroscope with sub-prad phase resolution

Optical gyroscopes based on the Sagnac effect are the cornerstone of precision orientation and navigation. However, their bulky form factors prevent deployment in emerging mobile and autonomous systems. On nanophotonic platforms, the Sagnac signal plummets under aggressive miniaturization. Consequently, the signal is easily swamped by refractive-index fluctuations, rendering navigation-grade sensitivity within just a few square millimeters a notoriously elusive goal. Here, we demonstrate a noise-resilient nanophotonic optical gyroscope by exploiting a two-chain decoupling architecture to effectively isolate the rotation signal from channel noise. Implemented on a 3 mm^2 passive silicon nitride chip, the proof-of-concept device achieves a bias instability of 1.42 deg/h and an angle random walk of 0.001 deg/\sqrt{h}, representing improvements of 4 and 6 orders of magnitude, respectively, over the representative nanophotonic gyroscope of similar footprint (ref. 27). In the broader context of integrated optical gyroscopes, our approach bridges the long-standing size-performance gap by two to three orders of magnitude, moving chip-scale devices into a previously inaccessible regime and pointing toward navigation-relevant precision for monolithic microsystems. This architecture further enables sub-prad phase resolution with general applicability, establishing a foundational framework for the next generation of robust, monolithically integrated photonic sensing systems.

physics.optics↗

arXiv2026

Research on the central region of quasars based on variability and structure function

Quasars,asextremelyluminousanddistantspecialcelestialbodiesintheuniverse,aredrivenbyacomplexsystemcomposedof supermassiveblackholesandsurroundingaccretiondisks.Thispaperadoptsatime-domainobservationstrategyandcombines the analysis of light curves with the construction of structure functions to indirectly reveal the physical essence of the central regionofquasarsfromtheperspectiveofvariability.Theresearchdataarederivedfromthelargesampleobservationdataofthe SloanDigitalSkySurvey(SDSS).Throughextensivedatastatisticsandcorrelationanalysis,aseriesofimportantfindingshave been obtained: the characteristic parameters of the structure function of quasars show significant correlations with luminosity, black hole mass, and Eddington ratio. That is, quasars with higher luminosity, larger black hole mass, and larger Eddington ratiohavelargerstructurefunctions.Forquasarsofthesameluminosity,thelargertheEddingtonratio,thesmallerthestructure function. However, the correlation between the structure function and redshift or rest wavelength is not significant, indicating that the variabilitycharacteristicsofquasars aremainly determined bytheir own physical propertiesandareminimallyaffected by the cosmologicalredshifteffect.

astro-ph.GA↗

arXiv2026

The characteristics of variability of AGNs based on the structure function

Variability is one of the classic features of active galactic nuclei (AGNs). The normalized structure function was applied to distinguish variability samples from OVRO, ASAS-SN and Fermi. A power-law function model was selected to fit the structure functions of samples of three bands. We present the available samples of three bands, and by integrating two parameters, we obtain ideal discrimination results for three bands. Meanwhile, the differences between BL Lacs and FSRQs of Fermi and non-Fermi samples are well verified. The results show that the improved structure function can effectively distinguish samples of radio, optical, and gamma-ray. Additionally, BL Lacs and FSRQs in both Fermi and non-Fermi samples can be distinguished. The conclusion obtained through the distinction of structural functions in different bands supports that the variability in the three bands are caused by different physical mechanisms respectively: the samples in the optical band are radio quiet AGNs, and their variability is mainly caused by the fluctuations of the accretion disk, and the samples of radio band and gamma-ray band are radio loud AGNs whose variability is mainly caused by relativistic jet radiation. This conclusion conforms to the unified standard interpretation of variability about AGNs. Using these two parameters, we verify that there is no fundamental difference between Fermi and non-Fermi BL Lacs, while significant differences exist between FSRQs. However, the power exponent of the two can well distinguish BL Lacs.

astro-ph.HE↗

arXiv2026

State-dependent broadband X-ray Timing Reconfiguration in the Changing-look AGN NGC 1566

NGC 1566 has shown dramatic X-ray spectral changes during its recent changing-look outburst, but the evolution of its broadband X-ray timing properties remains poorly constrained. We combine long-term Swift/XRT monitoring with high-time-resolution XMM-Newton observations to construct one pre-outburst Dim broadband PSD and two outburst broadband reconstructions associated with the O1 peak and O2 decay observations. In the outburst reconstructions, the same Swift/XRT up-state monitoring segment provides the low-frequency constraint, while the O1 and O2 XMM-Newton observations provide phase-specific high-frequency constraints. Using PSRESP forward modelling with the observed sampling windows, we test bending-power-law PSD models in the soft (0.3-2 keV) and hard (2-10 keV) bands. The Dim and O2-associated reconstructions are acceptably described by bending-power-law solutions, whereas the O1 peak observation does not yield a robust bend-frequency measurement. For the accepted Dim and O2-associated solutions, the preferred bend frequency shifts from about 2.0 x 10^-5 to about 2.7 x 10^-7 Hz in the soft band, and from about 2.1 x 10^-5 to about 2.7 x 10^-7 Hz in the hard band, implying a substantially longer characteristic variability timescale in the O2-associated reconstruction. This consistent shift in both energy bands suggests that the timing evolution is not confined to the soft-excess component alone, but reflects a broader change in the X-ray variability structure. Together with previous spectral studies, these results point to a transient reconfiguration of the disc-corona variability timescale during the changing-look transition in NGC 1566.

astro-ph.HE↗

arXiv2026

Timescale-dependent Optical Variability of Turn-on Changing-look Active Galactic Nuclei

Changing-look active galactic nuclei (CL AGNs) provide a valuable opportunity to study optical variability associated with changes in accretion state. We investigate the optical variability of turn-on CL AGNs, selected through the emergence or strengthening of broad emission lines, using g-band light curves from the Zwicky Transient Facility. For a final sample of 106 objects, we measure structure-function amplitudes at three fixed rest-frame timescales, SF30, SF150 and SF300, and examine their dependence on optical luminosity, Eddington ratio, black-hole mass and rest-frame wavelength using Spearman-rank correlations and multivariate regressions. The strongest trends are found on monthly timescales. SF30 is significantly anti-correlated with both optical luminosity and Eddington ratio, with Spearman coefficients of rho = -0.39 and rho = -0.33, respectively. These negative trends remain in multivariate regressions after accounting for black-hole mass and rest-frame wavelength. The dependence weakens at longer timescales: SF150 shows only weak evidence for luminosity or Eddington-ratio dependence, while SF300 shows no robust dependence. Black-hole mass shows no robust single-parameter correlation, and its multivariate coefficients depend on the model form, indicating that its apparent role is affected by covariance with luminosity and Eddington ratio. The rest-frame wavelength term is generally negative, but cannot be separated from redshift in this single-band analysis. These results suggest that monthly optical variability in turn-on CL AGNs is more closely linked to bright-state accretion properties than variability on half-year to year-long timescales.

astro-ph.GA↗

arXiv2025

Transformational astrophysics and exoplanet science with Habitable Worlds Observatory's High Resolution Imager

Habitable Worlds Observatory (HWO) will be NASA's flagship space telescope of the 2040s, designed to search for life on other planets and to transform broad areas of astrophysics. NASA are seeking international partners, and the UK is well-placed to lead the design and construction of its imaging camera - which is likely to produce the mission's most visible public impact. Early participation in the mission would return investment to UK industry, and bring generational leadership for the UK in space science, space technology, and astrophysics.

astro-ph.IM↗

arXiv2025

Local Proton Disorder Induced Intermolecular H-H Coupling in Ionization of Dense Ammonia

Under cold compression, hydrogen bonding was considered to dominate intermolecular interaction during the ionization of ammonia. Here, we provide experimental and theoretical evidence of intermolecular HH coupling in dense ammonia. Ab initio molecular dynamics simulations (AIMD) reveal an increasing degree of proton disorder in ammonia with increasing pressure, which promotes intermolecular H-H coupling. At pressure below the ionization phase transition pressure (135 GPa), intermolecular HH coupling gives rise to a unique dissociation pathway in ammonia. Sporadic molecular hydrogen was observed without laser heating, accompanied by the absence of molecular nitrogen. At pressure above 135 GPa, intermolecular HH coupling serves as an intermediate state in the ionization of ammonia. Two fingerprint Raman modes previously assigned to the ionic phase disappear upon further compression or heating. Together with proton transfer based on hydrogen bond, a dual path mechanism exists in the ionization of ammonia. Our results demonstrate a case of hydrides phase transition pathway that occurs independently of hydrogen bonding under high pressure.

physics.chem-ph↗

arXiv2025

Observation of Iron Oxide to Nitride Conversion via Liquid Liquid Phase Separation in High pressure Borate Melt

High pressure chemistry provides a powerful route to materials that are inaccessible or difficult to synthesize under ambient conditions. However, high pressure chemical reaction processes and mechanisms remain largely unexplored because of the challenges associated with in situ characterization under high pressure and high temperature, particularly within the deeply enclosed sample environment of a large volume press. Here, we employ the state of the art real time synchrotron X ray radiography to image a high pressure chemical reaction at 5.4 GPa and 1700 K within a large volume press. Using Fe2O3 and BN as precursors, we capture the complete dynamic metal oxide to nitride conversion and show that it differs fundamentally from conventional solid state diffusion controlled nitridation. Synchrotron X ray radiography clearly revealed that this conversion involves a two stage liquid liquid separation process (LLPS), including fluid nitrogen and fluid Fe N alloy. On the basis of these observations, we propose a nitrogen driven mechanism for LLPS in borate melts. Specifically, nitrogen reduces metal cations in the borate network, altering their coordination environments and triggering a substantial reorganization of the melt structure. This coordination induced restructuring destabilizes the borate melt and promotes the LLPS of fluid Fe N alloy. Our in-situ observations suggest a general pathway for high pressure metal oxide to nitride conversion. This study provides a direct visualization of a pres-sure-enabled chemical reaction that is inaccessible under ambient conditions, offering fundamental in-sight into how high pressure reshapes chemical reaction pathways and enables the synthesis of metal nitrides.

physics.chem-ph↗

arXiv2025

Nanosecond-latency all-optical fiber sensing with in-sensor computing

Optical fiber sensing plays a crucial role in modern measurement systems and holds significant promise for a wide range of applications. This potential, though, has been fundamentally constrained by the intrinsic latency and power limitations associated with electronic signal processing. Here, we propose an all-optical fiber sensing architecture with in-sensor computing (AOFS-IC) that achieves fully optical-domain sensing signal demodulation at the speed of light. By integrating a scattering medium with an optimized diffractive optical network, AOFS-IC enables linear mapping of physical perturbations to detected intensity, and sensing results can be directly read out without electronic processing. The proposed system maintains high accuracy across various sensing tasks, providing sub-nano strain resolution and 100% torsional angle classification accuracy, as well as multiplexed sensing of multiple physical quantities, and performing multi-degree-of-freedom robot arm monitoring. AOFS-IC eliminates computing hardware requirements while providing <3 ns demodulation delay, which is more than 2 orders of magnitude faster than conventional fiber optic sensing systems. This work demonstrates the potential of next-generation optical sensing systems empowered by all-optical computing, and paves the way for expanded applications of fiber sensing through the integration of fully optical components, ultrafast measurement speed, and low power consumption.

physics.optics↗

arXiv2025

Dual Optical Hyperbolicity of PdCoO$_2$ and PdCrO$_2$ Delafossite Single Crystals

Hyperbolic materials exhibit a very peculiar optical anisotropy with simultaneously different signs of the dielectric tensor components. This anisotropy allows the propagation of exotic surface-wave excitations like hyperbolic phonons and plasmon polaritons. While hyperbolic materials hold promise for applications in subwavelength photonics and enhanced light-matter interactions, their natural occurrence is limited to few materials, often accompanied by significant dielectric losses and limited hyperbolic spectral bandwidth. Focusing on PdCoO$_2$ and PdCrO$_2$ delafossite transition-metal oxides, in this paper we demonstrate their unique dual hyperbolic regimes: one localized around a phonon absorption in the mid-infrared spectral region, and the other extending into the visible range. Both hyperbolic regimes show exceptional properties including low dissipation and high hyperbolic quality factors. These results pave the way for innovative applications of delafossite layered metals in subwavelength photonics, imaging, and sensing.

cond-mat.mtrl-sci↗

arXiv2023

Crystal-Chemical Origins of the Ultrahigh Conductivity of Metallic Delafossites

Despite their highly anisotropic complex-oxidic nature, certain delafossite compounds (e.g., PdCoO2, PtCoO2) are the most conductive oxides known, for reasons that remain poorly understood. Their room-temperature conductivity can exceed that of Au, while their low-temperature electronic mean-free-paths reach an astonishing 20 microns. It is widely accepted that these materials must be ultrapure to achieve this, although the methods for their growth (which produce only small crystals) are not typically capable of such. Here, we first report a new approach to PdCoO2 crystal growth, using chemical vapor transport methods to achieve order-of-magnitude gains in size, the highest structural qualities yet reported, and record residual resistivity ratios (>440). Nevertheless, the first detailed mass spectrometry measurements on these materials reveal that they are not ultrapure, typically harboring 100s-of-parts-per-million impurity levels. Through quantitative crystal-chemical analyses, we resolve this apparent dichotomy, showing that the vast majority of impurities are forced to reside in the Co-O octahedral layers, leaving the conductive Pd sheets highly pure (~1 ppm impurity concentrations). These purities are shown to be in quantitative agreement with measured residual resistivities. We thus conclude that a previously unconsidered "sublattice purification" mechanism is essential to the ultrahigh low-temperature conductivity and mean-free-path of metallic delafossites.

cond-mat.mtrl-sci↗

arXiv2023

Investigating the magneto-elastic properties in FeSn and Fe$_{3}$Sn$_{2}$ flat band metals

Topological quantum magnets FeSn and Fe$_{3}$Sn$_{2}$ were studied using neutron scattering and first-principles calculations. Both materials are metallic but host dispersionless flat bands with Dirac nodes at the $K$ point in reciprocal space. The local structure determined from the pair density function analysis of the neutron diffraction data provided no evidence for electron localization in both compounds, consistent with their metallic nature. At the same time, in FeSn, an anomalous suppression in the $c$-axis lattice constant coupled with changes in the phonon spectra were observed across T$_{N}$ indicating the presence of magneto-elastic coupling and spin-phonon interactions. In addition, it was observed that spin waves persisted well above T$_{N}$, suggesting that the in-plane ferromagnetic spin correlations survive at high temperatures. In contrast, no lattice anomaly was observed in Fe$_{3}$Sn$_{2}$. The inelastic signal could be mostly accounted for by phonons, determined from density functional theory, showing typical softening on warming.

cond-mat.mtrl-sci↗

arXiv2022

Emergence of Layer Stacking Disorder in c-axis Confined MoTe$_2$

The layer stacking order in 2D materials strongly affects functional properties and holds promise for next generation electronic devices. In bulk, octahedral MoTe$_2$ possesses two stacking arrangements, the Weyl semimetal T$_d$ phase, and the higher-order topological insulator 1T' phase; however, it remains unclear if thin exfoliated flakes of MoTe$_2$ follow the T$_d$, 1T', or an alternative stacking sequence. Here, we resolve this debate using atomic-resolution imaging within the transmission electron microscope. We find that the layer stacking in thin flakes of MoTe$_2$ is highly disordered and pseudo-random, which we attribute to intrinsic confinement effects. Conversely, WTe$_2$, which is isostructural and isoelectronic to MoTe$_2$, displays ordered stacking even for thin exfoliated flakes. Our results are important for understanding the quantum properties of MoTe$_2$ devices, and suggest that thickness may be used to alter the layer stacking in other 2D materials.

cond-mat.mtrl-sci↗

arXiv2021

Lattice and magnetic dynamics in YVO$_{3}$ Mott insulator studied by neutron scattering and first-principles calculations

The Mott insulator YVO$_{3}$ with $T_{N}$ = 118 K is revisited to explore the role of spin, lattice and orbital correlations across the multiple structural and magnetic transitions observed as a function of temperature. Upon cooling, the crystal structure changes from orthorhombic to monoclinic at 200 K, and back to orthorhombic at 77 K, followed by magnetic transitions. From the paramagnetic high temperature phase, C-type ordering is first observed at 118 K, followed by a G-type spin re-orientation transition at 77 K. The dynamics of the transitions were investigated via inelastic neutron scattering and first principles calculations. An overall good agreement between the neutron data and calculated spectra was observed. From the magnon density of states, the magnetic exchange constants were deduced to be $J_{ab}$ = $J_{c}$ = -5.8 meV in the G-type spin phase, and $J_{ab}$ = -3.8 meV, $J_{c}$ = 7.6 meV at 80 K and $J_{ab}$ = -3.0 meV, $J_{c}$ = 6.0 meV at 100 K in the C-type spin phase. Paramagnetic scattering was observed in the spin ordered phases, well below the C-type transition temperature, that continuously increased above the transition. Fluctuations in the temperature dependence of the phonon density of states were observed between 50 and 80 K as well, coinciding with the G-type to C-type transition. These fluctuations are attributed to optical oxygen modes above 40 meV, from first principles calculations. In contrast, little change in the phonon spectra is observed across $T_{N}$.

cond-mat.str-el↗

arXiv2021

Large change of interlayer vibrational coupling with stacking in Mo$_{1-x}$W$_{x}$Te$_{2}$

Stacking variations in quasi-2D materials can have an important influence on material properties, such as changing the topology of the band structure. Unfortunately, the weakness of van der Waals interactions makes it difficult to compute the stacking dependence of properties, and even in a material as simple as graphite the stacking energetics remain unclear. Mo$_{1-x}$W$_{x}$Te$_{2}$ is a material in which three differently-stacked phases are conveniently accessible by temperature changes: $1T^{\prime}$, $T^*_d$, and the reported Weyl semimetal phase $T_d$. The transitions proceed via layer sliding, and the corresponding interlayer shear mode (ISM) is relevant not just for the stacking energetics, but for understanding the relationship between the Weyl physics and structural changes. However, the interlayer interactions of Mo$_{1-x}$W$_{x}$Te$_{2}$ are not well understood, with wide variation in computed properties. We report inelastic neutron scattering of the ISM in a Mo$_{0.91}$W$_{0.09}$Te$_{2}$ crystal. The ISM energies are generally consistent with the linear chain model (LCM), as expected given the weak interlayer interaction, though there are some discrepancies from predicted intensities. However, the interlayer force constants $K_x$ in the $T^*_d$ and $1T^{\prime}$ phases are substantially weaker than that of $T_d$, at 76(3)% and 83(3)%, respectively. Considering that the relative positioning of atoms in neighboring layers is approximately the same regardless of overall stacking, our results suggest that longer-range influences, such as stacking-induced band structure changes, may be responsible for the substantial change in the interlayer vibrational coupling. These findings should elucidate the stacking energetics of Mo$_{1-x}$W$_{x}$Te$_{2}$ and other van der Waals layered materials.

cond-mat.mtrl-sci↗

arXiv2021

Gapless Dirac magnons in CrCl$_{3}$

Bosonic Dirac materials are testbeds for dissipationless spin-based electronics. In the quasi two-dimensional honeycomb lattice of CrX$_{3}$ (X=Cl, Br, I), Dirac magnons have been predicted at the crossing of acoustical and optical spin waves, analogous to Dirac fermions in graphene. Here we show that, distinct from CrBr$_{3}$ and CrI$_{3}$, gapless Dirac magnons are present in bulk CrCl$_{3}$, with inelastic neutron scattering intensity at low temperatures approaching zero at the Dirac $K$ point. Upon warming, magnon-magnon interactions induce strong renormalization and decreased lifetimes, with a ~25% softening of the upper magnon branch intensity from 5 to 50 K, though magnon features persist well above T$_{N}$. Moreover, an unusual negative thermal expansion (NTE) of the $a$-axis lattice constant and anomalous phonon behavior are observed below 50 K, indicating magnetoelastic and spin-phonon coupling arising from an increase in the in-plane spin correlations that begins tens of Kelvin above T$_{N}$.

cond-mat.mtrl-sci↗

arXiv2021

Insiders and Outsiders in Research on Machine Learning and Society

A subset of machine learning research intersects with societal issues, including fairness, accountability and transparency, as well as the use of machine learning for social good. In this work, we analyze the scholars contributing to this research at the intersection of machine learning and society through the lens of the sociology of science. By analyzing the authorship of all machine learning papers posted to arXiv, we show that compared to researchers from overrepresented backgrounds (defined by gender and race/ethnicity), researchers from underrepresented backgrounds are more likely to conduct research at this intersection than other kinds of machine learning research. This state of affairs leads to contention between two perspectives on insiders and outsiders in the scientific enterprise: outsiders being those outside the group being studied, and outsiders being those who have not participated as researchers in an area historically. This contention manifests as an epistemic question on the validity of knowledge derived from lived experience in machine learning research, and predicts boundary work that we see in a real-world example.

cs.CY↗