The Counterintuitive "One-Enhanced, One-Suppressed" Bifurcation Phenomenon of Spin Mobility under Weak Spin-Orbit Coupling in Helices
The chiral-induced spin selectivity (CISS) effect poses a longstanding puzzle: how weak spin-orbit coupling (SOC) within a helical molecule produces strong spin polarization. We uncover a counterintuitive phenomenon, a "one-enhanced, one-suppressed" bifurcation of spin-resolved mobility relative to the SOC-free case. We trace this phenomenon to an analytical sign reversal of spin-dependent transmission and identify it as the microscopic origin of CISS. The phenomenon is found absent in achiral systems and single-stranded DNA, validating our theoretical picture. Our findings resolve the core puzzle and establish the origin of CISS.