arXiv subjects

Yu-Yuan Chen

Publications and source records attributed to Yu-Yuan Chen.

12 recordsLinked to original sources

arXiv2025

Hybrid quantum surface acoustic wave with skyrmion qubit for quantum information processing

Surface acoustic wave (SAW) devices are key components of classical communication systems and recently studied for quantum information processing. We here propose and study a hybrid quantum system composed of skyrmion qubit and a SAW cavity, which supports a number of long-lived phononic modes. The results show that the system allows for strong coupling between skyrmion qubit and single phonon of different modes. By manipulating the qubit(s) through a static magnetic field and a time-dependent modulation magnetic field, we further study the interaction between skyrmion qubit and individual phononic modes, phonon-phonon interaction, and qubit-qubit interaction, which operates in strong-coupling regime. The controllability of nanoscale skyrmion qubit and the dense phononic modes of single SAW cavity would make our system have promising applications in large-scale quantum communication and computing.

quant-ph↗

arXiv2024

Manipulation of magnetic systems by quantized surface acoustic wave via piezomagnetic effect

The quantized surface acoustic wave (SAW) in the piezoelectric medium has recently been studied, and is used to control electric dipoles of quantum systems via the electric field produced through piezoelectric effect. However, it is not easy and convenient to manipulate magnetic moments directly by the electric field. We here study a quantum theory of SAW in the piezomagnetic medium. We show that the intrinsic properties of the piezomagnetic medium enable the SAW in the piezomagnetic medium to directly interact with magnetic moments of quantum systems via magnetic field induced by piezomagnetic effect. By taking the strip SAW waveguide made of piezomagnetic medium as an example, we further study the coupling strengths between different magnetic quantum systems with magnetic moments and the quantized single-mode SAW in the waveguide. Based on this, we discuss the interaction between magnetic quantum systems mediated by the quantized multi-mode SAW in piezomagnetic waveguide. Our study provides a convenient way to directly control magnetic quantum systems by quantized SAW, and offers potential applications to on-chip information processing based on solid-state quantum systems via quantized acoustic wave.

quant-ph↗

arXiv2022

Enantiodiscrimination of chiral molecules via quantum correlation function

We propose a method to realize enantiodiscrimination of chiral molecules based on quantum correlation function in a driven cavity-molecule system, where the chiral molecule is coupled with a quantized cavity field and two classical light fields to form a cyclic three-level model. According to the inherent properties of electric-dipole transition moments of chiral molecules, there is a $π$-phase difference in the overall phase of the cyclic three-level model for the left- and right-handed chiral molecules. Thus, the correlation function depends on this overall phase and is chirality-dependent. The analytical and numerical results indicate that the left- and right-handed chiral molecules can be discriminated by detecting quantum correlation function. Our work opens up a promising route to discriminate molecular chirality, which is an extremely important task in pharmacology and biochemistry.

quant-ph↗

arXiv2021

Enantio-detection of cyclic three-level chiral molecules in a driven cavity

We propose an enantio-detection method of chiral molecules in a cavity with external drive. The chiral molecules are coupled with a quantized cavity field and two classical light fields to form the cyclic three-level systems. The chirality-dependent cavity-assisted three-photon process in the three-level systems leads to the generation of intracavity photons. Simultaneously, the drive field also results in the chirality-independent process of the generation of intracavity photons. Based on the interference between the intracavity photons generated from these two processes, one can detect the enantiomeric excess of chiral mixture via monitoring the transmission rate of the drive field.

quant-ph↗

arXiv2021

Enantio-detection via cavity-assisted three-photon processes

We propose a method for enantio-detection of chiral molecules based on a cavity-molecule system, where the left- and right-handed molecules are coupled with a cavity and two classical light fields to form cyclic three-level models. Via the cavity-assisted three-photon processes based on the cyclic three-level model, photons are generated continuously in the cavity even in the absence of external driving to the cavity. However, the photonic fields generated from the three-photon processes of left- and right-handed molecules differ with the phase difference π according to the inherent properties of electric-dipole transition moments of enantiomers. This provides a potential way to detect the enantiomeric excess of chiral mixture by monitoring the output field of the cavity.

quant-ph↗

arXiv2021

Enantio-conversion of chiral mixtures via optical pumping

Enantio-conversion with the help of electromagnetic fields is an essential issue due to the chirality-dependence of many chemical, biological, and pharmaceutical processes. Here, we propose a method for this issue based on a five-level double-$Δ$ model of chiral molecules. By utilizing the breaking of left-right symmetry in the two $Δ$-type sub-structures, we can establish the chiral-state-selective excitation with one chiral ground state being excited to an achiral excited state and the other one being undisturbed. In the meanwhile, the achiral excited state will relax to the two chiral ground states. The two effects simultaneously acting on the chiral mixtures can convert molecules of different chiralities to the ones of the same chirality, i.e., the enantio-conversion via optical pumping. With typical parameters in gas-phase experiments, we numerically show that highly efficient enantio-conversion can be achieved. Our method works in the appearance of decoherences and without the precise control of pulse-durations (pulse-areas) and/or pulse-shapes. These advantages offer it promising features in promoting the future exploring of enantio-conversion.

quant-ph↗

arXiv2021

Improved laser-distillation method for complete enantio-conversion of chiral mixtures

Laser-assisted enantio-conversion is an ambitious issue related to chiral molecules in the atomic, molecular, and optical physics. The theoretical laser-distillation method had been proposed to realize enantio-conversion based on a four-level double-$Δ$ model of two degenerated chiral ground states and two achiral excited states. Here, we re-investigate and improve the laser-distillation method so that a chiral mixture can be converted to an enantiopure sample of the desired chirality, i.e., complete enantio-conversion, which has not been discussed in the previous theoretical works of the laser-distillation method. Since the undesired chirality may be inefficient or even cause serious side effects in pharmacology, our work plays as an important improvement to the original theoretical works of the laser-assisted enantio-conversion.

physics.chem-ph↗

arXiv2020

Evading thermal population influence in enantiomeric-specific state transfer based on a cyclic three-level system via ro-vibrational transitions

Optical methods of enantiomeric-specific state transfer had been proposed theoretically based on a cyclic three-level system of chiral molecule. According to these theoretical methods, recently the breakthrough progress has been reported in experiments [S. Eibenberger et al., Phys. Rev. Lett. 118, 123002 (2017); C. Pérez et al., Angew. Chem. Int. Ed. 56, 12512 (2017)] for cold gaseous chiral molecules but with low state-specific enantiomeric enrichment. One of the limiting factors is the influence of the thermal population in the selected three purely rotational states in experiment. Here, we theoretically propose an improved optical method of enantiomeric-specific state transfer to effectively evade such an adverse impact of thermal population by introducing ro-vibrational transitions for the cyclic three-level system of chiral molecules. Then, at the typical temperature in experiments approximately only the lowest state in the chosen three-level system is thermally occupied and the optical method of enantiomeric-specific state transfer works well. Comparing with the case of purely rotational transitions where all the three states are thermally occupied, this modification will remarkably increase the obtained state-specific enantiomeric enrichment with enantiomeric excess approximately 100%.

quant-ph↗

arXiv2020

Enantio-discrimination via light deflection effect

We propose a theoretical method for enantio-discrimination based on the light deflection effect in four-level models of chiral molecules. This four-level model consists of a cyclic three-level subsystem coupled by three strong driving fields and an auxiliary level connected to the cyclic three-level subsystem by a weak probe field. It is shown that the induced refractive index for the weak probe field is chirality-dependent. Thus it will lead to chirality-dependent light deflection when the intensities of two of the three strong driving fields are spatially inhomogeneous. As a result, the deflection angle of the weak probe light can be utilized to detect the chirality of pure enantiomers and enantiomeric excess of chiral mixture. Therefore, our method may act as a tool for enantio-discrimination.

physics.optics↗

arXiv2020

Fast enantioconversion of chiral mixtures based on a four-level double-$Δ$ model

Based on the four-level double-$Δ$ model composed of two degenerated (left- and right-handed) chiral ground states and two achiral excited states, we propose a purely optical method for enantio-conversion of chiral mixture. By choosing appropriate parameters, the original four-level model will be simplified to two effective two-level sub-systems with each of them involving one chiral ground state. Then, with the help of well-designed optical operations, the initial unwanted and wanted chiral ground states are converted, respectively, to the wanted chiral ground state and an auxiliary chiral excited state with the wanted chirality, i.e., achieving the enantioconversion of the chiral mixture. Comparing with the original work of enantioconversion based on the four-level double-$Δ$ model with the requirement of the time-consuming relaxation step and repeated operations, our method can be three orders of magnitude faster since we use only purely optical operations. Thus, it offers a promising candidate for fast enantioconversion when the total operation time is limited due to the racemization and/or experimental conditions.

physics.optics↗

arXiv2019

Effective two-level models for highly efficient inner-state enantio-separation based on cyclic three-level systems of chiral molecules

Based on cyclic three-level systems of chiral molecules, we propose two methods to realize highly efficient inner-state enantio-separations of a chiral mixture with the two enantiomers initially prepared in their ground states. Our methods work in the region where the evolutions of the two enantiomers can be described by their corresponding effective two-level models, simultaneously. The approximately $100\%$-efficiency inner-state enantio-separations can be realized when the probability occupying the ground state of one enantiomer becomes $0$ by experiencing half-integer periods of its corresponding on-resonance Rabi oscillation and in the meanwhile the other one still stays approximately in the ground state, under the conditions that the two enantiomers are governed by the effective on-resonance and large-detuning two-level models, respectively. Alternatively, the exactly $100\%$-efficiency inner-state enantio-separation can be obtained when the probabilities occupying the ground states of the two enantiomers simultaneously experience half-integer and integer periods of their corresponding on-resonance and detuned (instead of largely-detuned) Rabi oscillations with final $0$ and $1$ probabilities occupying the ground state, respectively.

physics.optics↗

arXiv2019

Determination of enantiomeric excess with chirality-dependent AC Stark effects in cyclic three-level models

Determination of enantiomeric excess is important and remains challenges. We theoretically propose a new spectroscopic method for this issue based on the chirality-dependent AC Stark effects in cyclic three-level models under the three-photon resonance condition. The enantiomeric excess of the chiral mixture is determined by comparing the amplitudes of the two chosen AC Stark peaks in the Fourier transform spectrum of the induced polarizations, which are (approximately) proportional to the molecule numbers of the two enantiomers, respectively. Comparing with current spectroscopic methods based on the interference between the electric- and (usually weak) magnetic-dipole transition moments and/or with the need for enantio-pure samples, our method only involves electric-dipole transitions and does not require the enantio-pure samples. Therefore, it will give strong chiral signals and can be applied to the determinations of enantiomeric excess for chiral molecules whose enantio-pure samples are still challenging to achieve.

physics.optics↗