Yu-chen Karen Chen-Wiegart

arXiv2026

Dynamic Coherent Diffractive Imaging Using Only a Support Constraint in the Complex Plane

We show that a bounded temporal increment prior on the sample dynamics is sufficient to reconstruct a time-varying phase object from a near-field diffraction movie, under the thin-film approximation. The time evolution of the field is parameterized by a multiplicative inter-frame update factor, and a bound on its complex-plane support enforces a bounded phase increment and a passive amplitude constraint. Reconstruction of the dynamic field is thereby converted into a feasibility problem with two projection operators: a measurement-domain modulus projection and an object-domain circular-sector projection. We validate the approach experimentally using a spatial light modulator as a calibrated dynamic sample in two cases: a reaction--diffusion phase pattern with spatially expanding extent, and a growing phase pattern whose accumulated phase reaches $10π$. In both cases the reconstructed phase trajectory agrees well with the ground truth. We then apply the same framework, without modification, to in-situ monitoring of a photo-polymer 3D printing process, recovering the spatiotemporal phase induced by polymerization under a spatially patterned blue light. The reconstructed phase trajectory provides an observable for photo-chemical system identification and process control.

physics.optics↗

arXiv2025

Accelerating Discovery of Solid-State Thin-Film Metal Dealloying for 3D Nanoarchitecture Materials Design through Laser Thermal Gradient Treatment

Thin-film solid-state metal dealloying (thin-film SSMD) is a promising method for fabricating nanostructures with controlled morphology and efficiency, offering advantages over conventional bulk materials processing methods for integration into practical applications. Although machine learning (ML) has facilitated the design of dealloying systems, the selection of key thermal treatment parameters for nanostructure formation remains largely unknown and dependent on experimental trial and error. To overcome this challenge, a workflow enabling high-throughput characterization of thermal treatment parameters while probing local nanostructures of thin-film samples is needed. In this work, a laser-based thermal treatment is demonstrated to create temperature gradients on single thin-film samples of Nb-Al/Sc and Nb-Al/Cu. This continuous thermal space enables observation of dealloying transitions and the resulting nanostructures of interest. Through synchrotron X-ray multimodal and high-throughput characterization, critical transitions and nanostructures can be rapidly captured and subsequently verified using electron microscopy. The key temperatures driving chemical reactions and morphological evolutions are clearly identified within this framework. While the oxidation process may contribute to nanostructure formation during thin-film treatment, the dealloying process at the dealloying front involves interactions solely between the dealloying elements, highlighting the availability and viability of the selected systems. This approach enables efficient exploration of the dealloying process and validation of ML predictions, thereby accelerating the discovery of thin-film SSMD systems with targeted nanostructures.

cond-mat.mtrl-sci↗