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Yu-ping Sun

Publications and source records attributed to Yu-ping Sun.

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Effect of Stacking Order on the Electronic State of 1T-TaS$_2$

New theoretical proposals and experimental findings on transition metal dichalcogenide 1T-TaS$_2$ have revived interests in its possible Mott insulating state. We perform a comprehensive scanning tunneling microscopy and spectroscopy experiment on different single-step areas in pristine 1T-TaS$_2$. After accurately determining the relative displacement of Star-of-David super-lattices in two layers, we find different stacking orders can correspond to the similar large-gap spectrum on the upper terrace. When the measurement is performed away from the step edge, the large gap spectrum can always be maintained. The stacking order seems rarely disturb the large-gap spectrum in the ideal bulk material. We conclude that the large insulating gap is from the single-layer property, which is a correlation-induced Mott gap based on the single-band Hubbard model. Specific stacking orders can perturb the state and induce a small-gap or metallic spectrum for a limited area around the step edge, which we attribute to a surface and edge phenomenon. Our work provides more evidence about the surface electronic state and deepens our understanding of the Mott insulating state in 1T-TaS$_2$.

cond-mat.str-el

Reconcile the Bulk Metallic and Surface Insulating state in 1T-TaSe$_2$

The transition metal dichalcogenides 1T-TaS$_2$ and 1T-TaSe$_2$ have been extensively studied for the complicated correlated electronic properties. The origin of different surface electronic states remains controversial. We apply scanning tunneling microscopy and spectroscopy to restudy the surface electronic state of bulk 1T-TaSe$_2$. Both insulating and metallic states are identified in different areas of the same sample. The insulating state is similar to that in 1T-TaS$_2$, concerning both the dI/dV spectrum and the orbital texture. With further investigations in single-step areas, the discrepancy of electronic states is found to be associated with different stacking orders. The insulating state is most possibly a single-layer property, modulated to a metallic state in some particular stacking orders. Both the metallic and large-gap insulating spectra, together with their corresponding stacking orders, are dominant in 1T-TaSe$_2$. The connected metallic areas lead to the metallic transport behavior. We then reconcile the bulk metallic and surface insulating state in 1T-TaSe$_2$. The rich phenomena in 1T-TaSe$_2$ deepen our understanding of the correlated electronic state in bulk 1T-TaSe$_2$ and 1T-TaS$_2$.

cond-mat.str-el