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Yu. A. Litvinov

Publications and source records attributed to Yu. A. Litvinov.

At least 37 records · Page 2Linked to original sources

Exploring isospin-nonconserving effects in the upper $fp$ shell with new mass measurements

Nuclear mass measurements have recently been extended conspicuously to proton-rich region in the upper $fp$ shell. The new data are utilized to study isospin symmetry breaking phenomena}using Coulomb displacement energy (CDE) and triplet displacement energy (TDE) as probes. The new mass data, either measured for the first time or with greatly improved accuracy, removed several previously found ``anomalies" in the systematical behavior in the $fp$ shell. Remarkably, more regular odd-even staggering patterns can be established in both CDE and TDE, calling for a uniform explanation in terms of isospin-nonconserving (INC) forces across the $sd$, $f_{7/2}$, and upper $fp$ shells. By extending the large-scale shell-model calculation [Phys. Rev. Lett. \textbf{110}, 172505 (2013)] to the upper $fp$-shell region, we found that, in order to describe the new data, the same INC force is required as previously used for the $f_{7/2}$ shell. Especially, we propose the $T=1$ TDE for those triplet nuclei, that have $pp$, $nn$, and $pn$ pairs on top of a common even-even $N=Z$ core, to be a good indicator for the isotensor component of isospin violating interactions, which is estimated here to be 150 keV.

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First measurement of the neutron-emission probability with a surrogate reaction in inverse kinematics at a heavy-ion storage ring

Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the 208Pb(p,p') reaction as a surrogate for neutron capture on 207Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of 208Pb. We have used this probability to select different descriptions of the gamma-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of 207Pb at energies for which no experimental data exist.

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Isochronous mass spectrometry at the RIKEN Rare-RI Ring facility

A dedicated isochronous storage ring, named the Rare-RI Ring, was constructed at the RI Beam Factory of RIKEN, aiming at precision mass measurements of nuclei located in uncharted territories of the nuclear chart. The Rare-RI Ring employs the isochronous mass spectrometry technique with the goal to achieve a relative mass precision of $10^{-6}$ within a measurement time of less than 1 ms. The performance of the facility was demonstrated through mass measurements of neutron-rich nuclei with well-known masses. Velocity or magnetic rigidity is measured for every particle prior to its injection into the ring, wherein its revolution time is accurately determined. The latter quantity is used to determine the mass of the particle, while the former one is needed for non-isochronicity corrections. Mass precisions on the order of $10^{-5}$ were achieved in the first commissioning, which demonstrates that Rare-RI Ring is a powerful tool for mass spectrometry of short-lived nuclei.

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Observation and spectroscopy of proton-unbound nucleus $^{21}$Al

We report on the observation of previously-unknown isotope $^{21}$Al, the first unbound aluminum isotope located beyond the proton dripline. The $^{21}$Al nucleus decays by one-proton (1p) emission, and its in-flight decays were detected by tracking trajectories of all decay products with micro-strip silicon detectors. The 1p-emission processes were studied by analyses of the measured angular correlations of decay products $^{20}$Mg+p. The 1p-decay energies of ground and low-lying excited states of $^{21}$Al, its mass excess and proton separation energy value $S_p$=$-1.1(1)$ MeV were determined.

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Neutron radius determination of 133Cs and its impact on the interpretation of CEvNS-CsI measurement

Proton-$^{133}$Cs elastic scattering at low momentum transfer is performed using an in-ring reaction technique at the Cooler Storage Ring at the Heavy Ion Research Facility in Lanzhou. Recoil protons from the elastic collisions between the internal H$_2$-gas target and the circulating $^{133}$Cs ions at 199.4 MeV/u are detected by a silicon-strip detector. The matter radius of $^{133}$Cs is deduced by describing the measured differential cross sections using the Glauber model. Employing the adopted proton distribution radius, a point-neutron radius of 4.86(21) fm for $^{133}$Cs is obtained. With the newly determined neutron radius, the weak mixing angle sin$^2 θ_W$ is independently extracted to be 0.227(28) by fitting the coherent elastic neutrino-nucleus scattering data. Our work limits the sin$^2 θ_W$ value in a range smaller than the ones proposed by the previous independent approaches, and would play an important role in searching new physics via the high precision CE$ν$NS-CsI cross section data in the near future.

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A new approach for deducing rms proton radii from charge-changing reactions of neutron-rich nuclei and the reaction-target dependence

We report the charge-changing cross sections ($σ_{\text{cc}}$) of 24 $p$-shell nuclides on both hydrogen and carbon at about 900$A$ MeV, of which $^{8,9}$Li, $^{10\textendash12}$Be, $^{10,14,15}$B, $^{14,15,17\textendash22}$N and $^{16}$O on hydrogen and $^{8,9}$Li on carbon are for the first time. Benefiting from the data set,we found a new and robust relationship between the scaling factor of the Glauber model calculations and the separation energies of the nuclei of interest on both targets.This allows us to deduce proton radii ($R_p$) for the first time from the cross sections on hydrogen. Nearly identical $R_p$ values are deduced from both target data for the neutron-rich carbon isotopes, however, the $R_p$ from the hydrogen target is systematically smaller in the neutron-rich nitrogen isotopes.This calls for further experimental and theoretical investigations.

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Ground-state mass of $^{22}$Al and test of state-of-the-art \textit{ab initio} calculations

The ground-state mass excess of the $T_{z}=-2$ drip-line nucleus $^{22}$Al is measured for the first time to be $18103(10)$ keV using the newly-developed B$ρ$-defined isochronous mass spectrometry method at the cooler storage ring in Lanzhou. The new mass excess value allowed us to determine the excitation energies of the two low-lying $1^+$ states in $^{22}$Al with significantly reduced uncertainties of 51 keV. Comparing to the analogue states in its mirror nucleus $^{22}$F, the mirror energy differences of the two $1^+$ states in the $^{22}$Al-$^{22}$F mirror pair are determined to be $-625(51)$ keV and $-330(51)$ keV, respectively. The excitation energies and the mirror energy differences are used to test the state-of-the-art \textit{ab initio} valence-space in-medium similarity renormalization group calculations with four sets of interactions derived from the chiral effective field theory. The mechanism leading to the large mirror energy differences is investigated and attributed to the occupation of the $πs_{1/2}$ orbital.

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Measurement of the Isolated Nuclear Two-Photon Decay in $^{72}\mathrm{Ge}$

The nuclear two-photon or double-gamma ($2γ$) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the $2γ$ decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to $\sim100$\,keV and half-lives as short as $\sim10$\,ms. The half-life for the $2γ$ decay of the first-excited $0^+$ state in bare $^{72}\mathrm{Ge}$ ions was determined to be $23.9\left(6\right)$\,ms, which strongly deviates from expectations.

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Isomeric excitation energy for $^{99}$In$^{m}$ from mass spectrometry reveals constant trend next to doubly magic $^{100}$Sn

The excitation energy of the 1/2$^-$ isomer in $^{99}$In at ${N=50}$ is measured to be 671(37) keV and the mass uncertainty of the 9/2$^+$ ground state is significantly reduced using the ISOLTRAP mass spectrometer at ISOLDE/CERN. The measurements exploit a major improvement in the resolution of the multi-reflection time-of-flight mass spectrometer. The results reveal an intriguing constancy of the $1/2^-$ isomer excitation energies in neutron-deficient indium that persists down to the $N = 50$ shell closure, even when all neutrons are removed from the valence shell. This trend is used to test large-scale shell model, \textit{ab initio}, and density functional theory calculations. The models have difficulties describing both the isomer excitation energies and ground-state electromagnetic moments along the indium chain.

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Storage, Accumulation and Deceleration of Secondary Beams for Nuclear Astrophysics

Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.

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Executive Summary of the Topical Program: Nuclear Isomers in the Era of FRIB

We report on the Facility for Rare Isotope Beams (FRIB) Theory Alliance topical program "Nuclear Isomers in the Era of FRIB". We outline the many ways isomers influence and contribute to nuclear science and technology, especially in the four FRIB pillars: properties of rare isotopes, nuclear astrophysics, fundamental symmetries, and applications for the nation and society. We conclude with a resolution stating our recommendation that the nuclear physics community actively pursue isomer research. A white paper is forthcoming.

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$Bρ$-defined isochronous mass spectrometry: a new approach for high-precision mass measurements of short-lived nuclei

A novel technique for broadband high-precision mass measurements of short-lived exotic nuclides is reported. It is based on the isochronous mass spectrometry (IMS) and realizes simultaneous determinations of revolution time and velocity of short-lived stored ions at the cooler storage ring CSRe in Lanzhou. The new technique, named as the $Bρ$-defined IMS or $Bρ$-IMS, boosts the efficiency, sensitivity, and accuracy of mass measurements, and is applied here to measure masses of neutron-deficient $fp$-shell nuclides. In a single accelerator setting, masses of $^{46}$Cr, $^{50}$Fe and $^{54}$Ni are determined with relative uncertainties of (5~-~6)$\times10^{-8}$, thereby improving the input data for testing the unitarity of the Cabibbo-Kobayashi-Maskawa quark mixing matrix. This is the technique of choice for future high-precision measurements of the most rarely produced shortest-lived nuclides.

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$Bρ$-defined Isochronous Mass Spectrometry and Mass Measurements of $^{58}$Ni Fragments

A novel isochronous mass spectrometry, termed as $Bρ$-defined IMS, is established at the experimental cooler-storage ring CSRe in Lanzhou. Its potential has been studied through high precision mass measurements of $^{58}$Ni projectile fragments. Two time-of-flight detectors were installed in one of the straight sections of CSRe, thus enabling simultaneous measurements of the velocity and the revolution time of each stored short-lived ion. This allows for calculating the magnetic rigidity $Bρ$ and the orbit length $C$ of each ion. The accurate $Bρ(C)$ function has been constructed, which is a universal calibration curve used to deduce the masses of the stored nuclides. The sensitivity to single stored ions, quickness, and background-free characteristics of the method are ideally suited to address nuclides with very short lifetimes and tiniest production yields. In the limiting case of just a single particle, the attained mass resolving power allows one us to determine its mass-over-charge ratio $m/q$ with a remarkable precision of merely $\sim5$ keV. Masses of $T_z = -3/2$ fp-shell nuclides are re-determined with high accuracy, and the validity of the isospin multiplet mass equation is tested up to the heaviest isospin quartet with $A = 55$. The new masses are also used to investigate the mirror symmetry of empirical residual proton-neutron interactions.

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Proton distribution radii of $^{16-24}$O: signatures of new shell closures and neutron skin

The root mean square radii of the proton density distribution in $^{16-24}$O derived from measurements of charge changing cross sections with a carbon target at $\sim$900$A$ MeV together with the matter radii portray thick neutron skin for $^{22 - 24}$O despite $^{22,24}$O being doubly magic. Imprints of the shell closures at $N$ = 14 and 16 are reflected in local minima of their proton radii that provide evidence for the tensor interaction causing them. The radii agree with it ab initio calculations employing the chiral NNLO$_{\mathrm{sat}}$ interaction, though skin thickness predictions are challenged. Shell model predictions agree well with the data.

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Systematic study of Δ(1232) resonance excitations using single isobaric charge-exchange reactions induced by medium-mass projectiles of Sn

The fragment separator FRS has been for the first time used to measure the (n,p) and (p,n)-type isobaric charge-exchange cross sections of stable 112,124Sn isotopes accelerated at 1A GeV with an uncertainty of 3% and to separate quasi-elastic and inelastic components in the missing-energy spectra of the ejectiles. The inelastic contribution can be associated to the excitation of isobar Δ(1232) resonances and to the pion emission in s-wave, both in the target and projectile nuclei, while the quasi-elastic contribution is associated to the nuclear spin-isospin response of nucleon-hole excitations. The data lead to interesting results where we observe a clear quenching of the quasi-elastic component and their comparisons to theoretical calculations demonstrate that the baryonic resonances can be excited in the target and projectile nuclei. To go further in this investigation, we propose to study the excitation of baryonic resonances taking advantage of the combination of high-resolving power magnetic spectrometers with the WASA calorimeter. These new measurements will allow us to determine the momenta of the ejectiles and pions emitted in coincidence after the single isobaric charge-exchange collisions, providing us unique opportunities to study the evolution of the baryonic resonance dynamics with the neutron-proton asymmetry through the use of exotic radioactive ion beams.

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First application of mass measurement with the Rare-RI Ring reveals the solar r-process abundance trend at A=122 and A=123

The Rare-RI Ring (R3) is a recently commissioned cyclotron-like storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory (RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF, $^{127}$Sn, $^{126}$In, $^{125}$Cd, $^{124}$Ag, $^{123}$Pd, were injected in R3. Masses of $^{126}$In, $^{125}$Cd, and $^{123}$Pd were measured whereby the mass uncertainty of $^{123}$Pd was improved. This is the first reported measurement with a new storage ring mass spectrometery technique realized at a heavy-ion cyclotron and employing individual injection of the pre-identified rare nuclei. The latter is essential for the future mass measurements of the rarest isotopes produced at RIBF. The impact of the new $^{123}$Pd result on the solar $r$-process abundances in a neutron star merger event is investigated by performing reaction network calculations of 20 trajectories with varying electron fraction $Y_e$. It is found that the neutron capture cross section on $^{123}$Pd increases by a factor of 2.2 and $β$-delayed neutron emission probability, $P_\mathrm{1n}$, of $^{123}$Rh increases by 14\%. The neutron capture cross section on $^{122}$Pd decreases by a factor of 2.6 leading to pileup of material at $A=122$, thus reproducing the trend of the solar $r$-process abundances. The trend of the two-neutron separation energies (S$_\mathrm{2n}$) was investigated for the Pd isotopic chain. The new mass measurement with improved uncertainty excludes large changes of the S$_\mathrm{2n}$ value at $N=77$. Such large increase of the S$_\mathrm{2n}$ values before $N=82$ was proposed as an alternative to the quenching of the $N=82$ shell gap to reproduce $r$-process abundances in the mass region of $A=112-124$.

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Single and double $K$-shell vacancy production in slow Xe$^\textrm{54+,53+}$-Xe collisions

We present an experimental and theoretical study of symmetric $\textrm{Xe}^{54+}+\textrm{Xe}$ collisions at 50, 30, and 15 MeV/u, corresponding to strong perturbations with $v_K/v_\text{p}$ = 1.20, 1.55, and 2.20, respectively ($v_K$: classical $K$-shell orbital velocity, $v_\text{p}$: projectile velocity), as well as $\textrm{Xe}^{53+}+\textrm{Xe}$ collisions at 15 MeV/u. For each of these systems, x-ray spectra were measured under a forward angle of $35^\circ$ with respect to the projectile beam. Target satellite and hypersatellite radiation, $Kα_{2,1}^\mathrm{s}$ and $Kα_{2,1}^\mathrm{hs}$, respectively, were analyzed and used to derive cross section ratios for double-to-single target $K$-shell vacancy production. We compare our experimental results to relativistic time-dependent two-center calculations.

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Charge resolution in the isochronous mass spectrometry and the mass of $^{51}$Co

Isochronous mass spectrometry (IMS) of heavyion storage rings is a powerful tool for the mass measurements of short-lived nuclei. In IMS experiments, masses are determined through precision measurements of the revolution times of the ions stored in the ring. However, the revolution times cannot be resolved for particles with nearly the same mass-to-charge (m/q) ratios. To overcome this limitation and to extract the accurate revolution times for such pairs of ion species with very close m/q ratios, in our early work on particle identification, we analyzed the amplitudes of the timing signals from the detector based on the emission of secondary electrons. Here, the previous data analysis method is further improved by considering the signal amplitudes, detection efficiencies, and number of stored ions in the ring. A sensitive Z-dependent parameter is introduced in the data analysis, leading to a better resolution of $^{34}$Ar$^{18+}$ and $^{51}$Co$^{27+}$ with A/Z=17/9. The mean revolution times of $^{34}$Ar$^{18+}$ and $^{51}$Co$^{27+}$ are deduced, although their time difference is merely 1.8 ps. The uncorrected, overlapped peak of these ions has a full width at half maximum of 7.7 ps. The mass excess of $^{51}$Co was determined to be -27332(41) keV, which is in agreement with the previous value of -27342(48) keV.

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