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Yu. A. Litvinov

Publications and source records attributed to Yu. A. Litvinov.

At least 91 records · Page 5Linked to original sources

A method to measure the transition energy $γ_{t}$ of the isochronously tuned storage ring

The Isochronous Mass Spectrometry (IMS) is a powerful technique developed in heavy-ion storage rings for measuring masses of very short-lived exotic nuclei. The IMS is based on the isochronous setting of the ring. One of the main parameters of this setting is the transition energy $γ_{t}$. %The transition energy $γ_{t}$ plays an important role in the isochronous mass spectrometry (IMS). It has been a challenge to determine the $γ_{t}$ and especially to monitor the variation of $γ_{t}$ during experiments. In this paper we introduce a method to measure the $γ_{t}$ online during IMS experiments by using the acquired experimental data. Furthermore, since the storage ring has (in our context) a relatively large momentum acceptance, the variation of the $γ_{t}$ across the ring acceptance is a source of systematic uncertainty of measured masses. With the installation of two time-of-flight (TOF) detectors, the velocity of each stored ion and its revolution time are simultaneously available for the analysis. These quantities enabled us to determine the $γ_{t}$ as a function of orbital length in the ring. The presented method is especially important for future IMS experiments planned at the new-generation storage ring facilities FAIR in Germany and HIAF in China.

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Isochronous mass measurements of $T_z=-1$ $fp$-shell nuclei from projectile fragmentation of $^{58}$Ni

Atomic masses of seven $T_z=-1$, $fp$-shell nuclei from $^{44}$V to $^{56}$Cu and two low-lying isomers, $^{44m}$V ($J^π=6^+$) and $^{52m}$Co ($J^π=2^+$), have been measured with relative precisions of $1-4\times 10^{-7}$ with Isochronous Mass Spectrometry (IMS) at CSRe. The masses of $^{56}$Cu, $^{52g,52m}$Co, and $^{44m}$V were measured for the first time in this experiment. The Mass Excesses ($ME^{\prime}$s) of $^{44}$V, $^{48}$Mn, $^{50}$Fe, and $^{54}$Ni are determined with an order of magnitude improved precision compared to the literature values. $^{52g,52m}$Co and $^{56}$Cu are found to be $370$~keV and $400$~keV more bound, respectively, while $^{44g,44m}$V are $\sim 300$~keV less bound than the extrapolations in the Atomic-Mass Evaluation 2012 (AME$^{\prime}$12). The masses of the four $T_z=-1/2$ nuclei $^{45}$V, $^{47}$Cr, $^{49}$Mn, and $^{51}$Fe are re-determined to be in agreement, within the experimental errors, with the recent JYFLTRAP measurements or with the previous IMS measurements in CSRe. Details of the measurements and data analysis are described, and the impact of the new $ME$ values on different aspects in nuclear structure are investigated and discussed.

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Deep excursion beyond the proton dripline. I. Argon and chlorine isotope chains

The proton-unbound argon and chlorine isotopes have been studied by measuring trajectories of their decay-in-flight products by using a tracking technique with micro-strip detectors. The proton ($1p$) and two-proton ($2p$) emission processes have been detected in the measured angular correlations "heavy-fragment"+$p$ and "heavy-fragment"+$p$+$p$, respectively. The ground states of the previously unknown isotopes $^{30}$Cl and $^{28}$Cl have been observed for the first time, providing the $1p$-separation energies $S_p$ of $-0.48(2)$ and $-1.60(8)$ MeV, respectively. The relevant systematics of $1p$ and $2p$ separations energies have been studied theoretically in the core+$p$ and core+$p$+$p$ cluster models. The first-time observed excited states of $^{31}$Ar allow to infer the $2p$-separation energy $S_{2p}$ of 6(34) keV for its ground state. The first-time observed state in $^{29}$Ar with $S_{2p} = -5.50(18)$ MeV can be identified either as a ground or an excited state according to different systematics.

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Deep excursion beyond the proton dripline. II. Toward the limits of existence of nuclear structure

Prospects of experimental studies of argon and chlorine isotopes located far beyond the proton dripline are studied by using systematics and cluster models. The deviations from the widespread systematics observed in $^{28,29}$Cl and $^{29,30}$Ar have been theoretically substantiated, and analogous deviations predicted for the lighter chlorine and argon isotopes. The limits of nuclear structure existence are predicted for Ar and Cl isotopic chains, with $^{26}$Ar and $^{25}$Cl found to be the lightest sufficiently long-living nuclear systems. By simultaneous measurements of protons and $γ$-rays following decays of such systems as well as their $β$-delayed emission, an interesting synergy effect may be achieved, which is demonstrated by the example of $^{30}$Cl and $^{31}$Ar ground state studies. Such synergy effect may be provided by the new EXPERT setup (EXotic Particle Emission and Radioactivity by Tracking), being operated inside the fragment separator and spectrometer facility at GSI, Darmstadt.

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The Masses of the $T_z=-3/2$ Nuclei $^{27}$P and $^{29}$S

Isochronous mass spectrometry has been applied in the storage ring CSRe to measure the masses of the $T_z=-3/2$ nuclei $^{27}$P and $^{29}$S. The new mass excess value $ME$($^{29}$S) $=-3094(13)$~keV is 66(52)~keV larger than the result of the previous $^{32}$S($^3$He,$^{6}$He)$^{29}$S reaction measurement in 1973 and a factor of 3.8 more precise. The new result for $^{29}$S, together with those of the $T=3/2$ isobaric analog states (IAS) in $^{29}$P, $^{29}$Si, and $^{29}$Al, fit well into the quadratic form of the Isobaric Multiplet Mass Equation IMME. The mass excess of $^{27}$P has been remeasured to be $ME(^{27}$P$)=-685(42)$ keV. By analyzing the linear and quadratic coefficients of the IMME in the $T_z=-3/2$ $sd$-shell nuclei, it was found that the ratio of the Coulomb radius parameters is $R\approx0.96$ and is nearly the same for all $T=3/2$ isospin multiplets. Such a nearly constant $R$-value, apparently valid for the entire light mass region with $A>9$, can be used to set stringent constraints on the isovector and isotensor components of the isospin non-conserving forces in theoretical calculations.

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First application of combined isochronous and Schottky mass spectrometry: Half-lives of fully ionized 49Cr24+ and 53Fe26+ atoms

Lifetime measurements of b -decaying highly charged ions have been performed in the storage ring CSRe by applying the isochronous Schottky mass spectrometry. The fully ionized 49Cr and 53Fe ions were produced in projectile fragmentation of 58Ni primary beam and were stored in the CSRe tuned into the isochronous ion-optical mode. The new resonant Schottky detector was applied to monitor the intensities of stored uncooled 49Cr24+ and 53Fe26+ ions. The extracted half-lives T1/2(49Cr24+) = 44.0(27) min and T1/2(53Fe26+) = 8.47(19) min are in excellent agreement with the literature half-life values corrected for the disabled electron capture branchings. This is an important proof-of-principle step towards realizing the simultaneous mass and lifetime measurements on exotic nuclei at the future storage ring facilities.

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Mass Measurements of Neutron-Deficient Y, Zr, and Nb Isotopes and Their Impact on $rp$ and $νp$ Nucleosynthesis Processes

Using isochronous mass spectrometry at the experimental storage ring CSRe in Lanzhou, the masses of $^{82}$Zr and $^{84}$Nb were measured for the first time with an uncertainty of $\sim 10$ keV, and the masses of $^{79}$Y, $^{81}$Zr, and $^{83}$Nb were re-determined with a higher precision. %The latter differ significantly from their literature values. The latter are significantly less bound than their literature values. Our new and accurate masses remove the irregularities of the mass surface in this region of the nuclear chart. Our results do not support the predicted island of pronounced low $α$ separation energies for neutron-deficient Mo and Tc isotopes, making the formation of Zr-Nb cycle in the $rp$-process unlikely. The new proton separation energy of $^{83}$Nb was determined to be 490(400)~keV smaller than that in the Atomic Mass Evaluation 2012. This partly removes the overproduction of the $p$-nucleus $^{84}$Sr relative to the neutron-deficient molybdenum isotopes in the previous $νp$-process simulations.

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Halo structure of $^8$B determined from intermediate energy proton elastic scattering in inverse kinematics

The absolute differential cross section for small-angle proton elastic scattering on the proton-rich $^8$B nucleus has been measured in inverse kinematics for the first time. The experiment was performed using a secondary radioactive beam with an energy of 0.7 GeV/u at GSI, Darmstadt. The active target, namely hydrogen-filled time projection ionization chamber IKAR, was used to measure the energy, angle and vertex point of the recoil protons. The scattering angle of the projectiles was simultaneously determined by the tracking detectors. The measured differential cross section is analyzed on the basis of the Glauber multiple scattering theory using phenomenological nuclear-density distributions with two free parameters. The radial density distribution deduced for $^8$B exhibits a halo structure with the root-mean-square (rms) matter radius $R_{\rm m} = 2.58 (6)$ fm and the rms halo radius $R_{\rm h} = 4.24 (25)$ fm. The results on $^8$B are compared to those on the mirror nucleus $^8$Li investigated earlier by the same method. A comparison is also made with previous experimental results and theoretical predictions for both nuclei.

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Spectroscopy of excited states of unbound nuclei $^{30}$Ar and $^{29}$Cl

Several states of proton-unbound isotopes $^{30}$Ar and $^{29}$Cl were investigated by measuring their in-flight decay products, $^{28}$S+proton+proton and $^{28}$S+proton, respectively. A refined analysis of $^{28}$S-proton angular correlations indicates that the ground state of $^{30}$Ar is located at $2.45^{+0.05}_{-0.10}$ MeV above the two-proton emission threshold. The theoretical investigation of the $^{30}$Ar ground state decay demonstrates that its mechanism has the transition dynamics with a surprisingly strong sensitivity of the correlation patterns of the decay products to the two-proton decay energy of the $^{30}$Ar ground state and the one-proton decay energy as well as the one-proton decay width of the $^{29}$Cl ground state. The comparison of the experimental $^{28}$S-proton angular correlations with those resulting from Monte Carlo simulations of the detector response illustrates that other observed $^{30}$Ar excited states decay by sequential emission of protons via intermediate resonances in $^{29}$Cl. Based on the findings, the decay schemes of the observed states in $^{30}$Ar and $^{29}$Cl were constructed. For calibration purposes and for checking the performance of the experimental setup, decays of the previously-known states of a two-proton emitter $^{19}$Mg were remeasured. Evidences for one new excited state in $^{19}$Mg and two unknown states in $^{18}$Na were found.

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$β$-decay half-lives and $β$-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb and Bi, beyond N=126

$Background:$ Previous measurements of $β$-delayed neutron emitters comprise around 230 nuclei, spanning from the $^{8}$He up to $^{150}$La. Apart from $^{210}$Tl, with a minuscule branching ratio of 0.007\%, no other neutron emitter is measured yet beyond $A=150$. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at $A\sim195$. $Purpose:$ To measure both, $β$-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond $N=126$. $Method:$ Ions of interest are produced by fragmentation of a $^{238}$U beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) is used to measure ion-implants and $β$-decays. An array of 30 $^3$He tubes embedded in a polyethylene matrix (BELEN) is used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time-correlations. The latter are analyzed with an analytical model and results for the half-lives and neutron-branching ratios are derived using the binned Maximum-Likelihood method. $Results:$ Twenty new $β$-decay half-lives are reported for $^{204-206}$Au, $^{208-211}$Hg,$^{211-216}$Tl,$^{215-218}$Pb and $^{218-220}$Bi, nine of them for the first time. Neutron emission probabilities are reported for $^{210,211}$Hg and $^{211-216}$Tl. $Conclusions:$ The new $β$-decay half-lives are in good agreement with previous measurements in this region. The measured neutron emission probabilities are comparable or smaller than values predicted by global models like RHB+RQRPA.

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Identification of the Lowest $T=2$, $J^{π=}0^+$ Isobaric Analog State in $^{52}$Co and Its Impact on the Understanding of $β$-Decay Properties of $^{52}$Ni

Masses of $^{52g,52m}$Co were measured for the first time with an accuracy of $\sim 10$ keV, an unprecedented precision reached for short-lived nuclei in the isochronous mass spectrometry. Combining our results with the previous $β$-$γ$ measurements of $^{52}$Ni, the $T=2$, $J^π=0^+$ isobaric analog state (IAS) in $^{52}$Co was newly assigned, questioning the conventional identification of IASs from the $β$-delayed proton emissions. Using our energy of the IAS in $^{52}$Co, the masses of the $T=2$ multiplet fit well into the Isobaric Multiplet Mass Equation. We find that the IAS in $^{52}$Co decays predominantly via $γ$ transitions while the proton emission is negligibly small. According to our large-scale shell model calculations, this phenomenon has been interpreted to be due to very low isospin mixing in the IAS.

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Proton distribution radii of $^{12-19}$C illuminate features of neutron halos

Proton radii of $^{12-19}$C densities derived from first accurate charge changing cross section measurements at 900$A$ MeV with a carbon target are reported. A thick neutron surface evolves from $\sim$ 0.5 fm in $^{15}$C to $\sim$ 1 fm in $^{19}$C. The halo radius in $^{19}$C is found to be 6.4$\pm$0.7 fm as large as $^{11}$Li. Ab initio calculations based on chiral nucleon-nucleon and three-nucleon forces reproduce well the radii.

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Observation of Large Enhancement of Charge Exchange Cross Sections with Neutron-Rich Carbon Isotopes

Production cross sections of nitrogen isotopes from high-energy carbon isotopes on hydrogen and carbon targets have been measured for the first time for a wide range of isotopes. The fragment separator FRS at GSI was used to deliver C isotope beams. The cross sections of the production of N isotopes were determined by charge measurements of forward going fragments. The cross sections show a rapid increase with the number of neutrons in the projectile. Since the production of nitrogen is mostly due to charge exchange reactions below the proton separation energies, the present data suggests a concentration of Gamow-Teller and Fermi transition strength at low excitation energies for neutron-rich isotopes. It was also observed that the cross sections were enhanced much more strongly for neutron rich isotopes in the C-target data.

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An improvement of isochronous mass spectrometry: Velocity measurements using two time-of-flight detectors

Isochronous mass spectrometry (IMS) in storage rings is a powerful tool for mass measurements of exotic nuclei with very short half-lives down to several tens of microseconds, using a multicomponent secondary beam separated in-flight without cooling. However, the inevitable momentum spread of secondary ions limits the precision of nuclear masses determined by using IMS. Therefore, the momentum measurement in addition to the revolution period of stored ions is crucial to reduce the influence of the momentum spread on the standard deviation of the revolution period, which would lead to a much improved mass resolving power of IMS. One of the proposals to upgrade IMS is that the velocity of secondary ions could be directly measured by using two time-of-flight (double TOF) detectors installed in a straight section of a storage ring. In this paper, we outline the principle of IMS with double TOF detectors and the method to correct the momentum spread of stored ions.

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Precision Mass Measurements of 129-131Cd and Their Impact on Stellar Nucleosynthesis via the Rapid Neutron Capture Process

Masses adjacent to the classical waiting-point nuclide 130Cd have been measured by using the Penning- trap spectrometer ISOLTRAP at ISOLDE/CERN. We find a significant deviation of over 400 keV from earlier values evaluated by using nuclear beta-decay data. The new measurements show the reduction of the N = 82 shell gap below the doubly magic 132Sn. The nucleosynthesis associated with the ejected wind from type-II supernovae as well as from compact object binary mergers is studied, by using state-of-the-art hydrodynamic simulations. We find a consistent and direct impact of the newly measured masses on the calculated abundances in the A = 128 - 132 region and a reduction of the uncertainties from the precision mass input data.

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Toward precision mass measurements of neutron-rich nuclei relevant to $r$-process nucleosynthesis

The open question of where, when, and how the heavy elements beyond iron enrich our Universe has triggered a new era in nuclear physics studies.\ Of all the relevant nuclear physics inputs, the mass of very neutron-rich nuclides is a key quantity for revealing the origin of heavy elements beyond iron.\ Although the precise determination of this property is a great challenge, enormous progress has been made in recent decades, and it has contributed significantly to both nuclear structure and astrophysical nucleosynthesis studies.\ In this review, we first survey our present knowledge of the nuclear mass surface, emphasizing the importance of nuclear mass precision in $r$-process calculations.\ We then discuss recent progress in various methods of nuclear mass measurement with a few selected examples.\ For each method, we focus on recent breakthroughs and discuss possible ways of improving the weighing of $r$-process nuclides.

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Conceptual design of elliptical cavities for intensity and position sensitive beam measurements in storage rings

Position sensitive beam monitors are indispensable for the beam diagnostics in storage rings. Apart from their applications in the measurements of beam parameters, they can be used in non-destructive in-ring decay studies of radioactive ion beams as well as enhancing precision in the isochronous mass measurement technique. In this work, we introduce a novel approach based on cavities with elliptical cross-section, in order to compensate for existing limitations in ion storage rings. The design is aimed primarily for future heavy ion storage rings of the FAIR project. The conceptual design is discussed together with simulation results.

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\b{eta}-delayed three-proton decay of 31Ar

The beta decay of 31Ar, produced by fragmentation of a 36Ar beam at 880 MeV/nucleon, was investigated. Identified ions of 31Ar were stopped in a gaseous time projection chamber with optical readout allowing to record decay events with emission of protons. In addition to \b{eta}-delayed emission of one and two protons we have clearly observed the beta-delayed three-proton branch. The branching ratio for this channel in 31Ar is found to be 0.07(2)%.

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