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Yuanhong Teng

Publications and source records attributed to Yuanhong Teng.

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Oxygen-vacancy quantum spin defects in silicon carbide

Optically addressable spin defects in wide-bandgap semiconductors are promising building blocks for quantum sensing and quantum networks. Establishing their atomic structure is essential for understanding functionality and enabling controlled engineering. In 4H-SiC, the PL5 and PL6 centers have long been recognized for their exceptional charge stability and room-temperature optically detected magnetic resonance (ODMR) performance, but their structural origin has remained elusive for over a decade. Here, we provide direct evidence for their oxygen-vacancy (${\rm O_C V_{Si}}$) origins through a combined chemical and isotopic control strategy. Under oxygen ion implantation, we observe over tenfold enhancement in the yield of PL5 and PL6 compared to nitrogen ion implantation. Furthermore, implantation with $^{17}{\rm O}$ ions produces PL5 and PL6 defects that exhibit a characteristic six-fold $^{17}{\rm O}$ hyperfine splitting in their ODMR spectra. These results affirm PL6 as the ${\rm O_C V_{Si}}$ defect in the $hh$ configuration. For PL5, the oxygen-related evidence, together with \textit{ab initio} calculations and additional measurements of the zero-field splitting and hyperfine structure, establishes it as the ${\rm O_C V_{Si}}$ defect in the $kh$ configuration. This unambiguous structural identification, achieved through materials-level chemical control, provides the microscopic foundation for deterministic engineering of these defects, paving the way for scalable photonic devices and high-sensitivity ensemble quantum sensors based on oxygen-vacancy centers.

cond-mat.mtrl-sci

Quantum Noise Spectroscopy of Nanoscale Charge Defects in Silicon Carbide at Room Temperature

The nanoscale charge environment critically influences semiconductor physics and device performance. While conventional bulk characterization techniques provide volume-averaged defect properties, they lack the spatial resolution to resolve nanoscale charge heterogeneity and identify microscopic noise sources. Here, we utilize single PL5 centers in 4H-SiC as room-temperature broadband quantum sensors to fill in the gap. We report the first real-time, nanoscale observation of singlecharge tunneling dynamics in a commercial semiconductor at room temperature, by monitoring the random telegraph noise using optically detected magnetic resonance (ODMR). This capability enables an electrical noise imaging technique, showing distinct noise variations across different wafer substrates. By employing dynamical decoupling, we extend noise spectroscopy from near-DC to MHz frequencies, uncovering significant noise spectral density correlations across frequency bands. Finally, we probe MHz-GHz noise and identify its origin via T1 relaxation spectroscopy, obtaining the first nanoscale electron paramagnetic resonance (EPR) spectroscopic fingerprint of charge defects in SiC. These techniques open avenues for characterizing noise environments in semiconductor devices, providing critical insights for optimizing SiC fabrication processes, defect control, and advancing quantum technologies.

quant-ph

Single-molecule Scale Nuclear Magnetic Resonance Spectroscopy using a Robust Near-Infrared Spin Sensor

Nuclear magnetic resonance (NMR) at the single-molecule level with atomic resolution holds transformative potential for structural biology and surface chemistry. Near-surface solid-state spin sensors with optical readout ability offer a promising pathway toward this goal. However, their extreme proximity to target molecules demands exceptional robustness against surface-induced perturbations. Furthermore, life science applications require these sensors to operate in biocompatible spectral ranges that minimize photodamage. In this work, we demonstrate that the PL6 quantum defect in 4H silicon carbide (4H-SiC) can serve as a robust near-infrared spin sensor. This sensor operates at tissue-transparent wavelengths and exhibits exceptional near-surface stability even at depth of 2 nm. Using shallow PL6 centers, we achieve nanoscale NMR detection of proton ($\mathrm{^{1}H}$) spins in immersion oil and fluorine ($\mathrm{^{19}F}$) spins in Fomblin, attaining a detection volume of $\mathrm{(3~nm)^3}$ and a sensitivity reaching the requirement for single-proton spin detection. This work establishes 4H-SiC quantum sensors as a compelling platform for nanoscale magnetic resonance, with promising applications in probing low-dimensional water phases, protein folding dynamics, and molecular interactions.

quant-ph

Varying primordial state fractions in exo- and endothermic SIDM simulations of Milky Way-mass haloes

Self-interacting dark matter (SIDM) is increasingly studied as a potential solution to small-scale discrepancies between simulations of cold dark matter (CDM) and observations. We examine a physically motivated two-state SIDM model with both elastic and inelastic scatterings. In particular, endothermic, exothermic, and elastic scattering occur with equal probability at high relative velocities ($v_{\rm rel}\gtrsim400~{\rm km/s})$. In a suite of cosmological zoom-in simulation of Milky Way-size haloes, we vary the primordial state fractions to understand the impact of inelastic dark matter self-interactions on halo structure and evolution. In particular, we test how the initial conditions impact the present-day properties of dark matter haloes. Depending on the primordial state fraction, scattering reactions will be dominated by either exothermic or endothermic effects for high and low initial excited state fractions respectively. We find that increasing the initial excited fraction reduces the mass of the main halo, as well as the number of subhaloes on all mass scales. The main haloes are cored, with lower inner densities and higher outer densities compared with CDM. Additionally, we find that the shape of the main halo becomes more spherical the higher the initial excited state fraction is. Finally, we show that the number of satellites steadily decreases with initial excited state fraction across all satellite masses.

astro-ph.CO