arXiv subjects

Yuanji Li

Publications and source records attributed to Yuanji Li.

10 recordsLinked to original sources

arXiv2026

Magnetic-field-tunable commensurate multi-q charge orders on UTe2 (011) surface

The heavy-fermion superconductor UTe2 has attracted intense interest as a candidate for spin-triplet pairing. Recent scanning tunneling microscopy (STM) studies have reported complex charge orders (COs) on its (011) surface, but their origin and relationship with superconductivity remain controversial. Here, by performing temperature-, magnetic field-, and sample-dependent STM measurements, we identify multiple new CO wave vectors beyond those previously reported. All these CO wave vectors are strictly locked to integer multiples of 1/14 and 1/4 of the reciprocal lattice vectors of the UTe2 (011) surface, and multiple of them coexist in real space, collectively revealing a family of field-tunable, commensurate multi-q COs. These COs exist within an energy range much larger than the superconducting energy scale, their emergence suppresses the density of states near EF, yet show negligible coupling to bulk superconductivity and magnetic vortices. Our findings strongly disfavor the Fermi surface nesting or primary pair-density-wave pictures, but are consistent with a surface parent spin order.

cond-mat.supr-con↗

arXiv2026

Distinguishing impurity-induced bound states from Majorana-like zero-energy peaks in strained CsCa2Fe4As4F2 by scanning tunneling microscopy

Iron-based superconductors offer a versatile platform for exploring topological superconductivity and Majorana zero modes (MZMs), with experimental confirmations in Fe(Te,Se), (Li,Fe)OHFeSe and CaKFe4As4 at ambient pressure, as well as in LiFeAs under local strain. The related properties in other iron-based superconductors still need to be explored, especially under the application of local strain. In this study, we conduct scanning tunneling microscopy/spectroscopy measurements on CsCa2Fe4As4F2 crystals under unidirectional local strain. A fully developed superconducting gap with multiple pairs of coherence peaks are observed, and the gap sizes can be significantly modulated by local strain. Spectroscopic measurements on various types of defects including the nonmagnetic Cs-site vacancies consistently reveal pair-breaking effects. These phenomena support a fully gapped multiband superconductivity scenario with sign-changing. Notably, a sharp zero-energy conductance peak (ZECP) is universally observed on a particular type of defects by using a metallic tip, resembling the MZMs observed at interstitial Fe atoms in Fe(Te,Se) [Nat. Phys. 11, 543 (2015)]. However, by using a superconducting tip to enhance energy resolution as well as by studying the ZECP evolution as functions of magnetic field and tunneling transmissivity, we demonstrate that the ZECP originates from nearly degenerate Yu-Shiba-Rusinov states rather than MZMs. Our study not only provides more insights into the superconducting pairing symmetry of CsCa2Fe4As4F2, but also establishes systematic experimental methods for identifying weak impurity state signals and discerning the physical origins of ZECPs.

cond-mat.supr-con↗

arXiv2026

Scanning tunneling microscopy study of helimagnetic monolayer CrBr2 on s-wave superconductor NbSe2: a topologically trivial system due to weak interfacial coupling

Hybrid magnet-superconductor heterostructures attract significant interest for their potential to host unconventional superconductivity, topological superconductivity, and Majorana physics. Transition metal dihalides (MX2, M = transition metal, X = Cl, Br, I) are compelling magnetic candidates due to their novel magnetic structures and possible ferroelectricity. Here, we employ low-temperature scanning tunneling microscopy/spectroscopy to investigate the interfaces fabricated by growing helimagnet candidate CrBr2 on s-wave superconductor NbSe2. Our results reveal that the monolayer CrBr2 is insulating, the measured low-energy electronic states on it derive entirely from the NbSe2 substrate. The superconducting properties of CrBr2/NbSe2 are nearly identical to the bare NbSe2, manifested by the superconducting gap spectra and their temperature and magnetic field dependence, as well as the spatial distribution and bound states of magnetic vortices. Furthermore, in-gap excitations appear only at the dirty edges of CrBr2 islands and are absent from clean edges, suggesting the lack of intrinsic edge states. Taken together, these findings establish the topologically trivial nature of the helimagnetic insulator/s-wave superconductor system CrBr2/NbSe2, attributable to the absence of interfacial superconducting proximity and weak magnetic coupling.

cond-mat.supr-con↗

arXiv2025

Yin-Yang vortex on UTe2 (011) surface

UTe2 is a promising candidate for spin-triplet superconductor, yet its exact superconducting order parameter remains highly debated. Here, via scanning tunneling microscopy/spectroscopy, we observe a novel type of magnetic vortex with distinct dark-bright contrast in local density of states on UTe2 (011) surface under a perpendicular magnetic field, resembling the conjugate structure of Yin-Yang diagram in Taoism. Each Yin-Yang vortex contains a quantized magnetic flux, and the boundary between the Yin and Yang parts aligns with the crystallographic a-axis of UTe2. The vortex states exhibit intriguing behaviors -- a sharp zero-energy conductance peak exists at the Yang part, while a superconducting gap with pronounced coherence peaks exists at the Yin part, which is even sharper than those measured far from the vortex core or in the absence of magnetic field. By theoretical modeling, we show that the Yin-Yang vortices on UTe2 (011) surface can be explained by the asymmetric vortex-derived local distortion of the zero-energy surface states associated with spin-triplet pairing with appropriate d-vectors. Therefore, the observation of Yin-Yang vortex confirms the spin-triplet pairing in UTe2 and imposes constraints on the candidate d-vector for the spin-triplet pairing.

cond-mat.supr-con↗

arXiv2025

Direct Visualization of an Incommensurate Unidirectional Charge Density Wave in La$_4$Ni$_3$O$_{10}$

Superconductivity emerges in both La$_3$Ni$_2$O$_7$ and La$_4$Ni$_3$O$_{10}$ under high pressure by suppressing their density-wave transitions, but critical temperature (Tc) differs significantly between these two compounds. To gain deeper insights into the distinct superconducting states, it is essential to unravel the nature of the density-wave states at ambient pressure, a topic that remains largely unexplored. Here, using scanning tunneling microscopy/spectroscopy (STM/STS), we report the direct visualization of an incommensurate unidirectional charge density wave (CDW) in La$_4$Ni$_3$O$_{10}$ in real space. The density of states (DOS) is strongly depleted near $E_F$, indicating the opening of a CDW gap of $2{\Delta} \approx 71$ meV, which is unfavorable for the formation of superconductivity at ambient pressure. We propose that the CDW arises from Fermi surface nesting, and is likely a subsidiary phase of a spin density wave. Compared to La$_3$Ni$_2$O$_7$, the weaker electronic correlation in La$_4$Ni$_3$O$_{10}$ is likely one reason for the lower $T_c$.

cond-mat.supr-con↗

arXiv2024

Observation of Yu-Shiba-Rusinov-like states at the edge of CrBr3/NbSe2 heterostructure

The hybrid ferromagnet-superconductor heterostructures have attracted extensive attention as they potentially host topological superconductivity. Relevant experimental signatures have recently been reported in CrBr3/NbSe2 ferromagnet-superconductor heterostructure, but controversies remain. Here, we reinvestigate CrBr3/NbSe2 by an ultralow temperature scanning tunneling microscope with higher spatial and energy resolutions. We find that the single-layer CrBr3 film is insulating and acts likely as a vacuum barrier, the measured superconducting gap and vortex state on it are nearly the same as those of NbSe2 substrate. Meanwhile, in-gap features are observed at the edges of CrBr3 island, which display either a zero-energy conductance peak or a pair of particle-hole symmetric bound states. They are discretely distributed at the edges of CrBr3 film, and their appearance is found closely related to the atomic lattice reconstruction near the edges. By increasing tunneling transmissivity, the zero-energy conductance peak quickly splits, while the pair of nonzero in-gap bound states first approach each other, merge, and then split again. These behaviors are unexpected for Majorana edge modes, but in consistent with the conventional Yu-Shiba-Rusinov states. Our results provide critical information for further understanding the interfacial coupling in CrBr3/NbSe2 heterostructure.

cond-mat.supr-con↗

arXiv2023

Discovery of a long-ranged charge order with 1/4 Ge1-dimerization in an antiferromagnetic Kagome metal

Exotic quantum states arise from the interplay of various degrees of freedom such as charge, spin, orbital, and lattice. Recently, a novel short-ranged charge order (CO) was discovered deep inside the antiferromagnetic phase of Kagome magnet FeGe, exhibiting close relationships with magnetism. Despite extensive investigations, the CO mechanism remains controversial, mainly because the short-ranged behavior hinders precise identification of CO superstructure. Here, combining multiple experimental techniques, we report the observation of a long-ranged CO in high-quality FeGe samples, which is accompanied with a first-order structural transition. With these high-quality samples, the distorted 2 * 2 * 2 CO superstructure is characterized by a strong dimerization along the c-axis of 1/4 of Ge1-sites in Fe3Ge layers, and in response to that, the 2 * 2 in-plane charge modulations are induced. Moreover, we show that the previously reported short-ranged CO might be related to large occupational disorders at Ge1-site, which upsets the equilibrium of the CO state and the ideal 1 * 1 * 1 structure with very close energies, inducing nanoscale coexistence of these two phases.Our study provides crucial clues for further understanding the CO properties in FeGe and helps to identify the CO mechanism.

cond-mat.str-el↗

arXiv2023

Charge order driven by multiple-Q spin fluctuations in heavily electron-doped iron selenide superconductors

Intertwined spin and charge orders have been widely studied in high-temperature superconductors, since their fluctuations may facilitate electron pairing; however, they are rarely identified in heavily electron-doped iron selenides. Here, using scanning tunneling microscopy, we show that when the superconductivity of (Li0.84Fe0.16OH)Fe1-xSe is suppressed by introducing Fe-site defects, a short-ranged checkerboard charge order emerges, propagating along the Fe-Fe directions with an approximately 2aFe period. It persists throughout the whole phase space tuned by Fe-site defect density, from a defect-pinned local pattern in optimally doped samples to an extended order in samples with lower Tc or non-superconducting. Intriguingly, our simulations indicate that the charge order is likely driven by multiple-Q spin density waves originating from the spin fluctuations observed by inelastic neutron scattering. Our study proves the presence of a competing order in heavily electron-doped iron selenides, and demonstrates the potential of charge order as a tool to detect spin fluctuations.

cond-mat.supr-con↗

arXiv2023

Instability of the charge density wave in Kagome magnet FeGe

Kagome metals show rich competing quantum phases due to geometry frustration, flat bands, many-body effects, and non-trivial topology. Recently, a novel charge density wave (CDW) was discovered deep inside the antiferromagnetic phase of FeGe, attracting intense attention due to close relation with magnetism. Here, via a scanning tunneling microscope (STM), we find the 2*2 CDW in FeGe is very fragile and can be readily disrupted into the initial 1*1 phase; Small sqrt3*sqrt3 CDW puddles are found to coexist with the 2*2 CDW in as-grown samples, and can also be induced in the intermediate process of CDW disruption, which will eventually transform into the initial 1*1 phase. Moreover, an exotic intermediate CDW state and standalone CDW nuclei appear unexpectedly during the disruption process. Our first-principle calculations find equal softening of a flat optical phonon mode in a large momentum region around the CDW wave vector, corresponding to numerous competing CDWs with close energies. This might lead to strong instability of the CDW ground state, responsible for STM observations. Our findings provide more novel experimental aspects to understand the CDW in FeGe and suggest FeGe-like Kagome metals are ideal platforms for studying the physics of competing CDW instabilities.

cond-mat.str-el↗

arXiv2021

Multiband superconductivity with sign-preserving order parameter in kagome superconductor CsV3Sb5

The superconductivity of a kagome superconductor CsV3Sb5 is studied by scanning tunneling microscopy / spectroscopy at an ultralow temperature with high resolution. Two kinds of superconducting gaps with multiple sets of coherent peaks and residual zero-energy density of states are observed on both half-Cs and Sb surfaces, implying multiband superconductivity with gap nodes. Sixfold star-shaped magnetic vortex is observed with conventional Caroli-de Gennes-Matricon bound states inside. Magnetic impurities suppress the superconductivity, while nonmagnetic impurities do not, suggesting the absence of sign-change in the superconducting order parameter. Moreover, the interplay between charge density waves and superconductivity differs on various bands, resulting in different density of state distributions. Our study provides critical clues for further understanding the superconductivity and its relation to charge density waves in CsV3Sb5.

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