arXiv subjects

Yue Chai

Publications and source records attributed to Yue Chai.

3 recordsLinked to original sources

arXiv2026

Extending the operating window of scanning electron microscopy through an integrated electron-optical architecture for high-temperature and near-ambient-pressure environments

Scanning electron microscopy (SEM) under simultaneously high-temperature, near-ambient-pressure (NAP), and reactive-gas environments requires coordinated control of vacuum isolation, electron-beam transmission, signal generation, and thermal management, constraints that have long limited the operating window of environmental scanning electron microscopy (ESEM). Here we establish an integrated electron-optical architecture that combines a multistage differential-pressure pathway, front-stage pressure transition, detector optimization, thermal management, and a gas-focusing sampling architecture into a unified ESEM platform. Pressure distribution and electron-beam transmission are quantitatively validated through computational fluid dynamics (CFD), Monte Carlo electron-gas scattering analysis, and direct beam-current measurements, while detector optimization and thermionic-electron suppression preserve stable imaging under elevated pressure and temperature. The resulting system enables stable SEM imaging at pressures up to 20,000 Pa and high-temperature imaging up to 1,400 degrees C, continuous observation of hydrated biological specimens, and synchronized SEM-QMS operando characterization using local gas sampling. These developments establish a general electron-optical framework for extending ESEM toward realistic operando environments where elevated temperature, reactive gases, structural evolution, and gas-phase chemistry can be investigated simultaneously.

physics.app-ph↗

arXiv2026

Controllable Lateral Optical Forces on Janus Particles in Fluid Media

Optical forces - studied since the earliest days of laser physics - continue to reveal rich dynamics and enable powerful tools for manipulation of objects on micro- and nanoscales, and even individual atoms. Lateral optical forces, which act perpendicular to the direction of beam propagation, are particularly intriguing but have largely been restricted to interface geometries such as air - water boundaries. Here, we realize tunable lateral optical force entirely within a fluid environment by using Janus particles: dielectric microspheres half-coated with gold. We show that the lateral optical force arises from scattering asymmetry induced by the asymmetric structure of the particles; it can be tuned by adjusting the polarization angle of a linearly polarized beam, but also particle parameters including their size and orientation. Experimentally, we directly observe fully reversible lateral propulsion of Janus particles in water merely by rotating the polarization direction, in excellent agreement with theoretical predictions. These results establish a new mechanism for programmable, polarization-controlled optical manipulation, with promising implications for biophotonics, microfluidics, and active soft-matter systems.

physics.optics↗

arXiv2025

Non-Euclidean interfaces decode the continuous landscape of graphene-induced surface reconstructions

Interfacial reconstruction between two-dimensional (2D) materials and metal substrates fundamentally governs heterostructure properties, yet conventional flat substrates fail to capture the continuous crystallographic landscape. Here, we overcome this topological limitation using non-Euclidean interfaces-curved 2D graphene-copper surfaces as a model system-to traverse the infinite spectrum of lattice orientations. By integrating multimodal microscopy with a deep-learning-enhanced dimensional upscaling framework, we translate 2D scanning electron microscopy (SEM) contrast into quantitative three-dimensional (3D) morphologies with accurate facet identification. Coupling these observations with machine-learning-assisted density functional theory, we demonstrate that reconstruction is governed by a unified thermodynamic mechanism where high-index facets correspond to specific local minima in the surface energy landscape. This work resolves the long-standing complexity of graphene-copper faceting and establishes non-Euclidean surface topologies as a generalizable paradigm for decoding and controlling interfacial reconstruction in diverse metal-2D material systems.

cond-mat.mes-hall↗