Searcharxiv⌕ Search

arXiv subjects

Yuhe Zhang

Publications and source records attributed to Yuhe Zhang.

At least 37 records · Page 2Linked to original sources

Development of crystal optics for Multi-Projection X-ray Imaging for synchrotron and XFEL sources

X-ray Multi-Projection Imaging (XMPI) is an emerging technology that allows for the acquisition of millions of 3D images per second in samples opaque to visible light. This breakthrough capability enables volumetric observation of fast stochastic phenomena, which were inaccessible due to the lack of a volumetric X-ray imaging probe with kHz to MHz repetition rate. These include phenomena of industrial and societal relevance such as fractures in solids, propagation of shock waves, laser-based 3D printing, or even fast processes in the biological domain. Indeed, the speed of traditional tomography is limited by the shear forces caused by rotation, to a maximum of 1000 Hz in state-of-the-art tomography. Moreover, the shear forces can disturb the phenomena in observation, in particular with soft samples or sensitive phenomena such as fluid dynamics. XMPI is based on splitting an X-ray beam to generate multiple simultaneous views of the sample, therefore eliminating the need for rotation. The achievable performances depend on the characteristics of the X-ray source, the detection system, and the X-ray optics used to generate the multiple views. The increase in power density of the X-ray sources around the world now enables 3D imaging with sampling speeds in the kilohertz range at synchrotrons and megahertz range at X-ray Free-Electron Lasers (XFELs). Fast detection systems are already available, and 2D MHz imaging was already demonstrated at synchrotron and XFEL. In this work, we explore the properties of X-ray splitter optics and XMPI schemes that are compatible with synchrotron insertion devices and XFEL X-ray beams. We describe two possible schemes designed to permit large samples and complex sample environments. Then, we present experimental proof of the feasibility of MHz-rate XMPI at the European XFEL.

physics.ins-det↗

Development towards high-resolution kHz-speed rotation-free volumetric imaging

X-ray multi-projection imaging (XMPI) provides rotation-free 3D movies of optically opaque samples. The absence of rotation enables superior imaging speed and preserves fragile sample dynamics by avoiding the shear forces introduced by conventional rotary tomography. Here, we present our XMPI observations at the ID19 beamline (ESRF, France) of 3D dynamics in melted aluminum with 1000 frames per second and 8 $μ$m resolution per projection using the full dynamical range of our detectors. Since XMPI is a method under development, we also provide different tests for the instrumentation of up to 3000 frames per second. As the flux of X-ray sources grows globally, XMPI is a promising technique for current and future X-ray imaging instruments.

physics.ins-det↗

Ultrasound cavitation and exfoliation dynamics of 2D materials re-vealed in operando by X-ray free electron laser megahertz imaging

Ultrasonic liquid phase exfoliation is a promising method for the production of two-dimensional (2D) layered materials. A large number of studies have been made in investigating the underlying ultrasound exfoliation mechanisms. However, due to the experimental challenges for capturing the highly transient and dynamic phenomena in real-time at sub-microsecond time and micrometer length scales simultaneously, most theories reported to date still remain elusive. Here, using the ultra-short X-ray Free Electron Laser pulses (~25ps) with a unique pulse train structure, we applied MHz X-ray Microscopy and machine-learning technique to reveal unambiguously the full cycles of the ultrasound cavitation and graphite layer exfoliation dynamics with sub-microsecond and micrometer resolution. Cyclic fatigue shock wave impacts produced by ultrasound cloud implosion were identified as the dominant mechanism to deflect and exfoliate graphite layers mechanically. For the graphite flakes, exfoliation rate as high as ~5 angstroms per shock wave impact was observed. For the HOPG graphite, the highest exfoliation rate was ~0.15 angstroms per impact. These new findings are scientifically and technologically important for developing industrial upscaling strategies for ultrasonic exfoliation of 2D materials.

cond-mat.mtrl-sci↗

Megahertz X-ray Multi-projection imaging

X-ray time-resolved tomography is one of the most popular X-ray techniques to probe dynamics in three dimensions (3D). Recent developments in time-resolved tomography opened the possibility of recording kilohertz-rate 3D movies. However, tomography requires rotating the sample with respect to the X-ray beam, which prevents characterization of faster structural dynamics. Here, we present megahertz (MHz) X-ray multi-projection imaging (MHz-XMPI), a technique capable of recording volumetric information at MHz rates and micrometer resolution without scanning the sample. We achieved this by harnessing the unique megahertz pulse structure and intensity of the European X-ray Free-electron Laser with a combination of novel detection and reconstruction approaches that do not require sample rotations. Our approach enables generating multiple X-ray probes that simultaneously record several angular projections for each pulse in the megahertz pulse burst. We provide a proof-of-concept demonstration of the MHz-XMPI technique's capability to probe 4D (3D+time) information on stochastic phenomena and non-reproducible processes three orders of magnitude faster than state-of-the-art time-resolved X-ray tomography, by generating 3D movies of binary droplet collisions. We anticipate that MHz-XMPI will enable in-situ and operando studies that were impossible before, either due to the lack of temporal resolution or because the systems were opaque (such as for MHz imaging based on optical microscopy).

eess.IV↗

Online dynamic flat-field correction for MHz Microscopy data at European XFEL

The X-ray microscopy technique at the European X-ray free-electron laser (EuXFEL), operating at a MHz repetition rate, provides superior contrast and spatial-temporal resolution compared to typical microscopy techniques at other X-ray sources. In both online visualization and offline data analysis for microscopy experiments, baseline normalization is essential for further processing steps such as phase retrieval and modal decomposition. In addition, access to normalized projections during data acquisition can play an important role in decision-making and improve the quality of the data. However, the stochastic nature of XFEL sources hinders the use of existing flat-flied normalization methods during MHz X-ray microscopy experiments. Here, we present an online dynamic flat-field correction method based on principal component analysis of dynamically evolving flat-field images. The method is used for the normalization of individual X-ray projections and has been implemented as an online analysis tool at the Single Particles, Clusters, and Biomolecules and Serial Femtosecond Crystallography (SPB/SFX) instrument of EuXFEL.

physics.ins-det↗

Saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride molecules

We report an experimental investigation on the Doppler-free saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride (BaF) molecules in a 4~K cryogenic cell. The obtained spectra with a resolution of 19~MHz, much smaller than previously observed in absorption spectroscopy, clearly resolve the hyperfine transitions. Moreover, we use these high-resolution spectra to fit the hyperfine splittings of excited $A(v=0)$ state and find the hyperfine splitting of the laser-cooling-relevant $A^2Π_{1/2}(v=0, J=1/2, +)$ state is about 18 MHz, much higher than the previous theoretically predicted value. This provides important missing information for laser cooling of BaF molecules.

physics.atom-ph↗

EPCS: Endpoint-based Part-aware Curve Skeleton Extraction for Low-quality Point Clouds

The curve skeleton is an important shape descriptor that has been utilized in various applications in computer graphics, machine vision, and artificial intelligence. In this study, the endpoint-based part-aware curve skeleton (EPCS) extraction method for low-quality point clouds is proposed. The novel random center shift (RCS) method is first proposed for detecting the endpoints on point clouds. The endpoints are used as the initial seed points for dividing each part into layers, and then the skeletal points are obtained by computing the center points of the oriented bounding box (OBB) of the layers. Subsequently, the skeletal points are connected, thus forming the branches. Furthermore, the multi-vector momentum-driven (MVMD) method is also proposed for locating the junction points that connect the branches. Due to the shape differences between different parts on point clouds, the global topology of the skeleton is finally optimized by removing the redundant junction points, re-connecting some branches using the proposed MVMD method, and applying an interpolation method based on the splitting operator. Consequently, a complete and smooth curve skeleton is achieved. The proposed EPCS method is compared with several state-of-the-art methods, and the experimental results verify its robustness, effectiveness, and efficiency. Furthermore, the skeleton extraction and model segmentation results on the point clouds of broken Terracotta also highlight the utility of the proposed method.

cs.CV↗

On geography of symplectic fillings of contact branched covers

In this paper, we determine the Euler characteristics and signatures of the exact symplectic fillings of the contact double, 3-fold or 4-fold cyclic covers of the standard contact 3-sphere branched over certain transverse quasi-positive links. These links include all quasi-positive knots with crossing numbers smaller than 11 and all quasi-positive links with crossing numbers smaller than 12 and nonzero nullity.

math.GT↗

ONIX: an X-ray deep-learning tool for 3D reconstructions from sparse views

Three-dimensional (3D) X-ray imaging techniques like tomography and confocal microscopy are crucial for academic and industrial applications. These approaches access 3D information by scanning the sample with respect to the X-ray source. However, the scanning process limits the temporal resolution when studying dynamics and is not feasible for some applications, such as surgical guidance in medical applications. Alternatives to obtaining 3D information when scanning is not possible are X-ray stereoscopy and multi-projection imaging. However, these approaches suffer from limited volumetric information as they only acquire a small number of views or projections compared to traditional 3D scanning techniques. Here, we present ONIX (Optimized Neural Implicit X-ray imaging), a deep-learning algorithm capable of retrieving 3D objects with arbitrary large resolution from only a set of sparse projections. ONIX, although it does not have access to any volumetric information, outperforms current 3D reconstruction approaches because it includes the physics of image formation with X-rays, and it generalizes across different experiments over similar samples to overcome the limited volumetric information provided by sparse views. We demonstrate the capabilities of ONIX compared to state-of-the-art tomographic reconstruction algorithms by applying it to simulated and experimental datasets, where a maximum of eight projections are acquired. We anticipate that ONIX will become a crucial tool for the X-ray community by i) enabling the study of fast dynamics not possible today when implemented together with X-ray multi-projection imaging, and ii) enhancing the volumetric information and capabilities of X-ray stereoscopic imaging in medical applications.

eess.IV↗

Doppler cooling of buffer-gas-cooled Barium monofluoride molecules

We demonstrate one-dimensional Doppler cooling of a beam of buffer-gas cooled Barium monofluoride (BaF) molecules. The dependences of the cooling efficiency with the laser detuning, the bias filed and the laser intensity are carefully measured. We numerical simulate our experiment with a Monte Carlo method, and find the theoretic predictions consists with our experimental data. This result represents a key step towards further cooling and trapping of BaF molecules.

physics.atom-ph↗

PyPhase -- a Python package for X-ray phase imaging

X-ray propagation-based imaging techniques are well-established at synchrotron radiation and laboratory sources. However, most reconstruction algorithms for such image modalities, also known as phase retrieval algorithms, have been developed specifically for one instrument by and for experts, making the development and spreading of the use of such techniques difficult. Here, we present PyPhase, a free and open-source package for propagation-based near-field phase reconstructions, which is distributed under the CeCILL license. PyPhase implements some of the most popular phase-retrieval algorithms in a highly-modular framework supporting the deployment on large-scale computing facilities. This makes the integration, the development of new phase-retrieval algorithms, and the deployment on different computing infrastructures straight-forward. To demonstrate its capabilities and simplicity, we present its application to data acquired at synchrotron MAX~IV (Lund, Sweden).

eess.IV↗

PhaseGAN: A deep-learning phase-retrieval approach for unpaired datasets

Phase retrieval approaches based on DL provide a framework to obtain phase information from an intensity hologram or diffraction pattern in a robust manner and in real time. However, current DL architectures applied to the phase problem rely i) on paired datasets, i.e., they are only applicable when a satisfactory solution of the phase problem has been found, and ii) on the fact that most of them ignore the physics of the imaging process. Here, we present PhaseGAN, a new DL approach based on Generative Adversarial Networks, which allows the use of unpaired datasets and includes the physics of image formation. Performance of our approach is enhanced by including the image formation physics and provides phase reconstructions when conventional phase retrieval algorithms fail, such as ultra-fast experiments. Thus, PhaseGAN offers the opportunity to address the phase problem when no phase reconstructions are available, but good simulations of the object or data from other experiments are available, enabling us to obtain results not possible before.

eess.IV↗

A general Zeeman slower for type-II transitions and polar molecules

We proposed a general Zeeman slower scheme applicable to the majority of the laser-coolable molecules. Different from previous schemes, the key idea of our scheme lies in that the compensation of the detuning with the magnetic field is done for the repumping laser instead of the cooling laser. Only atoms or molecules with the right velocity will be repumped and laser slowed. Such scheme is more feasible for molecules with complex energy sturcutres. We apply this scheme for molecules with large Landé g-factor of the excited states and polyatomic molecules, and it shows a better slowing efficiency.

physics.atom-ph↗

Laser cooling with adiabatic passage for diatomic molecules

We present a magnetically enhanced laser cooling scheme applicable to multi-level type-II transitions and further diatomic molecules with adiabatic transfer. An angled magnetic field is introduced to not only remix the dark states, but also decompose the multi-level system into several two-level sub-systems in time-ordering, hence allowing multiple photon momentum transfer. For complex multi-level diatomic molecules, although the enhancement gets weakened, our simulations still predict a $\sim 4\times$ larger value of the maximum achievable cooling force and a wider coolable velocity range compared to the conventional Doppler cooling. A reduced dependence on spontaneous emission of this scheme makes laser cooling a molecule with leakage channels become a feasibility.

physics.atom-ph↗

Crystallization in the Fractional Quantum Hall Regime Induced by Landau-level Mixing

The interplay between strongly correlated liquid and crystal phases for two-dimensional electrons exposed to a high transverse magnetic field is of fundamental interest. Through the non-perturbative fixed phase diffusion Monte Carlo method, we determine the phase diagram of the Wigner crystal in the $ν-κ$ plane, where $ν$ is the filling factor and $κ$ is the strength of Landau level mixing. The phase boundary is seen to exhibit a striking $ν$ dependence, with the states away from the magic filling factors $ν=n/(2pn+1)$ being much more susceptible to crystallization due to Landau level mixing than those at $ν=n/(2pn+1)$. Our results explain the qualitative difference between the experimental behaviors observed in n-doped and p-doped GaAs quantum wells, and, in particular, the existence of an insulating state for $ν<1/3$ and also for $1/3 <ν< 2/5$ in low density p-doped systems. We predict that in the vicinity of $ν=1/5$ and $ν=2/9$, increasing LL mixing causes a transition not into an ordinary electron Wigner crystal but rather into a strongly correlated crystal of composite fermions carrying two vortices.

cond-mat.str-el↗

Surprising robustness of particle-hole symmetry for composite fermion liquids

We report on fixed phase diffusion Monte Carlo calculations that show that, even for a large amount of Landau level mixing, the energies of the Pfaffian and anti-Pfaffian phases remain very nearly the same, as also do the excitation gaps at $1/3$ and $2/3$. These results, combined with previous theoretical and experimental investigations, indicate that particle hole (PH) symmetry for composite fermion states is much more robust than a priori expected, emerging even in models that explicitly break PH symmetry. We provide insight into this fact by showing that the low energy physics of a generic repulsive 3-body interaction is captured, to a large extent and over a range of filling factors, by a mean field approximation that maps it into a PH symmetric 2-body interaction. This explains why Landau level mixing, which effectively generates such a generic 3-body interaction, is inefficient in breaking PH symmetry. As a byproduct, our results provide a systematic construction of a 2-body interaction which produces, to a good approximation, the Pfaffian wave function as its ground state.

cond-mat.str-el↗

Tunnel transport and interlayer excitons in bilayer fractional quantum Hall systems

In a bilayer system consisting of a composite-fermion Fermi sea in each layer, the tunnel current is exponentially suppressed at zero bias, followed by a strong peak at a finite bias voltage $V_{\rm max}$. This behavior, which is qualitatively different from that observed for the electron Fermi sea, provides fundamental insight into the strongly correlated non-Fermi liquid nature of the CF Fermi sea and, in particular, offers a window into the short-distance high-energy physics of this state. We identify the exciton responsible for the peak current and provide a quantitative account of the value of $V_{\rm max}$. The excitonic attraction is shown to be quantitatively significant, and its variation accounts for the increase of $V_{\rm max}$ with the application of an in-plane magnetic field. We also estimate the critical Zeeman energy where transition occurs from a fully spin polarized composite fermion Fermi sea to a partially spin polarized one, carefully incorporating corrections due to finite width and Landau level mixing, and find it to be in satisfactory agreement with the Zeeman energy where a qualitative change has been observed for the onset bias voltage [Eisenstein et al., Phys. Rev. B 94, 125409 (2016)]. For fractional quantum Hall states, we predict a substantial discontinuous jump in $V_{\rm max}$ when the system undergoes a transition from a fully spin polarized state to a spin singlet or a partially spin polarized state.

cond-mat.str-el↗

Landau-Level Mixing and Particle-Hole Symmetry Breaking for Spin Transitions in the Fractional Quantum Hall Effect

The spin transitions in the fractional quantum Hall effect provide a direct measure of the tiny energy differences between differently spin-polarized states, and thereby serve as an extremely sensitive test of the quantitative accuracy of the theory of the fractional quantum Hall effect, and, in particular, of the role of Landau-level mixing in lifting the particle-hole symmetry. We report on an accurate quantitative study of this physics, evaluating the effect of Landau-level mixing in a nonperturbative manner using a fixed-phase diffusion Monte Carlo method. We find excellent agreement between our calculated critical Zeeman energies and the experimentally measured values. In particular, we find, as also do experiments, that the critical Zeeman energies for fractional quantum Hall states at filling factors $ν=2-n/(2n\pm 1)$ are significantly higher than those for $ν=n/(2n\pm 1)$, a quantitative signature of the lifting of particle-hole symmetry due to Landau-level mixing.

cond-mat.str-el↗