arXiv subjects

Yuji Hamamoto

Publications and source records attributed to Yuji Hamamoto.

10 recordsLinked to original sources

arXiv2026

Mechanical bistability and hysteresis in graphene-CNT hybrid systems: from atomistic simulations to macroscale structural responses

Hybrid systems composed of graphene (Gr) and carbon nanotubes (CNTs), such as films and aerogels, have attracted broad attention for applications in electronics, mechanics, energy, and environmental science. Since the microstructures of Gr-CNT hybrids strongly affect their properties, it is essential to establish mechanical principles that govern these structures. In this study, we investigated the structural stability and mechanical behavior of Gr-CNT hybrid systems by combining molecular dynamics (MD) simulations and nanoindentation experiments. MD simulations of stacked Gr-CNT structures, in which two Gr layers confine CNTs between them, identified the energetically stable configurations and their governing parameters, i.e., intertube spacing, CNT diameter, and wall number. Specifically, under certain conditions, the structures exhibit mechanical bistability with two stable configurations: adhesion and separation of the Gr layers, arising from the competition between interlayer van der Waals attraction and elastic deformation of Gr and CNTs. Simulated loading--unloading curves display hysteresis and energy dissipation related to the stable configurations. In addition, reduced graphene oxide (rGO)-CNT hybrid films were experimentally fabricated as macroscopic assemblies of the unit structures modeled in the simulations. Atomic force microscopy-based nanoindentation measurements on the rGO-CNT films exhibit clear hysteresis and higher dissipation energy compared with pure rGO, in good agreement with the simulation results. These results provide valuable insights into Gr-CNT hybrid systems and offer guidance for designing microstructures with enhanced properties for advanced applications.

cond-mat.mtrl-sci↗

arXiv2023

Reduction of Interlayer Interaction in Multilayer Stacking Graphene with Carbon Nanotube Insertion: Insights from Experiment and Simulation

The creation of multilayer graphene (Gr), while preserving the brilliant properties of monolayer Gr derived from its unique band structure, can expand the application field of Gr to the macroscale. However, the energy-favorable AB stacking structure in the multilayer Gr induces a strong interlayer interaction and alters the band structure. Consequently, the intrinsic properties of each monolayer are degraded. In this work, we insert carbon nanotubes (CNTs) as nanospacers to modulate the microstructure of multilayer stacking Gr. Nanospacers can increase the interlayer distance and reduce the interlayer interaction. The Gr/CNT stacking structure is experimentally fabricated using a dry transfer method in a layer-by-layer manner. Raman spectroscopy verifies the reduction in the interlayer interaction within the stacking structure. Atomic force microscopy shows an increase in the interlayer distance, which can explain the weakening of the interlayer interactions. The microstructure of the stacked Gr and CNTs is studied by molecular dynamics simulation to systematically investigate the effect of CNT insertion. We found that the distribution distance, size, and arrangement of the CNT can modulate the interlayer distance. These results will help us to understand and improve the properties of the composite systems consisting of Gr and CNTs.

cond-mat.mes-hall↗

arXiv2016

Self-consistent van der Waals density functional study of benzene adsorption on Si(100)

The adsorption of benzene on the Si(100) surface is studied theoretically using the self-consistent van der Waals density functional (vdW-DF) method. The adsorption energies of two competing adsorption structures, butterfly (BF) and tight-bridge (TB) structures, are calculated with several vdW-DFs at saturation coverage. Our results show that recently proposed vdW-DFs with high accuracy all prefer TB to BF, in accord with more accurate calculations based on exact exchange and correlation within the random phase approximation. Detailed analyses reveal the important roles played by the molecule-surface interaction and molecular deformation upon adsorption, and we suggest that their precise description is prerequisite for accurate prediction of the most stable adsorption structure of organic molecules on semiconductor surfaces.

cond-mat.mtrl-sci↗

arXiv2013

Spin-resoloved chiral condensate as a spin-unpolarized \nu=0 quantum Hall state in graphene

Motivated by the recent experiments indicating a spin-unpolarized \nu=0 quantum Hall state in graphene, we theoretically investigate the ground state based on the many-body problem projected onto the n=0 Landau level. For an effective model with the on-site Coulomb repulsion and antiferromagnetic exchange couplings, we show that the ground state is a doubly-degenerate spin-resolved chiral condensate in which all the zero-energy states with up spin are condensed into one chirality, while those with down spin to the other. This can be exactly shown for an Ising-type exchange interaction. The charge gap due to the on-site repulsion in the ground state is shown to grow linearly with the magnetic field, in qualitative agreement with the experiments.

cond-mat.mes-hall↗

arXiv2012

Chiral Symmetry and Many-Body Effect in Multilayer Graphene

Influence of the chiral symmetry on the many-body problem in multilayer graphene in magnetic fields is investigated. For a spinless electron model on the honeycomb lattice the many-body ground state is shown to be a doubly-degenerate chiral condensate irrespective of the number of layers. The energy spectrum calculated numerically with the exact diagonalization method reveals for ABC-stacked multilayer graphenes that the many-body gap decreases monotonically with the number of layers.

cond-mat.mes-hall↗

arXiv2012

Chiral condensate with topological degeneracy in graphene and its manifestation in edge states

Role of chiral symmetry in many-body states of graphene in strong magnetic fields is theoretically studied with the honeycomb lattice model. For a spin-split Landau level where the leading electron-electron interaction is the nearest-neighbor repulsion, a chiral condensate is shown to be, within the subspace of n = 0 Landau level, an exact many-body ground state with a finite gap, for which calculation of Chern numbers reveals that the ground state is a Hall insulator with a topological degeneracy of two. The topological nature of the ground state is shown to manifest itself as a Kekul\'ean bond order along armchair edges, while the pattern melts in the bulk due to quantum fluctuations. The whole story can be regarded as a realization of the bulk-edge correspondence peculiar to the chiral symmetry.

cond-mat.mes-hall↗

arXiv2010

Quantum phase transition of dynamical resistance in a mesoscopic capacitor

We study theoretically dynamic response of a mesoscopic capacitor, which consists of a quantum dot connected to an electron reservoir via a point contact and capacitively coupled to a gate voltage. A quantum Hall edge state with a filling factor nu is realized in a strong magnetic field applied perpendicular to the two-dimensional electron gas. We discuss a noise-driven quantum phase transition of the transport property of the edge state by taking into account an ohmic bath connected to the gate voltage. Without the noise, the charge relaxation for nu>1/2 is universally quantized at R_q=h/(2e^2), while for nu<1/2, the system undergoes the Kosterlitz-Thouless transtion, which drastically changes the nature of the dynamical resistance. The phase transition is facilitated by the noisy gate voltage, and we see that it can occur even for an integer quantum Hall edge at nu=1. When the dissipation by the noise is sufficiently small, the quantized value of R_q is shifted by the bath impedance.

cond-mat.mes-hall↗

arXiv2009

Dynamic response of a mesoscopic capacitor in the presence of strong electron interactions

We consider a one dimensional mesoscopic capacitor in the presence of strong electron interactions and compute its admittance in order to probe the universal nature of the relaxation resistance. We use a combination of perturbation theory, renormalization group arguments, and quantum Monte Carlo calculation to treat the whole parameter range of dot-lead coupling. The relaxation resistance is universal even in the presence of strong Coulomb blockade when the interactions in the wire are sufficiently weak. We predict and observe a quantum phase transition to an incoherent regime for a Luttinger parameter $K<1/2$. Results could be tested using a quantum dot coupled to an edge state in the fractional quantum Hall effect.

cond-mat.mes-hall↗

arXiv2008

Numerical study of the Coulomb blockade in an open quantum dot

The Coulomb blockade in an open quantum dot connected to a bulk lead by a single mode point contact is studied numerically using the path-integral Monte Carlo method. The Coulomb oscillation of the average charge and capacitance of the dot is investigated, and is compared with the analytic expression for strong tunneling. At the degeneracy point, we observe logarithmic divergence of the capacitance for strong backscattering at the point contact. This observation supports the conjecture that the nature of the present system at the degeneracy point is described by the two-channel Kondo problem for an arbitrary strength of tunneling.

cond-mat.mes-hall↗

arXiv2007

Numerical study of transport through a single impurity in a spinful Tomonaga-Luttinger liquid

The single impurity problem in a spinful Tomonaga-Luttinger liquid is studied numerically using path-integral Monte Carlo methods. The advantage of our approach is that the system allows for extensive analyses of charge and spin conductance in the non-perturbative regime. By closely examining the behavior of conductances at low temperatures, in the presence of a finite backward scattering barrier due to the impurity, we identified four distinct phases characterized by either perfect transmission or reflection of charge and spin channels. Our phase diagram for an intermediate scattering strength is consistent with the standard perturbative renormalization group (RG) analysis in the limit of weak and strong backward scattering, in the sense that all our phase boundaries interpolate the two limiting cases. Further investigations show, however, that precise location and form of our phase boundaries are not trivially explained by the standard RG analysis, e.g., some part of the phase diagram looks much similar to the weak backscattering limit, whereas some other part is clearly derived from the opposite limit. In order to give a more intuitive interpretation of such behaviors, we also reconsidered our impurity problem from the viewpoint of a quantum Brownian motion picture.

cond-mat.mes-hall↗