arXiv subjects

Yun-Feng Xiao

Publications and source records attributed to Yun-Feng Xiao.

At least 19 recordsLinked to original sources

arXiv2025

Integrated soliton microcombs beyond the turnkey limit

Soliton microcombs generated in optical microresonators are accelerating the transition of optical frequency combs from laboratory instruments to industrial platforms. Self injection locking (SIL) enables direct driving of soliton microcombs by integrated lasers, providing turnkey initiation and improved coherence, but it also pins the pump close to resonance, limiting both spectral span and tuning flexibility. Here we theoretically and experimentally demonstrate that introducing a thermally tunable auxiliary microresonator extends the bandwidth of SIL soliton microcombs. By engineering hybridization of the pumped resonance, we achieve deterministic access to single soliton states and then push operation into a far detuned regime inaccessible to direct initiation. The resulting combs reach a near 200 nm span at a 25 GHz repetition rate, while preserving the SIL-enabled noise suppression throughout. Moreover, the added degree of freedom afforded by the coupled resonator architecture enables orthogonal control of the comb's repetition rate and center frequency. These advances expand the spectral reach and controllability of integrated soliton microcombs for information processing and precision metrology.

physics.optics↗

arXiv2025

Raman-induced dynamics of ultrafast microresonator solitons

Soliton microcombs are evolving towards octave-spanning for $f$-$2f$ self-referencing and expanding applications in spectroscopy and timekeeping. As spectra broaden and pulses shorten, the Raman-induced soliton self-frequency shift (SSFS) becomes a principal limitation: it reduces pump-to-comb conversion efficiency, constrains achievable span, and can, in extremes, preclude stationary operation. We develop a complementary theory of SSFS in microresonators that remains valid when the soliton duration $τ_s$ is shorter than the Raman response timescale. The theory predicts a reduced dependence of the SSFS on $τ_s$ which also expands the soliton existence range. Such predictions are validated by numerical simulations and by experiments on Si$_3$N$_4$ microresonators. Our results provide practical guidelines for engineering efficient and broadband soliton microcombs.

physics.optics↗

arXiv2025

Compact Turnkey Soliton Microcombs at Microwave Rates via Wafer-Scale Fabrication

Soliton microcombs generated in nonlinear microresonators facilitate the photonic integration of timing, frequency synthesis, and astronomical calibration functionalities. For these applications, low-repetition-rate soliton microcombs are essential as they establish a coherent link between optical and microwave signals. However, the required pump power typically scales with the inverse of the repetition rate, and the device footprint scales with the inverse of square of the repetition rate, rendering low-repetition-rate soliton microcombs challenging to integrate within photonic circuits. This study designs and fabricates silicon nitride microresonators on 4-inch wafers with highly compact form factors. The resonator geometries are engineered from ring to finger and spiral shapes to enhance integration density while attaining quality factors over 10^7. Driven directly by an integrated laser, soliton microcombs with repetition rates below 10 GHz are demonstrated via turnkey initiation. The phase noise performance of the synthesized microwave signals reaches -130 dBc/Hz at 100 kHz offset frequency for 10 GHz carrier frequencies. This work enables the high-density integration of soliton microcombs for chip-based microwave photonics and spectroscopy applications.

physics.optics↗

arXiv2024

Toward ultimate-efficiency frequency conversion in nonlinear optical microresonators

Integrated nonlinear photonics has emerged as a transformative platform, enabling nanoscale nonlinear optical processes with significant implications for sensing, computation, and metrology. Achieving efficient nonlinear frequency conversion in optical microresonators is paramount to fully unlocking this potential, yet the absolute conversion efficiency (ACE) of many processes, such as second-harmonic generation (SHG), remains fundamentally constrained by dissipative losses and intrinsic nonlinear effects in the device. In this work, we establish a unified theoretical framework for SHG in microresonators, identifying a decisive factor M that predicts the upper limit of ACE under the nonlinear critical coupling (NCC) condition. Using this framework, we fabricate integrated periodically poled lithium niobate microresonators and address the dispersive and dissipative suppression to approach the NCC condition. We achieve a record-high experimental ACE of 61.3% with milliwatt-level pump powers toward the ultimate efficiency, with the potential for even higher efficiency as the M factor increases. These results provide a versatile paradigm for high-efficiency nonlinear optical devices, offering new opportunities for advancements across classical and quantum photonic applications.

physics.optics↗

arXiv2024

Steering Non-Equilibrium Molecular Dynamics in Optical Cavities

Optical resonators have shown outstanding abilities to tailor chemical landscapes through enhanced light-matter interaction between confined optical modes and molecule vibrations. We propose a theoretical model to study cooperative vibrational strong coupling in an open quantum system. The non-equilibrium stochastic molecular dynamics in an optical cavity with an auxiliary ensemble is investigated. It shows that coupling with a cavity mode introduces an additional colored noise and a negative feedback, both of which enable control over thermalization rates (i.e. the lifetime of excitation) of reactive molecules. Our work offers a pathway to steer stability of chemical bonds for chemical reactivity under cooperative vibrational strong coupling.

physics.optics↗

arXiv2023

Single-particle vibrational spectroscopy using optical microresonators

Vibrational spectroscopy is a ubiquitous technology that derives the species, constituents, and morphology of an object from its natural vibrations. However, the vibrational spectra of mesoscopic particles - including most biological cells - have remained hidden from existing technologies. These particles are expected to vibrate faintly at megahertz to gigahertz rates, imposing unpractical sensitivity and resolution for current optical and piezoelectric spectroscopy. Here we demonstrate the real-time measurement of natural vibrations of single mesoscopic particles using an optical microresonator, extending the reach of vibrational spectroscopy to a new spectral window. Conceptually, a spectrum of vibrational modes of the particles is stimulated photoacoustically, and correlated to a high-quality-factor optical resonance for the ultrasensitive readout. Experimentally, this scheme is testified by measuring mesoscopic particles with different constituents, sizes, and internal structures, showing an unprecedented signal-to-noise ratio of 50 dB and detection bandwidth over 1 GHz. This new technology is further applied for the biomechanical fingerprinting of single microbial cells with different species and living states. The present method opens up new avenues to study single-particle mechanical properties in vibrational degrees of freedom, and may find applications in photoacoustic sensing and imaging, cavity optomechanics and biomechanics.

physics.optics↗

arXiv2023

Atom-referenced on-chip soliton microcomb

For the applications of the frequency comb in microresonators, it is essential to obtain a fully frequency-stabilized microcomb laser source. Here, we demonstrate an atom-referenced stabilized soliton microcomb generation system based on the integrated microring resonator. The pump light around $1560.48\,\mathrm{nm}$ locked to an ultra-low-expansion (ULE) cavity, is frequency-doubled and referenced to the atomic transition of $^{87}\mathrm{Rb}$. The repetition rate of the soliton microcomb is injection-locked to an atomic-clock-stabilized radio frequency (RF) source, leading to mHz stabilization at $1$ seconds. As a result, all comb lines have been frequency-stabilized based on the atomic reference and could be determined with very high precision reaching $\sim18\,\mathrm{Hz}$ at 1 second, corresponding to the frequency stability of $9.5\times10^{-14}$. Our approach provides an integrated and fully stabilized microcomb experiment scheme with no requirement of $f-2f$ technique, which could be easily implemented and generalized to various photonic platforms, thus paving the way towards the portable and ultraprecise optical sources for high precision spectroscopy.

physics.optics↗

arXiv2023

Phase-transition microcavity laser

Liquid-crystal microcavity lasers have attracted considerable attention because of their extraordinary tunability and sensitive response to external stimuli, and they operate generally within a specific phase. Here, we demonstrate a liquid-crystal microcavity laser operated in the phase transition, in which the reorientation of liquid-crystal molecules occurs from aligned to disordered states. A significant wavelength shift of the microlaser is observed, resulting from the dramatic changes in the refractive index of liquid-crystal microdroplets during the phase transition. This phase-transition microcavity laser is then exploited for sensitive thermal sensing, enabling two-order-of-magnitude enhancement in sensitivity compared with the nematic-phase microlaser operated far from the transition point. Experimentally, we demonstrate an exceptional sensitivity of -40 nm/K and an ultrahigh resolution of 320 uK. The phase-transition microcavity laser features compactness, softness, and tunability, showing great potential for high-performance sensors, optical modulators, and soft matter photonics.

physics.optics↗

arXiv2022

Integrated vortex soliton microcombs

The frequency and orbital angular momentum (OAM) are independent physical properties of light that both offer unbounded degrees of freedom. However, creating, processing, and detecting high-dimensional OAM states have been a pivot and long-lasting task, as the complexity of the required optical systems scales up drastically with the OAM dimension. On the other hand, mature toolboxes -- such as optical frequency combs -- have been developed in the frequency domain for parallel measurements with excellent fidelity. Here we correlate the two dimensions into an equidistant comb structure on a photonic chip. Dissipative optical solitons formed in a nonlinear microresonator are emitted through the engraved angular gratings with each comb line carrying distinct OAM. Such one-to-one correspondence between the OAM and frequencies manifests state-of-the-art extinction ratios over 18.5 dB, enabling precision spectroscopy of optical vortices. The demonstrated vortex soliton microcombs provide coherent light sources that are multiplexed in the spatial and frequency domain, having the potential to establish a new modus operandi of high-dimensional structured light.

physics.optics↗

arXiv2022

Electron microscopy probing electron-photon interactions in SiC nanowires with ultra-wide energy and momentum match

Nanoscale materials usually can trap light and strongly interact with it leading to many photonic device applications. The light-matter interactions are commonly probed by optical spectroscopy, which, however, have some limitations such as diffraction-limited spatial resolution, tiny momentum transfer and non-continuous excitation/detection. In this work, using scanning transmission electron microscopy-electron energy loss spectroscopy (STEM-EELS) with ultra-wide energy and momentum match and sub-nanometer spatial resolution, we study the optical microcavity resonant spectroscopy in a single SiC nanowire. The longitudinal Fabry-Perot (FP) resonating modes and the transverse whispering-gallery modes (WGMs) are simultaneously excited and detected, which span from near-infrared (~ 1.2 μm) to ultraviolet (~ 0.2 μm) spectral regime and the momentum transfer can be ranging up to 108 cm{^{-1}}. The size effects on the resonant spectra of nanowires are also revealed. Moreover, the nanoscale decay length of resonant EELS is revealed, which is contributed by the strongly localized electron-photon interactions in the SiC nanowire. This work provides a new alternative technique to investigate the optical resonating spectroscopy of a single nanowire structure and to explore the light-matter interactions in dielectric nanostructures, which is also promising for modulating free electrons via photonic structures.

cond-mat.mes-hall↗

arXiv2022

Non-reciprocal frequency conversion and mode routing in a microresonator

The transportation of photons and phonons typically obeys the principle of reciprocity. Breaking reciprocity of these bosonic excitations will enable the corresponding non-reciprocal devices, such as isolators and circulators. Here, we use two optical modes and two mechanical modes in a microresonator to form a four-mode plaquette via radiation pressure force. The phase-controlled non-reciprocal routing between any two modes with completely different frequencies is demonstrated, including the routing of phonon to phonon (MHz to MHz), photon to phonon (THz to MHz), and especially photon to photon with frequency difference of around 80 THz for the first time. In addition, one more mechanical mode is introduced to this plaquette to realize a phononic circulator in such single microresonator. The non-reciprocity is derived from interference between multi-mode transfer processes involving optomechanical interactions in an optomechanical resonator. It not only demonstrates the non-reciprocal routing of photons and phonons in a single resonator but also realizes the non-reciprocal frequency conversion for photons and circulation for phonons, laying a foundation for studying directional routing and thermal management in an optomechanical hybrid network.

physics.optics↗

arXiv2021

Ground-state cooling of multiple near-degenerate mechanical modes

We propose a general and experimentally feasible approach to realize simultaneous ground-state cooling of arbitrary number of near-degenerate, or even fully degenerate mechanical modes, overcoming the limit imposed by the formation of mechanical dark modes. Multiple optical modes are employed to provide different dissipation channels that prevent complete destructive interference of the cooling pathway, and thus eliminating the dark modes. The cooling rate and limit are explicitly specified, in which the distinguishability of the optical modes to the mechanical modes is found to be critical for an efficient cooling process. In a realistic multi-mode optomechanical system, ground-state cooling of all mechanical modes is demonstrated by sequentially introducing optical drives, proving the feasibility and scalability of the proposed scheme. The work may provide new insights in preparing and manipulating multiple quantum states in macroscopic systems.

quant-ph↗

arXiv2021

Spectrally multiplexed and ultrabright entangled photon pairs in a lithium niobate microresonator

On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum source generated in a lithium niobate microresonator system.Without introducing the conventional domain poling, the on-chip microdisk produces entangled photon pairs covering a broad bandwidth promised by natural phase matching in spontaneous parametric down conversion.Experimentally, the multiplexed photon pairs are characterized by $30\ \rm nm$ bandwidth limited by the filtering system, which can be furthered enlarged.Meanwhile, the generation rate reaches $5.13\ {\rm MHz}/\upmu \rm W$ with a coincidence-to-accidental ratio up to $804$.Besides, the quantum source manifests the prominent purity with heralded single photon correlation $g_H^{(2)}(0)=0.0098\pm0.0021$ and energy-time entanglement with excellent interference visibility of $96.5\%\pm1.9\%$. Such quantum sources at the telecommunication band pave the way for high-dimensional entanglement and future integrated quantum information systems.

quant-ph↗

arXiv2021

Vibrational Kerr solitons in an optomechanical microresonator

Soliton microcombs based on Kerr nonlinearity in microresonators have been a prominent miniaturized coherent light source. Here, for the first time, we demonstrate the existence of Kerr solitons in an optomechanical microresonator, for which a nonlinear model is built by incorporating a single mechanical mode and multiple optical modes. Interestingly, an exotic vibrational Kerr soliton state is found, which is modulated by a self-sustained mechanical oscillation. Besides, the soliton provides extra mechanical gain through the optical spring effect, and results in phonon lasing with a red-detuned pump. Various nonlinear dynamics is also observed, including limit cycle, higher periodicity, and transient chaos. This work provides a guidance for not only exploring many-body nonlinear interactions, but also promoting precision measurements by featuring superiority of both frequency combs and optomechanics.

physics.optics↗

arXiv2020

Gain-assisted chiral soliton microcombs

The emerging microresonator-based frequency combs revolutionize a broad range of applications from optical communications to astronomical calibration. Despite of their significant merits, low energy efficiency and the lack of all-optical dynamical control severely hinder the transfer of microcomb system to real-world applications. Here, by introducing active lasing medium into the soliton microcomb, for the first time, we experimentally achieve the chiral soliton with agile on-off switch and tunable dual-comb generation in a packaged microresonator. It is found that such a microresonator enables a soliton slingshot effect, the rapid soliton formation arising from the extra energy accumulation induced by inter-modal couplings. Moreover, tuning the erbium gain can generate versatile multi-soliton states, and extend the soliton operation window to a remarkable range over 18 GHz detuning. Finally, the gain-assisted chirality of counterpropagating soliton is demonstrated, which enables an unprecedented fast on-off switching of soliton microcombs. The non-trivial chiral soliton formation with active controllability inspires new paradigms of miniature optical frequency combs and brings the fast tunable soliton tools within reach.

physics.optics↗

arXiv2020

Reconfigurable photon sources based on quantum plexcitonic systems

A single photon in a strongly nonlinear cavity is able to block the transmission of the second photon, thereby converting incident coherent light into anti-bunched light, which is known as photon blockade effect. On the other hand, photon anti-pairing, where only the entry of two photons is blocked and the emission of bunches of three or more photons is allowed, is based on an unconventional photon blockade mechanism due to destructive interference of two distinct excitation pathways. We propose quantum plexcitonic systems with moderate nonlinearity to generate both anti-bunched and anti-paired photons. The proposed plexitonic systems benefit from subwavelength field localizations that make quantum emitters spatially distinguishable, thus enabling a reconfigurable photon source between anti-bunched and anti-paired states via tailoring the energy bands. For a realistic nanoprism plexitonic system, two schemes of reconfiguration are suggested: (i) the chemical means by partially changing the type of the emitters; or (ii) the optical approach by rotating the polarization angle of the incident light to tune the coupling rate of the emitters. These results pave the way to realize reconfigurable nonclassical photon sources in a simple quantum plexcitonic platform with readily accessible experimental conditions.

quant-ph↗

arXiv2020

Chip-to-chip quantum teleportation and multi-photon entanglement in silicon

Exploiting semiconductor fabrication techniques, natural carriers of quantum information such as atoms, electrons, and photons can be embedded in scalable integrated devices. Integrated optics provides a versatile platform for large-scale quantum information processing and transceiving with photons. Scaling up the integrated devices for quantum applications requires highperformance single-photon generation and photonic qubit-qubit entangling operations. However, previous demonstrations report major challenges in producing multiple bright, pure and identical single-photons, and entangling multiple photonic qubits with high fidelity. Another notable challenge is to noiselessly interface multiphoton sources and multiqubit operators in a single device. Here we demonstrate on-chip genuine multipartite entanglement and quantum teleportation in silicon, by coherently controlling an integrated network of microresonator nonlinear single-photon sources and linear-optic multiqubit entangling circuits. The microresonators are engineered to locally enhance the nonlinearity, producing multiple frequencyuncorrelated and indistinguishable single-photons, without requiring any spectral filtering. The multiqubit states are processed in a programmable linear circuit facilitating Bell-projection and fusion operation in a measurement-based manner. We benchmark key functionalities, such as intra-/inter-chip teleportation of quantum states, and generation of four-photon Greenberger-HorneZeilinger entangled states. The production, control, and transceiving of states are all achieved in micrometer-scale silicon chips, fabricated by complementary metal-oxide-semiconductor processes. Our work lays the groundwork for scalable on-chip multiphoton technologies for quantum computing and communication.

quant-ph↗

arXiv2020

Diabolical Points in Coupled Active Cavities with Quantum Emitters

In single microdisks, embedded active emitters intrinsically affect the cavity mode of microdisks, which results in a trivial symmetric backscattering and a low controllability. Here we propose a macroscopical control of the backscattering direction by optimizing the cavity size. The signature of positive and negative backscattering directions in each single microdisk is confirmed with two strongly coupled microdisks. Furthermore, the diabolical points are achieved at the resonance of two microdisks, which agrees well with the theoretical calculations considering backscattering directions. The diabolical points in active optical structures pave a way to implement quantum information processing with geometric phase in quantum photonic networks.

physics.optics↗