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Yuqian Zhao

Publications and source records attributed to Yuqian Zhao.

At least 19 recordsLinked to original sources

Spiral spin liquid resilient to quantization in the frustrated honeycomb antiferromagnet GdZnPO

Frustrated magnets host strong quantum fluctuations that can suppress conventional magnetic order and give rise to exotic quantum phases such as spin liquids. In some cases, however, quantum fluctuations lift classical degeneracies and stabilize ordered states via an order-by-quantum-disorder mechanism. The spin-7/2 honeycomb antiferromagnet GdZnPO has recently been proposed as a spiral spin-liquid candidate arising from cooperative fluctuations among a subextensively degenerate manifold of spiral states. Here, we investigate the local magnetization and spin dynamics in GdZnPO using nuclear magnetic resonance. In an intermediate field regime between $\sim$3 T and the saturation field ($\sim$12 T), we observe a spatially uniform magnetization and persistent low-energy spin dynamics down to 0.033 K, with no detectable symmetry breaking, providing spectroscopic evidence for a spin-liquid state. At lower fields below $\sim$3 T, a weak stripe order emerges below $\sim$0.25 K; however, strong fluctuations persist, as indicated by a nearly temperature-independent and unusually large spin-lattice relaxation rate in the low-temperature limit. Our results demonstrate that spin-7/2 quantization weakly lifts the spiral degeneracy, stabilizing subtle magnetic order while preserving robust dynamics and spin-liquid phenomenology. These findings establish GdZnPO as a promising platform for exploring spin liquids in high-spin frustrated magnets down to the lowest accessible temperatures.

cond-mat.str-el

Itinerant and topological excitations in a honeycomb spiral spin liquid candidate

The frustrated insulating magnet can stabilize a spiral spin liquid, arising from cooperative fluctuations among a subextensively degenerate manifold of spiral configurations, with ground-state wave vectors forming a continuous contour or surface in reciprocal space. The atomic-mixing-free honeycomb antiferromagnet GdZnPO has recently emerged as a promising spiral spin-liquid candidate, hosting nontrivial topological excitations. Despite growing interest, the transport and topological properties of spiral spin liquids remain largely unexplored experimentally. Here, we report transport measurements on high-quality, electrically insulating GdZnPO single crystals. We observe a giant low-temperature magnetic thermal conductivity down to $\sim$50 mK, described by $\kappa_{xx}^\mathrm{m}$ $\sim$ $\kappa_0+\kappa_1T$, where both $\kappa_0$ and $\kappa_1$ are positive constants associated with excitations along and off the spiral contour in reciprocal space, respectively. This behavior parallels the magnetic specific heat, underscoring the presence of mobile low-energy excitations intrinsic to the putative spiral spin liquid. Furthermore, the observed positive thermal Hall effect confirms the topological nature of at least some of these excitations. Our findings provide key insights into the itinerant and topological properties of low-lying spin excitations in the spiral spin-liquid candidate.

cond-mat.str-el

Giant Magnetocaloric Effect in a Honeycomb Spiral Spin-Liquid Candidate

Unlike conventional magnetic states, which lack degeneracy, the spiral spin liquid (SSL) fluctuates among degenerate spiral configurations, with ground-state wave vectors forming a continuous contour or surface in reciprocal space. At low temperatures, the field-induced crossover from the polarized ferromagnetic state to the SSL results in a large entropy increase and decalescence, indicating its potential for magnetic cooling. However, magnetic cooling using a SSL has yet to be reported. Here, we investigate the magnetocaloric effect and cooling performance of single-crystal GdZnPO, a spin-7/2 honeycomb-lattice SSL candidate, under a magnetic field $H$ $<$ $H_\mathrm{c}$ ($\mu_0H_\mathrm{c}$ $\sim$ 12 T) applied perpendicular to the honeycomb plane and below the crossover temperature ($\sim$2 K). For $H$ $\geq$ $H_\mathrm{c}$, GdZnPO enters a polarized non-degenerate ferromagnetic state. Our results demonstrate that GdZnPO exhibits a giant low-temperature magnetocaloric effect near $H_\mathrm{c}$, surpassing other magnetocaloric materials. This giant magnetocaloric effect is well-explained by the frustrated honeycomb spin model of GdZnPO, suggesting the stability of the SSL below $H_\mathrm{c}$ down to very low temperatures. Additionally, its magnetic cooling performance remains robust up to at least 4.5 K, making GdZnPO a promising candidate for magnetic refrigeration down to $\sim$36 mK through cycling the applied magnetic field within a narrow range.

cond-mat.str-el

Detecting multiple change points in linear models with heteroscedasticity

The problem of detecting change points in the parameters of a linear regression model with errors and covariates exhibiting heteroscedasticity is considered. Asymptotic results for weighted functionals of the cumulative sum (CUSUM) processes of model residuals are established when the model errors are weakly dependent and non-stationary, allowing for either abrupt or smooth changes in their variance. These theoretical results illuminate how to adapt standard change point test statistics for linear models to this setting. We studied such adapted change-point tests in simulation experiments, along with a finite sample adjustment to the proposed testing procedures. The results suggest that these methods perform well in practice for detecting multiple change points in the linear model parameters and controlling the Type I error rate in the presence of heteroscedasticity. We illustrate the use of these approaches in applications to test for instability in predictive regression models and explanatory asset pricing models.

econ.EM

Spiral spin liquid in a frustrated honeycomb antiferromagnet: A single-crystal study of GdZnPO

The frustrated honeycomb spin model can stabilize a subextensively degenerate spiral spin liquid with nontrivial topological excitations and defects, but its material realization remains rare. Here, we report the experimental realization of this model in the structurally disorder-free compound GdZnPO. Using a single-crystal sample, we find that spin-7/2 rare-earth Gd$^{3+}$ ions form a honeycomb lattice with dominant second-nearest-neighbor antiferromagnetic and first-nearest-neighbor ferromagnetic couplings, along with easy-plane single-site anisotropy. This frustrated model stabilizes a unique spiral spin liquid with a degenerate contour around the $\mathrm{K}$$\{$1/3,1/3$\}$ point in reciprocal space, consistent with our experiments down to 30 mK, including the observation of a giant residual specific heat. Our results establish GdZnPO as an ideal platform for exploring the stability of spiral spin liquids and their novel properties, such as the emergence of low-energy topological defects on the sublattices.

cond-mat.str-el

Quantum annealing of a frustrated magnet

Quantum annealing, which involves quantum tunnelling among possible solutions, has state-of-the-art applications not only in quickly finding the lowest-energy configuration of a complex system, but also in quantum computing. Here we report a single-crystal study of the frustrated magnet $α$-CoV$_2$O$_6$, consisting of a triangular arrangement of ferromagnetic Ising spin chains without evident structural disorder. We observe quantum annealing phenomena resulting from time-reversal symmetry breaking in a tiny transverse field. Below $\sim$ 1 K, the system exhibits no indication of approaching the lowest-energy state for at least 15 hours in zero transverse field, but quickly converges towards that configuration with a nearly temperature-independent relaxation time of $\sim$ 10 seconds in a transverse field of $\sim$ 3.5 mK. Our many-body simulations show qualitative agreement with the experimental results, and suggest that a tiny transverse field can profoundly enhance quantum spin fluctuations, triggering rapid quantum annealing process from topological metastable Kosterlitz-Thouless phases, at low temperatures.

cond-mat.str-el

Proximate Tomonaga-Luttinger liquid in a spin-1/2 ferromagnetic XXZ chain compound

The spin-1/2 ferromagnetic XXZ chain is a prototypical many-body quantum model, exactly solvable via the integrable Bethe ansatz method, hosting a Tomonaga-Luttinger spin liquid. However, its clear experimental realizations remain absent. Here, we present a thorough investigation of the magnetism of the structurally disorder-free compound LuCu(OH)$_3$SO$_4$. By conducting magnetization and electron-spin-resonance measurements on the single-crystal sample, we establish that the title compound approximates the spin-1/2 ferromagnetic XXZ chain model with a nearest-neighbor exchange strength of $J_1$ $\sim$ 65 K and an easy-plane anisotropy of $\sim$ 0.994. The specific heat demonstrates a distinctive power-law behavior at low magnetic fields (with energy scales $\leq$ 0.02$J_1$) and low temperatures ($T$ $\leq$ 0.03$J_1$). This behavior is consistent with the expectations of the ideal spin-1/2 ferromagnetic XXZ chain model, thereby supporting the formation of a gapless Tomonaga-Luttinger spin liquid in LuCu(OH)$_3$SO$_4$.

cond-mat.str-el

Influence of dark matter equation of state on the axial gravitational ringing of supermassive black holes

In this work, we explore the effects of surrounding dark matter featuring different equations of state on the axial gravitational quasinormal modes of supermassive black holes situated at the center of galaxies. Our attention primarily rests on dark matter exhibiting a spike structure, originating from relativistic Bondi accretion through an adiabatic process, which diminishes at a certain distance from the black hole. We analyze how varying the equation of state of the dark matter influences the properties of the spacetime in the black hole's vicinity. Our findings reveal that different states of dark matter spikes correspondingly affect the black hole's quasinormal modes. In particular, we identify deviations in both the ringing frequency and damping time, reaching magnitudes of up to $10^{-3}$ for certain parameter values. These variations can potentially be detected by upcoming space-borne detectors. Our findings thus indicate the feasibility of discerning and limiting the essential properties of dark matter surrounding supermassive black holes using future gravitational wave detections, particularly in the case of extreme mass ratio inspiral systems.

gr-qc

Expanded-plane bilayer thermal concentrator for improving thermoelectric conversion efficiency

Thermoelectric devices are pivotal in the energy sector, with enhancing their conversion efficiency being a longstanding focal point. While progress has been made, overcoming the inherent low efficiency and heat management issues remains challenging. The advent of thermal metamaterials, particularly thermal concentrators, holds promise for improved thermoelectric efficiency. The concentrator has the potential to amplify the temperature gradient within the working region without altering the temperature gradient of the background, thereby enhancing thermoelectric conversion efficiency through this concentrating effect. Nevertheless, the efficacy of this effect is contingent upon the structural parameters of the concentrator. Systematically investigating the impact of metamaterials on thermoelectric conversion efficiency, particularly in terms of quantifying the enhancement, presents a significant challenge. Additionally, the intrinsic thermal conductivity of the material imposes constraints on the applicability of the concentrator in this regard. In this context, drawing inspiration from the recently proposed passive ultra-conductive heat transport scheme, we have devised expanded-plane bilayer thermal concentrators. We substantiate the prospective performance of our design through analytical demonstration, further validated through finite-element simulations and experiments. Notably, through direct calculation, we illustrate an efficiency improvement of about 38\% when utilizing the expanded-plane concentrator comparing with not using expanded-plane structure. The expanded-plane geometrical configuration of the outer layer can also attain large-scale value. These findings not only present a novel avenue for the functional transformation of thermal metamaterials but also hold significant implications for the field of thermoelectrics.

physics.app-ph

Thermal conduction force under standing and quasi-standing temperature field

Thermal conduction force plays a crucial role in manipulating the local thermal conductivity of crystals. However, due to the diffusive nature of thermal conduction, investigating the force effect is challenging. Recently, researchers have explored the force effect based on the wave-like behavior of thermal conduction, specifically second sound. However, their focus has been primarily on the progressive case, neglecting the more complex standing temperature field case. Additionally, establishing a connection between the results obtained from the progressive case and the standing case poses a challenging problem. In this study, we investigate the force effect of standing and quasi-standing temperature fields, revealing distinct characteristics of thermal conduction force. Moreover, we establish a link between the progressive and standing cases through the quasi-standing case. Our findings pave the way for research in more intricate scenarios and provide an additional degree of freedom for manipulating the local thermal conductivity of dielectric crystals.

physics.app-ph

Intraday FX Volatility-Curve Forecasting with Functional GARCH Approaches

This paper seeks to forecast intraday volatility curves for major foreign exchange (FX) currencies using functional GARCH models. Intraday return curves are observed at a daily frequency, yet preserve the full high-frequency trading structure, enabling volatility analysis at the intraday level. We demonstrate that the USD/EUR, USD/GBP, and USD/JPY intraday return curves exhibit strong cross-dependence, while individually they are serially uncorrelated but display long-range conditional heteroskedasticity. Embedding cross-currency dependence via multi-level functional principal component analysis and adding intraday bid-ask spread curves as exogenous drivers significantly improves intraday and day-ahead volatility forecasts relative to functional and realised-volatility baselines. The precise volatility forecasts motivate the construction of intraday Value-at-Risk (VaR). An intraday risk management application highlights that predicted intraday VaR curves can help mitigate dramatic losses in intraday trading strategies, showcasing their practical economic benefits in FX markets.

stat.ME

Ultrasonic investigation of the Kondo semimetal CeBi

We report the elastic properties of the Kondo semimetal CeBi by resonant ultrasound spectroscopy measurements at zero magnetic field. Clear elastic softening is found in bulk modulus $C_B$ below $\sim 60$ K. Such a softening in $C_B$, in addition to the anomalous temperature dependent Poisson's ratio, is hardly attributable to multipolar response for stable localized $4f$ orbital, but can be well described by a two-band model arising from the hybridization between conduction- and $4f$- electrons. These results probably are consequences of the valence fluctuations in this Kondo semimetal as originally suggested by a Fermi-surface expansion observed in a previous angle-resolved photoemission spectroscopy study [P. Li \textit{et al.}, Phys. Rev. B $\mathbf{100}$, 155110 (2019)].

cond-mat.str-el

CancerUniT: Towards a Single Unified Model for Effective Detection, Segmentation, and Diagnosis of Eight Major Cancers Using a Large Collection of CT Scans

Human readers or radiologists routinely perform full-body multi-organ multi-disease detection and diagnosis in clinical practice, while most medical AI systems are built to focus on single organs with a narrow list of a few diseases. This might severely limit AI's clinical adoption. A certain number of AI models need to be assembled non-trivially to match the diagnostic process of a human reading a CT scan. In this paper, we construct a Unified Tumor Transformer (CancerUniT) model to jointly detect tumor existence & location and diagnose tumor characteristics for eight major cancers in CT scans. CancerUniT is a query-based Mask Transformer model with the output of multi-tumor prediction. We decouple the object queries into organ queries, tumor detection queries and tumor diagnosis queries, and further establish hierarchical relationships among the three groups. This clinically-inspired architecture effectively assists inter- and intra-organ representation learning of tumors and facilitates the resolution of these complex, anatomically related multi-organ cancer image reading tasks. CancerUniT is trained end-to-end using a curated large-scale CT images of 10,042 patients including eight major types of cancers and occurring non-cancer tumors (all are pathology-confirmed with 3D tumor masks annotated by radiologists). On the test set of 631 patients, CancerUniT has demonstrated strong performance under a set of clinically relevant evaluation metrics, substantially outperforming both multi-disease methods and an assembly of eight single-organ expert models in tumor detection, segmentation, and diagnosis. This moves one step closer towards a universal high performance cancer screening tool.

eess.IV

The Axial Gravitational Ringing of a Spherically Symmetric Black Hole Surrounded by Dark Matter Spike

Supermassive black holes at the center of each galaxy may be surrounded by dark matter. Such dark matter admits a spike structure and vanishes at a certain distance from the black hole. This dark matter will impact the spacetime near the black hole and the related ringing gravitational waves can show distinguished features of the black hole without dark matter. In the present work, we focus on the quasi-normal modes of the axial gravitational perturbation who dominate the ringdown process of the perturbed black holes surrounded by dark matter spikes. The relativistic modification results in less impact on QNMs. And the relative ringing frequency difference between the black holes with and without dark matter can be as large as $10^{-2}$. These features can be used in future gravitational wave detection about extremal mass ratio inspiral systems to probe the existence of dark matter around supermassive black holes.

gr-qc

IMKGA-SM: Interpretable Multimodal Knowledge Graph Answer Prediction via Sequence Modeling

Multimodal knowledge graph link prediction aims to improve the accuracy and efficiency of link prediction tasks for multimodal data. However, for complex multimodal information and sparse training data, it is usually difficult to achieve interpretability and high accuracy simultaneously for most methods. To address this difficulty, a new model is developed in this paper, namely Interpretable Multimodal Knowledge Graph Answer Prediction via Sequence Modeling (IMKGA-SM). First, a multi-modal fine-grained fusion method is proposed, and Vgg16 and Optical Character Recognition (OCR) techniques are adopted to effectively extract text information from images and images. Then, the knowledge graph link prediction task is modelled as an offline reinforcement learning Markov decision model, which is then abstracted into a unified sequence framework. An interactive perception-based reward expectation mechanism and a special causal masking mechanism are designed, which "converts" the query into an inference path. Then, an autoregressive dynamic gradient adjustment mechanism is proposed to alleviate the insufficient problem of multimodal optimization. Finally, two datasets are adopted for experiments, and the popular SOTA baselines are used for comparison. The results show that the developed IMKGA-SM achieves much better performance than SOTA baselines on multimodal link prediction datasets of different sizes.

cs.AI

Quasi Normal Modes of Black Holes and Detection in Ringdown Process

Quasi-normal modes (QNMs) of a black hole (BH) are the eigen modes describing the dissipative oscillation of various fields in that spacetime, which can be intrinsically produced by the linear perturbation theory. With the discovery of the first gravitational waves (GWs) event, GW150914, a new window into the universe has been opened, allowing for the detection of QNMs associated to the ringdown process, which will enable more accurate measurements of the BHs parameters as well as further testing of general relativity. This article discusses the linear perturbation theory of BHs and provides review of several QNMs calculation methods including the newly developed methods. We will also focus on the connection between QNMs and the detection of GWs as well as some recent advancements in this area.

gr-qc

Electrical transport and magnetic properties of the triangular-lattice compound Zr$_2$NiP$_2$

We report the first investigation of the electrical and magnetic properties of the triangular-lattice compound Zr$_2$NiP$_2$ (space group $P$6$_3$/$mmc$). The temperature evolution of electrical resistivity follows the Bloch-Grüneisen-Mott law, and exhibits a typically metallic behavior. No transition is visible by both electrical and magnetic property measurements, and nearly no magnetization is detected ($M_0$ $<$ 0.002$μ_\mathrm{B}$/Ni) down to 1.8 K up to 7 T. The metallic and nonmagnetic characters are well understood by the first-principles calculations for Zr$_2$NiP$_2$.

cond-mat.mtrl-sci

Possible coexistence of short-range resonating-valence-bond and long-range stripe correlations in the spatially anisotropic triangular-lattice quantum magnet Cu$_2$(OH)$_3$NO$_3$

We show that short-range resonating-valence-bond correlations and long-range order can coexist in the ground state (GS) of a frustrated spin system. Our study comprises a comprehensive investigation of the quantum magnetism on the structurally disorder-free single crystal of Cu$_2$(OH)$_3$NO$_3$, which realizes the $s$ = 1/2 Heisenberg model on a spatially anisotropic triangular lattice. Competing exchange interactions determined by fitting the magnetization measured up to 55 T give rise to an exotic GS wavefunction with coexistence of the dominant short-range resonating-valence-bond correlations and weak long-range stripe order (ordered moment $M_0$ = $|\langle s_i^z\rangle|$ $\sim$ 0.02). At low temperatures, a first-order spin-flop transition is visible at $\sim$ 1-3 T. As the applied field further increases, another two magnetic-field-induced quantum phase transitions are observed at $\sim$ 14-19 and $\sim$ 46-52 T, respectively. Simulations of the Heisenberg exchange model show semi-quantitative agreement with the magnetic-field modulation of these unconventional phases, as well as the absence of visible magnetic reflections in neutron diffraction, thus supporting the GS of the spin system of Cu$_2$(OH)$_3$NO$_3$ may be approximate to a quantum spin liquid. Our study establishes structurally disorder-free magnetic materials with spatially anisotropic exchange interactions as a possible arena for spin liquids.

cond-mat.str-el