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Yuri Aikawa

Publications and source records attributed to Yuri Aikawa.

At least 145 records · Page 8Linked to original sources

Chemistry in a forming protoplanetary disk: main accretion phase

We investigate the chemistry in a radiation-hydrodynamics model of star-forming core which evolves from a cold ($\sim 10$ K) prestellar core to the main accretion phase in $\sim 10^5$ yr. A rotationally-supported gravitationally unstable disk is formed around a protostar. We extract the temporal variation of physical parameters in $\sim 1.5 \times 10^3$ SPH particles which end up in the disk, and perform post-processing calculations of the gas-grain chemistry adopting a three-phase model. Inside the disk, the SPH particles migrate both inward and outward. Since a significant fraction of volatiles such as CO can be trapped in the water-dominant ice in the three-phase model, the ice mantle composition depends not only on the current position in the disk but also on whether the dust grain has ever experienced higher temperatures than the water sublimation temperature. Stable molecules such as H$_2$O, CH$_4$, NH$_3$ and CH$_3$OH are already abundant at the onset of gravitational collapse and simply sublimated as the fluid parcels migrate inside the water snow line. On the other hand, various molecules such as carbon chains and complex organic molecules (COMs) are formed in the disk. COMs abundance sensitively depends on the outcomes of photodissociation and diffusion rates of photofragments in bulk ice mantle. As for S-bearing species, H$_2$S ice is abundant in the collapse phase. In the warm regions in the disk, H$_2$S is sublimated to be destroyed, while SO, H$_2$CS, OCS and SO$_2$ become abundant.

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ALMA reveals the anatomy of the mm-sized dust and molecular gas in the HD 97048 disk

Transitional disks show a lack of excess emission at infrared wavelengths due to a large dust cavity, that is often corroborated by spatially resolved observations at ~ mm wavelengths. We present the first spatially resolved ~ mm-wavelength images of the disk around the Herbig Ae/Be star, HD 97048. Scattered light images show that the disk extends to ~640 au. The ALMA data reveal a circular-symmetric dusty disk extending to ~350 au, and a molecular disk traced in CO J=3-2 emission, extending to ~750 au. The CO emission arises from a flared layer with an opening angle ~ 30 deg - 40 deg. HD 97048 is another source for which the large (~ mm-sized) dust grains are more centrally concentrated than the small (~ μm-sized) grains and molecular gas, likely due to radial drift. The images and visibility data modelling suggests a decrement in continuum emission within ~50 au, consistent with the cavity size determined from mid-infrared imaging (34 +/- 4 au). The extracted continuum intensity profiles show ring-like structures with peaks at ~50, 150, and 300 au, with associated gaps at ~100 and 250 au. This structure should be confirmed in higher-resolution images (FWHM ~ 10 - 20 au). These data confirm the classification of HD 97048 as a transitional disk that also possesses multiple ring-like structures in the dust continuum emission. Additional data are required at multiple and well-separated frequencies to fully characterise the disk structure, and thereby constrain the mechanism(s) responsible for sculpting the HD 97048 disk.

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Discovery of a Hot Corino in the Bok Globule B335

We report the first evidence of a hot corino in a Bok globule. This is based on the ALMA observations in the 1.2 mm band toward the low-mass Class 0 protostar IRAS 19347+0727 in B335. Saturated complex organic molecules (COMs), CH$_3$CHO, HCOOCH$_3$, and NH$_2$CHO, are detected in a compact region within a few 10 au around the protostar. Additionally, CH$_3$OCH$_3$, C$_2$H$_5$OH, C$_2$H$_5$CN, and CH$_3$COCH$_3$ are tentatively detected. Carbon-chain related molecules, CCH and c-C$_3$H$_2$, are also found in this source, whose distributions are extended over a few 100 au scale. On the other hand, sulfur-bearing molecules CS, SO, and SO$_2$, have both compact and extended components. Fractional abundances of the COMs relative to H$_2$ are found to be comparable to those in known hot-corino sources. Though the COMs lines are as broad as 5-8 km s$^{-1}$, they do not show obvious rotation motion in the present observation. Thus, the COMs mainly exist in a structure whose distribution is much smaller than the synthesized beam (0."58 x 0."52).

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Spectral Line Survey toward a Molecular Cloud in IC10

We have conducted a spectral line survey observation in the 3 mm band toward the low-metallicity dwarf galaxy IC10 with the 45 m radio telescope of Nobeyama Radio Observatory to explore its chemical composition at a molecular-cloud scale (~80 pc). The CS, SO, CCH, HCN, HCO+, and HNC lines are detected for the first time in this galaxy in addition to the CO and 13CO lines, while c-C3H2, CH3OH, CN, C18O, and N2H+ lines are not detected. The spectral intensity pattern is found to be similar to those observed toward molecular clouds in the Large Magellanic Cloud, whose metallicity is as low as IC10. Nitrogen-bearing species are deficient in comparison with the Galactic molecular clouds due to a lower elemental abundance of nitrogen. CCH is abundant in comparison with Galactic translucent clouds, whereas CH3OH may be deficient. These characteristic trends for CCH and CH3OH are also seen in the LMC, and seem to originate from photodissociation regions more extended in peripheries of molecular clouds due to the lower metallicity condition.

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First detection of gas-phase methanol in a protoplanetary disk

The first detection of gas-phase methanol in a protoplanetary disk (TW Hya) is presented. In addition to being one of the largest molecules detected in disks to date, methanol is also the first disk organic molecule with an unambiguous ice chemistry origin. The stacked methanol emission, as observed with ALMA, is spectrally resolved and detected across six velocity channels ($>3 σ$), reaching a peak signal-to-noise of $5.5σ$, with the kinematic pattern expected for TW~Hya. Using an appropriate disk model, a fractional abundance of $3\times 10^{-12} - 4 \times 10^{-11}$ (with respect to H$_2$) reproduces the stacked line profile and channel maps, with the favoured abundance dependent upon the assumed vertical location (midplane versus molecular layer). The peak emission is offset from the source position suggesting that the methanol emission has a ring-like morphology: the analysis here suggests it peaks at $\approx 30$~AU reaching a column density $\approx 3-6\times10^{12}$~cm$^{-2}$. In the case of TW Hya, the larger (up to mm-sized) grains, residing in the inner 50~AU, may thus host the bulk of the disk ice reservoir. The successful detection of cold gas-phase methanol in a protoplanetary disk implies that the products of ice chemistry can be explored in disks, opening a window to studying complex organic chemistry during planetary system formation.

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Detection of a hot molecular core in the Large Magellanic Cloud with ALMA

We report the first detection of a hot molecular core outside our Galaxy based on radio observations with ALMA toward a high-mass young stellar object (YSO) in a nearby low metallicity galaxy, the Large Magellanic Cloud (LMC). Molecular emission lines of CO, C17O, HCO+, H13CO+, H2CO, NO, SiO, H2CS, 33SO, 32SO2, 34SO2, and 33SO2 are detected from a compact region (0.1 pc) associated with a high-mass YSO, ST11. The temperature of molecular gas is estimated to be higher than 100 K based on rotation diagram analysis of SO2 and 34SO2 lines. The compact source size, warm gas temperature, high density, and rich molecular lines around a high-mass protostar suggest that ST11 is associated with a hot molecular core. We find that the molecular abundances of the LMC hot core are significantly different from those of Galactic hot cores. The abundances of CH3OH, H2CO, and HNCO are remarkably lower compared with Galactic hot cores by at least 1-3 orders of magnitude. We suggest that these abundances are characterized by the deficiency of molecules whose formation requires the hydrogenation of CO on grain surfaces. In contrast, NO shows a high abundance in ST11 despite the notably low abundance of nitrogen in the LMC. A multitude of SO2 and its isotopologue line detections in ST11 imply that SO2 can be a key molecular tracer of hot core chemistry in metal-poor environments. Furthermore, we find molecular outflows around the hot core, which is the second detection of an extragalactic protostellar outflow. In this paper, we discuss physical and chemical characteristics of a hot molecular core in the low metallicity environment.

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Subarcsecond Analysis of Infalling-Rotating Envelope around the Class I Protostar IRAS 04365+2535

Sub-arcsecond images of the rotational line emission of CS and SO have been obtained toward the Class I protostar IRAS 04365$+$2535 in TMC-1A with ALMA. A compact component around the protostar is clearly detected in the CS and SO emission. The velocity structure of the compact component of CS reveals infalling-rotating motion conserving the angular momentum. It is well explained by a ballistic model of an infalling-rotating envelope with the radius of the centrifugal barrier (a half of the centrifugal radius) of 50 AU, although the distribution of the infalling gas is asymmetric around the protostar. The distribution of SO is mostly concentrated around the radius of the centrifugal barrier of the simple model. Thus a drastic change in chemical composition of the gas infalling onto the protostar is found to occur at a 50 AU scale probably due to accretion shocks, demonstrating that the infalling material is significantly processed before being delivered into the disk.

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Spectral Line Survey toward Molecular Clouds in the Large Magellanic Cloud

Spectral line survey observations of 7 molecular clouds in the Large Magellanic Cloud (LMC) have been conducted in the 3 mm band with the Mopra 22 m telescope to reveal chemical compositions in low metallicity conditions. Spectral lines of fundamental species such as CS, SO, CCH, HCN, HCO+, and HNC are detected in addition to those of CO and 13CO, while CH3OH is not detected in any source and N2H+ is marginally detected in two sources. The molecular-cloud scale (10 pc scale) chemical composition is found to be similar among the 7 sources regardless of different star formation activities, and hence, it represents the chemical composition characteristic to the LMC without influences of star formation activities. In comparison with chemical compositions of Galactic sources, the characteristic features are (1) deficient N-bearing molecules, (2) abundant CCH, and (3) deficient CH3OH. The feature (1) is due to a lower elemental abundance of nitrogen in the LMC, whereas the features (2) and (3) seem to originate from extended photodissociation regions and warmer temperature in cloud peripheries due to a lower abundance of dust grains in the low metallicity condition. In spite of general resemblance of chemical abundances among the seven sources, the CS/HCO+ and SO/HCO+ ratios are found to be slightly higher in a quiescent molecular cloud. An origin of this trend is discussed in relation to possible depletion of sulfur along molecular cloud formation.

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Methane clathrates in the Solar System

We review the reservoirs of methane clathrates that may exist in the different bodies of the Solar System. Methane was formed in the interstellar medium prior to having been embedded in the protosolar nebula gas phase. This molecule was subsequently trapped in clathrates that formed from crystalline water ice during the cooling of the disk and incorporated in this form in the building blocks of comets, icy bodies, and giant planets. Methane clathrates may play an important role in the evolution of planetary atmospheres. On Earth, the production of methane in clathrates is essentially biological, and these compounds are mostly found in permafrost regions or in the sediments of continental shelves. On Mars, methane would more likely derive from hydrothermal reactions with olivine-rich material. If they do exist, martian methane clathrates would be stable only at depth in the cryosphere and sporadically release some methane into the atmosphere via mechanisms that remain to be determined.

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Double DCO+ rings reveal CO ice desorption in the outer disk around IM Lup

In a protoplanetary disk, a combination of thermal and non-thermal desorption processes regulate where volatiles are liberated from icy grain mantles into the gas phase. Non-thermal desorption should result in volatile-enriched gas in disk-regions where complete freeze-out is otherwise expected. We present ALMA observations of the disk around the young star IM Lup in 1.4 mm continuum, C18O 2-1, H13CO+ 3-2 and DCO+ 3-2 emission at ~0".5 resolution. The images of these dust and gas tracers are clearly resolved. The DCO+ line exhibits a striking pair of concentric rings of emission that peak at radii of ~0".6 and 2" (~90 and 300 AU, respectively). Based on disk chemistry model comparison, the inner DCO+ ring is associated with the balance of CO freeze-out and thermal desorption due to a radial decrease in disk temperature. The outer DCO+ ring is explained by non-thermal desorption of CO ice in the low-column-density outer disk, repopulating the disk midplane with cold CO gas. The CO gas then reacts with abundant H2D+ to form the observed DCO+ outer ring. These observations demonstrate that spatially resolved DCO+ emission can be used to trace otherwise hidden cold gas reservoirs in the outmost disk regions, opening a new window onto their chemistry and kinematics.

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ALMA Observations of the Transition from Infall Motion to Keplerian Rotation around the Late-phase Protostar TMC-1A

We have observed the Class I protostar TMC-1A with Atacama Millimeter/submillimeter Array (ALMA) in 12CO and C18O (J=2-1), and 1.3-mm dust continuum emission. Continuum emission with a deconvolved size of 0.50"x0.37", perpendicular to the 12CO outflow, is detected. It most likely traces a circumstellar disk around TMC-1A, as previously reported. In contrast, a more extended structure is detected in C18O although it is still elongated with a deconvolved size of 3.3"x2.2", indicating that C18O traces mainly a flattened envelope surrounding the disk and the central protostar. C18O shows a clear velocity gradient perpendicular to the outflow at higher velocities, indicative of rotation, while an additional velocity gradient along the outflow is found at lower velocities. The radial profile of the rotational velocity is analyzed in detail, finding that it is given as a power-law \propto r^{-a} with an index of ~0.5 at higher velocities. This suggests that the rotation at higher velocities can be explained as Keplerian rotation orbiting a protostar with a dynamical mass of 0.68 Mo (inclination-corrected). The additional velocity gradient of C18O along the outflow is considered to be mainly infall motions in the envelope. Position-Velocity diagrams made from models consisting of an infalling envelope and a Keplerian disk are compared with the observations, revealing that the observed infall velocity is ~0.3 times smaller than the free fall velocity yielded by the dynamical mass of the protostar. Magnetic fields could be responsible for the slow infall velocity. A possible scenario of Keplerian disk formation is discussed.

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Analytical Formulas of Molecular Ion Abundances and N2H+ Ring in Protoplanetary Disks

We investigate the chemistry of ion molecules in protoplanetary disks, motivated by the detection of N$_2$H$^+$ ring around TW Hya. While the ring inner radius coincides with the CO snow line, it is not apparent why N$_2$H$^+$ is abundant outside the CO snow line in spite of the similar sublimation temperatures of CO and N$_2$. Using the full gas-grain network model, we reproduced the N$_2$H$^+$ ring in a disk model with millimeter grains. The chemical conversion of CO and N$_2$ to less volatile species (sink effect hereinafter) is found to affect the N$_2$H$^+$ distribution. Since the efficiency of the sink depends on various parameters such as activation barriers of grain surface reactions, which are not well constrained, we also constructed the no-sink model; the total (gas and ice) CO and N$_2$ abundances are set constant, and their gaseous abundances are given by the balance between adsorption and desorption. Abundances of molecular ions in the no-sink model are calculated by analytical formulas, which are derived by analyzing the full-network model. The N$_2$H$^+$ ring is reproduced by the no-sink model, as well. The 2D (R-Z) distribution of N$_2$H$^+$, however, is different among the full-network model and no-sink model. The column density of N$_2$H$^+$ in the no-sink model depends sensitively on the desorption rate of CO and N$_2$, and the flux of cosmic ray. We also found that N$_2$H$^+$ abundance can peak at the temperature slightly below the CO sublimation, even if the desorption energies of CO and N$_2$ are the same.

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The cometary composition of a protoplanetary disk as revealed by complex cyanides

Observations of comets and asteroids show that the Solar Nebula that spawned our planetary system was rich in water and organic molecules. Bombardment brought these organics to the young Earth's surface, seeding its early chemistry. Unlike asteroids, comets preserve a nearly pristine record of the Solar Nebula composition. The presence of cyanides in comets, including 0.01% of methyl cyanide (CH3CN) with respect to water, is of special interest because of the importance of C-N bonds for abiotic amino acid synthesis. Comet-like compositions of simple and complex volatiles are found in protostars, and can be readily explained by a combination of gas-phase chemistry to form e.g. HCN and an active ice-phase chemistry on grain surfaces that advances complexity[3]. Simple volatiles, including water and HCN, have been detected previously in Solar Nebula analogues - protoplanetary disks around young stars - indicating that they survive disk formation or are reformed in situ. It has been hitherto unclear whether the same holds for more complex organic molecules outside of the Solar Nebula, since recent observations show a dramatic change in the chemistry at the boundary between nascent envelopes and young disks due to accretion shocks[8]. Here we report the detection of CH3CN (and HCN and HC3N) in the protoplanetary disk around the young star MWC 480. We find abundance ratios of these N-bearing organics in the gas-phase similar to comets, which suggests an even higher relative abundance of complex cyanides in the disk ice. This implies that complex organics accompany simpler volatiles in protoplanetary disks, and that the rich organic chemistry of the Solar Nebula was not unique.

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Evidence for DCO+ as a probe of ionization in the warm disk surface

In this Letter we model the chemistry of DCO$^{+}$ in protoplanetary disks. We find that the overall distribution of the DCO$^{+}$ abundance is qualitatively similar to that of CO but is dominated by thin layer located at the inner disk surface. To understand its distribution, we investigate the different key gas-phase deuteration pathways that can lead to the formation of DCO$^{+}$. Our analysis shows that the recent update in the exothermicity of the reaction involving CH$_2$D$^{+}$ as a parent molecule of DCO$^{+}$ favors deuterium fractionation in warmer conditions. As a result the formation of DCO$^{+}$ is enhanced in the inner warm surface layers of the disk where X-ray ionization occurs. Our analysis points out that DCO$^{+}$ is not a reliable tracer of the CO snow line as previously suggested. We thus predict that DCO$^{+}$ is a tracer of active deuterium and in particular X-ray ionization of the inner disk.

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ALMA Observations of the IRDC Clump G34.43+00.24 MM3: DNC/HNC Ratio

We have observed the clump G34.43+00.24 MM3 associated with an infrared dark cloud in DNC $J$=3--2, HN$^{13}$C $J$=3--2, and N$_2$H$^+$ $J$=3--2 with the Atacama Large Millimeter/submillimeter Array (ALMA). The N$_2$H$^+$ emission is found to be relatively weak near the hot core and the outflows, and its distribution is clearly anti-correlated with the CS emission. This result indicates that a young outflow is interacting with cold ambient gas. The HN$^{13}$C emission is compact and mostly emanates from the hot core, whereas the DNC emission is extended around the hot core. Thus, the DNC and HN$^{13}$C emission traces warm regions near the protostar differently. The DNC emission is stronger than the HN$^{13}$C emission toward most parts of this clump. The DNC/HNC abundance ratio averaged within a $15^{\prime\prime} \times 15^{\prime\prime}$ area around the phase center is higher than 0.06. This ratio is much higher than the value obtained by the previous single-dish observations of DNC and HN$^{13}$C $J$=1--0 ($\sim$0.003). It seems likely that the DNC and HNC emission observed with the single-dish telescope traces lower density envelopes, while that observed with ALMA traces higher density and highly deuterated regions. We have compared the observational results with chemical-model results in order to investigate the behavior of DNC and HNC in the dense cores. Taking these results into account, we suggest that the low DNC/HNC ratio in the high-mass sources obtained by the single-dish observations are at least partly due to the low filling factor of the high density regions.

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Evaporation of grain-surface species by shock waves in proto-planetary disk

Recent ALMA (Atacama Large Millimeter/submillimeter Array) observations of young protostellar objects detected warm SO emission, which could be associated with a forming protostellar disk. In order to investigate if such warm gas can be produced by accretion shock onto the forming disk, we calculate the sputtering and thermal desorption of various grain surface species in one dimensional shock waves. We find that thermal desorption is much more efficient than the sputtering in the post-shock region. While H$_{2}$O can be thermally desorbed, if the accretion velocity is larger than 8 km s$^{-1}$ with the pre-shock gas number density of 10$^{9}$ cm$^{-3}$, SO is desorbed, if the accretion velocity $\gtrsim$ 2 km s$^{-1}$ and $\gtrsim$ 4km s$^{-1}$, with the pre-shock density of 10$^{9}$ cm$^{-3}$ and 10$^{8}$ cm$^{-3}$, respectively. We also find that the column density of hydrogen nuclei in warm post-shock gas is $N_{\rm warm} \sim 10^{21}$ cm$^{-2}$.

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ALMA Observations of the IRDC Clump G34.43+00.24 MM3: 278 GHz Class I Methanol Masers

We have observed a molecular clump (MM3) associated with the infrared dark cloud G34.43+00.24 in the CH3OH J_K=9_{-1}--8_0 E, 5_0-4_0 E, and 5_{-1}-4_{-1} E lines at sub-arcsecond resolution by using the Atacama Large Millimeter/submillimeter Array. By comparing the CH3OH J_K=9_{-1}-8_0 E emission with the CH3OH 5_0-4_0 E and 5_{-1}-4_{-1} E emission, we have found that the CH3OH J_K=9_{-1}-8_0 E emission is masing. We have clearly shown that the CH3OH J_K=9_{-1}-8_0 masers arise from the post shocked gas in the interacting regions between the outflows and ambient dense gas. Toward the strongest peak of the CH3OH maser emission, SiO J=6-5 emission is very weak. This indicates that the CH3OH maser emission traces relatively old shocks or weak shocks.

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Formation of a Keplerian disk in the infalling envelope around L1527 IRS: transformation from infalling motions to Kepler motions

We report Atacama Large Millimeter/submillimeter Array (ALMA) cycle 0 observations of C$^{18}$O ($J=2-1$), SO ($J_N= 6_5-5_4$) and 1.3mm dust continuum toward L1527 IRS, a class 0 solar-type protostar surrounded by an infalling and rotating envelope. C$^{18}$O emission shows strong redshifted absorption against the bright continuum emission associated with L1527 IRS, strongly suggesting infall motions in the C$^{18}$O envelope. The C$^{18}$O envelope also rotates with a velocity mostly proportional to $r^{-1}$, where $r$ is the radius, while the rotation profile at the innermost radius (54 AU) may be shallower than $r^{-1}$, suggestive of formation of a Keplerian disk around the central protostar of 0.3 Mo in dynamical mass. SO emission arising from the inner part of the C$^{18}$O envelope also shows rotation in the same direction as the C$^{18}$O envelope. The rotation is, however, rigid-body like which is very different from the differential rotation shown by C$^{18}$O. In order to explain the line profiles and the position-velocity (PV) diagrams of C$^{18}$O and SO observed, simple models composed of an infalling envelope surrounding a Keplerian disk of 54 AU in radius orbiting a star of 0.3 Mo are examined. It is found that in order to reproduce characteristic features of the observed line profiles and PV diagrams, the infall velocity in the model has to be smaller than the free-fall velocity yielded by a star of 0.3 Mo. Possible reasons for the reduced infall velocities are discussed.

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