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Yuri Myasoedov

Publications and source records attributed to Yuri Myasoedov.

34 records · Page 2Linked to original sources

Imaging of super-fast dynamics and flow instabilities of superconducting vortices

Quantized magnetic vortices driven by electric current determine key electromagnetic properties of superconductors. While the dynamic behavior of slow vortices has been thoroughly investigated, the physics of ultrafast vortices under strong currents remains largely unexplored. Here we use a nanoscale scanning superconducting quantum interference device to image vortices penetrating into a superconducting Pb film at rates of tens of GHz and moving with velocities up to tens of km/s, which are not only much larger than the speed of sound but also exceed the pair-breaking speed limit of superconducting condensate. These experiments reveal formation of mesoscopic vortex channels which undergo cascades of bifurcations as the current and magnetic field increase. Our numerical simulations predict metamorphosis of fast Abrikosov vortices into mixed Abrikosov-Josephson vortices at even higher velocities. This work offers an insight into the fundamental physics of dynamic vortex states of superconductors at high current densities, crucial for many applications.

cond-mat.supr-con↗

Effects of uniaxial pressure on the quantum tunneling of magnetization in a high-symmetry Mn12 single-molecule magnet

The symmetry of single-molecule magnets dictates their spin quantum dynamics, influencing how such systems relax via quantum tunneling of magnetization (QTM). By reducing a system's symmetry, through the application of a magnetic field or uniaxial pressure, these dynamics can be modified. We report measurements of the magnetization dynamics of a crystalline sample of the high-symmetry [Mn12O12(O2CMe)16(MeOH)4]MeOH single-molecule magnet as a function of uniaxial pressure applied either parallel or perpendicular to the sample's "easy" magnetization axis. At temperatures between 1.8 and 3.3 K, magnetic hysteresis loops exhibit the characteristic steplike features that signal the occurrence of QTM. After applying uniaxial pressure to the sample in situ, both the magnitude and field position of the QTM steps changed. The step magnitudes were observed to grow as a function of pressure in both arrangements of pressure, while pressure applied along (perpendicular to) the sample's easy axis caused the resonant-tunneling fields to increase (decrease). These observations were compared with simulations in which the system's Hamiltonian parameters were changed. From these comparisons, we determined that parallel pressure induces changes to the second-order axial anisotropy parameter as well as either the fourth-order axial or fourth-order transverse parameter, or to both. In addition, we find that pressure applied perpendicular to the easy axis induces a rhombic anisotropy E ~ D/2000 per kbar that can be understood as deriving from a symmetry-breaking distortion of the molecule.

cond-mat.mes-hall↗

Electrically tunable multi-terminal SQUID-on-tip

We present a new nanoscale superconducting quantum interference device (SQUID) whose interference pattern can be shifted electrically in-situ. The device consists of a nanoscale four-terminal/four-junction SQUID fabricated at the apex of a sharp pipette using a self-aligned three-step deposition of Pb. In contrast to conventional two-terminal/two-junction SQUIDs that display optimal sensitivity when flux biased to about a quarter of the flux quantum, the additional terminals and junctions allow optimal sensitivity at arbitrary applied flux, thus eliminating the magnetic field "blind spots". We demonstrate spin sensitivity of 5 to 8 $μ_B/\text{Hz}^{1/2}$ over a continuous field range of 0 to 0.5 T, with promising applications for nanoscale scanning magnetic imaging.

cond-mat.supr-con↗

Emergent nanoscale superparamagnetism at oxide interfaces

Atomically sharp oxide heterostructures exhibit a range of novel physical phenomena that do not occur in the parent bulk compounds. The most prominent example is the appearance of highly conducting and superconducting states at the interface between the band insulators LaAlO3 and SrTiO3. Here we report a new emergent phenomenon at the LaMnO3/SrTiO3 interface in which an antiferromagnetic insulator abruptly transforms into a magnetic state that exhibits unexpected nanoscale superparamagnetic dynamics. Upon increasing the thickness of LaMnO3 above five unit cells, our scanning nanoSQUID-on-tip microscopy shows spontaneous formation of isolated magnetic islands of 10 to 50 nm diameter, which display random moment reversals by thermal activation or in response to an in-plane magnetic field. Our charge reconstruction model of the polar LaMnO3/SrTiO3 heterostructure describes the sharp emergence of thermodynamic phase separation leading to nucleation of metallic ferromagnetic islands in an insulating antiferromagnetic matrix. The model further suggests that the nearby superparamagnetic-ferromagnetic transition can be gate tuned, holding potential for applications in magnetic storage and spintronics.

cond-mat.str-el↗

Probing dynamics and pinning of single vortices in superconductors at nanometer scales

The dynamics of quantized magnetic vortices and their pinning by materials defects determine electromagnetic properties of superconductors, particularly their ability to carry non-dissipative currents. Despite recent advances in the understanding of the complex physics of vortex matter, the behavior of vortices driven by current through a multi-scale potential of the actual materials defects is still not well understood, mostly due to the scarcity of appropriate experimental tools capable of tracing vortex trajectories on nanometer scales. Using a novel scanning superconducting quantum interference microscope we report here an investigation of controlled dynamics of vortices in lead films with sub-Angstrom spatial resolution and unprecedented sensitivity. We measured, for the first time, the fundamental dependence of the elementary pinning force of multiple defects on the vortex displacement, revealing a far more complex behavior than has previously been recognized, including striking spring softening and broken-spring depinning, as well as spontaneous hysteretic switching between cellular vortex trajectories. Our results indicate the importance of thermal fluctuations even at 4.2 K and of the vital role of ripples in the pinning potential, giving new insights into the mechanisms of magnetic relaxation and electromagnetic response of superconductors.

cond-mat.supr-con↗

A three-junction SQUID-on-tip with tunable in-plane and out-of-plane magnetic field sensitivity

Nanoscale superconducting quantum interference devices (SQUIDs) demonstrate record sensitivities to small magnetic moments, but are typically sensitive only to the field component that is normal to the plane of the SQUID and out-of-plane with respect to the scanned surface. We report on a nanoscale three-junction Pb SQUID which is fabricated on the apex of a sharp tip. Because of its three-dimensional structure, it exhibits a unique tunable sensitivity to both in-plane and out-of-plane fields. We analyze the two-dimensional interference pattern from both numerical and experimental points of view. This device is integrated into a scanning microscope and its ability to independently measure the different components of the magnetic field with outstanding spin sensitivity better than $5\ \frac{μ_B}{\mathrm{Hz}^{1/2}}$ is demonstrated. This highlights its potential as a local probe of nanoscale magnetic structures.

cond-mat.supr-con↗

Energy emanating from the molecular nanomagnet Fe$_{8}$ revisited

In the molecular nanomagnet Fe$_{8}$ tunneling can occur from a metastable state to an excited state followed by a transition to the ground state. This transition is accompanied by an energy release of $115.6$GHz. We constructed an experimental setup to measure whether this energy is released in the form of thermal or electromagnetic energy. Contrary to a previous publication we find no evidence for release of electromagnetic radiation. Our results for transitions between the first and second excited states to the ground state are consistent with a release of only thermal energy. This energy release extends for a longer time for the second excited state than for the first excited state.

cond-mat.mes-hall↗

Quantum avalanche in the Fe$_{8}$ Molecular-Magnet

We report spatially resolved, time-dependent, magnetization reversal measurements of an Fe$_{8}$ single molecular magnet using a microscopic Hall bar array. We found that under some conditions the molecules reverse their spin direction at a resonance field in the form of an avalanche. The avalanche front velocity is of the order of $1$m/sec and is sensitive to field gradients and sweep rates. We also measured the propagation velocity of a heat pulse and found that it is much slower than the avalanche velocity. We therefore conclude that in Fe$_{8}$, the avalanche front propagates without thermal assistance.

cond-mat.mes-hall↗

Scanning nano-SQUID with single electron spin sensitivity

One of the critical milestones in the intensive pursuit of quantitative nanoscale magnetic imaging tools is achieving the level of sensitivity required for detecting the field generated by the spin magnetic moment μB of a single electron. Superconducting quantum interference devices (SQUIDs), which were traditionally the most sensitive magnetometers, could not hitherto reach this goal because of their relatively large effective size (of the order of 1 μm). Here we report self-aligned fabrication of nano-SQUIDs with diameters as small as 46 nm and with an extremely low flux noise of 50 nΦ0/Hz^1/2, representing almost two orders of magnitude improvement in spin sensitivity, down to 0.38 μB/Hz^1/2. In addition, the devices operate over a wide range of magnetic fields with 0.6 μB/Hz^1/2 sensitivity even at 1 T. We demonstrate magnetic imaging of vortices in type II superconductor that are 120 nm apart and scanning measurements of AC magnetic fields down to 50 nT. The unique geometry of these nano-SQUIDs that reside on the apex of a sharp tip allows approaching the sample to within a few nm, which paves the way to a new class of single-spin resolved scanning probe microscopy.

cond-mat.supr-con↗

Lamellar mesophase nucleated by Josephson vortices at the melting of the vortex lattice in $Bi_2Sr_2CaCu_2O_{8+delta}$

The local effect of the Josephson vortices on the vortex lattice melting process in \BSCCO crystals in the presence of an in-plane field $H_{ab}$ is studied by differential magneto-optical imaging. The melting process is found to commence along the Josephson vortex stacks, forming a mesomorphic phase of periodic liquid and solid lamellas, the direction and spacing of which are controlled by $H_{ab}$. The reduction of the local melting field $H_m$ along the Josephson vortex stacks is more than an order of magnitude larger than the reduction of the average bulk $H_m$ by $H_{ab}$.

cond-mat.supr-con↗

Suppression of geometrical barrier in $Bi_2Sr_2CaCu_2O_{8+δ}$ crystals by Josephson vortex stacks

Differential magneto-optics are used to study the effect of dc in-plane magnetic field on hysteretic behavior due to geometrical barriers in $Bi_2Sr_2CaCu_2O_{8+δ}$ crystals. In absence of in-plane field a vortex dome is visualized in the sample center surrounded by barrier-dominated flux-free regions. With in-plane field, stacks of Josephson vortices form vortex chains which are surprisingly found to protrude out of the dome into the vortex-free regions. The chains are imaged to extend up to the sample edges, thus providing easy channels for vortex entry and for drain of the dome through geometrical barrier, suppressing the magnetic hysteresis. Reduction of the vortex energy due to crossing with Josephson vortices is evaluated to be about two orders of magnitude too small to account for the formation of the protruding chains. We present a model and numerical calculations that qualitatively describe the observed phenomena by taking into account the demagnetization effects in which flux expulsion from the pristine regions results in vortex focusing and in the chain protrusion. Comparative measurements on a sample with narrow etched grooves provide further support to the proposed model.

cond-mat.supr-con↗

Self-aligned nanoscale SQUID on a tip

A nanometer-sized superconducting quantum interference device (nanoSQUID) is fabricated on the apex of a sharp quartz tip and integrated into a scanning SQUID microscope. A simple self-aligned fabrication method results in nanoSQUIDs with diameters down to 100 nm with no lithographic processing. An aluminum nanoSQUID with an effective area of 0.034 $μ$m$^2$ displays flux sensitivity of 1.8$\cdot 10^{-6}$ $Φ_0/\mathrm{Hz}^{1/2} and operates in fields as high as 0.6 T. With projected spin sensitivity of 65 $μ_B/\mathrm{Hz}^{1/2}$ and high bandwidth, the SQUID on a tip is a highly promising probe for nanoscale magnetic imaging and spectroscopy.

cond-mat.supr-con↗

Multiple Changes of Order of the Vortex Melting Transition in BSCCO with Dilute Columnar Defects

A low concentration of columnar defects is reported to transform a first-order vortex lattice melting line in BSCCO crystals into alternating segments of first-order and second-order transitions separated by two critical points. As the density of CDs is increased, the critical points shift apart and the range of the intermediate second-order transition expands. A third, low temperature critical point was also observed in one sample. The measurement of equilibrium magnetization and the mapping of the melting line down to 27K was made possible by employment of the shaking technique.

cond-mat.supr-con↗

Instabilities in the vortex matter and the peak effect phenomenon

In single crystals of 2H-NbSe2, we identify for the first time a crossover from weak collective to strong pinning regime in the vortex state which is not associated with the peak effect phenomenon. Instead, we find the crossover is associated with anomalous history dependent magnetization response. In the field (Bdc) - temperature (T) vortex matter phase diagram we demarcate this pinning crossover boundary. We also delineate another boundary which separates the strong pinning region from a thermal fluctuation dominated regime, and find that PE appears on this boundary.

cond-mat.supr-con↗

First-order disorder-driven transition and inverse melting of the vortex lattice

Vortex matter phase transitions in the high-temperature superconductor Bi2Sr2CaCu2O8 were studied using local magnetization measurements combined with a vortex 'shaking' technique. The measurements revealed thermodynamic evidence of a first-order transition along the second magnetization peak line, at temperatures below the apparent critical point Tcp. We found that the first-order transition line does not terminate at Tcp, but continues down to at least 30 K. This observation suggests that the ordered vortex lattice phase is destroyed through a unified first-order transition that changes its character from thermally induced melting at high temperatures to a disorder-induced transition at low temperatures. At intermediate temperatures the transition line shows an upturn, which implies that the vortex matter displays 'inverse' melting behavior.

cond-mat.supr-con↗

Inverse melting of the vortex lattice

Inverse melting, in which a crystal reversibly transforms into a liquid or amorphous phase upon decreasing the temperature, is considered to be very rare in nature. The search for such an unusual equilibrium phenomenon is often hampered by the formation of nonequilibrium states which conceal the thermodynamic phase transition, or by intermediate phases, as was recently shown in a polymeric system. Here we report a first-order inverse melting of the magnetic flux line lattice in Bi2Sr2CaCu2O8 superconductor. At low temperatures, the material disorder causes significant pinning of the vortices, which prevents observation of their equilibrium properties. Using a newly introduced 'vortex dithering' technique we were able to equilibrate the vortex lattice. As a result, direct thermodynamic evidence of inverse melting transition is found, at which a disordered vortex phase transforms into an ordered lattice with increasing temperature. Paradoxically, the structurally ordered lattice has larger entropy than the disordered phase. This finding shows that the destruction of the ordered vortex lattice occurs along a unified first-order transition line that gradually changes its character from thermally-induced melting at high temperatures to a disorder-induced transition at low temperatures.

cond-mat.supr-con↗