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Yurii E. Lozovik

Publications and source records attributed to Yurii E. Lozovik.

At least 19 recordsLinked to original sources

Bose-Einstein condensation of THz photons in an optical microcavity with Landau-quantized electrons

We present a theoretical model for a coherent terahertz radiation source based on Bose-Einstein condensate of incoherently pumped microcavity photons. Energy relaxation is provided by inelastic photon scattering on a two-dimensional electron gas in magnetic field. The proposed setup evades the standard lasing mechanisms: neither population inversion nor light wave amplification is utilized. We study the kinetics of photon condensation and describe a semiconductor-crystal based device.

cond-mat.quant-gas↗

Restriction of macroscopic structural superlubricity due to structure relaxation by the example of twisted graphene bilayer

The effect of structure relaxation on the potential energy surface (PES) of interlayer interaction of twisted graphene bilayer is studied for a set of commensurate moiré systems using the registry-dependent empirical potential of Kolmogorov and Crespi. It is found that the influence of structure relaxation on the amplitude of PES corrugations (determining static friction) depends on the unit cell size (or related twist angle) of the moiré system. For moiré systems with the smallest unit cells, the amplitudes of PES corrugations calculated with and without account of structure relaxation are approximately the same. However, for large unit cell sizes, the structure relaxation can lead to an increase of PES corrugations by orders of magnitude. This means that structure relaxation can provide the main contribution into the static friction of a superlubric system under certain conditions (such as the contact size and twist angle). Moreover, the change of the PES type because of structure relaxation from a trigonal lattice of maxima to a trigonal lattice of minima is observed for the systems with the moiré patterns (5,1) and (5,3). Based on the results obtained, possible crossovers between static friction modes taking place upon changing the twist angle in a macroscopic superlubric system consisting of identical layers are discussed. Additionally it is shown that the PES for relaxed structures can still be approximated by the first Fourier harmonics compatible with symmetries of twisted layers analogously to the PES for rigid layers.

cond-mat.mes-hall↗

Photon Bose-Condensate as a Tunable Terahertz Laser Source without Inversion

We develop a theoretical model for a tunable coherent terahertz radiation source based on the long-lived Bose condensate of photons. In the device we propose, the original photon pumping is performed incoherently by a blackbody radiation emitter. The photons thus produced Bose-condense by the inelastic relaxation on a two-dimensional electron gas in a perpendicular magnetostatic field. The process involves neither population inversion nor light wave amplification the standard laser sources are built on. The coherence and tunability of the light emitted by such a photon condensate are provided and supported by the discrete spectrum of the electron gas in the quantizing magnetic field. The device is a compact-size semiconductor crystal. We propose the design and perform the realistic calculations of the physical properties and limiting factors for the terahertz photon Bose-condensate resonator. We show that our terahertz source can deliver the highly coherent light emission in the frequency range of 3-30 THz for the magnetic field induction of the order of 2 T, with the upper emission frequency limit adjustable by the strength of the magnetic field applied.

cond-mat.quant-gas↗

Magnetic and electronic properties of 1D hybrid nanoobjects composed of alternating polycyclic hydrocarbon regions and double carbon chains

It has been proposed recently that 1D hybrid nanoobjects consisting of alternating double carbon chains and polycyclic carbon regions can be obtained from graphene nanoribbons of alternating width by electron irradiation. Here, based on density functional theory calculations, we show that magnetic and electronic properties of such nanoobjects can be changed dramatically by modifying the chain length and edge structure of polycyclic regions and this opens wide possibilities for spintronic applications. Nanoobjects composed of polycyclic regions with dangling bonds and even chains are found to behave as magnetic semiconductors that can generate spin-polarized currents. Band gaps of nanoobjects with odd chains change considerably upon switching between magnetic states making them promising for magnetic tunnel junctions. We also demonstrate that use of a hybrid exchange-correlation functional is important to properly describe stability of magnetic states, band gaps and synergistic effects of nanoobject components leading, for example, to magnetism in even chains.

cond-mat.mes-hall↗

Bose-Einstein condensation in canonical ensemble with fixed total momentum

We consider Bose-Einstein condensation of noninteracting homogeneous three-dimensional gas in canonical ensemble when both particle number $N$ and total momentum $\mathbf{P}$ of all particles are fixed. Using the saddle point method, we derive the large-$N$ analytical approximations for partition function, free energy, and statistical distributions of occupation numbers of different single-particle energy levels. At temperatures below the critical point of phase transition, we predict, in some ranges of $\mathbf{P}$, fragmentation of the condensate, when more than one single-particle level is macroscopically occupied. The occupation number distributions have approximately Gaussian shapes for the levels hosting the condensate, and exponential shapes for other, noncondensate levels. Our analysis demonstrates breaking of Galilean invariance of moving finite-temperature many-particle system in the presence of Bose-Einstein condensation and extends the theory of moving and rotating quantum systems to the finite-temperature large-$N$ limit.

cond-mat.quant-gas↗

Finite-frequency normal and superfluid drag effects in two-component atomic Bose-Einstein condensates

Two-component systems consisting of mutually interacting particles can demonstrate both intracomponent transport effects and intercomponent entrainment (or drag) effects. In the presence of superfluidity, the intracomponent transport is characterized by dissipative conductivity and superfluid weight in the framework of two-fluid model, and intercomponent entrainment gives rise to normal and nondissipative drag effects. We present unified treatment of all these effects for spatially homogeneous two-component atomic Bose-Einstein condensates based on the Bogoliubov theory, focusing specifically on the drag effects. Calculating finite-frequency intra- and intercomponent conductivities with taking into account quasiparticle damping, we derive and numerically check analytical Drude-like approximations applicable at low frequencies, and Lorentz-like approximations applicable at higher frequencies in vicinity of the resonant energy of spin-to-density Bogoliubov quasiparticle conversion. As possible physical realizations of two-component atomic systems, we consider three-dimensional Bose-Bose mixtures and closely spaced two-layered systems of magnetic dipolar atoms.

cond-mat.quant-gas↗

Quantum entanglement of multiple excitons in strained graphene

We studied the effects arising from a coherent source of photons on the entanglement between excitons in a strained graphene monolayer. The graphene layer was considered to be embedded in an imperfect optical microcavity. In our investigation, we have studied the entanglement dynamics of systems consisting of up to five excitons, which are treated as atomic-like qubits. Entangled states of multiple qubits are useful in quantum error correction codes. We have monitored the time evolution of the concurrence, three-$π$, mutual information, and especially the negativity. We have demonstrated that coherent pumping can create lasting entanglement between the excitons. However, the entanglement only persists when the rate at which photons are pumped is smaller than the decay rate of the cavity. Our results show that the degree in entanglement between the excitons is increased with the intensity of the strain-induced pseudomagnetic field in the graphene sheet. Additionally, we have shown that a maximum amount of entanglement occurs at a finite number of excitons in the system which depends on the parameters describing the structure.

cond-mat.mes-hall↗

Drift velocity of edge magnetoplasmons due to magnetic edge channels

Edge magnetoplasmons arise on a boundary of conducting layer in perpendicular magnetic field due to an interplay of electron cyclotron motion and Coulomb repulsion. Lateral electric field, which confines electrons inside the sample, drives their spiraling motion in magnetic field along the edge with the average drift velocity contributing to the total magnetoplasmon velocity. We revisit this classical picture by developing fully quantum theory of drift velocity starting from analysis of magnetic edge channels and their electrodynamic response. We derive the quantum-mechanical expression for the drift velocity, which arises in our theory as a characteristic of such response and can be calculated as harmonic mean of group velocities of edge channels crossing the Fermi level. Using the Wiener-Hopf method to solve analytically the edge mode electrodynamic problem, we demonstrate that the edge channel response effectively enhances the bulk Hall response of the conducting layer and thus increases the edge magnetoplasmon velocity. In the long-wavelength limit of our model, the drift velocity is simply added to the total magnetoplasmon velocity, in agreement with the classical picture.

cond-mat.mes-hall↗

Interlayer interaction, shear vibrational mode, and tribological properties of two-dimensional bilayers with a commensurate moiré pattern

The potential energy surface (PES) of interlayer interaction of infinite twisted bilayer graphene is calculated for a set of commensurate moiré patterns using the registry-dependent Kolmogorov-Crespi empirical potential. The calculated PESs have the same shape for all considered moiré patterns with the unit cell size of the PES which is inversely related to the unit cell size of the moiré pattern. The amplitude of PES corrugations is found to decrease exponentially upon increasing the size of the moiré pattern unit cell. An analytical expression for such a PES including the first Fourier harmonics compatible with the symmetries of both layers is derived. It is shown that the calculated PESs can be approximated by the derived expression with the accuracy within 1%. This means that different physical properties associated with relative in-plane motion of graphene layers are interrelated and can be expressed analytically as functions of the amplitude of PES corrugations. In this way, we obtain the shear mode frequency, shear modulus, shear strength and barrier for relative rotation of the commensurate twisted layers to a fully incommensurate state for the considered moiré patterns. This barrier may possibly lead to the macroscopic robust superlubricity for twisted graphene bilayer with a commensurate moiré pattern. The conclusions made should be valid for diverse 2D systems of twisted commensurate layers.

cond-mat.mes-hall↗

Tunable Bose-Einstein condensation and roton-like excitation spectra with dipolar exciton-polaritons in crossed fields

We develop the many-body theory of dipolar exciton-polaritons in an optical microcavity in crossed transverse electric and in-plane magnetic fields. Even for relatively weak fields, we reveal the existence of two minima in the bare lower-polariton dispersion, which give rise to the tuneable transition between the polariton Bose-Einstein condensate and that of excitons, produced by the competition between these minima. We predict that such dipolar condensate exhibits a roton-maxon character of the excitation spectrum, never before observed for polaritons. We show that upon the transition between the two condensation regimes, the weak correlations in the polariton gas give way to the intermediate interparticle correlations characteristic for excitons, and that the transition is accompanied by a sharp quenching of photoluminescence as the lifetime is increased by several orders of magnitude. While in the polariton regime, the luminescence peak corresponding to the condensate is shifted to a non-zero angle. The angular dependence of the two-photon decay time in the Hanbury Brown and Twiss experiment is calculated and used as a tool to evidence the formation of the macroscopically-coherent state. Our proposal opens opportunities towards manipulating the superfluid properties and extended-range dipole-dipole correlations of exciton-polariton condensates.

cond-mat.quant-gas↗

Coupled system of electrons and exciton-polaritons: Screening, dynamical effects, and superconductivity

Bose-Fermi systems such as mixtures of electrons with excitons or exciton-polaritons are extensively discussed as candidates to host a variety of intriguing phenomena, including polaron formation, drag effects, supersolidity, and superconductivity. In this work, assuming the strong-coupling regime between the semiconductor excitons and cavity photons, we develop the many-body theory approach addressing the interplay of different types of interaction among various species in such a mixture, wherein we take into account dynamical density responses of both the Bose-condensed exciton-polaritons and the two-dimensional electron gas inside an optical microcavity. As was anticipated previously, at high enough polariton densities the lower hybrid mode of the system's excitation spectrum acquires a roton minimum, making the system prone to superconducting pairing in the vicinity of the roton instability. We analyze the possibility of polariton-BEC-mediated superconductivity in the electron gas taking into account full momentum and frequency dependence of the gap, as well as in the Eliashberg approach where the momentum dependence is neglected, and in the Bardeen-Cooper-Schrieffer approach that discards the frequency dependence and dynamical effects. Considering the interaction screening in Thomas-Fermi and in random-phase approximations, we estimate the critical temperatures of superconductivity to be not larger than 0.1 K in the vicinity of instability. As possible realizations of the coupled polariton-electron system, semiconductor quantum wells and two-dimensional transition metal dichalcogenides are considered.

cond-mat.mes-hall↗

Superconductor-polariton non-dissipative drag in optical microcavity

We consider non-dissipative drag between Bose-condensed exciton polaritons in optical microcavity and embedded superconductors. This effect consists in induction of a non-dissipative electric current in the superconductor by motion of polariton Bose condensate due to electron-polariton interaction, or vice versa. Using many-body theory, we calculate the drag density, characterizing magnitude of this effect, with taking into account dynamical screening of the interaction. Hoping to diminish the interaction screening and microcavity photon absorption, we consider atomically-thin superconductors (both conventional s-wave and copper-oxide d-wave) of planar and nanoribbon shapes. Our estimates show that in realistic conditions the drag effect could be rather weak but observable in accurate experiments in the case of dipolar interlayer excitons in transition metal dichalcogenide bilayers. Use of spatially direct excitons, semiconductor quantum wells as the host for excitons, or thin films of bulk metallic superconductors considerably lowers the drag density.

cond-mat.mes-hall↗

Magnetic-Field-Induced Wigner Crystallization of Charged Interlayer Excitons in van der Waals Heterostructures

We develop the theory of the magnetic-field-induced Wigner crystallization effect for charged interlayer excitons (CIE) discovered recently in transition-metal-dichalcogenide (TMD) heterobilayers. We derive the ratio of the average potential interaction energy to the average kinetic energy for the many-particle CIE system subjected to the perpendicular magnetic field of an arbitrary strength, analyze the weak and strong field regimes, and discuss the 'cold' crystallization phase transition for the CIE system in the strong field regime. We also generalize the effective g-factor concept previously formulated for interlayer excitons, to include the formation of CIEs in electrostatically doped TMD heterobilayers. We show that magnetic-field-induced Wigner crystallization and melting of CIEs can be observed in strong-field magneto-photoluminescence experiments with TMD heterobilayes of systematically varied electron-hole doping concentrations. Our results advance the capabilities of this new family of transdimensional quantum materials.

cond-mat.mes-hall↗

Superfluid drag between excitonic polaritons and superconducting electron gas

The Andreev-Bashkin effect, or superfluid drag, is predicted in a system of Bose-condensed excitonic polaritons in optical microcavity coupled by electron-exciton interaction with a superconducting layer. Two possible setups with spatially indirect dipole excitons or direct excitons are considered. The drag density characterizing a magnitude of this effect is found by many-body calculations with taking into account dynamical screening of electron-exciton interaction. For the superconducting electronic layer, we assume the recently proposed polaritonic mechanism of Cooper pairing, although the preexisting thin-film superconductor should also demonstrate the effect. According to our calculations, the drag density can reach considerable values in realistic conditions, with excitonic and electronic layers made from GaAs-based quantum wells or two-dimensional transition metal dichalcogenides. The predicted nondissipative drag could be strong enough to be observable as induction of a supercurrent in the electronic layer by a flow of polariton Bose condensate.

cond-mat.mes-hall↗

Quantum entanglement between excitons in two-dimensional materials

The quantum entanglement between two excitons in two-dimensional materials, embedded in an optical microcavity, was investigated. The energy eigenstates of a Jaynes-Cummings like Hamiltonian for two qubits coupled to a single cavity mode have been calculated. The quantum entanglement between such states was estimated by calculating the concurrence between two qubits in each of these eigenstates. According to the results of our calculations, if the system is allowed to decay only through the emission of cavity photons at low temperatures, there is a maximally entangled eigenstate, protected from decay. We demonstrated that the existence of such a state results in the counter-intuitive conclusion that, for some initial states of the system, the fact that the cavity is leaky can actually lead to an increase in the average concurrence on the timescales of the average photonic lifetime. In addition, we calculated the time evolution of the concurrence between a pair of excitons in a strained graphene monolayer.

cond-mat.mes-hall↗

Electron pairing with gapless excitations in mixed double layers

We study the interlayer pairing states in layered systems of two different 2d electronic subsystems, one with relativistic linear and the other with non-relativistic parabolic spectrum. The complex order parameter of the paired state has a two component structure. We investigate the pairing state formation on the mean-field level, determine the critical interaction strength and evaluate the effective potential. The anisotropic three-band spectrum of quasiparticles depends explicitly on the phase difference of the order parameter components, rotates in momentum space as it changes. It is subject to the strong band deformation due to the pairing. It leads to the fusion and hybridization of initially decoupled bands. The quasiparticle spectrum has the shape of deformed Dirac cones in the vicinity of the two touching points between neighboring bands. The density of states exhibits a number of specific features due to band deformation, such as a van Hove singularity.

cond-mat.supr-con↗

Organic single-photon switch

The recent progress in nanotechnology [1,2] and single-molecule spectroscopy [3-5] paves the way for cost-effective organic quantum optical technologies emergent with a promise to real-life devices operating at ambient conditions. In this letter, we harness $π$-conjugated segments of an organic ladder-type polymer strongly coupled to a microcavity forming correlated collective dressed states of light, so-called of exciton-polariton condensates. We explore an efficient way for all-optical ultra-fast control over the macroscopic condensate wavefunction via a single photon. Obeying Bose statistics, exciton-polaritons exhibit an extreme nonlinearity undergoing bosonic stimulation [6] which we have managed to trigger at the single-photon level. Relying on the nature of organic matter to sustain stable excitons dressed with high energy molecular vibrations we have developed a principle that allows for single-photon nonlinearity operation at ambient conditions opening the door for practical implementations like sub-picosecond switching, amplification and all-optical logic at the fundamental limit of single light quanta.

cond-mat.mes-hall↗

Exact analytical solution for density matrix of a non-equilibrium polariton Bose-Einstein condensate

In this letter, we give an analytical quantum description of a non-equilibrium polariton Bose-Einstein condensate (BEC) based on the solution of the master equation for the full polariton density matrix in the limit of fast thermalization. We find the density matrix of a non-equilibrium BEC, that takes into account quantum correlations between all polariton states. We show that the formation of BEC is accompanied by the build-up of cross-correlations between the ground state and the excited states reaching their highest values at the condensation threshold. Despite the non-equilibrium nature of polariton systems, we show the average population of polariton states exhibits the Bose-Einstein distribution with an almost zero effective chemical potential above the condensation threshold similar to an equilibrium BEC. We demonstrate that above threshold the effective temperature of polariton condensate drops below the reservoir temperature.

cond-mat.quant-gas↗