arXiv subjects

Yuta Murakami

Publications and source records attributed to Yuta Murakami.

At least 37 records · Page 2Linked to original sources

arXiv2023

Non-thermal superconductivity in photo-doped multi-orbital Hubbard systems

Superconductivity in laser-excited correlated electron systems has attracted considerable interest due to reports of light-induced superconducting-like states. Here we explore the possibility of non-thermal superconducting order in strongly interacting multi-orbital Hubbard systems, using non-equilibrium dynamical mean field theory. We find that a staggered $η$-type superconducting phase can be realized on a bipartite lattice in the high photo-doping regime, if the effective temperature of the photo-carriers is sufficiently low. The $η$ superconducting state is stabilized by Hund coupling - a positive Hund coupling favors orbital-singlet spin-triplet $η$ pairing, whereas a negative Hund coupling stabilizes spin-singlet orbital-triplet $η$ pairing.

cond-mat.str-el↗

arXiv2023

Multiscale space-time ansatz for correlation functions of quantum systems based on quantics tensor trains

Correlation functions of quantum systems -- central objects in quantum field theories -- are defined in high-dimensional space-time domains. Their numerical treatment thus suffers from the curse of dimensionality, which hinders the application of sophisticated many-body theories to interesting problems. Here, we propose a multi-scale space-time ansatz for correlation functions of quantum systems based on quantics tensor trains (QTT), ``qubits'' describing exponentially different length scales. The ansatz then assumes a separation of length scales by decomposing the resulting high-dimensional tensors into tensor trains (known also as matrix product states). We numerically verify the ansatz for various equilibrium and nonequilibrium systems and demonstrate compression rates of several orders of magnitude for challenging cases. Essential building blocks of diagrammatic equations, such as convolutions or Fourier transforms are formulated in the compressed form. We numerically demonstrate the stability and efficiency of the proposed methods for the Dyson and Bethe-Salpeter equations. {The QTT representation} provides a unified framework for implementing efficient computations of quantum field theories.

cond-mat.str-el↗

arXiv2023

Spin, charge and $η$-spin separation in one-dimensional photo-doped Mott insulators

We show that effectively cold metastable states in one-dimensional photo-doped Mott insulators described by the extended Hubbard model exhibit spin, charge and $η$-spin separation. Namely, their wave functions in the large on-site Coulomb interaction limit can be expressed as $|Ψ\rangle =|Ψ_{\rm charge}\rangle|Ψ_{\rm spin}\rangle |Ψ_{\rm η-spin}\rangle$, which is analogous to the Ogata-Shiba states of the doped Hubbard model in equilibrium. Here $η$-spin represents the type of the photo-generated pseudeparticles (doublon or holon). $|Ψ_{\rm charge}\rangle$ is determined by spinless free fermions, $|Ψ_{\rm spin}\rangle$ by the isotropic Heisenberg model in the squeezed spin space, and $|Ψ_{\rm η-spin}\rangle$ by the XXZ model in the squeezed $η$-spin space. In particular, the metastable $η$-pairing and charge-density-wave (CDW) states correspond to the gapless and gapful states of the XXZ model. The specific form of the wave function allows us to accurately determine the exponents of correlation functions. The form also suggests that the central charge of the $η$-pairing state is 3 and that of the CDW phase is 2, which we numerically confirm. Our study provides analytic and intuitive insights into the correlations between active degrees of freedom in photo-doped strongly correlated systems.

cond-mat.str-el↗

arXiv2023

Majorana Gap Formation in the Anisotropic Kitaev Model with Ordered Flux Configuration

We study the Kitaev model with direction dependent interactions to investigate how the flux configuration and/or the anisotropy in the exchanges affect the Majorana excitations. Systematic numerical calculations demonstrate how the anisotropy of the exchange couplings and flux configuration make the Majorana excitation gapped. The induced gapped quantum spin liquid states are distinct from the gapped one realized in the large anisotropic limit. The nature of gapped states can be explained by the superlattice potential due to flux configuration.

cond-mat.str-el↗

arXiv2023

Dynamical mean-field theory for the Hubbard-Holstein model on a quantum device

Recent developments in quantum hardware and quantum algorithms have made it possible to utilize the capabilities of current noisy intermediate-scale quantum devices for addressing problems in quantum chemistry and condensed matter physics. Here we report a demonstration of solving the dynamical mean-field theory (DMFT) impurity problem for the Hubbard-Holstein model on the IBM 27-qubit Quantum Falcon Processor Kawasaki, including self-consistency of the DMFT equations. This opens up the possibility to investigate strongly correlated electron systems coupled to bosonic degrees of freedom and impurity problems with frequency-dependent interactions. The problem involves both fermionic and bosonic degrees of freedom to be encoded on the quantum device, which we solve using a recently proposed Krylov variational quantum algorithm to obtain the impurity Green's function. We find the resulting spectral function to be in good agreement with the exact result, exhibiting both correlation and plasmonic satellites and significantly surpassing the accuracy of standard Trotter-expansion approaches. Our results provide an essential building block to study electronic correlations and plasmonic excitations on future quantum computers with modern ab initio techniques.

quant-ph↗

arXiv2022

Anomalous temperature dependence of high-harmonic generation in Mott insulators

We reveal the crucial effect of strong spin-charge coupling on high-harmonic generation (HHG) in Mott insulators. In a system with antiferromagnetic correlations, the HHG signal is drastically enhanced with decreasing temperature, even though the gap increases and the production of charge carriers is suppressed. This anomalous behavior, which has also been observed in recent HHG experiments on Ca$_2$RuO$_4$, originates from a cooperative effect between the spin-charge coupling and the thermal ensemble, and the strongly temperature-dependent coherence between charge carriers. We argue that the peculiar temperature dependence of HHG is a generic feature of Mott insulators, which can be controlled via the Coulomb interaction and dimensionality of the system. Our results demonstrate that correlations between different degrees of freedom, which are a characteristic feature of strongly correlated solids, have significant and nontrivial effects on nonlinear optical responses.

cond-mat.str-el↗

arXiv2022

Optical response of the tightbinding model on the Fibonacci chain

We theoretically study the optical conductivity of the tightbinding model which has two types of the hopping integrals arranged in the Fibonacci sequence. Due to the lack of the translational symmetry, many peak structures appear in the optical conductivity as well as the density of states. When the ratio of two hopping integrals is large, the self-similar structure appears in the optical conductivity. This implies that the optical response between the high-energy bands is related to that within the low-energy bands, which should originate from critical behavior in the wave functions. The effects of disorders on the optical conductivity are also analyzed in order to show the absence of the self-similarity in the tightbinding model with the random sequence.

cond-mat.mes-hall↗

arXiv2022

High-harmonic generation in the Rice-Mele model: Role of intraband current originating from interband transition

We consider high-harmonic generation (HHG) in the Rice-Mele model to study the role of the intraband current originating from the change of the intraband dipole via interband transition. This contribution, which has been often neglected in previous works, is necessary for the consistent theoretical formulation of the light-matter coupling. We demonstrate that the contribution becomes crucial when the gap is smaller than or comparable to the excitation frequency and the system is close to the half filling.

cond-mat.mes-hall↗

arXiv2022

Doping and gap-size dependence of high-harmonic generation in graphene : Importance of consistent formulation of light-matter coupling

High-harmonic generation (HHG) in solids is a fundamental nonlinear phenomenon, which can be efficiently controlled by modifying system parameters such as doping-level and temperature. In order to correctly predict the dependence of HHG on these parameters, consistent theoretical formulation of the light-matter coupling is crucial. Recently, contributions to the current that are often missing in the HHG analysis based on the semiconductor Bloch equations have been pointed out [J. Wilhelm, et.al. PRB 103 125419 (2021)]. In this paper, by systematically analyzing the doping and gap-size dependence of HHG in gapped graphene, we discuss the practical impact of such terms. In particular, we focus on the role of the current $J_{\rm ra}^{(2)}$, which originates from the change of the intraband dipole via interband transition. When the gap is small and the system is close to half filling, intraband and interband currents mostly cancel, thus suppressing the HHG signal - an important property that is broken when neglecting $J_{\rm ra}^{(2)}$. Furthermore, without $J_{\rm ra}^{(2)}$, the doping and gap-size dependence of HHG becomes qualitatively different from the full evaluation. Our results demonstrate the importance of the consistent expression of the current to study the parameter dependence of HHG for the small gap systems.

cond-mat.mes-hall↗

arXiv2022

Second-order magnetic responses in quantum magnets: Magnetization under ac magnetic fields

We investigate second-order magnetic responses of quantum magnets against ac magnetic fields. We focus on the case where the $z$ component of the spin is conserved in the unperturbed Hamiltonian and the driving field is applied in the $xy$ plane. We find that linearly polarized driving fields induce a second-harmonic response, while circularly polarized fields generate only a zero-frequency response, leading to a magnetization with a direction determined by the helicity. Employing an unbiased numerical method, we demonstrate the nonlinear magnetic effect driven by the circularly polarized field in the XXZ model and show that the magnitude of the magnetization can be predicted by the dynamical spin structure factor in the linear response regime.

cond-mat.str-el↗

arXiv2022

Scattering phenomena for spin transport in Kitaev spin liquid

The Kitaev model exhibits a canonical quantum spin liquid as a ground state and hosts two fractional quasiparticles, itinerant Majorana fermion and localized flux excitation. The former can carry heat and spin modulations in the quantum spin liquid, but the role of the latter remains unknown for the transport phenomena. Here, we focus on spin transport in the presence of excited fluxes and report that they yield strong interference in the propagation of the Majorana fermions, which feel gauge-like potential emergent around the fluxes. We examine the transient spin dynamics triggered by a pulsed magnetic field at an edge. In the absence of excited fluxes, the magnetic-field pulse creates the plane wave of the Majorana fermions, which flows in the quantum spin liquid. Although this wave does not accompany the change of local spin moments in bulk, it induces local moments at the side opposite to the edge under the magnetic-field pulse. We observe the spatial modulation of induced spin moments when fluxes are excited in the bulk region. This behavior is more striking than the case of lattice defects. Moreover, we find that, although the amplitude of the spatial change is almost independent of the distance between lattice defects, it is strongly enhanced by increasing the distance for the case of excited fluxes. The difference is understood from the influence on the itinerant Majorana fermions; the lattice defects change the system locally, but flux excitations alter all the transfer integrals on the string connecting them. The present results will provide another route to observing intrinsic flux excitations distinguished from extrinsic effects such as lattice defects.

cond-mat.str-el↗

arXiv2022

Thermally enhanced Majorana-mediated spin transport in the Kitaev model

We study how stable the Majorana-mediated spin transport in a quantum spin Kitaev model is against thermal fluctuations. Using the time-dependent thermal pure quantum state method, we examine finite-temperature spin dynamics in the Kitaev model. The model exhibits two characteristic temperatures $T_L$ and $T_H$, which correspond to energy scales of the local flux and the itinerant Majorana fermion, respectively. At low temperatures $(T\ll T_L)$, an almost flux-free state is realized and the spin excitation propagates in a similar way to that for the ground state. Namely, after the magnetic pulse is introduced at one of the edges, the itinerant Majorana fermions propagate the spin excitations even through the quantum spin liquid state region, and oscillations in the spin moment appear in the other edge with a tiny magnetic field. When $T\sim T_L$, larger oscillations in the spin moments are induced in the other edge, compared to the results at the ground state. At higher temperatures, excited $Z_2$ fluxes disturb the coherent motion of the itinerant Majorana fermions, which suppresses the spin propagation. Our results demonstrate a crucial role of thermal fluctuations in the Majorana-mediated spin transport.

cond-mat.str-el↗

arXiv2021

Photoinduced Phase Transition in Two-Band model on Penrose Tiling

We study the effects of the photo irradiation on the band insulating state in the two-band Hubbard model on the Penrose tiling. Examining the time- and site-dependent physical quantities, we find that the excitionic state is dynamically induced with site-dependent order parameters. It is also clarified that, in the excitonic state induced by the photo irradiation, local oscillatory behavior appears in the electron number as well as in the order parameter, which should be characteristic of the quasiperiodic lattice.

cond-mat.str-el↗

arXiv2021

Unveiling the underlying interactions in Ta2NiSe5 from photo-induced lifetime change

We present a generic procedure for quantifying the interplay of electronic and lattice degrees of freedom in photo-doped insulators through a comparative analysis of theoretical many-body simulations and time- and angle-resolved photoemission spectroscopy (TR-ARPES) of the transient response of the candidate excitonic insulator Ta2NiSe5. Our analysis demonstrates that the electron-electron interactions dominate the electron-phonon ones. In particular, a detailed analysis of the TRARPES spectrum enables a clear separation of the dominant broadening (electronic lifetime) effects from the much smaller bandgap renormalization. Theoretical calculations show that the observed strong spectral broadening arises from the electronic scattering of the photo-excited particle-hole pairs and cannot be accounted for in a model in which electron-phonon interactions are dominant. We demonstrate that the magnitude of the weaker subdominant bandgap renormalization sensitively depends on the distance from the semiconductor/semimetal transition in the high-temperature state, which could explain apparent contradictions between various TR-ARPES experiments. The analysis presented here indicates that electron-electron interactions play a vital role (although not necessarily the sole one) in stabilizing the insulating state.

cond-mat.str-el↗

arXiv2021

Exploring nonequilibrium phases of photo-doped Mott insulators with Generalized Gibbs ensembles

Photo-excited strongly correlated systems can exhibit intriguing non-thermal phases, but the theoretical investigation of them poses significant challenges. In this work, we introduce a generalized Gibbs ensemble type description for long-lived photo-doped states in Mott insulators. This framework enables systematic studies of photo-induced phases based on equilibrium methods, as demonstrated here for the one-dimensional extended Hubbard model. We determine the nonequilibrium phase diagram, which features $η$-pairing and charge density wave phases in a wide doping range, and reveal physical properties of these phases. We show that the peculiar kinematics of photo-doped carriers, and the interaction between them, play an essential role in the formation of the non-thermal phases, and we clarify the differences between photo-doped Mott insulators, chemically-doped Mott insulators and photo-doped semiconductors. Our results demonstrate a new path for the systematic exploration of nonequilibrium strongly correlated systems and show that photo-doped Mott insulators host different phases than conventional semiconductors.

cond-mat.str-el↗

arXiv2021

Bulk Photovoltaic Effect Driven by Collective Excitations in a Correlated Insulator

We investigate the bulk photovoltaic effect, which rectifies light into electric current, in a collective quantum state with correlation driven electronic ferroelectricity. We show via explicit real-time dynamical calculations that the effect of the applied electric field on the electronic order parameter leads to a strong enhancement of the bulk photovoltaic effect relative to the values obtained in a conventional insulator. The enhancements include both resonant enhancements at sub-band-gap frequencies, arising from excitation of optically active collective modes, and broadband enhancements arising from nonresonant deformations of the electronic order. The deformable electronic order parameter produces an injection current contribution to the bulk photovoltaic effect that is entirely absent in a rigid-band approximation to a time-reversal symmetric material. Our findings establish that correlation effects can lead to the bulk photovoltaic effect and demonstrate that the collective behavior of ordered states can yield large nonlinear optical responses.

cond-mat.str-el↗

arXiv2021

Photo-induced Dynamics of Quasicrystalline Excitonic Insulator

We study the photo-induced dynamics of the excitonic insulator in the two-band Hubbard model on the Penrose tiling by means of the time-dependent real-space mean-field approximation. We show that, with a single-cycle electric-field pulse, the bulk (spatially averaged) excitonic order parameter decreases in the BCS regime, while it increases in the BEC regime. To clarify the dynamics peculiar to the Penrose tiling, we examine the coordination number dependence of observables and analyze the perpendicular space. In the BEC regime, characteristic oscillations of the electron number at each site are induced by the pulse, which are not observed in normal crystals. On the other hand, the dynamics in the BCS regime is characterized by drastic change in the spatial pattern of the excitonic order parameter.

cond-mat.str-el↗

arXiv2021

Imaging the coherent propagation of collective modes in the excitonic insulator candidate Ta$_2$NiSe$_5$ at room temperature

Excitonic insulators host a condensate of electron-hole pairs at equilibrium, giving rise to collective many-body effects. Although several materials have emerged as excitonic insulator candidates, evidence of long-range coherence is lacking and the origin of the ordered phase in these systems remains controversial. Here, using ultrafast pump-probe microscopy, we investigate the possible excitonic insulator Ta$_2$NiSe$_5$. Below 328 K, we observe the anomalous micrometer-scale propagation of coherent modes at velocities of the order of $\sim10^5$ m/s, which we attribute to the hybridization between phonon modes and the phase mode of the condensate. We develop a theoretical framework to support this explanation and propose that electronic interactions provide a significant contribution to the ordered phase in Ta$_2$NiSe$_5$. These results allow us to understand how the condensate's collective modes transport energy and interact with other degrees of freedom. Our study provides a unique paradigm for the investigation and manipulation of these properties in strongly correlated materials.

cond-mat.str-el↗