arXiv subjects

Yuto Ishii

Publications and source records attributed to Yuto Ishii.

14 recordsLinked to original sources

arXiv2026

$5/9-$Magnetization Plateau and Spin Supersolidity in YCu$_3$(OD)$_{7-x}$Br$_{2+x}$ under Magnetic Fields up to 120~T

We performed high-precision magnetization measurements up to 120~T on three compositions of the newly discovered kagome antiferromagnet YCu$_3$(OD)$_{7-x}$Br$_{2+x}$ (YCOB), revealing a previously unobserved 5/9 fractional magnetization plateau. All YCOB samples with different Br$^-$ concentrations exhibit nearly identical magnetization curves below 60~T, whereas the 5/9 plateau appears at markedly different fields in the ultrahigh-field regime. By modeling the experimental data using tensor-network calculations, we derive the effective spin Hamiltonians for the YCOB family with three spatially anisotropic Heisenberg couplings (the 3$J$-type model), which quantitatively reproduces the measured magnetization processes and captures the composition-dependent evolution of the 5/9 plateau. Furthermore, our theoretical analysis suggests the emergence of a spin supersolid phase in the field window between the 1/3 and 5/9 plateaus, which is sensitive to spin exchange parameters and accounts for the significant variation in the critical fields of the 5/9 plateau observed among different YCOB compositions.

cond-mat.str-el↗

arXiv2026

Non-linear diffusion and inhomogeneity of the magnetic field in single-turn coils: Insights from 3D multiphysics modeling

The single-turn coil method is a destructive pulsed magnet for generating over 100 T with a few $μ$-second pulse duration, and it inevitably causes the coil to explode. The temporal and spatial distributions of the electric current and magnetic field are highly inhomogeneous, arising from the skin effect, rapid temperature rise, and coil deformation. To grasp the dynamic phenomena in the single-turn coil, we conducted a finite element analysis using multiphysics simulation. We employed finite element method calculations using a fully 3D model of the single-turn coil with broken cylindrical symmetry. The calculated result revealed highly nonlinear diffusion of electric current, temperature, and magnetic fields, which are the sources of the inhomogeneous magnetic fields inside the single-turn coil in time and space.

cond-mat.mtrl-sci↗

arXiv2026

Efficiency in a repetitive pulse magnet

A repetitive-pulse magnet is a promising tool when combined with repetitive excitations, such as pulsed lasers. Technically, the repetition and the magnetic field values in a repetitive-pulse magnet are limited by the Joule heating in the coil. Here, we analytically examine the relationship between the coil's dimensions and its efficiency, assuming negligible heating of the coil, to design an optimized high-repetition, high-magnetic-field coil. We calculated the dependence of the maximum magnetic field, energy loss, pulse duration, form factor, impedance, and maximum current on the coil's geometry. We found that the smaller the coil, the more pulses and the more intense the magnetic fields we can obtain under a given condition. We argue that the obtained trend arises from a complex interplay among various parameters.

physics.app-ph↗

arXiv2026

Large magnetostriction and first-order phase transition induced by ultrahigh magnetic fields in V$_6$O$_{13}$

V$_6$O$_{13}$ exhibits the metal-insulator transition (MIT) at around 150 K with the formation of vanadium-vanadium (V-V) dimers. We measured the magnetostriction of V$_6$O$_{13}$ along the crystallographic $b$-axis in ultrahigh magnetic fields up to 186 T at various temperatures. An abrupt and large negative magnetostriction of $ΔL / L \sim 10^{-3}$ was observed above 120 T below 150 K which is attributed to the collapse of the V-V dimer. A pronounced hysteresis exceeding 50 T was observed, indicating a first-order phase transition. The field-induced collapse of the V-V dimer is expected to be accompanied by the insulator-to-metal transition. The robustness of the insulating phase against magnetic fields was discussed based on thermodynamics and the comparison with the case of VO$_2$.

cond-mat.str-el↗

arXiv2025

Fate of Pomeranchuk effect in ultrahigh magnetic fields

The Pomeranchuk effect is a counterintuitive phenomenon where liquid helium-3 (3He) solidifies under specific pressures, not when cooled, but when heated. This behaviour originates from the magnetic entropy of nuclear spins, suggesting a magnetic field should influence it. However, its detailed response to magnetic fields remains elusive due to the small nuclear magneton of 3He and lack of analogous fermion systems. Here, we show that an electron system also exhibit the Pomeranchuk effect, where the Fermi liquid state solidifies in a high magnetic field, unlike conventional electron systems where a field melts an electron solid into a metal. Remarkably, the electron system displays a reentrant liquid state in ultrahigh fields. These responses are explained by changes in magnetic entropy and magnetisation, extending the underlying physics to 3He. Our findings clarify magnetic-field impact on the Pomeranchuk effect and open avenues for magnetic control of chemical interactions.

cond-mat.str-el↗

arXiv2025

Possible evidence for Harper broadening in the yellow exciton series of Cu2O at ultrahigh magnetic fields

Hydrogen-like systems in ultra-high magnetic fields are of significant interest in interdisciplinary research. Previous studies have focused on the exciton wavefunction shrinkage under magnetic fields down to artificial crystal lattices (e.g., quantum wells, superlattices), where the effective mass approximation remains valid. However, further compression toward the natural crystal lattice scale remains experimentally challenging. In this study, we report magneto-absorption measurements on the yellow-exciton series in Cu2O using pulsed magnetic fields of up to 500 T. The strong low energy absorption features are assigned to the spin Zeeman split 2p0 and 3p0 exciton states. The high field data provides a value for the reduced effective mass of the exciton u* = 0.415 \pm 0.01me. Intriguingly, the broadening of the 2p0 ground state transition exhibits a sudden increase for ultrahigh magnetic fields above 300 T, providing possible evidence for Harper broadening - an indication of the breakdown of the effective mass approximation when the magnetic length becomes comparable to the lattice constant of the crystal.

cond-mat.mtrl-sci↗

arXiv2025

X-ray free-electron laser observation of giant and anisotropic magnetostriction in $β$-O$_{2}$ at 110 Tesla

In strong magnetic fields beyond 100 T, the significant Zeeman energy competes with the lattice interactions, where a considerable magnetostriction is expected. However, the microscopic observation of the magnetostriction above 100 T has been hindered due to the short pulse duration of $μ$-seconds and the coil's destruction. Here, we report the observation of the giant and anisotropic magnetostriction of $\sim 1$ % at 110 T in the spin-controlled crystal, $β$-O$_{2}$, by combining the single-shot diffraction of x-ray free-electron laser (XFEL) and the newly developed portable 100 T generator (PINK-02). The very soft and anisotropic response of $β$-O$_{2}$ should originate in the competing van der Waals force and exchange interaction, and also the frustration of spin and lattice on the triangular network. The XFEL experiment above 100 T using PINK-02 enables microscopic investigations on materials' properties at high magnetic fields, providing insights into how spins contribute to the stability of crystal structures.

cond-mat.str-el↗

arXiv2025

Longitudinal Magnetoresistance in YBa$_2$Cu$_3$O$_7$ at High Magnetic Fields of up to 100 T

The investigation of transport characteristics in high-temperature superconductors under magnetic fields is one of the most important topics in condensed matter physics and transport applications. For YBa$_2$Cu$_3$O$_7$ (YBCO), the measurements of magnetoresistance under a high magnetic field are technically challenging because the required magnetic field ($B$) to suppress the superconductivity is 100~T class. The low temperature (from 52 to 150 K) longitudinal magnetoresistance ($B$$\parallel$ab-plane$\parallel$$J$, where $J$ is an electrical current) was measured up to 103~T in optimally doped YBCO thin films. A radio frequency reflection method and the single-turn coil technique were employed. The electrical resistivity $ρ_{ab}$ exhibited a non-saturating magnetoresistance behavior until the highest field region, with the slope $β(=d ρ/d B)$ showing a pronounced deviation compared to the transverse magnetoresistance ($B$$\parallel$c-axis) case. These findings suggest a potential contribution due to the non-orbital origin in the high field phase of YBCO, because the quasiparticle orbital motion is expected to be absent in the longitudinal magnetoresistance.

cond-mat.str-el↗

arXiv2024

Phonon hydrodynamic regimes in sapphire

When an ideal insulator is cooled, four regimes of thermal conductivity are expected to emerge one after another. Two of these, the Ziman and the Poiseuille, are hydrodynamic regimes in which collision among phonons are mostly Normal. It has been difficult to observe them, save for a few insulators with high levels of isotopic and chemical purity. Our thermal transport measurements, covering four decades of temperatures between 0.1 K and 900 K, reveal that sapphire displays all four regimes, despite its isotopic impurity. In the Ziman regime, the thermal conductivity exponentially increases attaining an amplitude as large as 35,000 W/Km. We show that the peak thermal conductivity of ultra-pure, simple insulators, including diamond, silicon and solid helium, is set by a universal scaling depending on isotropic purity. The thermal conductivity of sapphire is an order of magnitude higher than what is expected by this scaling. We argue that this may be caused by the proximity of optical and acoustic phonon modes, as a consequence of the large number of atoms in the primitive cell.

cond-mat.mtrl-sci↗

arXiv2024

Geometric frustration and Dzyaloshinskii-Moriya interactions in a quantum star lattice hybrid copper sulfate

We study the magnetism of a layered, spin-$\frac12$ organic-inorganic copper sulfate, which is a close realization of the star lattice antiferromagnet, one of the playgrounds of geometric frustration and resonating valence bond physics in two spatial dimensions. Our thermodynamic measurements show no ordering down to 0.1 K and a characteristic field-induced entropic shift, revealing the presence of an infinite number of competing states down to very low energy scales. The response to external magnetic fields shows, in addition, a peculiar anisotropy, reflected in the formation of a 1/3 magnetization plateau (stable up to full saturation around 105 T) and a paramagnetic, Curie-like susceptibility for one direction of the field (${\bf H}\parallel{\bf c}$), and a completely different response in other field directions. Our first-principles density functional theory calculations and exact diagonalizations show that these experimental puzzles are distinctive signatures of a strong interplay between geometric frustration and sizable Dzyaloshinskii-Moriya interactions, and the emergence of a continuous U(1) symmetry at low energy scales.

cond-mat.str-el↗

arXiv2023

Signature of spin-triplet exciton condensations in LaCoO$_{3}$ at ultrahigh magnetic fields up to 600 T

Bose-Einstein condensation of electron-hole pairs, exciton condensation, has been effortfully investigated since predicted 60 years ago. Irrefutable evidence has still been lacking due to experimental difficulties in verifying the condensation of the charge neutral and non-magnetic spin-singlet excitons. Whilst, condensation of spin-triplet excitons is a promising frontier because spin supercurrent and spin-Seebeck effects will be observable. A canonical cobaltite LaCoO$_{3}$ under very high magnetic fields is a propitious candidate, yet to be verified. Here, we unveil the exotic phase diagram of LaCoO$_{3}$ up to 600 T generated using the electromagnetic flux compression method and the state-of-the-art magnetostriction gauge. We found the continuous magnetostriction curves and a bending structure, which suggest the emergence of two distinct spin-triplet exciton condensates. By constructing a phenomenological model, we showed that quantum fluctuations of excitons are crucial for the field-induced successive transitions. The spin-triplet exciton condensation in a cobaltite, which is three-dimensional and thermally equilibrated, opens up a novel venue for spintronics technologies with spin-supercurrent such as a spin Josephson junction.

cond-mat.str-el↗

arXiv2022

Ferroelectric transition of a chiral molecular crystal BINOL2DMSO

We report dielectric, thermodynamical, acoustic, and optical properties of a chiral molecular crystal, 1,1'-bi-2-naphthol 2-dimethylsulfoxide (BINOL2DMSO). We find two successive phase transitions at Tc1=190 K and Tc2=125 K. The first transition at Tc1 is characterized by an order-disorder transition of the guest molecules DMSO along with ferroelectricity. At the second transition of Tc2, the crystal structure deforms from tetragonal to monoclinic, leading to domain formation. Low-temperature x-ray diffraction suggests that the space group changes from P4_12_12 (P4_32_12) to P4_1 (P4_3) at Tc1, and down to P112_1 at Tc2.

cond-mat.mtrl-sci↗

arXiv2022

Generating 77 T using a portable pulse magnet for single shot quantum beam experiments

We devised a portable system that generates pulsed high magnetic fields up to 77 T with 3 $μ$s duration. The system employs the single turn coil method, a destructive way of field generation. The system consists of a capacitor of 10.4 $μ$F, a 30 kV charger, a mono air-gap switch, a triggering system, and a magnet clamp, which weighs less than 1.0 tons in total and is transportable. The system offers opportunities for single-shot experiments at ultrahigh magnetic fields in combinations with novel quantum beams. The single-shot x-ray diffraction experiment using x-ray free-electron laser at 65 T is presented. We comment on the possible update of the system for the generation of 100 T.

cond-mat.str-el↗

arXiv2021

Magnetic properties of the Shastry-Sutherland lattice material BaNd$_2$ZnO$_5$

We investigate the physical properties of the Shastry-Sutherland lattice material BaNd$_2$ZnO$_5$. Neutron diffraction, magnetic susceptibility, and specific heat measurements reveal antiferromagnetic order below 1.65 K. The magnetic order is found to be a 2-$\boldsymbol{Q}$ magnetic structure with the magnetic moments lying in the Shastry-Sutherland lattice planes comprising the tetragonal crystal structure of BaNd$_2$ZnO$_5$. The ordered moment for this structure is 1.9(1) $μ_B$ per Nd ion. Inelastic neutron scattering measurements reveal that the crystal field ground state doublet is well separated from the first excited state at 8 meV. The crystal field Hamiltonian is determined through simultaneous refinement of models with both the LS coupling and intermediate coupling approximations to the inelastic neutron scattering and magnetic susceptibility data. The ground state doublet indicates that the magnetic moments lie primarily in the basal plane with magnitude consistent with the size of the determined ordered moment.

cond-mat.str-el↗