arXiv subjects

Yuuki Yasui

Publications and source records attributed to Yuuki Yasui.

8 recordsLinked to original sources

arXiv2026

Individual Characterization of Fast-Responding Trap States at the NO-Annealed SiO$_2$/4H-SiC Interface

Fast-responding trap states introduced by NO-annealing are suspected to limit the channel mobility of 4H-SiC MOSFETs, yet their microscopic characterization remains challenging because conventional electrical methods are spatially averaged and do not readily isolate such fast processes. Here, we visualize and analyze individual fast-responding trap states at the NO-annealed SiO$_2$/4H-SiC interface using the energy dissipation signal in frequency-modulation atomic force microscopy (FM-AFM), which selectively probes charge-exchange dynamics on sub-$\mu$s time scales. Ring-shaped dissipation patterns were observed in the NO-annealed sample but not in the control sample without NO-annealing, indicating that the detected states are associated with nitridation. Spectroscopic measurements were also performed to determine the dependence of energy dissipation on the tip bias and the tip-sample distance. Combined with finite-element electrostatic calculations, this analysis allowed us to determine trap energies relative to the Fermi level, $E_t - E_f$, and revealed that the trap-energy distribution extends toward the interfacial conduction-band edge. These results provide microscopic evidence that NO-annealing generates fast-responding trap states near the SiO$_2$/4H-SiC interface.

cond-mat.mtrl-sci↗

arXiv2025

Force-Based Reading and Writing of Individual Single-Atom Magnets

The integration of single-atom bits enables the realization of the highest data-density memory. Reading and writing information to these bits through mechanical interactions opens the possibility of operating the magnetic devices with low heat generation and high density recording. To achieve this visionary goal, we demonstrate the use of magnetic exchange force microscopy to read and write the spin orientation of individual holmium adatoms on MgO thin films. The spin orientation of the holmium adatom is stabilized by the strong uniaxial anisotropy of the adsorption site and can be read out by measuring the exchange forces between the magnetic tip and the atom. The spin orientation can be written by approaching the tip closer to the holmium adatom.We explain this writing mechanism by the symmetry reduction of the adsorption site of the Ho adatom. These findings demonstrate the potential for information storage with minimal energy loss and pave the way for a new field of atomic-scale mechano-spintronics.

physics.app-ph↗

arXiv2024

Closing of the Mott gap near step edges in NiS2

A prototypical charge-transfer type Mott insulator NiS2 pyrite exhibits a metal-insulator transition with bandwidth control. Recent discoveries on surface-specific electronic states on other 3d transition-metal disulfide pyrites motivate us to further investigate the surface of NiS2, where metallic surface conduction is discussed. Here, the spectroscopic-imaging scanning-tunneling-microscopy observations revealed that the surface is not metallic, contrary to the expectation. Instead, the Mott gap is closed near step edges, suggesting possible electrical conduction from one-dimensional channels. The edge anomaly was observed irrespective of its magnetic order and is limited to the insulator phases.

cond-mat.str-el↗

arXiv2024

Atomic observation on diamond (001) surfaces with non-contact atomic force microscopy

To achieve atomic-level characterization of the diamond (001) surface, persistent efforts have been made over the past few decades. The motivation behind the pursuit extends beyond investigating surface defects and adsorbates; it also involves unraveling the mystery of the smooth growth of diamond. However, the inherently low conductivity and the short C-C bonds render atomic resolution imaging exceptionally challenging. Here, we successfully overcame these challenges by employing non-contact atomic force microscopy with reactive Si tips. Atomic resolution imaging was achieved even at room temperature. With density-functional-theory calculations, we clarified that the critical factors for atomic resolution are in the formation of tilted C-Si bonds between scanning probes and surfaces, along with reordering of the surface C-C dimers. Implications of the findings extend beyond the realm of surface characterization. The present atomic-resolution microscopies drive future advancements in diamond technologies by providing avenues for identifying dopants and constructing artificial nanostructures.

cond-mat.mtrl-sci↗

arXiv2024

Unveiling unconventional magnetism at the surface of Sr$_2$RuO$_4$

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered oxide perovskite Sr$_2$RuO$_4$ is a strongly correlated electron material that has been intensively investigated since its discovery due to its unusual physical properties. Whilst recent experiments have reopened the debate on the exact symmetry of the superconducting state in Sr$_2$RuO$_4$, a deeper understanding of the Sr$_2$RuO$_4$ normal state appears crucial as this is the background in which electron pairing occurs. Here, by using low-energy muon spin spectroscopy we discover the existence of magnetism at the surface of Sr$_2$RuO$_4$ in its normal state. We detect static weak dipolar fields yet manifesting below a relatively high onset temperature larger than 50 K, which reveals the unconventional nature of the observed magnetism. We relate the origin of this phase breaking time reversal symmetry to electronic ordering in the form of orbital loop currents that originate at the reconstructed Sr$_2$RuO$_4$ surface. Our observations set a reference for the discovery of the same magnetic phase in other materials and unveil an electronic ordering mechanism that can influence unconventional electron pairing with broken time reversal symmetry in those materials where the observed magnetic phase coexists with superconductivity.

cond-mat.str-el↗

arXiv2020

Imaging the coupling between itinerant electrons and localised moments in the centrosymmetric skyrmion magnet GdRu2Si2

Magnetic skyrmions were thought to be stabilised only in inversion-symmetry breaking structures, but skyrmion lattices were recently discovered in inversion symmetric Gd-based compounds, spurring questions of the stabilisationmechanism. A natural consequence of a recent theoretical proposal, a coupling between itinerant electrons and localised magnetic moments, is that the skyrmions are amenable to detection using even non-magnetic probes such as spectroscopic-imaging scanning tunnellingmicroscopy (SI-STM). Here SI-STM observations of GdRu$_2$Si$_2$ reveal patterns in the local density of states that indeed vary with the underlying magnetic structures. These patterns are qualitatively reproduced by model calculations which assume exchange coupling between itinerant electrons and localised moments. These findings provide a clue to understand the skyrmion formation mechanism in GdRu$_2$Si$_2$.

cond-mat.str-el↗

arXiv2020

Spontaneous emergence of Josephson junctions in homogeneous rings of single-crystal Sr2RuO4

The chiral p-wave order parameter in Sr$_\mathsf{2}$RuO$_\mathsf{4}$ would make it a special case amongst the unconventional superconductors. A consequence of this symmetry is the possible existence of superconducting domains of opposite chirality. At the boundary of such domains, the locally supressed condensate can produce an intrinsic Josephson junction. Here, we provide evidence of such junctions using mesoscopic rings, structured from Sr$_\mathsf{2}$RuO$_\mathsf{4}$ single crystals. Our order parameter simulations predict such rings to host stable domain walls across their arms. Thisis verified with transport experiments on loops, with a sharp transition at 1.5 K, which show distinct critical current oscillations with periodicity corresponding to the flux quantum. In contrast, loops with broadened transitions at around 3 K are void of such junctions and show standard Little-Parks oscillations. Our analysis demonstrates the junctions are of intrinsic origin and makes a compelling case for the existence of superconducting domains.

cond-mat.supr-con↗

arXiv2017

Little-Parks oscillations with half-quantum fluxoid features in Sr2RuO4 micro rings

In a micro ring of a superconductor with a spin-triplet equal-spin pairing state, a fluxoid, a combined object of magnetic flux and circulating supercurrent, can penetrate as half-integer multiples of the flux quantum. A candidate material to investigate such half-quantum fluxoids is Sr$_\mathsf{2}$RuO$_\mathsf{4}$. We fabricated Sr$_\mathsf{2}$RuO$_\mathsf{4}$ micro rings using single crystals and measured their resistance behavior under magnetic fields controlled with a three-axes vector magnet. Proper Little-Parks oscillations in the magnetovoltage as a function of an axially applied field, associated with fluxoid quantization are clearly observed, for the first time using bulk single crystalline superconductors. We then performed magnetovoltage measurements with additional in-plane magnetic fields. By carefully analyzing both the voltages $V_+$ ($V_-$) measured at positive (negative) current, we find that, above an in-plane threshold field of about 10 mT, the magnetovoltage maxima convert to minima. We interpret this behavior as the peak splitting expected for the half-quantum fluxoid states.

cond-mat.supr-con↗