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Yuxuan Ye

Publications and source records attributed to Yuxuan Ye.

9 recordsLinked to original sources

General and scalable vapor etching and transformation platform for two-dimensional materials

Two-dimensional (2D) nanomaterials derived from non-van der Waals (non-vdW) solids offer exceptional physicochemical properties, yet their synthesis is impeded by intrinsic covalent/metallic bonding and high surface reactivity of the precursors. Here, we report a general vapor-phase etching and transformation platform for producing a library of 36 2D carbides, nitrides, and carbonitrides, exhibiting electrical conductivities spanning six orders of magnitude. Using reactive vapors like hydrogen chloride, we selectively remove A-layers from MAX phases to yield well-defined layers (MXenes), including previously inaccessible semiconducting Hf2CTx. By varying the reactive vapor environment, MXenes can be engineered at X-site and surface-termination site and even be transformed into non-vdW layers such as 2D MAX phases. This general and scalable vapor-phase platform reframes 2D material synthesis, opening new avenues for various applications.

cond-mat.mtrl-sci

Teaching Language Models to Check Grounded Claim Factuality with Human Test-Taking Strategies

Grounded claim factuality checking is important for large language model (LLM) applications such as retrieval-augmented generation, as it helps users assess the correctness of generated outputs. Existing metrics using entailment classifiers require dataset-specific threshold tuning, while LLM-based approaches often use direct prompting, which underutilises the reasoning capabilities of LLMs. We address this by formulating grounded claim factuality checking as a true/false reading comprehension task and prompting LLMs with explicit test-taking strategies for efficient reasoning. Our method reduces token usage by over 80% compared to unguided open-ended reasoning, and achieves competitive performance to more expensive alternatives across two factuality benchmarks, setting a new state of the art on one. To further reduce inference cost, we train small language models (SLMs) to replace LLMs in the checking pipeline. Using supervised fine-tuning (SFT) and a self-revision mechanism, the SLMs learn to improve their factuality judgements. Experimental results show that the resulting SLMs perform on par with strong baselines, combining low inference costs with generating supporting rationales to support interpretability. Code and datasets will be released upon acceptance.

cs.CL

Optimising Factual Consistency in Summarisation via Preference Learning from Multiple Imperfect Metrics

Reinforcement learning with evaluation metrics as rewards is widely used to enhance specific capabilities of language models. However, for tasks such as factually consistent summarisation, existing metrics remain underdeveloped, limiting their effectiveness as signals for shaping model behaviour.While individual factuality metrics are unreliable, their combination can more effectively capture diverse factual errors. We leverage this insight to introduce an automated training pipeline that improves factual consistency in summaries by aggregating scores from different weak metrics. Our approach avoids the need for complex reward shaping by mapping scores to preferences and filtering out cases with high disagreement between metrics. For each source document, we generate lexically similar summary pairs by varying decoding strategies, enabling the model to learn from factual differences caused by subtle lexical differences. This approach constructs a high-quality preference dataset using only source documents.Experiments demonstrate consistent factuality gains across models, ranging from early encoder-decoder architectures to modern large language models, with smaller models reaching comparable factuality to larger ones.

cs.CL

The Alpha Illusion: Reported Alpha from LLM Trading Agents Should Not Be Treated as Deployment Evidence

End-to-end LLM trading agents have moved quickly from research curiosity to a small ecosystem of named systems, including FinCon, FinMem, TradingAgents, FinAgent, QuantAgent, and FLAG-Trader. Several of these report headline Sharpe ratios that would be material if read at face value on a deployment desk, and associated benchmarks such as FinBen report trading-task Sharpe statistics in the same range. The gap between architecture research and deployment claim has been crossed too freely on both sides of the academia--industry divide. We take a position on that gap: reported alpha from end-to-end LLM trading agents should not be treated as deployment evidence. Before such returns can support claims of deployable trading capability, they must survive structural validity tests for temporal integrity, real-world frictions, counterfactual robustness, predictive calibration, numerical execution, and multi-agent disaggregation. Current public evidence cannot yet distinguish robust predictive ability from temporal contamination, unmodeled frictions, short-window Sharpe uncertainty, narrative fitting, and parametric priors. The problem is not only evaluative but structural. Language confidence is not tradable probability, narrative reasoning is not numerical execution, and model priors may become undisclosed implicit factor exposures. We contribute a minimum reporting protocol suite, P1--P6, with tiered applicability by claim strength, and a conservative modular alternative that uses LLMs as auditable information interfaces upstream of independent calibration, risk, and execution modules. Code and reproduction harness: \url{https://github.com/hj1650782738/Trading}.

cs.CE

Quantifying Compositionality of Classic and State-of-the-Art Embeddings

For language models to generalize correctly to novel expressions, it is critical that they exploit access compositional meanings when this is justified. Even if we don't know what a "pelp" is, we can use our knowledge of numbers to understand that "ten pelps" makes more pelps than "two pelps". Static word embeddings such as Word2vec made strong, indeed excessive, claims about compositionality. The SOTA generative, transformer models and graph models, however, go too far in the other direction by providing no real limits on shifts in meaning due to context. To quantify the additive compositionality, we formalize a two-step, generalized evaluation that (i) measures the linearity between known entity attributes and their embeddings via canonical correlation analysis, and (ii) evaluates additive generalization by reconstructing embeddings for unseen attribute combinations and checking reconstruction metrics such as L2 loss, cosine similarity, and retrieval accuracy. These metrics also capture failure cases where linear composition breaks down. Sentences, knowledge graphs, and word embeddings are evaluated and tracked the compositionality across all layers and training stages. Stronger compositional signals are observed in later training stages across data modalities, and in deeper layers of the transformer-based model before a decline at the top layer. Code is available at https://github.com/Zhijin-Guo1/quantifying-compositionality.

cs.CL

Two-dimensional materials as a multiproperty sensing platform

Two-dimensional (2D) materials have disrupted materials science due to the development of van der Waals technology. It enables the stacking of ultrathin layers of materials characterized by vastly different electronic structures to create man-made heterostructures and devices with rationally tailored properties, circumventing limitations of matching crystal structures, lattice constants, and geometry of constituent materials and supporting substrates. 2D materials exhibit extraordinary mechanical flexibility, strong light-matter interactions driven by their excitonic response, single photon emission from atomic centers, stable ferromagnetism in sub-nm thin films, fractional quantum Hall effect in high-quality devices, and chemoselectivity at ultrahigh surface-to-volume ratio. Consequently, van der Waals heterostructures with atomically flat interfaces demonstrate an unprecedented degree of intertwined mechanical, chemical, optoelectronic, and magnetic properties. This constitutes a foundation for multiproperty sensing, based on complex intra- and intermaterial interactions, and a robust response to external stimuli originating from the environment. Here, we review recent progress in the development of sensing applications with 2D materials, highlighting the areas where van der Waals heterostructures offer the highest sensitivity, simultaneous responses to multiple distinct externalities due to their atomic thickness in conjunction with unique material combinations, and conceptually new sensing methodology.

cond-mat.mes-hall

Using Similarity to Evaluate Factual Consistency in Summaries

Cutting-edge abstractive summarisers generate fluent summaries, but the factuality of the generated text is not guaranteed. Early summary factuality evaluation metrics are usually based on n-gram overlap and embedding similarity, but are reported fail to align with human annotations. Therefore, many techniques for detecting factual inconsistencies build pipelines around natural language inference (NLI) or question-answering (QA) models with additional supervised learning steps. In this paper, we revisit similarity-based metrics, showing that this failure stems from the comparison text selection and its granularity. We propose a new zero-shot factuality evaluation metric, Sentence-BERT Score (SBERTScore), which compares sentences between the summary and the source document. It outperforms widely-used word-word metrics including BERTScore and can compete with existing NLI and QA-based factuality metrics on the benchmark without needing any fine-tuning. Our experiments indicate that each technique has different strengths, with SBERTScore particularly effective in identifying correct summaries. We demonstrate how a combination of techniques is more effective in detecting various types of error.

cs.CL

Towards Abstractive Timeline Summarisation using Preference-based Reinforcement Learning

This paper introduces a novel pipeline for summarising timelines of events reported by multiple news sources. Transformer-based models for abstractive summarisation generate coherent and concise summaries of long documents but can fail to outperform established extractive methods on specialised tasks such as timeline summarisation (TLS). While extractive summaries are more faithful to their sources, they may be less readable and contain redundant or unnecessary information. This paper proposes a preference-based reinforcement learning (PBRL) method for adapting pretrained abstractive summarisers to TLS, which can overcome the drawbacks of extractive timeline summaries. We define a compound reward function that learns from keywords of interest and pairwise preference labels, which we use to fine-tune a pretrained abstractive summariser via offline reinforcement learning. We carry out both automated and human evaluation on three datasets, finding that our method outperforms a comparable extractive TLS method on two of the three benchmark datasets, and participants prefer our method's summaries to those of both the extractive TLS method and the pretrained abstractive model. The method does not require expensive reference summaries and needs only a small number of preferences to align the generated summaries with human preferences.

cs.LG

Metal-bonded Atomic Layers of Transition Metal Carbides (MXenes)

Although two-dimensional transition metal carbides and nitrides (MXenes) have fantastic physical and chemical properties as well as wide applications, it remains challenging to produce stable MXenes due to their rapid structural degradation. Here, unique metal-bonded atomic layers of transition metal carbides with high stabilities are produced via a simple topological reaction between chlorine-terminated MXenes and selected metals, where the metals enable to not only remove Cl terminations, but also efficiently bond with adjacent atomic MXene slabs, driven by the symmetry of MAX phases. The films constructed from Al-bonded Ti$_3$C$_2$Cl$_x$ atomic layers show high oxidation resistance up to 400 degrees centigrade and low sheet resistance of 9.3 ohm per square. Coupled to the multi-layer structure, the Al-bonded Ti$_3$C$_2$Cl$_x$ film displays a significantly improved EMI shielding capability with a total shielding effectiveness value of 39 dB at a low thickness of 3.1 micron, outperforming pure Ti$_3$C$_2$Cl$_x$ film.

cond-mat.mtrl-sci