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Z. -X. Shen

Publications and source records attributed to Z. -X. Shen.

At least 163 records · Page 9Linked to original sources

Surface electronic structure of Sr2RuO4

We have addressed the possibility of surface ferromagnetism in Sr2RuO4 by investigating its surface electronic states by angle-resolved photoemission spectroscopy (ARPES). By cleaving samples under different conditions and using various photon energies, we have isolated the surface from the bulk states. A comparison with band structure calculations indicates that the ARPES data are most readily explained by a nonmagnetic surface reconstruction.

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Electron-Like Fermi Surface and Remnant (pi,0) Feature in Overdoped La1.78Sr0.22CuO4

We have performed an angle-resolved photoemission study of overdoped La1.78Sr0.22CuO4, and have observed sharp nodal quasiparticle peaks in the second Brillouin zone that are comparable to data from Bi2Sr2CaCu2O8+d. The data analysis using energy distribution curves, momentum distribution curves and intensity maps all show evidence of an electron-like Fermi surface, which is well explained by band structure calculations. Evidence for many-body effects are also found in the substantial spectral weight remaining below the Fermi level around (pi,0), where the band is predicted to lie above EF.

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Superconducting Gap and Strong In-Plane Anisotropy in Untwinned YBa2Cu3O7-d

With significantly improved sample quality and instrumental resolution, we clearly identify in the (pi,0) ARPES spectra from YBa2Cu3O6.993, in the superconducting state, the long-sought `peak-dip-hump' structure. This advance allows us to investigate the large a-b anisotropy of the in-plane electronic structure including, in particular, a 50% difference in the magnitude of the superconducting gap that scales with the energy position of the hump feature. This anisotropy, likely induced by the presence of the CuO chains, raises serious questions about attempts to quantitatively explain the YBa2Cu3O7-d data from various experiments using models based on a perfectly square lattice.

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Bilayer Splitting in the Electronic Structure of Heavily Overdoped Bi2Sr2CaCu2O8+d

The electronic structure of heavily overdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ is investigated by angle-resolved photoemission spectroscopy. The long-sought bilayer band splitting in this two-plane system is observed in both normal and superconducting states, which qualitatively agrees with the bilayer Hubbard model calculations. The maximum bilayer energy splitting is about 88 meV for the normal state feature, while it is only about 20 meV for the superconducting peak. This anomalous behavior cannot be reconciled with the quasiparticle picture.

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Fermi surface of Sr2RuO4 from angle resolved photoemission

We investigated the low-energy electronic structure of Sr2RuO4 by angle-resolved photoemission spectroscopy (ARPES) focusing, in particular, on the controversial issues of the Fermi surface (FS) topology and of the extended van Hove singularity (evHs). A detailed study of temperature and photon energy dependence demonstrates the surface-state nature of the electronic band responsible for the evHs, and may suggest the presence of ferromagnetic correlations at the surface. In addition, we detected a replica of the primary FS that indicates a (sqrt2 x sqrt2) surface reconstruction, as confirmed by LEED. In light of these findings, the FS determined by ARPES is consistent with LDA and de Haas-van Alphen (dHvA) results, and it provides additional information on the detailed shape of the alpha, beta and gamma sheets. Also, at this stage, because of the strong sensitivity of the cleaved surface, we could not find any robust signature of the crossover from 2D to 3D Fermi liquid behavior in our ARPES measurements for T<130 K.

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Superconducting Gap Anisotropy in Nd$_{1.85}$Ce$_{0.15}$CuO$_4$: Results from Photoemission

We have performed angle resolved photoelectron spectroscopy on the electron doped cuprate superconductor Nd$_{1.85}$Ce$_{0.15}$CuO$_4$. A comparison of the leading edge midpoints between the superconducting and normal states reveals a small, but finite shift of 1.5-2 meV near the ($π$,0) position, but no observable shift along the zone diagonal near ($π$/2,$π$/2). This is interpreted as evidence for an anisotropic superconducting gap in the electron doped materials, which is consistent with the presence of d-wave superconducting order in this cuprate superconductor.

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Fermi surface, pseudogaps and dynamical stripes in La2-xSrxCuO4

Doping dependence of the electronic structure of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) has been systematically studied in a series of photoemission measurements. The unusual spectral features in the underdoped regime are attributed to the formation of dynamical stripes and the opening of large and small pseudogaps.

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Angle-resolved photoemission study of insulating and metallic Cu-O chains in PrBa$_2$Cu$_3$O$_7$ and PrBa$_2$Cu$_4$O$_8$

We compare the angle-resolved photoemission spectra of the hole-doped Cu-O chains in PrBa$_2$Cu$_3$O$_7$ (Pr123) and in PrBa$_2$Cu$_4$O$_8$ (Pr124). While, in Pr123, a dispersive feature from the chain takes a band maximum at $k_b$ (momentum along the chain) $\sim$ $π/4$ and loses its spectral weight around the Fermi level, it reaches the Fermi level at $k_b$ $\sim$ $π/4$ in Pr124. Although the chains in Pr123 and Pr124 are approximately 1/4-filled, they show contrasting behaviors: While the chains in Pr123 have an instability to charge ordering, those in Pr124 avoid it and show an interesting spectral feature of a metallic coupled-chain system.

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Fermi Surface, Surface States, and Surface Reconstruction in Sr2RuO4

The electronic structure of Sr2RuO4 is investigated by high angular resolution ARPES at several incident photon energies. We address the controversial issues of the Fermi surface (FS) topology and of the van Hove singularity at the M point, showing that a surface state and the replica of the primary FS due to (sqrt2 x sqrt2) surface reconstruction are responsible for previous conflicting interpretations. The FS thus determined by ARPES is consistent with the de Haas-van Alphen results, and it provides additional information on the detailed shape of the alpha, beta and gamma sheets.

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Signature of Superfluid Density in the Single-Particle Excitation Spectrum of Bi2Sr2CaCu2O8+delta

We report that the doping and temperature dependence of photoemission spectra near the Brillouin zone boundary of Bi2Sr2CaCu2O8+delta exhibit unexpected sensitivity to the superfluid density. In the superconducting state, the photoemission peak intensity as a function of doping scales with the superfluid density and the condensation energy. As a function of temperature, the peak intensity shows an abrupt behavior near the superconducting phase transition temperature where phase coherence sets in, rather than near the temperature where the gap opens. This anomalous manifestation of collective effects in single-particle spectroscopy raises important questions concerning the mechanism of high-temperature superconductivity.

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Dual Nature of the Electronic Structure of the Stripe Phase

High resolution angle-resolved photoemission measurements have been carried out on (La_1.4-xNd_0.6Sr_x)CuO_4, a model system with static stripes, and (La_1.85Sr_0.15)CuO_4, a high temperature superconductor (T_c=40K) with dynamic stripes. In addition to the straight segments near (pi, 0) and (0, pi) antinodal regions, we have identified the existence of nodal spectral weight and its associated Fermi surface in the electronic structure of both systems. The ARPES spectra in the nodal region show well-defined Fermi cut-off, indicating a metallic character of this charge-ordered state. This observation of nodal spectral weight, together with the straight segments near antinodal regions, reveals dual nature of the electronic structure of the stripes due to the competition of order and disorder.

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Angle resolved photoemission spectroscopy of Sr_2CuO_2Cl_2 - a revisit

We have investigated the lowest binding-energy electronic structure of the model cuprate Sr_2CuO_2Cl_2 using angle resolved photoemission spectroscopy (ARPES). Our data from about 80 cleavages of Sr_2CuO_2Cl_2 single crystals give a comprehensive, self-consistent picture of the nature of the first electron-removal state in this model undoped CuO_2-plane cuprate. Firstly, we show a strong dependence on the polarization of the excitation light which is understandable in the context of the matrix element governing the photoemission process, which gives a state with the symmetry of a Zhang-Rice singlet. Secondly, the strong, oscillatory dependence of the intensity of the Zhang-Rice singlet on the exciting photon-energy is shown to be consistent with interference effects connected with the periodicity of the crystal structure in the crystallographic c-direction. Thirdly, we measured the dispersion of the first electron-removal states along G->(pi,pi) and G->(pi,0), the latter being controversial in the literature, and have shown that the data are best fitted using an extended t-J-model, and extract the relevant model parameters. An analysis of the spectral weight of the first ionization states for different excitation energies within the approach used by Leung et al. (Phys. Rev. B56, 6320 (1997)) results in a strongly photon-energy dependent ratio between the coherent and incoherent spectral weight. The possible reasons for this observation and its physical implications are discussed.

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n(k) Structure and Matrix Elements in Photoemission: Results from Insulating Ca_2CuO_2Cl_2

The photon energy dependence of angle-resolved photoemission data on Ca_2CuO_2Cl_2 is presented, and the role of the matrix element is investigated. It is shown that despite strong variations in the matrix element, the loss in intensity as one crosses the antiferromagnetic zone boundary is a robust feature of the Mott insulator. As expected for a two dimensional system, the dispersion remains independent of the photon energy even when the matrix element does not.

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Electronic Structure of La2-xSrxCuO4 in the Vicinity of the Superconductor-Insulator Transition

We report on the result of angle-resolved photoemission (ARPES) study of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) from an optimally doped superconductor ($x=0.15$) to an antiferromagnetic insulator ($x=0$). Near the superconductor-insulator transition (SIT) $x\sim 0.05$, spectral weight is transferred with hole doping between two coexisting components, suggesting a microscopic inhomogeneity of the doped-hole distribution. For the underdoped LSCO ($x\leq 0.12$), the dispersive band crossing the Fermi level becomes invisible in the $(0,0)-(π,π)$ direction unlike Bi$_2$Sr$_2$CaCu$_2$O$_{8+y}$. These observations may be reconciled with the evolution of holes in the insulator into fluctuating stripes in the superconductor.

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Fermi Surface and Band Dispersion in La2-xSrxCuO4

Using angle-resolved photoemission spectroscopy (ARPES), we have observed the band structure, Fermi surface and their doping dependences in La2-xSrxCuO4. The results reveal that the Fermi surface undergoes a dramatic change: it is hole-like and centered at k=(pi,pi) in underdoped (x = 0.1) and optimally doped (x = 0.15) samples as in other cuprates while it is electron-like and centered at (0,0) in heavily overdoped (x = 0.3) ones. The peak in the ARPES spectra near (pi/2,pi/2) is broad and weak unlike in other cuprates. In the underdoped and optimally doped samples, a superconducting gap (Delta = 10 - 15 meV) is observed on the Fermi surface near (pi,0).

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Spin Liquid State around a Doped Hole in Insulating Cuprates

The numerically exact diagonalization study on small clusters of the t-J model with the second- and third- neighbor hopping terms shows that a novel spin liquid state is realized around a doped hole with momentum k=(pi,0) and energy \sim 2J compared with that with (pi/2,pi/2) in insulating cuprates, where the spin and charge degrees of freedom are approximately decoupled. Our finding implies that the excitations in the insulating cuprates are mapped onto the the d-wave resonating valence bond state.

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Fermi Surface of Bi2212: a Systematic Revisit and Identification of Almost Perfectly Nested Fermi Surface Segments

The Fermi surface of the Bi2212 system is systematically studied using a variety of photon energies. In addition to reconciling the conflicting reports on the Fermi surface of this important material, we identify almost perfectly nested Fermi surface segments parallel to the $(1,0)$ or $(0,1)$ direction. This general yet long overlooked feature of the Fermi surface is intriguingly similar to the Fermi surface of the $La_{1.48}Nd_{0.4}Sr_{0.12}CuO_4$ system.

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Angle-resolved photoemission study of untwinned PrBa$_2$Cu$_3$O$_7$: undoped CuO$_2$ plane and doped CuO$_3$ chain

We have performed an angle-resolved photoemission study on untwinned PrBa$_2$Cu$_3$O$_7$, which has low resistivity but does not show superconductivity. We have observed a dispersive feature with a band maximum around ($π$/2,$π$/2), indicating that this band is derived from the undoped CuO$_2$ plane. We have observed another dispersive band exhibiting one-dimensional character, which we attribute to signals from the doped CuO$_3$ chain. The overall band dispersion of the one-dimensional band agrees with the prediction of $t-J$ model calculation with parameters relevant to cuprates except that the intensity near the Fermi level is considerably suppressed in the experiment.

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