arXiv subjects

Z. D. Han

Publications and source records attributed to Z. D. Han.

5 recordsLinked to original sources

arXiv2026

Enhancement of metallicity by Na doping in La$_3$Ni$_2$O$_{7+{\delta}}$

The observation of high-$T_c$ superconductivity in bilayer nickelate La$_3$Ni$_2$O$_7$ under high pressure provides a new venue for exploring novel unconventional superconductors and elucidating the mechanism of high-$T_c$ superconductivity. Subsequently, numerous chemical substitution studies have been reported, aiming to stabilize superconductivity at ambient pressure, or significantly reduce the pressure threshold required for its occurrence. Here, we report the comprehensive study on sodium (Na) doping in the Ruddlesden-Popper nickelate La$_3$Ni$_2$O$_{7+{\delta}}$, where Na$^+$ substitutes for La$^{3+}$ at the A-site with varying doping concentrations. The structural, thermal, magnetic, and electronic transport properties of as-synthesized polycrystalline samples were systematically investigated. X-ray diffraction (XRD) analysis reveals that Na doping induces a structural transition from the '327' Amam phase to the '4310' Bmab phase when $x\geq0.075$, which is further corroborated by thermogravimetric analysis (TGA) measurements. Substitution of La$^{3+}$ with Na$^+$ gives rise to a gradual expansion of the '327' phase lattice. Meanwhile, resistivity measurements indicate that the density wave (DW) transition is marginally suppressed and metallicity is significantly enhanced. Upon the application of pressure, DW transition can be further suppressed, whereas the low-$T$ insulating behaviors remain insensitive to pressure. These results offer critical insights into the roles of elemental substitution and charge carrier doping in steering the competing electronic phases in layered nickelates.

cond-mat.supr-con↗

arXiv2020

Anisotropic and extreme magnetoresistance in the magnetic semimetal candidate Erbium monobismuthide

Rare-earth monopnictides display rich physical behaviors, featuring most notably spin and orbital orders in their ground state. Here, we grow ErBi single crystal and study its magnetic, thermal and electrical properties. An analysis of the magnetic entropy and magnetization indicates that the weak magnetic anisotropy in ErBi possibly derives from the mixing effect, namely the anisotropic ground state of Er3+ (4f11) mingles with the isotropic excited state through exchange interaction. At low temperature, an extremely large magnetoresistance (~104%) with a parabolic magnetic-field dependence is observed, which can be ascribed to the nearly perfect electron-hole compensation and ultrahigh carrier mobility. When the magnetic field is rotated in the ab (ac) plane and the current flows in the b axis, the angular magnetoresistance in ErBi shows a twofold (fourfold) symmetry. Similar case has been observed in LaBi where the anisotropic Fermi surface dominates the low-temperature transport. Our theoretical calculation suggests that near the Fermi level ErBi shares similarity with LaBi in the electronic band structures. These findings indicate that the angular magnetoresistance of ErBi could be mainly determined by its anisotropic Fermi surface topology. Besides, contributions from several other possibilities, including the spin-dependent scattering, spin-orbit scattering, and demagnetization correlation to the angular magnetoresistance of ErBi are also discussed.

cond-mat.mtrl-sci↗

arXiv2020

Magnetic-field-induced nontrivial electronic state in the Kondo-lattice semimetal CeSb

Synergic effect of electronic correlation and spin-orbit coupling is an emerging topic in topological materials. Central to this rapidly developing area are the prototypes of strongly correlated heavy-fermion systems. Recently, some Ce-based compounds are proposed to host intriguing topological nature, among which the electronic properties of CeSb are still under debate. In this paper, we report a comprehensive study combining magnetic and electronic transport measurements, and electronic band structure calculations of this compound to identify its topological nature. Quantum oscillations are clearly observed in both magnetization and magnetoresistance at high fields, from which one pocket with a nontrivial Berry phase is recognized. Angular-dependent magnetoresistance shows that this pocket is elongated in nature and corresponds to the electron pocket as observed in LaBi. Nontrivial electronic structure of CeSb is further confirmed by first-principle calculations, which arises from spin splitting in the fully polarized ferromagnetic state. These features indicate that magnetic-field can induce nontrivial topological electronic states in this prototypical Kondo semimetal.

cond-mat.mtrl-sci↗

arXiv2017

Enhanced electron correlations in the new binary stannide PdSn4: a homologue of the Dirac nodal arc semimetal PtSn4

The advent of nodal-line semi-metals, i.e. systems in which the conduction and valence bands cross each other along a closed trajectory (line or loop) inside the Brillouin zone, has opened up a new arena for the exploration of topological condensed matter in which, due to a vanishing density of states near the Fermi level, electron correlation effects may also play an important role. In spite of this conceptual richness however, material realization of nodal-line (loop) fermions is rare, with PbTaSe2, ZrSiS and PtSn4 the only promising known candidates. Here we report the synthesis and physical properties of a new compound PdSn4 that is isostructural with PtSn4 yet possesses quasiparticles with significantly enhanced effective masses. In addition, PdSn4 displays an unusual polar angular magnetoresistance which at a certain field orientation, varies linearly with field up to 55 Tesla. Our study suggests that, in association with its homologue PtSn4 whose low-lying excitations were recently claimed to possess Dirac node arcs, PdSn4 may be a promising candidate in the search for novel topological states with enhanced correlation effects.

cond-mat.mtrl-sci↗

arXiv2017

Topological Phase Transition Under Pressure in the Topological Nodal Line Superconductor PbTaSe$_2$

A first-order-like resistivity hysteresis is induced by a subtle structural transition under hydrostatic pressure in the topological nodal-line superconductor PbTaSe$_2$. This structure transition is quickly suppressed to zero at pressure $\sim$0.25 GPa. As a result, superconductivity shows a marked suppression, accompanied with fundamental changes in the magnetoresistance and Hall resistivity, suggesting a Lifshitz transition around $\sim$0.25 GPa. The first principles calculations show that the spin-orbit interactions partially gap out the Dirac nodal line around $K$ point in the Brillouin zone upon applying a small pressure, whilst the Dirac states around $H$ point are completely destroyed. The calculations further reveal a second structural phase transition under a pressure as high as $\sim$30 GPa, through which a transition from a topologically nontrivial phase to a trivial phase is uncovered, with a superconducting dome emerging under this high-pressure phase.

cond-mat.supr-con↗