arXiv subjects

Z. Fisk

Publications and source records attributed to Z. Fisk.

At least 73 records · Page 4Linked to original sources

arXiv2013

Angle-resolved photoemission spectroscopy observation of anomalous electronic states in EuFe$_2$As$_{2-x}$P$_x$

We used angle-resolved photoemission spectroscopy to investigate the electronic structure of EuFe$_2$As$_2$, EuFe$_2$As$_{1.4}$P$_{0.6}$ and EuFe$_2$P$_2$. We observed doubled core level peaks associated to the pnictide atoms, which are related to a surface state. Nevertheless, strong electronic dispersion along the $c$ axis, especially pronounced in EuFe$_2$P$_2$, is observed for at less one band, thus indicated that the Fe states, albeit probably affected at the surface, do not form pure two-dimensional surface states. However, this latter material shows reduced spectral weight near the Fermi level as compared to EuFe$_2$As$_2$ and EuFe$_2$As$_{1.4}$P$_{0.6}$. An anomalous jump is also found in the electronic states associated with the Eu$^{2+}$ $f$ states in EuFe$_2$P$_2$.

cond-mat.supr-con↗

arXiv2013

Hybridization gap and Fano resonance in SmB${_6}$

We present results of Scanning Tunneling Microscopy and Spectroscopy (STS) measurements on the "Kondo insulator" SmB$_6$. The vast majority of surface areas investigated was reconstructed but, infrequently, also patches of varying size of non-reconstructed, Sm- or B-terminated surfaces were found. On the smallest patches, clear indications for the hybridization gap and inter-multiplet transitions were observed. On non-reconstructed surface areas large enough for coherent co-tunneling we were able to observe clear-cut Fano resonances. Our locally resolved STS indicated considerable finite conductance on all surfaces independent of their structure.

cond-mat.str-el↗

arXiv2013

Single crystal growth and physical properties of a new uranium compound URhIn$_5$

We have grown the new uranium compound URhIn$_5$ with the tetragonal HoCoGa$_5$-type by the In self flux method. In contrast to the nonmagnetic ground state of the isoelectronic analogue URhGa$_5$, URhIn$_5$ is an antiferromagnet with antiferromagnetic transition temperature $T_{\rm N}$ = 98 K. The moderately large electronic specific heat coefficient $γ$ = 50 mJ/K$^2$mol demonstrates the contribution of 5$f$ electrons to the conduction band. On the other hand, magnetic susceptibility in the paramagnetic state roughly follows a Curie-Weiss law with a paramagnetic effective moment corresponding to a localized uranium ion. The crossover from localized to itinerant character at low temperature may occur around the characteristic temperature 150 K where the magnetic susceptibility and electrical resistivity show a marked anomaly.

cond-mat.str-el↗

arXiv2013

Weak Antilocalization and Linear Magnetoresistance in The Surface State of SmB6

Strongly correlated Kondo insulator SmB6 is known for its peculiar low temperature residual conduction, which has recently been demonstrated to arise from a robust metallic surface state, as predicted by the theory of topological Kondo insulator (TKI). Photoemission, quantum oscillation and magnetic doping experiments have provided evidence for the Dirac-like dispersion and topological protection. Questions arise as whether signatures of spin-momentum locking and electron interaction could be resolved in transport measurements. Here we report metallic conduction of surface state down to mK temperatures with saturation behaviors suggestive of Kondo effect. We observe in the surface state the weak-antilocalization (WAL) effect that is in agreement with a spin-momentum locked metallic surface. At larger perpendicular magnetic fields, the surface state exhibits an unusual linear magnetoresistance similar to those found in Bi-based topological insulators and in graphene. (Correspondence to: xia.jing@uci.edu)

cond-mat.str-el↗

arXiv2013

Topological surface state in the Kondo Insulator Samarium Hexaboride

Strongly correlated electron systems show many exotic properties such as unconventional superconductity, quantum criticality, and Kondo insulating behavior. In addition, the Kondo insulator SmB6 has been predicted theoretically to be a 3D topological insulator with a metallic surface state. We report here transport measurements on doped SmB6, which show that ~3% magnetic and non-magnetic dopants in SmB6 exhibit clearly contrasting behavior, evidence that the metallic surface state is only destroyed when time reversal symmetry is broken. We find as well a quantum percolation limit of impurity concentration which transform the topological insulator into a conventional band insulator by forming impurity band. Our careful thickness dependence results show that SmB6 is the first demonstatrated perfect 3D topological insulator with virtually zero residual bulk conductivity.

cond-mat.str-el↗

arXiv2013

Robust Surface Hall Effect and Nonlocal Transport in SmB6: Indication for an Ideal Topological Insulator

A topological insulator (TI) is an unusual quantum state in which the insulating bulk is topologically distinct from vacuum, resulting in a unique metallic surface that is robust against time-reversal invariant perturbations. These surface transport properties, however, remains difficult to be isolated from the bulk in existing TI crystals (Bi2Se3, Bi2Te3 and Sb2Te3) due to impurity caused bulk conduction. We report in large crystals of topological Kondo insulator (TKI) candidate material SmB6 the thickness-independent surface Hall effects and non- local transport, which are robust against perturbations including mechanical abrasion. These results serve as proof that at low temperatures SmB6 has a robust metallic surface that surrounds a truly insulating bulk, paving the way for transport studies of the surface state in this proposed TKI material. (xia.jing@uci.edu).

cond-mat.str-el↗

arXiv2013

Anomalous doping effect on the superconducting state in CeCoIn$_5$ at high magnetic fields

We investigated the effect of electron and hole doping on the high-field low-temperature superconducting state in CeCoIn$_5$ by measuring specific heat of CeCo(In$_{\rm 1-x}$M$_{\rm x}$)$_5$ with M=Sn, Cd and Hg and $x$ up to 0.33% at temperatures down to 0.1\,K and fields up to 14\,T. Although both Cd- and Hg-doping (hole-doping) suppresses the zero-field $T_c$ monotonically, $H_{c2}$ increases with small amounts of doping and has a maximum around $x$=0.2% (M=Cd). On the other hand, with Sn-doping (electron-doping) both zero-field $T_c$ and $H_{c2}$ decrease monotonically. The critical temperature for the high-field low-temperature superconducting state (so called {\it Q}-state) correlates with $H_{c2}$ and $T_c$, which we interpret in support of the superconducting origin of this state.

cond-mat.str-el↗

arXiv2013

Quantum oscillations in Kondo Insulator SmB$_6$

In Kondo insulator samarium hexaboride SmB$_6$, strong correlation and band hybridization lead to an insulating gap and a diverging resistance at low temperature. The resistance divergence ends at about 5 Kelvin, a behavior recently demonstrated to arise from the surface conductance. However, questions remain whether and where a topological surface state exists. Quantum oscillations have not been observed to map the Fermi surface. We solve the problem by resolving the Landau Level quantization and Fermi surface topology using torque magnetometry. The observed Fermi surface suggests a two dimensional surface state on the (101) plane. Furthermore, the tracking of the Landau Levels in the infinite magnetic field limit points to -1/2, which indicates a 2D Dirac electronic state.

cond-mat.str-el↗

arXiv2013

Surface electronic structure of a topological Kondo insulator candidate SmB6: insights from high-resolution ARPES

The Kondo insulator SmB6 has long been known to exhibit low temperature (T < 10K) transport anomaly and has recently attracted attention as a new topological insulator candidate. By combining low-temperature and high energy-momentum resolution of the laser-based ARPES technique, for the first time, we probe the surface electronic structure of the anomalous conductivity regime. We observe that the bulk bands exhibit a Kondo gap of 14 meV and identify in-gap low-lying states within a 4 meV window of the Fermi level on the (001)-surface of this material. The low-lying states are found to form electron-like Fermi surface pockets that enclose the X and the Gamma points of the surface Brillouin zone. These states disappear as temperature is raised above 15K in correspondence with the complete disappearance of the 2D conductivity channels in SmB6. While the topological nature of the in-gap metallic states cannot be ascertained without spin (spin-texture) measurements our bulk and surface measurements carried out in the transport-anomaly-temperature regime (T < 10K) are consistent with the first-principle predicted Fermi surface behavior of a topological Kondo insulator phase in this material.

cond-mat.str-el↗

arXiv2012

Electronic phase separation due to magnetic polaron formation in the semimetallic ferromagnet EuB$_6$ - A weakly-nonlinear-transport study

We report measurements of weakly nonlinear electronic transport, as measured by third-harmonic voltage generation $V_{3ω}$, in the low-carrier density semimetallic ferromagnet EuB$_6$, which exhibits an unusual magnetic ordering with two consecutive transitions at $T_{c_1} = 15.6$\,K and $T_{c_2} = 12.5$\,K. Upon cooling in zero magnetic field through the ferromagnetic transition, the dramatic drop in the linear resistivity at the upper transition $T_{c_1}$ coincides with the onset of nonlinearity, and upon further cooling is followed by a pronounced peak in $V_{3 ω}$ at the lower transition $T_{c_2}$. Likewise, in the paramagnetic regime, a drop of the material's magnetoresistance $R(H)$ precedes a magnetic-field-induced peak in nonlinear transport. A striking observation is a linear temperature dependence of $V_{3ω}^{\rm peak}(H)$. We suggest a picture where at the upper transition $T_{c_1}$ the coalescing MP form a conducting path giving rise to a strong decrease in the resistance. The MP formation sets in at around $T^\ast \sim 35$\,K below which these entities are isolated and strongly fluctuating, while growing in number. The MP then start to form links at $T_{c_1}$, where percolative electronic transport is observed. The MP merge and start forming a continuum at the threshold $T_{c_2}$. In the paramagnetic temperature regime $T_{c_1} < T < T^\ast$, MP percolation is induced by a magnetic field, and the threshold accompanied by charge carrier delocalization occurs at a single critical magnetization.

cond-mat.str-el↗

arXiv2012

Electronic tuning and uniform superconductivity in CeCoIn5

We report a globally reversible effect of electronic tuning on the magnetic phase diagram in CeCoIn_{5} driven by electron (Pt and Sn) and hole (Cd, Hg) doping. Consequently, we are able to extract the superconducting pair breaking component for hole and electron dopants with pressure and co-doping studies, respectively. We find that these nominally non-magnetic dopants have a remarkably weak pair breaking effect for a d-wave superconductor. The pair breaking is weaker for hole dopants, which induce magnetic moments, than for electron dopants. Furthermore, both Pt and Sn doping have a similar effect on superconductivity despite being on different dopant sites, arguing against the notion that superconductivity lives predominantly in the CeIn_{3} planes of these materials. In addition, we shed qualitative understanding on the doping dependence with density functional theory calculations.

cond-mat.supr-con↗

arXiv2012

Controllable chirality-induced geometrical Hall effect in a frustrated highly-correlated metal

A current of electrons traversing a landscape of localized spins possessing non-coplanar magnetic order gains a geometrical (Berry) phase which can lead to a Hall voltage independent of the spin-orbit coupling within the material--a geometrical Hall effect. We show that the highly-correlated metal UCu5 possesses an unusually large controllable geometrical Hall effect at T<1.2K due to its frustration-induced magnetic order. The magnitude of the Hall response exceeds 20% of the ν=1 quantum Hall effect per atomic layer, which translates into an effective magnetic field of several hundred Tesla acting on the electrons. The existence of such a large geometric Hall response in UCu5 opens a new field of inquiry into the importance of the role of frustration in highly-correlated electron materials.

cond-mat.str-el↗

arXiv2012

Probing the localized to itinerant behavior of the 4f electron in CeIn3-xSnx by Gd3+ electron spin resonance

The CeIn3-xSnx cubic heavy fermion system presents an antiferromagnetic transition at T_N = 10 K, for x = 0, that decreases continuously down to 0 K upon Sn substitution at a critical concentration of x_c ~ 0.65. In the vicinity of T_N -> 0 the system shows non-Fermi liquid behavior due to antiferromagnetic critical fluctuations. For a high Sn content, x > 2.2, intermediate valence effects are present. In this work we show that Gd3+-doped electron spin resonance (ESR) probes a change in the character of the Ce 4f electron, as a function of Sn substitution. The Gd3+ ESR results indicate a transition of the Ce 4f spin behavior from localized to itinerant. Near the quantum critical point, on the antiferromagnetic side of the magnetic phase diagram, both localized and itinerant behaviors coexist.

cond-mat.str-el↗

arXiv2012

Direct observation of the quantum critical point in heavy fermion CeRhSi$_3$

We report on muon spin rotation studies of the noncentrosymmetric heavy fermion antiferromagnet CeRhSi$_3$. A drastic and monotonic suppression of the internal fields, at the lowest measured temperature, was observed upon an increase of external pressure. Our data suggest that the ordered moments are gradually quenched with increasing pressure, in a manner different from the pressure dependence of the Néel temperature. At $\unit{23.6}{kbar}$, the ordered magnetic moments are fully suppressed via a second-order phase transition, and $T_{\rm{N}}$ is zero. Thus, we directly observed the quantum critical point at $\unit{23.6}{kbar}$ hidden inside the superconducting phase of CeRhSi$_3$.

cond-mat.str-el↗

arXiv2012

Magnetically-driven electronic phase separation in the semimetallic ferromagnet EuB$_6$

From measurements of fluctuation spectroscopy and weak nonlinear transport on the semimetallic ferromagnet EuB$_6$ we find direct evidence for magnetically-driven electronic phase separation consistent with the picture of percolation of magnetic polarons (MP), which form highly conducting magnetically-ordered clusters in a paramagnetic and 'poorly conducting' background. These different parts of the conducting network are probed separately by the noise spectroscopy/nonlinear transport and the conventional linear resistivity. We suggest a comprehensive and 'universal' scenario for the MP percolation, which occurs at a critical magnetization either induced by ferromagnetic order at zero field or externally applied magnetic fields in the paramagentic region.

cond-mat.str-el↗

arXiv2012

Pressure effects on the heavy-fermion antiferromagnet CeAuSb2

The f-electron compound CeAuSb2, which crystallizes in the ZrCuSi2-type tetragonal structure, orders antiferromagnetically between 5 and 6.8 K, where the antiferromagnetic transition temperature T_N depends on the occupancy of the Au site. Here we report the electrical resistivity and heat capacity of a high-quality crystal CeAuSb2 with T_N of 6.8 K, the highest for this compound. The magnetic transition temperature is initially suppressed with pressure, but is intercepted by a new magnetic state above 2.1 GPa. The new phase shows a dome shape with pressure and coexists with another phase at pressures higher than 4.7 GPa. The electrical resistivity shows a T^2 Fermi liquids behavior in the complex magnetic state, and the residual resistivity and the T^2 resistivity coefficient increases with pressure, suggesting the possibility of a magnetic quantum critical point at a higher pressure.

cond-mat.str-el↗

arXiv2011

Shubnikov-de Haas measurements on LuRh2Si2

We present Shubnikov-de Haas measurements on LuRh2Si2, the non-magnetic reference compound to the prototypical heavy-fermion system YbRh2Si2. We find an extensive set of orbits with clear angular dependences. Surprisingly, the agreement with non-correlated band structure calculations is limited. This may be related to an uncertainty in the calculations arising from a lack of knowledge about the exact Si atom position in the unit cell. The data on LuRh2Si2 provide an extensive basis for the interpretation of measurements on YbRh2Si2 indicative of discrepancies between the high-field Fermi surface of YbRh2Si2 and the "small" Fermi surface configuration.

cond-mat.str-el↗

arXiv2011

Electron spin resonance study of the LaIn3-xSnx superconducting system

The LaIn3-xSnx alloy system is composed of superconducting Pauli paramagnets. For LaIn3 the superconducting critical temperature T_c is approximately 0.7 K and it shows an oscillatory dependence as a function of Sn substitution, presenting its highest value T_c ~ 6.4 K for the LaSn3 end member. The superconducting state of these materials was characterized as being of the conventional type. We report our results for Gd3+ electron spin resonance (ESR) measurements in the LaIn3-xSnx compounds as a function of x. We show that the effective exchange interaction parameter J_fs between the Gd3+ 4f local moment and the s-like conduction electrons is almost unchanged by Sn substitution and observe microscopically that LaSn3 is a conventional superconductor.

cond-mat.supr-con↗