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Z. Halász

Publications and source records attributed to Z. Halász.

At least 19 recordsLinked to original sources

The dipole strength distribution of $^8$He and decay characteristics

The weak binding and spatially extended neutron densities characteristic of drip-line nuclei give rise to a distinctive low-energy dipole response. The drip-line nucleus $^8$He is the most neutron-rich bound nucleus with a mass-to-charge ratio of $A/Z=4$. We measure the dipole response of $^8$He, including for the first time the four-neutron decay channel. A total dipole strength of $\sum B(E1)(E^*<15$~MeV$)=0.95(16)~e^2$fm$^2$ and a dipole polarizability of $α_D = 0.61(1)$~fm$^3$ are extracted from the differential Coulomb-excitation cross section and compared to state-of-the-art theoretical calculations employing coupled cluster and three-body approaches. We find that the dipole continuum is dominated, even at high excitation energies well above the $4n$ decay threshold, by two-neutron emission, pointing to a $^6$He$+2n$ structure of the excited dipole mode. No indication was found for a $4n$ final-state correlation, while pronounced $nn$ and $^6$He-$n$ final-state correlations are apparent.

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Direct observation of three-neutron emission from $^7$He$^*$ and the search for the trineutron

Three-neutron emission from $^7$He has been directly measured for the first time, following neutron knockout from a $^8$He beam at 156 MeV/nucleon. A resonance-like structure at $2.08(4)$ MeV above the $^4$He+$3n$ threshold [$E_x=2.68(4)$ MeV] with a width of $3.9(2)$ MeV was observed and deduced to arise predominately from the predicted $J^π=3/2^{-}_2$ level. The three-neutron invariant-mass spectrum was reconstructed and found to peak at around 1 MeV and could, through complete simulations incorporating neutron-neutron correlations, be very well described by the sequential decay of $^7$He$^*$ via the $2_1^+$ excited state of $^6$He. No evidence was found for any significant three-neutron correlations beyond those expected from well-established two-body interactions, including a trineutron resonance.

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Gas-cell development for nuclear astrophysics motivated studies on noble gas targets and the $^3$He($α$,$γ$)$^7$Be reaction

In many astrophysical scenarios, alpha induced reactions on noble gas nuclei play a crucial role. Studying these reactions in the laboratory requires the noble gas atoms to be confined in a sufficient amount to allow the reactions. At Atomki thin-windowed gas-cell targets were developed and improved for studying alpha induced reactions on noble gases. Several stages of the gas-cell design used for activation experiments and lately a version to be used for particle scattering experiments will be presented. A new experimental study of the $^3$He($α$,$γ$)$^7$Be reaction with one of the activation gas-cell targets was performed. This reaction plays an important role both in the solar pp-chains and in big bang nucleosynthesis. The reaction cross section was measured in the past in several works, however, there are still energy regions lacking experimental data, rendering the extrapolations towards the astrophysically relevant energies uncertain. New experimental total cross section of the $^3$He($α$,$γ$)$^7$Be reaction was thus determined here in the energy range of $E_\mathrm{c.m.} = 2600-3000$ keV in about 50 keV energy steps. These results confirm the overall trend, and also the absolute scale set by the only one previous measurement in this energy range. In addition, two pilot experiments with the scattering cell were performed aiming to study the $^4$He($α$,$α$)$^4$He and $^{124}$Xe($α$,$α$)$^{124}$Xe reactions at $E_α= 18$ MeV. These studies benchmark the performance of the cell and detection system both for light and heavy noble gas targets.

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Continuous high-yield fast neutron generation with few-cycle laser pulses at 10 Hz for applications

We present a laser-based neutron source that produces $1.8 \times 10^5$ neutrons/s with a conversion rate of $7.8 \times 10^5$ neutrons/J. Laser pulses of 12 fs and 23 mJ were focused onto a 430-nm-thick heavy water liquid sheet at a 10 Hz repetition rate. The resulting peak intensity of $4 \times 10^{18}$ W/cm$^2$ accelerated deuterium ions from the target rear side to a kinetic energy of 1 MeV. This deuteron beam induced $^{2}$H(d,n)$^{3}$He fusion reactions in a deuterated polyethylene target, producing fast neutrons. The neutron yield was measured using two independent detection systems: the LILITH time-of-flight spectrometer, consisting of eight plastic scintillators covering nearly $180^\circ$, and a calibrated bubble detector spectrometer. The neutron yield per laser shot is 35 times higher than that recently achieved by lasers with comparable pulse energies, while the conversion rate is the highest ever achieved by continuously operating, sub-100 fs lasers. The generated neutrons are emitted from an area of 0.65 cm$^2$ corresponding to the deuteron beam spot on the catcher. Their angular distribution is peaked in forward and backward directions in agreement with the literature data on the angular distribution of $^{2}$H(d,n)$^{3}$He reaction. The system operated continuously for several hours per day with an unprecedented stability of 5%.

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Measurement of the E_p = 416.9 keV resonance strength in the 29Si(p,gamma)30P reaction

Silicon isotopic ratios measured in meteoritic presolar grains can provide useful information about the nucleosynthesis origin of these isotopes if the rates of nuclear reactions responsible for their production are known. One of the key reactions determining the Si isotopic abundances is 29Si(p,gamma)30P. Its reaction rate is not known with sufficient precision due in part to some ambiguous resonance strength values. In the present work, the strength of the E_p = 416.9 keV resonance has been measured with high precision using the activation technique. The new strength of omega_gamma = 219 +- 16 meV can be used in updated reaction rate estimations and astrophysical models.

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Low energy alpha-nucleus optical potential studied via (a,n) cross section measurements on Te isotopes

In several processes of stellar nucleosynthesis, like the astrophysical gamma-process, nuclear reactions involving alpha particles play an important role. The description of these reactions necessitates the knowledge of the alpha-nucleus optical model potential (AOMP) which is highly ambiguous at low, astrophysical energies. This ambiguity introduces a substantial uncertainty in the stellar models for predicting elemental and isotopic abundances. The experimental study of the AOMP is thus necessary which can be implemented by measuring the cross section of alpha-induced nuclear reactions. At low energies, (a,n) reactions are suitable for such a purpose. Therefore, in the present work, the (a,n) cross sections of four Te isotopes have been measured, mostly for the first time, and compared with theoretical predictions. The (a,n) cross sections of 120,122,124,130Te have been measured in the energy range between about 10 and 17 MeV using the activation method. The detection of the gamma radiation following the decay of the radioactive reaction products were used to determine the cross sections. The measured cross sections are compared with statistical model calculations obtained from the widely used TALYS nuclear reaction simulation code. Predictions using various available AOMPs are investigated. It is found that the recently developed Atomki-V2 AOMP provides the best description for all studied reactions and this potential also reproduces well the total reaction cross sections from elastic scattering experiments, when they are available in literature. We recommend therefore to use the astrophysical reaction rates based on this potential for nucleosynthesis models of heavy elements.

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Experimental determination of the $^3$He($α$,$γ$)$^7$Be reaction cross section above the $^7$Be proton separation threshold

The $^3$He($α$,$γ$)$^7$Be reaction plays a major role both in the BBN producing the majority of the primordial $^7$Li, and in the pp-chain, where it is the branching point. As a few-nucleon system, this reaction is often used to validate ab-initio theoretical calculations and/or test R-matrix theory and code implementations. For the latter, experimental data in an extended energy range is of crucial importance to test the fit and extrapolation capabilities of the different codes. The $^3$He($α$,$γ$)$^7$Be reaction cross section has been measured by several groups up to the first resonance ($E_{c.m.} \approx 3$ MeV) in the reaction. However, only one dataset exists above the $^7$Be proton separation threshold measured in a narrow energy range ($E_{c.m.} = 4.0-4.4$ MeV). In this work we extend the available experimental capture cross section database to the energy range of known $^7$Be levels. The activation method was used. The experiment was performed using a thin-window gas cell with two high-purity Al foils as entrance and exit windows. The activity of the $^7$Be nuclei implanted in the exit/catcher foil was measured by detecting the yield of the emitted $γ$~rays using shielded high-purity germanium detectors. New experimental $^3$He($α$,$γ$)$^7$Be reaction cross section data were obtained for the first time in the $E_{c.m.}=4.3-8.3$ MeV energy region. The new dataset with about 0.2 MeV step covers the energy range of known levels and particle separation thresholds. No prominent structures are observer around the $^7$Be levels. The reaction cross section is slowly increasing with increasing energy. Above the $^6$Li$+p_1$ threshold, a decrease starts in the cross section trend. The overall structure of the cross section suggest a broad resonance peaking around $E_x=7.5$ MeV $^7$Be excitation energy, with a width of 8 MeV.

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Cross section measurement of the 12C(p,gamma)13N reaction with activation in a wide energy range

The CNO cycle is one of the fundamental processes of hydrogen burning in stars. The first reaction of the cycle is the radiative proton capture on 12C and the rate of this 12C(p,gamma)13N reaction is related to the 12C/13C ratio observed e.g. in the Solar System. The low-energy cross section of this reaction was measured several times in the past, however, the experimental data are scarce in a wide energy range especially around the resonance at 1.7 MeV. In the present work the 12C(p,gamma)13N cross section was measured between 300 and 1900 keV using the activation method. This method was only used several decades ago in the low-energy region. As the activation method provides the total cross section and has uncertainties different from those of the in-beam gamma-spectroscopy technique, the present results provide a largely independent data set for future low-energy extrapolations and thus for astrophysical reaction rate calculations.

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Cross section measurement of the 144Sm(alpha,n)147Gd reaction for studying the alpha-nucleus optical potential at astrophysical energies

Nuclear reactions involving alpha particles play an important role in various astrophysical processes such as the gamma-process of heavy element nucleosynthesis. The poorly known low-energy alpha-nucleus optical (AOMP) potential is a key parameter to estimate the rates of these reactions. The AOMP can be tested by measuring the cross section of alpha-scattering as well as alpha-induced reactions. Low energy elastic alpha-scattering on 144Sm has recently been measured with high precision. The aim of the present work was to complement that work by measuring the (a,n) cross sections on 144Sm at low energies. The experimental data shall be used to constrain the AOMP. From this potential the 144Sm(a,g)148Gd reaction rate can be derived with reduced uncertainties. The 144Sm(a,n)147Gd reaction was studied by bombarding Sm targets with alpha-beams provided by the cyclotron accelerator of Atomki. The cross section was determined using the activation method. The gamma-radiation following the decay of the 147Gd reaction product was measured with a HPGe detector. The experimental data are analyzed within the statistical model. The cross section was measured in the alpha-energy range between 13 and 20 MeV in 1 MeV steps, i.e., from close above the (a,n) threshold. The results were compared with statistical model calculations using various approaches and parametrizations for the AOMP, and excellent agreement was obtained for two recent potentials. However, these potentials cannot reproduce literature data for the 144Sm(a,g)148Gd reaction with the same accuracy. Constraints for the AOMP were derived from an analysis of the new 144Sm(a,n)147Gd data and literature data for 144Sm(a,g)148Gd. These constraints enable a determination of the reaction rate of the 144Sm(a,g)148Gd reaction with significantly reduced uncertainties of less than a factor of two.

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Activation cross section measurement of the 14N(p,gamma)15O astrophysical key reaction

14N(p,gamma)15O is one of the key reactions of nuclear astrophysics playing a role in various stellar processes and influencing energy generation of stars, stellar evolution and nucleosynthesis. For a reliable reaction rate calculation the low energy cross section of 14N(p,gamma)15O must be known with high accuracy. Owing to the unmeasurable low cross sections, theoretical calculations are unavoidable. High precision experimental cross section data are needed in a wide energy range in order to provide the necessary basis for low energy extrapolations. In the present work the total 14N(p,gamma)15O cross section was measured with a method complementary to the available data sets. The cross section was measured with activation, based on the detection of the annihilation radiation following the beta+ decay of the reaction product 15O. This method, which provides directly the astrophysically important total cross section, was never used for the 14N(p,gamma)15O cross section measurement in the studied energy range. The non-resonant cross section was measured between 550 keV and 1400 keV center-of-mass energies with total uncertainty of about 10%. The results were compared with literature data using an R-matrix analysis. It is found that the cross sections measured in this work are in acceptable agreement with the two recent measurements only if the weak transitions - not measured in those works - are included. The present data set, being largely independent from the other available data, can be used to constrain the extrapolated cross sections to astrophysical energies and helps to make the astrophysical model calculations more reliable.

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Measurement of the 91Zr(p,gamma)92mNb cross section motivated by type Ia supernova nucleosynthesis

The synthesis of heavy, proton rich isotopes is a poorly understood astrophysical process. Thermonuclear (type Ia) supernova explosions are among the suggested sites and the abundance of some isotopes present in the early solar system may be used to test the models. 92Nb is such an isotope and one of the reactions playing a role in its synthesis is 91Zr(p,gamma)92Nb. As no experimental cross sections were available for this reaction so far, nucleosynthesis models had to solely rely on theoretical calculations. In the present work the cross section of 91Zr(p,gamma)92mNb has been measured at astrophysical energies by activation. The results excellently confirm the predictions of cross sections and reaction rates for 91Zr(p,gamma)92Nb, as used in astrophysical simulations.

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On the $β$-decay of $^{186}$Hg

The Gamow-Teller strength distribution of the decay of $^{186}$Hg into $^{186}$Au has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. The best description of the experimental beta strength is obtained with dominantly prolate components for both parent $^{186}$Hg and daughter $^{186}$Au. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.

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Cross section of $α$-induced reactions on $^{197}$Au at sub-Coulomb energies

Statistical model calculations have to be used for the determination of reaction rates in large-scale reaction networks for heavy-element nucleosynthesis. A basic ingredient of such a calculation is the a-nucleus optical model potential. Several different parameter sets are available in literature, but their predictions of a-induced reaction rates vary widely, sometimes even exceeding one order of magnitude. This paper presents the result of a-induced reaction cross-section measurements on gold which could be carried out for the first time very close to the astrophysically relevant energy region. The new experimental data are used to test statistical model predictions and to constrain the a-nucleus optical model potential. For the measurements the activation technique was used. The cross section of the (a,n) and (a,2n) reactions was determined from g-ray counting, while that of the radiative capture was determined via X-ray counting. The cross section of the reactions was measured below E$_a=20.0$~MeV. In the case of the $^{197}$Au(a,2n)$^{199}$Tl reaction down to 17.5~MeV with 0.5-MeV steps, reaching closer to the reaction threshold than ever before. The cross section of $^{197}$Au(a,n)$^{200}$Tl and $^{197}$Au(a,g)$^{201}$Tl was measured down to E$_a=13.6$ and 14.0~MeV, respectively, with 0.5-MeV steps above the (a,2n) reaction threshold and with 1.0-MeV steps below that. The new dataset is in agreement with the available values from the literature, but is more precise and extends towards lower energies. Two orders of magnitude lower cross sections were successfully measured than in previous experiments which used g-ray counting only, thus providing experimental data at lower energies than ever before. The new precision dataset allows us to find the best-fit a-nucleus optical model potential and to predict cross sections in the Gamow window with smaller uncertainties.

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Resonance strengths in the 14N(p,gamma)15O astrophysical key reaction measured with activation

The 14N(p,gamma)15O reaction plays a vital role in various astrophysical scenarios. Its reaction rate must be accurately known in the present era of high precision astrophysics. The cross section of the reaction is often measured relative to a low energy resonance, the strength of which must therefore be determined precisely. The activation method, based on the measurement of 15O decay, has not been used in modern measurements of the 14N(p,gamma)15O reaction. The aim of the present work is to provide strength data for two resonances in the 14N(p,gamma)15O reaction using the activation method. The obtained values are largely independent from previous data measured by in-beam gamma-spectroscopy and are free from some of their systematic uncertainties. Solid state TiN targets were irradiated with a proton beam provided by the Tandetron accelerator of Atomki using a cyclic activation. The decay of the produced 15O isotopes was measured by detecting the 511 keV positron annihilation gamma-rays. The strength of the Ep = 278 keV resonance was measured to be 13.4 +- 0.8 meV while for the Ep = 1058 keV resonance the strength is 442 +- 27 meV. The obtained Ep = 278 keV resonance strength is in fair agreement with the values recommended by two recent works. On the other hand, the Ep = 1058 keV resonance strength is about 20% higher than the previous value. The discrepancy may be caused in part by a previously neglected finite target thickness correction. As only the low energy resonance is used as a normalization point for cross section measurements, the calculated astrophysical reaction rate of the 14N(p,gamma)15O reaction and therefore the astrophysical consequences are not changed by the present results.

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Cross section of $^3$He($α$,$γ$)$^7$Be around the $^7$Be proton separation threshold

The $^3$He($α$,$γ$)$^7$Be reaction is a widely studied nuclear reaction; however, it is still not understood with the required precision. It has a great importance both in Big Bang nucleosynthesis and in solar hydrogen burning. The low mass number of the reaction partners makes it also suitable for testing microscopic calculations. Despite the high number of experimental studies, none of them addresses the $^3$He($α$,$γ$)$^7$Be reaction cross sections above 3.1-MeV center-of-mass energy. Recently, a previously unobserved resonance in the $^6$Li(p,$γ$)$^7$Be reaction suggested a new level in $^7$Be, which would also have an impact on the $^3$He($α$,$γ$)$^7$Be reaction in the energy range above 4.0 MeV. The aim of the present experiment is to measure the $^3$He($α$,$γ$)$^7$Be reaction cross section in the energy range of the proposed level. For this investigation the activation technique was used. A thin window gas-cell target confining $^3$He gas was irradiated using an $α$ beam. The $^7$Be produced was implanted into the exit foil. The $^7$Be activity was determined by counting the $γ$ rays following its decay by a well-shielded high-purity germanium detector. Reaction cross sections have been determined between $E_{cm} = 4.0 - 4.4$ MeV with 0.04-MeV steps covering the energy range of the proposed nuclear level. One lower-energy cross-section point was also determined to be able to compare the results with previous studies. A constant cross section of around 10.5 $μ$barn was observed around the $^7$Be proton separation energy. An upper limit of 45 neV for the strength of a $^3$He($α$,$γ$)$^7$Be resonance is derived.

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Study of multi-neutron systems with SAMURAI spectrometer

The tetraneutron has been drawing the attention of the nuclear physics community for decades, but a firm conclusion on its existence and properties is still far from being reached despite many experimental and theoretical efforts. New measurements have recently been performed at RIBF with the SAMURAI spectrometer by applying complementary reaction probes, which will help to pin down the properties of this four-neutron system.

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Half-life measurement of 65Ga with gamma-spectroscopy

The literature half-life value of 65Ga is based on only one experiment carried out more than 60 years ago and it has a relatively large uncertainty. In the present work this half-life is determined based on the counting of the gamma-rays following the beta-decay of 65Ga. Our new recommended half-life is 15.133 +- 0.028 min which is in agreement with the literature value but almost one order of magnitude more precise.

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Investigation of $α$-induced reactions on Sb isotopes relevant to the astrophysical $γ$-process

The aim of the present work is to measure the $^{121}$Sb($α,γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reaction cross sections. The $α$-induced reactions on natural and enriched antimony targets were investigated using the activation technique. The ($α$,$γ$) cross sections of $^{121}$Sb were measured and are reported for first time. To determine the cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reactions, the yields of $γ$-rays following the $β$-decay of the reaction products were measured. For the measurement of the lowest cross sections, the characteristic X-rays were counted with a LEPS (Low Energy Photon Spectrometer) detector. The cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I and $^{123}$Sb($α$,n)$^{126}$I reactions were measured with high precision in an energy range between 9.74 MeV to 15.48 MeV, close to the astrophysically relevant energy window. The results are compared with the predictions of statistical model calculations. The ($α$,n) data show that the $α$ widths are predicted well for these reactions. The ($α$,$γ$) results are overestimated by the calculations but this is due to the applied neutron- and $γ$ widths. Relevant for the astrophysical reaction rate is the $α$ width used in the calculations.While for other reactions the $α$ widths seem to have been overestimated and their energy dependence was not described well in the measured energy range, this is not the case for the reactions studied here. The result is consistent with the proposal that additional reaction channels, such as Coulomb excitation, may have led to the discrepancies found in other reactions.

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