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Z. Hatzopoulos

Publications and source records attributed to Z. Hatzopoulos.

At least 19 recordsLinked to original sources

Steady state oscillations of circular currents in concentric polariton condensates

Concentric ring exciton polariton condensates emerging under non-resonant laser pump in an annular trapping potential support persistent circular currents of polaritons. The trapping potential is formed by a cylindrical micropillar etched in a semiconductor microcavity with embedded quantum wells and a repulsive cloud of optically excited excitons under the pump spot. The symmetry of the potential is subject to external control via manipulation by its pump-induced component. In the manuscript, we demonstrate excitation of concentric ring polariton current states with predetermined vorticity which we trace using interferometry measurements with a spherical reference wave. We also observe the polariton condensate dynamically changing its vorticity during observation, which results in pairs of fork-like dislocations on the time-averaged interferogram coexisting with azimuthally homogeneous photoluminescence distribution in the micropillar.

cond-mat.mes-hall

Double ring polariton condensates with polariton vortices

We study formation of superfluid currents of exciton polaritons in annular polariton condensates in a cylindrical micropillar cavity under the spatially localised nonresonant optical pumping. Since polariton condensates are strongly nonequilibrium systems, the trapping potential for polaritons, formed by the pillar edge and the reservoir of optically induced incoherent excitons, is complex in general case. Its imaginary part includes the spatially distributed gain from the pump and losses of polaritons in the condensate. We show that engineering the gain-loss balance in the micropillar plane gives access to the excited states of the polariton condensate. We demonstrate both theoretically and experimentally formation of vortices in double concentric ring polariton condensates in the complex annular trap potential.

cond-mat.mes-hall

Stochastic circular persistent currents of exciton polaritons

We keep track of the orbital degree of freedom of an exciton polariton condensate, confined in an optical trap, and reveal the stochastic switching of persistent annular polariton currents in the pulse-periodic excitation regime.In an elliptic trap, the low-lying in energy polariton current states are inherent in a two-petalled density distribution and swirling phase. In the stochastic regime, the averaged over multiple excitation pulses density distribution gets homogenised in the azimuthal direction, while the weighted phase extracted from interference experiments experiences two compensating each other jumps, when varying around the center of the trap. Breaking the reciprocity of the system with a supplemental control optical pulse makes it possible to switch the system from the stochastic regime to the deterministic regime of an arbitrary polariton circulation.

cond-mat.mes-hall

Spin noise signatures of the self-induced Larmor precession

Bose-Einstein condensates of exciton-polaritons are known for their fascinating coherent and polarization properties. The spin state of the condensate is reflected in polarization of the exciton-polariton emission, with temporal fluctuations of this polarization being, in general, capable of reflecting quantum statistics of polaritons in the condensate. To study the polarization properties of optically trapped polariton condensates, we take advantage of the spin noise spectroscopy technique. The ratio between the noise of ellipticity of the condensate emission and its polarization plane rotation noise is found to be dependent, in a nontrivial way, on the intensity of CW nonresonant laser pumping. We show that the interplay between the ellipticity and the rotation noise can be explained in terms of the competition between the self-induced Larmor precession of the condensate pseudospin and the static polarization anisotropy of the microcavity.

cond-mat.mes-hall

Determination of polariton condensates' critical temperature

We investigate the thermal robustness of traveling polariton condensates. We create remote condensates that have never been in contact, and study their interference in momentum space, when they travel with the same velocity, by means of time-resolved photoluminescence. We determine the condensed to thermal, uncondensed polariton fraction, which shows a gradual decay with increasing temperature, and obtain the critical temperature for the Bose-Einstein-like condensate (BEC) phase transition. We tentatively compare our experimental findings with theoretical models, developed for atomic condensates, to describe the condensates' coherence fading with temperature.

cond-mat.mes-hall

Temperature dependence of the coherence in polariton condensates

We present a time-resolved experimental study of the temperature effect on the coherence of traveling polariton condensates. The simultaneous detection of their emission both in real- and reciprocal-space allows us to fully monitor the condensates' dynamics. We obtain fringes in reciprocal-space as a result of the interference between polariton wavepackets (WPs) traveling with the same speed. The periodicity of these fringes is inversely proportional to the spatial distance between the interfering WPs. In a similar fashion, we obtain interference fringes in real-space when WPs traveling in opposite directions meet. The visibility of both real- and reciprocal-space interference fringes rapidly decreases with increasing temperature and vanishes. A theoretical description of the phase transition, considering the coexistence of condensed and non-condensed particles, for an out of equilibrium condensate such as ours is still missing. Yet a comparison with theories developed for atomic condensates allows us to infer a critical temperature for the BEC-like transition when the visibility goes to zero.

cond-mat.mes-hall

Superfluid currents in half-moon polariton condensates

We excite exciton-polariton condensates in half-moon shapes by the non-resonant optical excitation of GaAs-based cylindrical pillar microcavities. In this geometry, the π-jump of the phase of the condensate wave function coexists with a gradual {\pm π} phase variation between two horns of the half-moon. We switch between clockwise and counter-clockwise phase currents by slightly shifting the excitation spot on the surface of the pillar. Half-moon condensates are expected to reveal features of two-level quantum systems similar to superconducting flux qubits

cond-mat.mes-hall

Synchronization crossover of polariton condensates in weakly disordered lattices

We demonstrate that the synchronization of a lattice of solid-state condensates when inter-site tunnelling is switched on, depends strongly on the weak local disorder. This finding is vital for implementation of condensate arrays as computation devices. The condensates here are nonlinear bosonic fluids of exciton-polaritons trapped in a weakly disordered Bose-Hubbard potential, where the nearest neighboring tunneling rate (Josephson coupling) can be dynamically tuned. The system can thus be tuned from a localized to a delocalized fluid as the number density, or the Josephson coupling between nearest neighbors increases. The localized fluid is observed as a lattice of unsynchronized condensates emitting at different energies set by the disorder potential. In the delocalized phase the condensates synchronize, and long-range order appears, evidenced by narrowing of momentum and energy distributions, new diffraction peaks in momentum space, and spatial coherence between condensates. Our work identifies similarities and differences of this nonequilibrium crossover to the traditional Bose-glass to superfluid transition in atomic condensates.

cond-mat.other

Strain-assisted optomechanical coupling of polariton condensate spin to a micromechanical resonator

We report spin and intensity coupling of an exciton-polariton condensate to the mechanical vibrations of a circular membrane microcavity. We optically drive the microcavity resonator at the lowest mechanical resonance frequency while creating an optically-trapped spin-polarized polariton condensate in different locations on the microcavity, and observe spin and intensity oscillations of the condensate at the vibration frequency of the resonator. Spin oscillations are induced by vibrational strain driving, whilst the modulation of the optical trap due to the displacement of the membrane causes intensity oscillations in the condensate emission. Our results demonstrate spin-phonon coupling in a macroscopically coherent condensate.

cond-mat.mes-hall

Optical bistability under non-resonant excitation in spinor polariton condensates

We realise bistability in the spinor of polariton condensates under non-resonant optical excitation and in the absence of biasing external fields. Numerical modelling of the system using the Ginzburg-Landau equation with an internal Josephson coupling between the two spin components of the condensate qualitatively describes the experimental observations. We demonstrate that polariton spin bistability persists for sweep times in the range of $[10 μsec,1 sec]$ offering a promising route to spin switches and spin memory elements.

cond-mat.mes-hall

Persistent circular currents of exciton-polaritons in cylindrical pillar microcavities

We have experimentally observed an eddy current of exciton polaritons arising in a cylindrical GaAs/AlGaAs pillar microcavity under the nonresonant optical pumping. The polariton current manifests itself in a Mach-Zehnder interferometry image as a characteristic spiral that occurs due to the interference of the light emitted by an exciton-polariton condensate with a spherical wave artificially shaped from the emission of the same condensate. We have experimentally observed the condensates with the topological charges m = +1, m = -1 and m = -2. The interference pattern corresponding to the m = -2 current represents the twin spiral emerging from the center of the micropillar.

cond-mat.mes-hall

Spin order and phase transitions in chains of polariton condensates

We demonstrate that multiply-coupled spinor polariton condensates can be optically tuned through a sequence of spin-ordered phases by changing the coupling strength between nearest neighbors. For closed 4-condensate chains these phases span from ferromagnetic (FM) to antiferromagnetic (AFM), separated by an unexpected crossover phase. This crossover phase is composed of alternating FM-AFM bonds. For larger 8 condensate chains, we show the critical role of spatial inhomogeneities and demonstrate a scheme to overcome them and prepare any desired spin state. Our observations thus demonstrate a fully controllable non-equilibrium spin lattice.

cond-mat.mes-hall

Inverse-phase Rabi oscillations in semiconductor microcavities

We study experimentally the oscillations of a non stationary transient signal of a semiconductor microcavity with embedded InGaAs quantum wells. The oscillations occur as a result of quantum beats between the upper and lower polariton modes due to the strong exciton-photon coupling in the microcavity sample (Rabi oscillations). The registration of spectrally resolved signal has allowed for separate observation of oscillations at the eigenfrequencies of two polariton modes. Surprisingly, the observed oscillations measured at the lower and upper polariton modes have opposite phases. We demonstrate theoretically that the opposite-phase oscillations are caused by the pump-induced modification of polariton Hopfield coefficients, which govern the ratio of exciton and photon components in each of the polartion modes. Such a behaviour is a fundamental feature of the quantum beats of coupled light-matter states. In contrast, the reference pump-probe experiment performed for the pure excitonic states in a quantum well heterostructure with no microcavity revealed the in-phase oscillations of the pump-probe signals measured at different excitonic levels.

cond-mat.mes-hall

Tunable magnetic alignment between trapped exciton-polariton condensates

Tunable spin correlations are found to arise between two neighboring trapped exciton-polariton condensates which spin-polarize spontaneously. We observe a crossover from an antiferromagnetic- to a ferromagnetic pair state by reducing the coupling barrier in real-time using control of the imprinted pattern of pump light. Fast optical switching of both condensates is then achieved by resonantly but weakly triggering only a single condensate. These effects can be explained as the competition between spin bifurcations and spin-preserving Josephson coupling between the two condensates, and open the way to polariton Bose-Hubbard ladders.

cond-mat.other

Robust platform for engineering pure-quantum-state transitions in polariton condensates

We report on pure-quantum-state polariton condensates in optical annular traps. The study of the underlying mechanism reveals that the polariton wavefunction always coalesces in a single pure-quantum-state that, counter-intuitively, is always the uppermost confined state with the highest overlap to the exciton reservoir. The tunability of such states combined with the short polariton lifetime allows for ultrafast transitions between coherent mesoscopic wavefunctions of distinctly different symmetries rendering optically confined polariton condensates a promising platform for applications such as many-body quantum circuitry and continuous-variable quantum processing.

cond-mat.quant-gas

Dynamics of the Energy Relaxation in a Parabolic Quantum Well Laser

We explore two parabolic quantum well (PQW) samples, with and without Bragg mirrors, in order to optimise the building blocks of a Bosonic Cascade Laser. The photoluminescence spectra of a PQW microcavity sample is compared against that of a conventional microcavity with embedded quantum wells (QWs) to demonstrate that the weak coupling lasing in a PQW sample can be achieved. The relaxation dynamics in a conventional QW microcavity and in the PQW microcavity was studied by a non-resonant pump-pump excitation method. Strong difference in the relaxation characteristics between the two samples was found. The semi-classical Boltzmann equations were adapted to reproduce the evolution of excitonic populations within the PQW as a function of the pump power and the output intensity evolution as a function of the pump-pump pulse delay. Fitting the PQW data confirms the anticipated cascade relaxation, paving the way for such a system to produce terahertz radiation.

cond-mat.mes-hall

Spontaneous spin bifurcations and ferromagnetic phase transitions in a spinor exciton-polariton condensate

We observe a spontaneous parity breaking bifurcation to a ferromagnetic state in a spatially trapped exciton-polariton condensate. At a critical bifurcation density under nonresonant excitation, the whole condensate spontaneously magnetizes and randomly adopts one of two elliptically polarized (up to 95% circularly-polarized) states with opposite handedness of polarization. The magnetized condensate remains stable for many seconds at 5 K, but at higher temperatures it can flip from one magnetic orientation to another. We optically address these states and demonstrate the inversion of the magnetic state by resonantly injecting 100-fold weaker pulses of opposite spin. Theoretically, these phenomena can be well described as spontaneous symmetry breaking of the spin degree of freedom induced by different loss rates of the linear polarizations.

cond-mat.mes-hall

Spin Selective Filtering of Polariton Condensate Flow

Spin-selective spatial filtering of propagating polariton condensates, using a controllable spin-dependent gating barrier, in a one-dimensional semiconductor microcavity ridge waveguide is reported. A nonresonant laser beam provides the source of propagating polaritons while a second circularly polarized weak beam imprints a spin dependent potential barrier, which gates the polariton flow and generates polariton spin currents. A complete spin-based control over the blocked and transmitted polaritons is obtained by varying the gate polarization.

cond-mat.mes-hall