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Zakaria Said

Publications and source records attributed to Zakaria Said.

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Cavity quantum electrodynamics with single perovskite quantum dots

Quantum emitters of single indistinguishable photons play a key role in quantum technologies. Among condensed matter systems, colloidal perovskite quantum dots have emerged as promising candidates, exhibiting high-purity single photon emission at room temperature and two-photon interference visibilities up to 0.5 at cryogenic temperatures. Achieving deterministic coupling of individual perovskite quantum dots to photonic structures is now a critical step towards harnessing cavity quantum electrodynamics (cQED) effects, such as the Purcell effect, to enhance single photon emission rate and indistinguishability. Here, we demonstrate the deterministic and reversible coupling of individual CsPbBr$_{3}$ perovskite quantum dots to a tunable, high-quality factor, low mode volume fiber-based Fabry-P\'erot microcavity at 10~\si{\kelvin}. By spatially and spectrally tuning the cavity mode in resonance with the quantum dot emission, we observe up to a twofold increase in single photon emission rates. We build on the original multiplet excitonic fine structure to assess the vacuum Rabi coupling strength ($g \simeq$ 40~\si{\micro eV}) from the shaping of the spectral profile of the emission upon increasing the electromagnetic confinement. This approach also made it possible to delineate the contributions of spectral diffusion and pure dephasing to the total linewidth of emission, paving the way to a fully optimized control of the emission properties of cavity coupled perovskite quantum dots.

quant-ph

Spectral fingerprint of quantum confinement in single CsPbBr$_3$ nanocrystals

Lead halide perovskite nanocrystals are promising materials for classical and quantum light emission. To understand these outstanding properties, a thorough analysis of the band-edge exciton emission is needed which is not reachable in ensemble and room temperature studies because of broadening effects. Here, we report on a cryogenic-temperature study of the photoluminescence of single CsPbBr$_3$ NCs in the intermediate quantum confinement regime. We reveal the size-dependence of the spectral features observed: the bright-triplet exciton energy splittings, the trion and biexciton binding energies as well as the optical phonon replica spectrum. In addition, we show that bright triplet energy splittings are consistent with a pure exchange model and that the variety of polarisation properties and spectra recorded can be rationalised simply by considering the orientation of the emitting dipoles and the populations of the emitting states.

cond-mat.mes-hall