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Zakhar A. Iakovlev

Publications and source records attributed to Zakhar A. Iakovlev.

5 recordsLinked to original sources

Magnetic-field control of Fermi polaron fine structure and polarization in strained monolayer semiconductors

The theory of attractive Fermi polaron energy spectrum fine structure and polarization in doped two-dimensional semiconductors in external magnetic field is developed. Fermi polaron $g$ factor renormalization due to correlations with the valley-polarized Fermi sea of resident charge carriers is calculated. We study the competition between Zeeman and strain-induced splittings in monolayers under uniaxial strain. The control of strain, magnetic field and electron density allows continuous tuning of energy splitting and eigenstate polarization. Linearly polarized strain-induced split doublet exhibits quadratic Zeeman shift changing to linear Zeeman splitting with elliptical polarization with the increase of magnetic field. We identify a critical magnetic field above which resident charge carriers become fully valley polarized and only one circularly polarized Fermi polaron state remains. Within the Green's function approach we calculate energy levels and Stokes parameters of attractive Fermi polaron states and introduce a simplified effective two-level model allowing us to study analytically the interplay of Zeeman and pseudo-Zeeman splitting. We calculate absorption and reflection spectra, including circular and linear dichroism in the trion spectral range. These results show that real and strain-induced pseudomagnetic fields provide complementary tools for controlling the optical response of many-body excitonic quasiparticles in two-dimensional semiconductors.

cond-mat.mes-hall↗

Boltzmann transport theory of magnon-exciton drag

We develop a microscopic theory of magnon-exciton drag effect in a bilayer van der Waals antiferromagnetic semiconductor CrSBr. Effective exciton-magnon coupling arises from an orbital mechanism: Magnons tilt the layer magnetizations, enabling charge carrier tunneling that mixes intra- and interlayer excitons and thereby modulate the exciton energy. We derive the effective Hamiltonian of exciton-magnon coupling, based on our calculation of the magnon spectrum taking into account short-range exchange interaction between Cr-ion spins, single-ion anisotropy, and long-range dipole-dipole interactions. The latter produces a negative group velocity of magnons at small wavevectors. We show that despite rather small renormalization of exciton's energy and effective mass by the exciton-magnon interaction, the three key two-magnon processes: exciton-magnon scattering, two-magnon absorption by exciton, and two-magnon emission are highly efficient. By solving the Boltzmann kinetic equation, we evaluate short exciton-magnon scattering time which is in the sub-ps range and strongly decreases with the increase of magnon population. Hence, exciton-magnon scattering is likely to be dominant over other scattering processes related to the exciton-phonon and exciton-disorder interactions. We demonstrate that magnons can efficiently drag excitons, resulting in a large and nearly isotropic exciton propagation that can significantly exceed the intrinsic anisotropic diffusion. Our results provide a theoretical basis for recent observations of anomalous exciton transport in CrSBr [F. Dirnberger, et al., Nat. Nano. (2025)] and establish magnon-exciton drag as a powerful mechanism for controlling exciton propagation in magnetic systems.

cond-mat.mes-hall↗

Exciton transport driven by spin excitations in an antiferromagnet

A new class of optical quasiparticles called magnetic excitons recently emerged in magnetic van der Waals materials. Akin to the highly effective strategies developed for electrons, the strong interactions of these excitons with the spin degree of freedom may provide innovative solutions for long-standing challenges in optics, such as steering the flow of energy and information. Here, we demonstrate transport of excitons by spin excitations in the van der Waals antiferromagnetic semiconductor CrSBr. Key results of our study are the observations of ultrafast, nearly isotropic exciton propagation substantially enhanced at the Neel temperature, transient contraction and expansion of the exciton clouds at low temperatures, as well as superdiffusive behavior in bilayer samples. These signatures largely defy description by commonly known exciton transport mechanisms and are related to the currents of incoherent magnons induced by laser excitation instead. We propose that the drag forces exerted by these currents can effectively imprint characteristic properties of spin excitations onto the motion of excitons. The universal nature of the underlying exciton-magnon scattering promises driving of excitons by magnons in other magnetic semiconductors and even in non-magnetic materials by proximity in heterostructures, merging the rich physics of magneto-transport with optics and photonics.

cond-mat.mes-hall↗

Control of atomic reconstruction and quasi-1D excitons in strain-engineered moiré heterostructures

In two-dimensional nearly commensurate heterostructures, strain plays a critical role in shaping electronic behavior. While previous studies have focused on random strain introduced during fabrication, achieving controlled structural design has remained challenging. Here, we demonstrate the deterministic creation of one-dimensional arrays from initially zero-dimensional triangular moiré patterns in MoSe$_2$-WSe$_2$ heterobilayers. This transformation, driven by the interplay of uniaxial strain and atomic reconstruction, results in one-dimensional confinement of interlayer excitons within domain walls, exhibiting near-unity linearly polarized emission related to the confinement-induced symmetry breaking. The width of the domain walls--and consequently the degree of exciton confinement--can be precisely tuned by the interlayer twist angle. By applying out-of-plane electric field, the confined excitons exhibit energy shifts exceeding 100~meV and changes in the fine-structure splitting by up to a factor of two. Our work demonstrates the potential of strain engineering for constructing designer moiré systems with programmable quantum properties, paving the way for future optoelectronic applications.

cond-mat.mes-hall↗

Excitons under large pseudomagnetic fields

Excitons in Transition Metal Dichalcogenides (TMDs) acquire a spin-like quantum number, a pseudospin, originating from the crystal's discrete rotational symmetry. Here, we break this symmetry using a tunable uniaxial strain, effectively generating a pseudomagnetic field exceeding 40 Tesla. Under this large field, we demonstrate pseudospin analogs of spintronic phenomena such as the Zeeman effect and Larmor precession. Moreover, we determine previously inaccessible fundamental properties of TMDs, including the strength of the depolarizing field responsible for the loss of exciton coherence. Finally, we uncover the bosonic -- as opposed to fermionic -- nature of many-body excitonic species using the pseudomagnetic equivalent of the $g$-factor spectroscopy. Our work is the first step toward establishing this spectroscopy as a universal method for probing correlated many-body states and realizing pseudospin analogs of spintronic devices.

cond-mat.mes-hall↗