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Zeeshawn Kazi

Publications and source records attributed to Zeeshawn Kazi.

7 recordsLinked to original sources

Momentum-resolved magnetic noise spectroscopy using ensembles of diamond quantum sensors

Spatiotemporal fluctuations across multiple scales govern and characterize the emergent properties, phase boundaries, and low-energy excitations of strongly correlated matter. However, capturing these dynamics has remained a major experimental challenge, as conventional probes typically offer either high spatial or temporal resolution, but not both simultaneously. Here, we leverage high-fidelity wide-field imaging of dense diamond nitrogen vacancy center ensembles to measure the momentum and frequency power spectral density of magnetic fluctuations. To access spatial wavevectors below the diffraction limit, we tune the sensing volume continuously through optical depletion. This approach enables study of equilibrium and driven fluctuations across three orders of magnitude in spatial scale and tunable frequency bands, providing a direct means to map low-energy, long-wavelength fluctuations in correlated systems.

quant-ph↗

Magnetic Microscopy of Skyrmions in Magnetic Thin Films with Chiral Overlayers

Topologically nontrivial magnetic textures such as skyrmions offer promising opportunities for spintronic applications. In recent years, it has been shown that the magnetic properties of layered materials can be affected by depositing chiral molecules on the surface, while the influence of chiral overlayers on skyrmion properties such as their stability and interactions remains largely unexplored. To address this challenge, we employ wide-field nitrogen-vacancy (NV) magnetometry to directly image skyrmions in chiral-molecule-functionalized magnetic thin films, enabling quantitative mapping of magnetic stray fields over extended areas under ambient conditions. Using pixel-resolved optically detected magnetic resonance (ODMR) combined with controlled magnetic fields, we reproducibly nucleate and probe skyrmion states in CoFeB ferromagnetic samples, enabling quantitative investigation of their properties. We find evidence for enantioselective and magnetic-field-polarity-dependent modifications of skyrmion diameter, spacing, and shape, pointing to a possibility of molecular control of topological spin textures via magneto-chiral coupling.

cond-mat.mtrl-sci↗

Massively multiplexed nanoscale magnetometry with diamond quantum sensors

Single nitrogen vacancy (NV) centers in diamond have been used extensively for high-sensitivity nanoscale sensing, but conventional approaches use confocal microscopy to measure individual centers sequentially, limiting throughput and access to non-local physical properties. Here we design and implement a multiplexed NV sensing platform that allows us to read out many single NV centers simultaneously using a low-noise camera. Using this platform, we coherently manipulate and read out the spin states of hundreds of individual NV centers in parallel, achieving comparable magnetic field sensitivity to confocal measurements. We also implement a parallelized version of spin-to-charge-conversion readout for low NV center spin state readout noise and use it to demonstrate multiplexed covariance magnetometry, in which we measure six two-point magnetic field correlators from four NV centers simultaneously. The number of correlators we can measure is limited only by the available laser power, opening the door to massively multiplexed covariance magnetometry. Our platform significantly increases the throughput and broadens the applications of nanoscale sensing using diamond quantum sensors.

quant-ph↗

Direct measure of DNA bending by quantum magnetic imaging of a nano-mechanical torque-balance

DNA flexibility is a key determinant of biological function, from nucleosome positioning to transcriptional regulation, motivating a direct measurement of the bend-torque response of individual DNA molecules. In this work, DNA bending is detected using a nano-mechanical torque balance formed by tethering a ferromagnetic nanoparticle probe by an individual DNA molecule to a diamond magnetic field imager. The torque exerted by the DNA in response to bending caused by an applied magnetic torque is measured using wide-field imaging of quantum defects near the surface of the diamond. Qualitative measurements of differences in DNA bio-mechanical binding configuration are demonstrated, and as a proof-of-principle, a quantitative measurement of the bend response is made for individual DNA molecules. This quantum-enabled measurement approach could be applied to characterize the bend response of biophysically relevant short DNA molecules as well as the sequence dependence of DNA bending energy.

physics.bio-ph↗

Impact of surface and laser-induced noise on the spectral stability of implanted nitrogen-vacancy centers in diamond

Scalable realizations of quantum network technologies utilizing the nitrogen vacancy center in diamond require creation of optically coherent NV centers in close proximity to a surface for coupling to optical structures. We create single NV centers by $^{15}$N ion implantation and high-temperature vacuum annealing. Origin of the NV centers is established by optically detected magnetic resonance spectroscopy for nitrogen isotope identification. Near lifetime-limited optical linewidths ($<$ 60 MHz) are observed for the majority of the normal-implant (7$^\circ$, $\approx$ 100 nm deep) $^{15}$NV centers. Long-term stability of the NV$^-$ charge state and emission frequency is demonstrated. The effect of NV-surface interaction is investigated by varying the implantation angle for a fixed ion-energy, and thus lattice damage profile. In contrast to the normal implant condition, NVs from an oblique-implant (85$^\circ$, $\approx$ 20 nm deep) exhibit substantially reduced optical coherence. Our results imply that the surface is a larger source of perturbation than implantation damage for shallow implanted NVs. This work supports the viability of ion implantation for formation of optically stable NV centers. However, careful surface preparation will be necessary for scalable defect engineering.

cond-mat.mes-hall↗

Wide-field dynamic magnetic microscopy using double-double quantum driving of a diamond defect ensemble

Wide-field magnetometry can be realized by imaging the optically-detected magnetic resonance of diamond nitrogen vacancy (NV) center ensembles. However, NV ensemble inhomogeneities significantly limit the magnetic-field sensitivity of these measurements. We demonstrate a double-double quantum (DDQ) driving technique to facilitate wide-field magnetic imaging of dynamic magnetic fields at a micron scale. DDQ imaging employs four-tone radio frequency pulses to suppress inhomogeneity-induced variations of the NV resonant response. As a proof-of-principle, we use the DDQ technique to image the dc magnetic field produced by individual magnetic-nanoparticles tethered by single DNA molecules to a diamond sensor surface. This demonstrates the efficacy of the diamond NV ensemble system in high-frame-rate magnetic microscopy, as well as single-molecule biophysics applications.

physics.app-ph↗

Probing topological spin structures using light-polarization and magnetic microscopy

We present an imaging modality that enables detection of magnetic moments and their resulting stray magnetic fields. We use wide-field magnetic imaging that employs a diamond-based magnetometer and has combined magneto-optic detection (e.g. magneto-optic Kerr effect) capabilities. We employ such an instrument to image magnetic (stripe) domains in multilayered ferromagnetic structures.

cond-mat.mtrl-sci↗