Searcharxiv⌕ Search

arXiv subjects

Zenghu Chang

Publications and source records attributed to Zenghu Chang.

12 recordsLinked to original sources
arXiv2026

Toroidal pulse enhanced XUV generation

Extreme ultraviolet (XUV) radiation plays a central role in a wide range of applications. Despite being a cornerstone of attosecond science, efficient XUV generation remains highly challenging. Here, we investigate XUV generation via nonlinear Thomson scattering driven by a toroidal pulse. Unlike conventional laser pulses, toroidal pulses possess intrinsically non-separable spatiotemporal field distributions. This unique field structure produces strongly asymmetric electron acceleration, resulting in substantially enhanced XUV emission that is 2-4 orders of magnitude stronger than that generated by a Gaussian pulse. Our results identify toroidal pulses as a promising route toward compact ultrafast XUV sources and advanced strong-field light-matter interaction studies.

physics.optics↗
arXiv2026

Roadmap on Attosecond Science

Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time. What began as a technological breakthrough - generating the shortest flashes ever produced - has evolved into a powerful approach for probing and steering electronic dynamics in atoms, molecules, and solids. This roadmap, authored by leading experts in the field, surveys the recent rapid progress in the generation and characterization of attosecond pulses, emerging attosecond measurement and control techniques, and their expanding range of applications. It reviews current and future developments in attosecond light sources, including novel laser technologies, waveform synthesizers, new schemes for high-order harmonic generation, attosecond pulse generation at free-electron lasers, and structured light. Advances in attosecond measurement methodologies are also discussed, encompassing all-attosecond pump-probe spectroscopy, attosecond four-wave mixing, attosecond microscopy, spectroscopy with light transients, and attosecond interferometry. Furthermore, the roadmap addresses applications of attosecond spectroscopy to reveal electron dynamics in molecules and condensed matter systems from both theoretical and experimental perspectives, and highlights emerging directions at the interface with quantum optics and quantum entanglement. Overall, this work aims to serve as a comprehensive resource for navigating the evolving landscape of attosecond science.

physics.optics↗
arXiv2024

Phase-Matched Generation of Coherent Soft-X-Rays

Phase-matched harmonic conversion of visible laser light into soft x-rays was demonstrated. The recently developed technique of guided-wave frequency conversion was used to upshift light from 800 nanometers to the range from 17 to 32 nanometers. This process increased the coherent x-ray output by factors of 10^2 to 10^3 compared to the non-phase-matched case. This source uses a small-scale (sub-millijoule) high repetition-rate laser and will enable a wide variety of new experimental investigations in linear and nonlinear x-ray science.

physics.optics↗
arXiv2022

High average power ultrafast laser technologies for driving future advanced accelerators

Large scale laser facilities are needed to advance the energy frontier in high energy physics and accelerator physics. Laser plasma accelerators are core to advanced accelerator concepts aimed at reaching TeV electron electron colliders. In these facilities, intense laser pulses drive plasmas and are used to accelerate electrons to high energies in remarkably short distances. A laser plasma accelerator could in principle reach high energies with an accelerating length that is 1000 times shorter than in conventional RF based accelerators. Notionally, laser driven particle beam energies could scale beyond state of the art conventional accelerators. LPAs have produced multi GeV electron beams in about 20 cm with relative energy spread of about 2 percent, supported by highly developed laser technology. This validates key elements of the US DOE strategy for such accelerators to enable future colliders but extending best results to date to a TeV collider will require lasers with higher average power. While the per pulse energies envisioned for laser driven colliders are achievable with current lasers, low laser repetition rates limit potential collider luminosity. Applications will require rates of kHz to tens of kHz at Joules of energy and high efficiency, and a collider would require about 100 such stages, a leap from current Hz class LPAs. This represents a challenging 1000 fold increase in laser repetition rates beyond current state of the art. This whitepaper describes current research and outlook for candidate laser systems as well as the accompanying broadband and high damage threshold optics needed for driving future advanced accelerators.

physics.acc-ph↗
arXiv2020

Ho:YLF amplifier with Ti:Sapphire frontend for pumping mid-infrared optical parametric amplifier

We present a Ho:YLF Chirped-Pulse Amplification (CPA) laser for pumping a longwave infrared Optical Parametric Chirped Pulse Amplifier (OPCPA) at a 1 kHz repetition rate. By utilizing a Ti:Sapphire laser as a frontend, 5-μJ seed pulses at 2051 nm laser pulse are generated in a Dual-Chirp Optical Parametric Amplifier (DC-OPA), which are amplified to 28 mJ pulses with a pulse duration of 6.8 ps. The scheme offers a potential driver for two-color (800 nm and 8 μm) high harmonic generation with an increased keV X-ray photon flux.

physics.optics↗
arXiv2019

Generation of 3 mJ, 44 fs, 2.5 micrometer pulses from a single-stage Cr2+:ZnSe amplifier

Lasers capable of generating attosecond X-ray pulses in the water window (282 to 533 eV) through high-order harmonic generation are normally based on inefficient, multi-stage optical parametric amplifiers or optical parametric chirped pulse amplifiers pumped by femtosecond or picosecond lasers. Here we report a very efficient single amplification stage laser based on traditional chirped pulse amplification capable of producing 3 mJ, near-transform limited 44 fs (<6 cycles), 1 kHz pulses centered at 2.5 micrometer. The 68 GW peak power is the highest value ever reached at this wavelength. In order to fully compress the laser pulses our system is built in a nitrogen box. Our system utilizes water cooled chromium doped zinc selenide (Cr2+:ZnSe) as the gain medium and is pumped by a commercial nanosecond holmium doped yttrium-aluminum-garnet (Ho:YAG) laser.

physics.optics↗
arXiv2019

Real-time observation of electronic, vibrational, and rotational dynamics in nitric oxide with attosecond soft X-ray pulses at 400 eV

Photoinduced quantum dynamics in molecules have hierarchical temporal structures with different energy scales that are associated with electron and nuclear motions. Femtosecond-to-attosecond transient absorption spectroscopy (TAS) using high-harmonic generation (HHG) with a photon energy below 300 eV has been a powerful tool to observe such electron and nuclear dynamics in a table-top manner. However, comprehensive measurements of the electronic, vibrational, and rotational molecular dynamics have not yet been achieved. Here, we demonstrate HHG-based TAS at the nitrogen K-edge (400 eV) for the first time, and observe all the electronic, vibrational, and rotational degrees of freedom in a nitric oxide molecule at attosecond to sub-picosecond time scales. This method of employing core-to-valence transitions offers an all-optical approach to reveal complete molecular dynamics in photochemical reactions with element and electronic state specificity.

physics.atom-ph↗
arXiv2019

Signal retrieval with measurement system knowledge using variational generative model

Signal retrieval from a series of indirect measurements is a common task in many imaging, metrology and characterization platforms in science and engineering. Because most of the indirect measurement processes are well-described by physical models, signal retrieval can be solved with an iterative optimization that enforces measurement consistency and prior knowledge on the signal. These iterative processes are time-consuming and only accommodate a linear measurement process and convex signal constraints. Recently, neural networks have been widely adopted to supersede iterative signal retrieval methods by approximating the inverse mapping of the measurement model. However, networks with deterministic processes have failed to distinguish signal ambiguities in an ill-posed measurement system, and retrieved signals often lack consistency with the measurement. In this work we introduce a variational generative model to capture the distribution of all possible signals, given a particular measurement. By exploiting the known measurement model in the variational generative framework, our signal retrieval process resolves the ambiguity in the forward process, and learns to retrieve signals that satisfy the measurement with high fidelity in a variety of linear and nonlinear ill-posed systems, including ultrafast pulse retrieval, coded aperture compressive video sensing and image retrieval from Fresnel hologram.

eess.IV↗
arXiv2019

Enhancing keV high harmonic signals generated by long-wave infrared lasers

It is demonstrated by single-atom simulations that X-ray signals in the 3.4 to 4 keV region from an 8 micron laser driven high harmonic generation can be increased by more than two orders of magnitude when a single-cycle pulse centered at 800 nm is added. The ionization probability of a helium atom by the two-pulse field is set to 4.56x10^-5, which is needed for balancing the index of refraction of free electrons with that of neutral helium atoms to achieve phase matching.

physics.atom-ph↗
arXiv2017

High-harmonic generation in amorphous solids

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to important applications such as all-optical methods to image valance charge density and reconstruction of electronic band structures, as well as compact XUV light sources. Previous HHG studies are confined on crystalline solids; therefore decoupling the respective roles of long-range periodicity and high density has been challenging. Here, we report the first observation of HHG from amorphous fused silica. We decouple the role of long-range periodicity by comparing with crystal quartz, which contains same atomic constituents but exhibits long-range periodicity. Our results advance current understanding of strong-field processes leading to high harmonic generation in solids with implications in robust and compact coherent XUV light sources.

physics.optics↗
arXiv2013

Broadband Isolated Attosecond Pulses: Generation, Characterization, and Applications

The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as light pulses in 2012, and broadband attosecond continua covering a wide range of extreme ultraviolet and soft x-ray wavelengths. Such pulses have been successfully applied in photoelectron/photoion spectroscopy and the recently developed attosecond transient absorption spectroscopy to study electron dynamics in matter. In this Review, we discuss the significant recent advancement in the generation, characterization, and application of ultrabroadband isolated attosecond pulses with spectral bandwidth comparable to the central frequency, which can in principle be compressed to a single optical cycle.

physics.optics↗