arXiv subjects

Zhangfeng Gao

Publications and source records attributed to Zhangfeng Gao.

10 recordsLinked to original sources

arXiv2026

Self-Synchronized Terahertz and X-Ray Free-Electron Lasers from a Single Pre-Bunched Electron Beam

Ultrafast pump-probe spectroscopy combining intense terahertz (THz) and X-ray pulses is a critical tool for investigating complex structural and electronic dynamics in materials. However, current setups combining THz sources and X-ray free-electron lasers (FELs) often suffer from high system complexity, inherent timing jitter, or limited THz pulse properties. Here, we experimentally demonstrate the generation of intrinsically synchronized, strong-field, narrow-band THz and X-ray FELs from a single pre-bunched electron beam. Sequentially passing the beam through X-ray and THz amplifiers reveals a highly synergistic process: the initial periodic THz density modulation notably boosts the X-ray FEL pulse energy, while robustly surviving the intense X-ray emission to drive high-power, narrow-band THz radiation. Originating from the same electron bunch, the two pulses inherently maintain a precise, constant time delay. This jitter-free scheme establishes a highly reliable platform tailored for both X-ray-pump/THz-probe and THz-pump/X-ray-probe experiments.

physics.acc-ph↗

arXiv2026

Theoretical and experimental studies of energy modulation to demodulation in seeded free-electron lasers

Laser manipulation plays a critical role in precisely tailoring relativistic electron beams through energy modulation, enabling the generation of coherent, intense, and ultrashort radiation in accelerator-based light sources such as synchrotron radiation facilities and free-electron lasers (FELs). However, laser-induced energy modulation inevitably degrades electron beam quality by increasing the energy spread, thereby limiting high-repetition-rate operation. Here, we investigate energy modulation and demodulation in a seeded FEL using two modulators separated by a tunable phase shifter. Analytical analysis and three-dimensional simulations show that a $π$ phase delay can nearly reverse the laser-beam interaction and substantially suppress the residual modulation. Diagnostics based on coherent undulator radiation and time-resolved measurements are established to characterize weak residual modulation, and a dedicated demodulation undulator is designed for controlled studies. Preliminary experiments performed at the Shanghai soft X-ray FEL facility using the existing seeding beamline demonstrate laser-induced energy-modulation suppression. Together with the analytical and numerical studies, these results establish a practical framework for investigating the transition from energy modulation to demodulation in seeded FELs, with potential applications in high-repetition-rate, fully coherent X-ray sources with improved preservation of electron beam quality.

physics.acc-ph↗

arXiv2026

Fully coherent short wavelength free-electron laser driven by a single sub-microjoule seed

High-repetition-rate, fully coherent extreme-ultraviolet (EUV) and X-ray free-electron lasers (FELs) are essential for advanced time-resolved ultrafast spectroscopies. While external seeding serves as the standard technique to achieve precise temporal coherence, conventional methods demand hundred-megawatt peak-power laser systems. Furthermore, advanced configurations like echo-enabled harmonic generation (EEHG) introduce the severe complexities of dual-laser synchronization. Together, these requirements fundamentally restrict operations to kilohertz repetition rates and compromise overall system stability. Here, we experimentally demonstrate a fully coherent EEHG-FEL driven by a single, sub-microjoule seed laser. By employing a direct-amplification enabled harmonic generation technique, we utilize an initial 0.4 microJ (2 MW peak power) ultraviolet seed to directly drive coherent lasing at nanometer wavelengths. By eliminating the need for extreme peak powers and multiple synchronized lasers, this approach significantly simplifies the seeding architecture and provides a practical and robust pathway toward megahertz-class, fully coherent EUV and X-ray light sources.

physics.acc-ph↗

arXiv2026

High-power beyond extreme ultraviolet FEL radiation with flexible polarization at SHINE

Linac-based free-electron lasers (FELs) feature high brightness, narrow bandwidth, controllable polarization, and wide wavelength tunability. With the rapid development of superconducting radio-frequency technology, linacs can now operate at MHz-level repetition rates, enabling FELs with both high repetition rates and high average power. Beyond extreme ultraviolet (BEUV) radiation is of great interest for scientific research and industrial applications, especially for next-generation lithography. Owing to the main design parameters of SHINE, the generation of BEUV radiation is a natural capability of the facility. The BEUV characteristics at SHINE are investigated and its achievable performance as a high-average-power light source is evaluated. By applying undulator tapering to enhance the energy extraction efficiency, kilowatt-level BEUV radiation with controllable polarization is shown to be achievable. These results demonstrate that SHINE can provide a high-performance BEUV source, offering a realistic pathway toward a high-average-power light source for next-generation high-resolution lithography.

physics.acc-ph↗

arXiv2026

Demonstration of High-Gain Harmonic Lasing in a Terahertz Free-Electron Laser

Compact Free-Electron Lasers (FELs) offering broad, continuous spectral tunability are traditionally constrained by fixed-parameter magnetic structures and the necessity for high-energy electron beams. High-gain Harmonic Lasing (HL) has long been proposed as a solution to overcome these limitations; however, a robust experimental verification of this principle has remained absent. Here, we report the first experimental demonstration of high-gain HL. By employing a frequency-tunable electron beam density modulation to dominate the fundamental instability, we achieved sustained FEL amplification at the 3rd and 5th harmonics of the wiggler. The HL mode generated output power comparable to conventional fundamental operation with enhanced stability and narrower spectral bandwidth. Notably, we demonstrate that HL extends the spectral coverage by a factor of two under fixed facility constraints, achieving pulse energies up to 540 μJ. These results establish high-gain HL as a versatile mechanism for advancing compact, wavelength-flexible FEL facilities.

physics.acc-ph↗

arXiv2025

NeutrSHINE: a high repetition rate ultrafast neutron source driven by SHINE electron beam

Neutrons serve as unique probes for exploring the microscopic structure of matter, with the performance of a neutron source fundamentally governing the depth of scientific exploration and the breadth of industrial applicability. To address application demands including nuclear data measurement in the ultra-high-energy region, fundamental particle physics research, highly efficient non-destructive neutron testing, and extreme environment simulation, an ultrafast neutron source driven by the 8 GeV electron beam from the Shanghai high-repetition-rate extreme light facility (SHINE) was conceptually proposed, named NeutrSHINE. Using multidisciplinary simulation tools, key neutronic parameters, thermal behavior of high-power neutron targets, and the factors affecting the time resolution of the source were analyzed. The results affirm the technical feasibility and promising application prospects of the NeutrSHINE concept.

physics.acc-ph↗

arXiv2025

First Lasing and Stable Operation of a Direct-Amplification Enabled Harmonic Generation Free-Electron laser

Seeded free-electron lasers (FELs) capable of operating at repetition rates up to the MHz level are in high demand for advanced time-resolved spectroscopies, which require both full longitudinal coherence and high average photon flux in the extreme ultraviolet (EUV) and x-ray regimes. However, conventional external-seed laser systems cannot sustain MHz operation with sufficient hundreds of megawatts peak power requirement due to their limited total power. Here, we report the first lasing and stable operation of a direct-amplification-enabled harmonic generation FEL driven by a weak seed laser with MW-level peak power. Beginning with an ultraviolet seed laser with only 0.75 μJ pulse energy, we demonstrate its direct amplification to over 10 μJ within an 8-meter-long modulator. We observe coherent harmonic generation up to the 12th harmonic of the seed and achieve saturation of the 7th harmonic in the radiator. These results represent a crucial milestone toward the realization of MHz-class, fully coherent EUV and x-ray light sources.

physics.acc-ph↗

arXiv2025

Enabling Continuous THz Band Coverage via Precise Electron Beam Tailoring in Free-electron Lasers

High-power, continuously tunable narrowband terahertz (THz) sources are essential for advancing nonlinear optics, THz-driven material dynamics, and ultrafast spectroscopy. Conventional techniques typically impose a trade-off between pulse energy and frequency tunability. Here, we introduce a novel free-electron laser approach that overcomes these limitations by pre-modulating a relativistic electron beam with a frequency-beating laser pulse and leveraging bunch compression along with collective effects to enhance microbunching. Experimental results demonstrate that this technique generates narrowband THz emission with continuous frequency tunability from 7.8 to 30.8THz, achieving pulse energies up to 385μJ while maintaining spectral bandwidths between 7.7% and 14.7%. Moreover, the method exhibits exceptional robustness and scalability, highlighting its unique ability to bridge the long-standing THz gap and offering a promising solution for diverse cutting-edge scientific applications.

physics.acc-ph↗

arXiv2023

Opportunities for Gas-Phase Science at Short-Wavelength Free-Electron Lasers with Undulator-Based Polarization Control

Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of accessible photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines.

physics.atom-ph↗

arXiv2021

Self-Amplification of Coherent Energy Modulation in Seeded Free-Electron Lasers

The spectroscopic techniques for time-resolved fine analysis of matter require coherent X-ray radiation with femtosecond duration and high average brightness. Seeded free-electron lasers (FELs), which use the frequency up-conversion of an external seed laser to improve temporal coherence, are ideal for providing fully coherent soft X-ray pulses. However, it is difficult to operate seeded FELs at a high repetition rate due to the limitations of present state-of-the-art laser systems. Here, we report the novel self-modulation method for enhancing laser-induced energy modulation, thereby significantly reducing the requirement of an external laser system. Driven by this scheme, we experimentally realize high harmonic generation in a seeded FEL using an unprecedentedly small energy modulation. An electron beam with a laser-induced energy modulation as small as 1.8 times the slice energy spread is used for lasing at the 7th harmonic of a 266-nm seed laser in a single-stage high-gain harmonic generation (HGHG) setup and the 30th harmonic of the seed laser in a two-stage HGHG setup. The results mark a major step towards a high-repetition-rate, fully coherent X-ray FEL.

physics.acc-ph↗