arXiv subjects

Zhangzhang Cui

Publications and source records attributed to Zhangzhang Cui.

3 recordsLinked to original sources

arXiv2026

Magnetic anisotropic pinning and symmetric breaking induced by interfacial coupling in topological-like ruthenate superlattices

Interfacial engineering enables various emergent effects such as spin reorientations and transport anisotropy. Noncollinear spin textures are essential for realizing many emergent quantum transport phenomena. However, driving such spin structures requires precise control of the interfacial magnetic coupling in complex oxide heterostructures. Here, by utilizing competing exchange interactions at the interface between ferromagnetic metal SrRuO3 and ferromagnetic insulator LaCoO3, we discovered a noncollinear spin configuration in SrRuO3 sublayers. Magnetic stripes were induced by out-of-plane rather than in-plane magnetic fields, indicating strong anisotropy pinning in our superlattices. The observed magneto-transport anisotropy is well explained by our proposed spin configurations, accounting for contributions from both bulk and interface of the SrRuO3 layers. More interestingly, magnetic skymionic textures were absent even at high magnetic fields. The interfacial exchange interaction overwhelms the Dzyaloshinskii-Moriya interaction (DMI) that stabilizes skyrmions, featuring a higher exchange coupling energy than that for the topological spin textures. Our work highlights the potential of interfacial engineering in tuning the spintronic properties by designing proper interfacial interactions.

cond-mat.str-el↗

arXiv2020

Correlation-driven eightfold magnetic anisotropy in a two-dimensional oxide monolayer

Engineering magnetic anisotropy in two-dimensional systems has enormous scientific and technological implications. The uniaxial anisotropy universally exhibited by two-dimensional magnets has only two stable spin directions, demanding 180 degrees spin switching between states. We demonstrate a novel eightfold anisotropy in magnetic SrRuO3 monolayers by inducing a spin reorientation in (SrRuO3)1/(SrTiO3)N superlattices, in which the magnetic easy axis of Ru spins is transformed from uniaxial <001> direction (N = 1 and 2) to eightfold <111> directions (N = 3, 4 and 5). This eightfold anisotropy enables 71 and 109 degrees spin switching in SrRuO3 monolayers, analogous to 71 and 109 degrees polarization switching in ferroelectric BiFeO3. First-principle calculations reveal that increasing the SrTiO3 layer thickness induces an emergent correlation-driven orbital ordering, tuning spin-orbit interactions and reorienting the SrRuO3 monolayer easy axis. Our work demonstrates that correlation effects can be exploited to substantially change spin-orbit interactions, stabilizing unprecedented properties in two-dimensional magnets and opening rich opportunities for low-power, multi-state device applications.

cond-mat.mtrl-sci↗

arXiv2019

Direct Imaging Revealing Halved Ferromagnetism in Tensile-Strained LaCoO3 Thin Films

The enigma of the emergent ferromagnetic state in tensile-strained LaCoO3 thin films remains to be explored because of the lack of a well agreed explanation. The direct magnetic imaging technique using a low-temperature magnetic force microscope (MFM) is critical to reveal new aspects of the ferromagnetism by investigating the lateral magnetic phase distribution. Here we show the experimental demonstration of the rare halved occupation of the ferromagnetic state in tensile-strained LaCoO3 thin films on SrTiO3 substrates using the MFM. The films have uniformly strained lattice structure and minimal oxygen vacancies (less than 2%) beyond the measurement limit. It is found that percolated ferromagnetic regions with typical sizes between 100 nm and 200 nm occupy about 50% of the entire film, even down to the lowest achievable temperature of 4.5 K and up to the largest magnetic field of 13.4 T. Preformed ferromagnetic droplets were still observed when the temperature is 20 K above the Curie temperature indicating the existence of possible Griffiths phase. Our study demonstrated a sub-micron level phase separation in high quality LaCoO3 thin films, which has substantial implications in revealing the intrinsic nature of the emergent ferromagnetism.

cond-mat.str-el↗