arXiv subjects

Zhao-Qi-Zhi Han

Publications and source records attributed to Zhao-Qi-Zhi Han.

13 recordsLinked to original sources

arXiv2026

Mid-infrared high-sensitive cavity-free in-situ CO gas sensing based on up-conversion detection

Carbon monoxide (CO) is a significant indicator gas with considerable application value in atmospheric monitoring, industrial production and medical diagnosis. Its fundamental vibrational band locates around 4.6 $\upmu$m and has larger absorption line strength than that of overtone band, which is more suitable for the precise identification and concentration detection of CO. In this paper, the up-conversion detection is employed to convert the mid-infrared absorption signal obtained by TDLAS to the visible light band, then a silicon-based detector is utilized for detection. By which, we can achieve the highest sensitivity of 79.6 ppb under the condition of cavity-free in-situ with an absorption range length of only 0.14 m. Furthermore, the single-photon level real-time detection of CO concentration after the diffuse reflection is realized by using SPAD. This work demonstrates the merits of the up-conversion detection in terms of its functionality at room temperature and capacity for sensitivity detection. Furthermore, it presents a design and optimization methodology that has the potential to underpin the advancement of the method towards more practical applications, like industrial process monitoring, medical diagnosis and so on.

physics.optics↗

arXiv2026

Broadband Tunable Photon-Pair Generation and Spectrum Measurement Based on Noncritical Lithium Niobate Crystals

Photon pairs play a vital role in modern science, driving extensive research into their generation. Yet, the narrow phase-matching bandwidth of conventional crystals has largely confined studies to specific wavelengths, leaving research on broadband tunable sources underexplored. Here, we employ a non-critical phase-matched lithium niobate (LN) crystal to generate widely tunable photon pairs. The generated near-infrared (NIR) photon pairs exhibit a high coincidence-to-accidental ratio (CAR > 20 dB) and are tunable across the 800-1600 nm range. We further showcase the utility of NIR photon pairs in spectroscopy by detecting carbon monoxide (CO) gas absorption. This approach will facilitate the design of advanced LN-based photonic experiments.

physics.optics↗

arXiv2026

Passive Incoherent Ultrafast Mid-Infrared Upconversion Imaging and Its Calibration

Ultrafast mid-infrared (MIR) imaging is a key enabling capability for monitoring transient thermal and plasma phenomena in scientific diagnostics and industrial safety. However, conventional cryogenic MIR cameras face a fundamental trade-off between frame rate, noise, and pixel format. Here we report a passive, incoherent MIR imaging platform that leverages sum-frequency upconversion in chirped periodically poled lithium niobate (CPLN) to translate broadband 3--5um scenes to the near-infrared, enabling ultrafast acquisition on a silicon-based intensified CCD (iCCD). In fast-kinetics mode we achieve a physical frame rate of 100kHz with microsecond-scale gate control, and we directly capture the full evolution of an air-breakdown electric arc, resolving its rapid ignition, expansion, and decay dynamics. Beyond demonstrating ultrafast passive imaging, we introduce a drift-aware calibration workflow based on Allan deviation analysis to quantitatively select the gate width and averaging strategy under realistic slow-drift and multiplicative noise. This combined capability -- ultrafast passive MIR imaging plus operationally meaningful calibration -- provides a practical route toward real-time thermal surveillance and early-warning systems for hazardous fast transients.

physics.optics↗

arXiv2025

High resolution up-conversion imaging in the 10 μm band under incoherent illumination

Long-wavelength infrared band exhibits significant utility in thermal signature acquisition and molecular spectral analysis, among other applications. The up-conversion detection technique enables effective signal transduction into the detection bandwidth of silicon-based photodetectors, thereby facilitating high-sensitivity photonic measurements. We realized high-resolution up-conversion imaging for incoherent thermal targets in the 10 μm spectral regime for the first time. Furthermore, this work presents the first derivation of analytical models characterizing depth of field and astigmatic aberration in up-conversion imaging systems, which show excellent agreement between theoretical and experimental results. The results demonstrate generalisability to various up-conversion imaging systems, thus providing critical insights for the design and optimisation of such systems.

physics.optics↗

arXiv2025

On Chip Quantum States Generation by Incoherent Light

On-chip quantum sources based on nonlinear processes are pivotal components in integrated photonics, driving significant advancements in quantum information technologies over recent decades. Usually, the pump coherence has been considered to be crucial for ensuring the quality of generated states, therefore incoherent light is rarely used in quantum information processing. In this work, we explore and reveal the constructive influence of pumped temporal incoherence on the quantum properties of photon sources. Taking silicon waveguides as nonlinear media, we theoretically show that temporal incoherence of light can improve pumping utilization efficiency, resulting in higher source brightness in a spontaneous four-wave mixing process, and the spectrally uncorrelated nature of incoherent light is transferred to the generated photon source, allowing high-purity state preparation. Experimentally, we obtain a higher photon pair generation rate and the lower heralded second-order autocorrelation with an Amplified Spontaneous Emission source. Additionally, we successfully generate a polarization-entangled state with Bell inequality violation of S = 2.64 and a fidelity of 95.7%. Our study reveals the mechanism behind incoherently pumped quantum states and presents a method for generating photon sources using an easily accessible incoherent light.

quant-ph↗

arXiv2025

An all optical broadband tunable quantum frequency shifter

A frequency shifter of the photon is a key component for frequency-multiplexed high-capacity quantum communications and frequency-encoded quantum computation. Existed methods for shifting the frequency of a photon based on electro-optical, or acousto-optical effect, however, suffer the limited frequency shift up to a few hundreds of GHz, furthermore, high-quality micro-wave electronics are required. The frequency of a photon can also be shifted with the frequency difference equal to the frequency of pump laser by using an all optical-wave-mixing approach, which is usually about tens of THz. So, there is a big frequency shifting gap between these methods. Here, we propose a new scheme of a quantum frequency shifter based on an all-optical wave-mixing process, which can theoretically achieve a frequency shift ranging from GHz to a few THz, therefore bridging the gap. As a principle of poof, by using two pump beams in a three-wave mixing cascading process, a heralded single photon is frequency-shifted more than 400GHz, and the shift can be tuned continuously over broadband by changing the frequency difference between two pump lasers. Besides, high coincidence to accidence ratio between the shifted photons and the heralded photon indicates the preserve of quantum properties. The present quantum frequency shifter is in analog to an electro-optical based shifter, but with much broader tuning ability. Our all-optical quantum frequency shifter will become a fundamental building block for high-speed quantum communication networks and frequency domain photonic quantum computation.

quant-ph↗

arXiv2024

In-Lab High Resolution Mid-infrared Up-conversion Stellar Interferometer Based on Synthetic Long Base-Line

Detecting mid-infrared (MIR) radiation has significant astronomical applications, although limited by unsatisfactory MIR detectors. Here we reported on the realization of a MIR up-conversion interferometer based on synthetic long base-line (SLBL) in the laboratory. The experimental system consisted of an interferometer and subsequent up-conversion detection part of mid-infrared signal, which streamlined the structure and enhanced the reliability of the system. By using a tungsten filament lamp as an imitated star, we not only achieved the single target angle resolution of 1.10 times 10^(-4) rad, but also obtained the field angle resolution of 3.0 times 10^(-4) rad of double star targets. The angular resolution is in inverse proportion to the length of baseline. The maximum length of simulated baseline in the laboratory is about 3cm. In a Keck Interferometer (KI) liked program, the base line can reach up to 85m leading to a corresponding angular resolution of 3.0 times 10^(-9) rad (about 1.8mas). The study will offer potential benefits in extending the usage of mid-infrared light in astronomical exploration.

astro-ph.IM↗

arXiv2024

Quantum key distribution based on mid-infrared and telecom band two-color entanglement source

Due to the high noise caused by solar background radiation, the existing satellite-based free-space quantum key distribution (QKD) experiments are mainly carried out at night, hindering the establishment of a practical all-day real-time global-scale quantum network. Given that the 3-5 μm mid-infrared (MIR) band has extremely low solar background radiation and strong scattering resistance, it is one of the ideal bands for free-space quantum communication. Here, firstly, we report on the preparation of a high-quality MIR (3370 nm) and telecom band (1555 nm) two-color polarization-entangled photon source, then we use this source to realize a principle QKD based on free-space and fiber hybrid channels in a laboratory. The theoretical analysis clearly shows that a long-distance QKD over 500 km of free-space and 96 km of fiber hybrid channels can be reached simultaneously. This work represents a significant step toward developing all-day global-scale quantum communication networks.

quant-ph↗

arXiv2024

Quantum-Enhanced Polarimetric Imaging

Polarimetric imaging, a technique that captures the invisible polarization-related properties of given materials, has broad applications from fundamental physics to advanced fields such as target recognition, stress detection, biomedical diagnosis and remote sensing. The introduction of quantum sources into classical imaging systems has demonstrated distinct advantages, yet few studies have explored their combination with polarimetric imaging. In this study, we present a quantum polarimetric imaging system that integrates polarization-entangled photon pairs into a polarizer-sample-compensator-analyzer (PSRA)-type polarimeter. Our system visualizes the birefringence properties of a periodical-distributed anisotropic material under decreasing illumination levels and diverse disturbing light sources. Compared to the classical system, the quantum approach reveals the superior sensitivity and robustness in low-light conditions, particularly useful in biomedical studies where the low illumination and non-destructive detection are urgently needed. The study also highlights the nonlocality of entangled photons in birefringence measurement, indicating the potential of quantum polarimetric system in the remote sensing domain.

physics.optics↗

arXiv2024

Effective multiband synthetic four-wave mixing by cascading quadratic processes

Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes in a periodically poled lithium niobate crystal (PPLN), which has a 110dB(at 3000nm) higher conversion efficiency than the FWM directly generated by third-order susceptibilities in bulk PPLN crystals. A general model of this process is developed that is in full agreement with the experimental verifications. The frequency difference between the new frequency components can be freely tuned by changing the frequency difference of the dual pump lasers. Furthermore, by increasing the conversion bandwidth and efficiency of the cascaded processes, it is feasible to generate frequency combs in three bands the visible, near-infrared and mid-infrared bands simultaneously through high-order cascaded processes. This work opens up a new avenue toward free-tuning multiband frequency comb generation with multi-octaves frequency spanning, which will have significant applications in fields such as mid-infrared gas sensing, lidar and precision spectroscopy.

physics.optics↗

arXiv2024

Polarization entanglement by two simultaneous backward phase-matching processes in a single crystal

Entanglement enables many promising applications in quantum technology. Devising new generation methods and harnessing entanglement are prerequisites for practical applications. Here we realize a distinct polarization-entangled source by simultaneously achieving type-0 and type-I backward quasi-phase matching (BQPM) through spontaneous parametric down-conversion in a single bulk crystal, which is different from all previous entangled-source configurations. Pumping the crystal with a single polarized beam generates a non-maximally polarization-entangled state, which can be further projected to a maximal Bell state with a pair of Brewster windows. Hong-Ou-Mandel interference experiments are done on polarization-degenerate photon pairs for both type-0 and type-I BQPM processes for the first time. The emitted photons in both processes have a bandwidth as narrow as 15.7 GHz. The high quality of this source is characterized by various methods. The rather simple configuration, narrow bandwidth, and high entanglement quality make the source very promising for many quantum information tasks.

quant-ph↗

arXiv2024

Quantum entanglement enabled ellipsometer for phase retardance measurement

An ellipsometer is a vital precision tool used for measuring optical parameters with wide applications in many fields, including accurate measurements in film thickness, optical constants, structural profiles, etc. However, the precise measurement of photosensitive materials meets huge obstacles because of the excessive input photons, therefore the requirement of enhancing detection accuracy under low incident light intensity is an essential topic in the precision measurement. In this work, by combining a polarization-entangled photon source with a classical transmission-type ellipsometer, the quantum ellipsometer with the PSA (Polarizer-Sample-Analyzer) and the Senarmount method is constructed firstly to measure the phase retardation of the birefringent materials. The experimental results show that the accuracy can reach to nanometer scale at extremely low input intensity, and the stability are within 1% for all specimens tested with a compensator involved. Our work paves the way for precision measurement at low incident light intensity, with potential applications in measuring photosensitive materials, active-biological samples and other remote monitoring scenarios.

quant-ph↗

arXiv2023

Mid-Infrared Upconversion Imaging Under Different Illumination Conditions

Converting the medium infrared field to the visible band is an effective image detection method. We propose a comprehensive theory of image up-conversion under continuous optical pumping, and discuss the relationship between the experimental parameters and imaging field of view, resolution, quantum efficiency, and conversion bandwidth. Theoretical predictions of upconversion imaging results are given based on numerical simulations, which show good agreement with experimental results. In particular, coherent and incoherent light illumination are studied separately and the advantages and disadvantages of their imaging performance are compared and analysed. This work provides a study of the upconversion image detection performance of the system, which is of great value in guiding the design of the detection system and bringing it to practical applications.

physics.optics↗