arXiv subjects

Zhao-Yang Dong

Publications and source records attributed to Zhao-Yang Dong.

34 records · Page 2Linked to original sources

arXiv2021

Topological magnon insulator spin excitations in the two-dimensional ferromagnet CrBr$_3$

Topological magnons are bosonic analogues of topological fermions in electronic systems. They have been studied extensively by theory but rarely realized by experiment. Here, by performing inelastic neutron scattering measurements on single crystals of a two-dimensional ferromagnet CrBr$_3$, which was classified as Dirac magnon semimetal featured by the linear bands crossing at the Dirac points, we fully map out the magnetic excitation spectra, and reveal that there is an apparent gap of $\sim$3.5~meV between the acoustic and optical branches of the magnons at the K point. By collaborative efforts between experiment and theoretical calculations using a five-orbital Hubbard model obtained from first-principles calculations to derive the exchange parameters, we find that a Hamiltonian with Heisenberg exchange interactions, next-nearest-neighbor Dzyaloshinskii-Moriya (DM) interaction, and single-ion anisotropy is more appropriate to describe the system. Calculations using the model show that the lower and upper magnon bands separated by the gap exhibit Chern numbers of $\pm1$. These results indicate that CrBr$_3$ is a topological magnon insulator, where the nontrivial gap is a result of the DM interaction.

cond-mat.str-el↗

arXiv2020

Disorder-induced spin-liquid-like behavior in kagome-lattice compounds

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental studies on two kagomé-lattice QSL candidates, Tm$_3$Sb$_3$Zn$_2$O$_{14}$ and Tm$_3$Sb$_3$Mg$_2$O$_{14}$, which are isostructural to each other but with strong and weak structural disorder, respectively, we show unambiguously that the disorder can induce spin-liquid-like features. In particular, both compounds show dominant antiferromagnetic interactions with a Curie-Weiss temperature of -17.4 and -28.7 K for Tm$_3$Sb$_3$Zn$_2$O$_{14}$ and Tm$_3$Sb$_3$Mg$_2$O$_{14}$, respectively, but remain disordered down to about 0.05 K. Specific heat results suggest the presence of gapless magnetic excitations characterized by a residual linear term. Magnetic excitation spectra obtained by inelastic neutron scattering (INS) at low temperatures display broad continua. All these observations are consistent with those of a QSL. However, we find in Tm$_3$Sb$_3$Zn$_2$O$_{14}$ which has strong disorder resulting from the random mixing of the magnetic Tm$^{3+}$ and nonmagnetic Zn$^{2+}$, that the low-energy magnetic excitations observed in the specific heat and INS measurements are substantially enhanced, compared to those of Tm$_3$Sb$_3$Mg$_2$O$_{14}$ which has much less disorder. We believe that the effective spins of the Tm$^{3+}$ ions in the Zn$^{2+}$/Mg$^{2+}$ sites give rise to the low-energy magnetic excitations, and the amount of the random occupancy determines the excitation strength. These results provide direct evidence of the mimicry of a QSL caused by disorder.

cond-mat.str-el↗

arXiv2020

Fractionalized Spin Excitations in the Edge Ferromagnetic State of Graphene: Signature of the Ferromagnetic Luttinger Liquid

The elementary excitations from the conventional magnetic ordered states, such as ferromagnets and antiferromagnets, are magnons. Here, we elaborate a case where the well-defined magnons are absent completely and the spin excitation spectra exhibit an entire continuum in the itinerant edge ferromagnetic state of graphene arising from the flatband edge electronic states. Based on the further studies of the entanglement entropy and finite-size analysis, we show that the continuum other than the Stoner part results from the spin-1/2 spinons deconfined from magnons. The spinon continuum in a magnetically ordered state is ascribed to a ferromagnetic Luttinger liquid in this edge ferromagnet. The investigation is carried out by using the numerical exact diagonalization method with a projection of the interacting Hamiltonian onto the flat band.

cond-mat.str-el↗

arXiv2020

Evidence for magnon-phonon coupling in the topological magnet Cu$_3$TeO$_6$

We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific heat and thermal conductivity results show that the thermal transport is dominated by phonons, the deviation of the thermal conductivity from a pure phononic model indicates that there is a strong coupling between magnons and phonons. In the INS measurements, we find a mode in the excitation spectra at 4.5 K, which exhibits a slight downward dispersion around the Brillouin zone center. This mode disappears above the Néel temperature, and thus cannot be a phonon. Furthermore, the dispersion is distinct from that of a magnon. Instead, it can be explained by the magnon-polaron mode, which is new collective excitations resulting from the hybridization between magnons and phonons. We consider the suppression of the thermal conductivity and emergence of the magnon-polaron mode to be evidence for magnon-phonon coupling in Cu$_3$TeO$_6$.

cond-mat.str-el↗

arXiv2020

Spin dynamics of a magnetic Weyl semimetal Sr$_{1-x}$Mn$_{1-y}$Sb$_2$

Dirac matters provide a platform for exploring the interplay of their carriers with other quantum phenomena. Sr$_{1-x}$Mn$_{1-y}$Sb$_2$ has been proposed to be a magnetic Weyl semimetal and provides an excellent platform to study the coupling between Weyl fermions and magnons. Here, we report comprehensive inelastic neutron scattering (INS) measurements on single crystals of Sr$_{1-x}$Mn$_{1-y}$Sb$_2$, which have been well characterized by magnetization and magnetotransport measurements, both of which demonstrate that the material is a topologically nontrivial semimetal. The INS spectra clearly show a spin gap of $\sim6$ meV. The dispersion in the magnetic Mn layer extends up to about 76 meV, while that between the layers has a narrow band width of 6 meV. We find that the linear spin-wave theory using a Heisenberg spin Hamiltonian can reproduce the experimental spectra with the following parameters: a nearest-neighbor ($SJ_1\sim28.0$ meV) and next-nearest-neighbor in-plane exchange interaction ($SJ_2\sim9.3$ meV) , interlayer exchange coupling ($SJ_c\sim-0.1$ meV), and spin anisotropy constant ($SD\sim-0.07$ meV). Despite the coexistence of Weyl fermions and magnons, we find no clear evidence that the magnetic dynamics are influenced by the Weyl fermions in Sr$_{1-x}$Mn$_{1-y}$Sb$_2$, possibly because that the Weyl fermions and magnons reside in the Sb and Mn layers separately, and the interlayer coupling is weak due to the quasi-two-dimensional nature of the material, as also evident from the small $SJ_c$ of -0.1 meV.

cond-mat.mtrl-sci↗

arXiv2019

Itinerant topological magnons in Haldane Hubbard model with a nearly-flat electron band

We elaborate the first theoretical realization of two dimensional itinerant topological magnons, based on the quarter filled Haldane-Hubbard model with a nearly-flat electron band. By using the exact diagonalization method with a projection onto this band, we obtain the spin wave excitations over the itinerant ferromagnetic ground state. In the flatband limit, the excitation exhibits similar dispersion to the free electron band with Dirac magnons. The nonflatness of the electron band opens a topological gap at Dirac points and leads to an acoustic magnon band with a nonzero Chern number. We further show that tuning the sublattice Hubbard interactions or the next-nearest-neighbor hopping can induce a topological transition characterized by the gap closing and reopening, and the existence of the in-gap magnons on magnetic domain walls. We find an exact set of bases for magnons in the flatband limit constructed from sublattice particle-hole vectors and derive an effective model to explore the origin of the topological magnon which is attributed to the ``mass inversion mechanism''.

cond-mat.str-el↗

arXiv2019

Ferromagnetism and spin excitations in topological Hubbard models with a flatband

We study the spin-1 excitation spectra of the flatband ferromagnetic phases in interacting topological insulators. As a paradigm, we consider a quarter filled square lattice Hubbard model whose free part is the $π$ flux state with topologically nontrivial and nearly-flat electron bands, which can realize either the Chern or $Z_2$ Hubbard model. By using the numerical exact diagonalization method with a projection onto the nearly-flat band, we obtain the ferromagnetic spin-1 excitation spectra for both the Chern and $Z_2$ Hubbard models, consisting of spin waves and Stoner continuum. The spectra exhibit quite distinct dispersions for both cases, in particular the spin wave is gapless for the Chern Hubbard model, while gapped for the $Z_2$ Hubbard model. Remarkably, in both cases, the nonflatness of the free electron bands introduces dips in the lower boundary of the Stoner continuum. It significantly renormalizes the energies of the spin waves around these dips downward and leads to roton-like spin excitations. We elaborate that it is the softening of the roton-like modes that destabilizes the ferromagnetic phase, and determine the parameter region where the ferromagnetic phase is stable.

cond-mat.str-el↗

arXiv2018

Discovery of coexisting Dirac and triply degenerate magnons in a three-dimensional antiferromagnet

Topological magnons are emergent quantum spin excitations featured by magnon bands crossing linearly at the points dubbed nodes, analogous to fermions in topological electronic systems. Experimental realization of topological magnons in three dimensions has not been reported so far. Here, by measuring spin excitations (magnons) of a three-dimensional antiferromagnet Cu$_{3}$TeO$_{6}$ with inelastic neutron scattering, we provide direct spectroscopic evidence for the coexistence of symmetry-protected Dirac and triply degenerate nodes, the latter involving three-component magnons beyond the Dirac-Weyl framework. Our theoretical calculations show that the observed topological magnon band structure can be well described by the linear-spin-wave theory based on a Hamiltonian dominated by the nearest-neighbour exchange interaction $J_1$. As such, we showcase Cu$_{3}$TeO$_{6}$ as an example system where Dirac and triply degenerate magnonic nodal excitations coexist, demonstrate an exotic topological state of matter, and provide a fresh ground to explore the topological properties in quantum materials.

cond-mat.str-el↗

arXiv2018

Topological Magnons in a One-dimensional Itinerant Flatband Ferromagnet

Different from previous scenarios that topological magnons emerge in local spin models, we propose an alternative that itinerant electron magnets can host topological magnons. A one-dimensional Tasaki model with a flat band is considered as the prototype. This model can be viewed as a quarter filled periodic Anderson model with impurities located in between and hybridizing with the nearest-neighbor conducting electrons, together with a Hubbard repulsion for these electrons. By increasing the Hubbard interaction, the gap between the acoustic and optical magnons closes and reopens while the Berry phase of the acoustic band changes from 0 to $π$, leading to the occurrence of a topological transition. After this transition, there always exist in-gap edge magnonic modes which is consistent with the bulk-edge correspondence. The Hubbard interaction driven transition reveals a new mechanism to realize non-trivial magnon bands.

cond-mat.str-el↗

arXiv2018

Spectral properties of the square-lattice antiferromagnetic J1-J2 Heisenberg model: confinement and deconfinement of spinons

Based on the mapping between $s=1/2$ spin operators and hard-core bosons, we extend the cluster perturbation theory to spin systems and study the whole excitation spectrum of the antiferromagnetic $J_{1}$-$J_{2}$ Heisenberg model on the square lattice. In the Néel phase for $J_{2}\lesssim0.4J_{1}$, in addition to the dominant magnon excitation, there is an obvious continuum close to $(π,0)$ in the Brillouin zone indicating the deconfined spin-1/2 spinon excitations. In the stripe phase for $J_{2}\gtrsim0.6J_{1}$, we find similar high-energy two-spinon continuums at $(π/2,π/2)$ and $(π/2,π)$, respectively. The intermediate phase is characterized by a spectrum with completely deconfined broad continuum, which is attributed to a $Z_{2}$ quantum spin liquid with the aid of a variational-Monte-Carlo analysis.

cond-mat.str-el↗

arXiv2018

Spin-glass ground state in a triangular-lattice compound YbZnGaO$_4$

We report on comprehensive results identifying the ground state of a triangular-lattice structured YbZnGaO$_4$ to be spin glass, including no long-range magnetic order, prominent broad excitation continua, and absence of magnetic thermal conductivity. More crucially, from the ultralow-temperature a.c. susceptibility measurements, we unambiguously observe frequency-dependent peaks around 0.1 K, indicating the spin-glass ground state. We suggest this conclusion to hold also for its sister compound YbMgGaO$_4$, which is confirmed by the observation of spin freezing at low temperatures. We consider disorder and frustration to be the main driving force for the spin-glass phase.

cond-mat.str-el↗

arXiv2017

Projective symmetry group classification of $Z_3$ parafermion spin liquids on a honeycomb lattice

To study exotic excitations described by parafermions in the possible spin liquid states of SU($n$) spin systems, we introduce a parafermion parton approach. The SU($n$) spin operators can be represented by clock and shift matrices, which are shown to be the polynomials of parafermion operators in the parafermion representation. We find that SU($n$) spins can be decomposed into $n$ parafermion matrices of degree one. In this decomposition, the spin has a $\{\bigotimes{\rm SU}(n)\}^{n-1}$ gauge symmetry. As an application, we study the one-dimensional three-state clock model and generalized Kitaev model by a mean-field theory, both of them have been proved to be related to parafermion excitations. We find that with the symmetries of translations, $6$-fold rotation and combination of parity and time reversal, there are $9$ types and $102$ solutions for two-dimensional $Z_3$ parafermion spin liquids on the honeycomb lattice. On the contrast, there are $9$ types and $36$ solutions if both parity and time-reversal symmetries are present. Our results provide a novel route for the systematic search of new types of spin liquids with exotic anyon excitations.

cond-mat.str-el↗

arXiv2017

SU($N$) spin-wave theory: Application to spin-orbital Mott insulators

We present the application of the SU($N$) ($N>2$) spin-wave theory to spin-orbital Mott insulators whose ground states exhibit magnetic orders. When taking both the spin and orbital degrees of freedom into account rather than projecting onto the Kramers doublet, the lowest spin-orbital locking energy levels, due to the inevitable spin-orbital multipole exchange interactions, the SU($N$) spin-wave theory should take the place of the SU($2$) one. To implement the application, we introduce an efficient general local mean field approach which involves all the local fluctuations into the SU($N$) linear spin-wave theory. Our approach is tested firstly by calculating the multipolar spin-wave spectra of the SU($4$) antiferromagnetic model. Then we apply it to spin-orbital Mott insulators. It is revealed that the Hund's coupling would influence the effectiveness of the isospin-$1/2$ representation when the spin orbital coupling is not large enough. Besides, we also calculate the spin-wave spectra based on the first principle calculations for two concrete materials, $α$-RuCl$_3$ and Sr$_2$IrO$_4$. The SU($N$) spin-wave theory appropriately depicts the low-energy magnons and the spin-orbital excitations qualitatively.

cond-mat.str-el↗

arXiv2017

Theoretical investigation of the magnetic dynamics in $α$-RuCl$_3$

We study the spin-wave excitations in $α$-RuCl$_3$ by the spin-wave theory. Starting from the five-orbital Hubbard model and the perturbation theory, we derive an effective isospin-$1/2$ model in the large Hubbard ($U$) limit. Based on the energy-band structure calculated from the first-principle method, we find that the effective model can be further reduced to the $K$-$Γ$ model containing a ferromagnetic nearest-neighbor (NN) Kitaev interaction ($K$) and a NN off-diagonal exchange interaction ($Γ$). With the spin-wave theory, we find that the $K$-$Γ$ model can give magnetic excitations which is consistent with the recent neutron scattering experiments.

cond-mat.str-el↗

arXiv2017

Spin-wave excitations evidencing the Kitaev interaction in single crystalline $α$-RuCl$_3$

Kitaev interactions underlying a quantum spin liquid have been long sought, but experimental data from which their strengths can be determined directly is still lacking. Here, by carrying out inelastic neutron scattering measurements on high-quality single crystals of $α$-RuCl$_3$, we observe spin-wave spectra with a gap of $\sim$2 meV around the M point of the two-dimensional Brillouin zone. We derive an effective-spin model in the strong-coupling limit based on energy bands obtained from first-principle calculations, and find that the anisotropic Kitaev interaction $K$ term and the isotropic antiferromagentic off-diagonal exchange interaction $Γ$ term are significantly larger than the Heisenberg exchange coupling $J$ term. Our experimental data can be well fit using an effective-spin model with $K=-6.8$ meV and $Γ=9.5$ meV. These results demonstrate explicitly that Kitaev physics is realized in real materials.

cond-mat.str-el↗

arXiv2014

Majorana Edge States and Braiding in an Exactly Solvable One-dimensional Spin Model

We derive an exactly solvable one-dimensional (1D) spin model from the three-band Hubbard model with a strong spin-orbit coupling by introducing U(1) gauge fields to the isospin states. We find that it has a topological nontrivial phase characterized by Majorana end modes which are protected by a new Z_2 topological invariant related to the parity of the lattice sites (odd or even number of sites) in the spin chain. With the protection of this Z_2 topological invariant, a novel braiding of two Majorana edge states in this strictly geometric 1D chain is realized. We also discuss the possible realization of the gauge fields.

cond-mat.mes-hall↗