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Zhe Qu

Publications and source records attributed to Zhe Qu.

At least 55 records · Page 3Linked to original sources

CDPA: Common and Distinctive Pattern Analysis between High-dimensional Datasets

A representative model in integrative analysis of two high-dimensional correlated datasets is to decompose each data matrix into a low-rank common matrix generated by latent factors shared across datasets, a low-rank distinctive matrix corresponding to each dataset, and an additive noise matrix. Existing decomposition methods claim that their common matrices capture the common pattern of the two datasets. However, their so-called common pattern only denotes the common latent factors but ignores the common pattern between the two coefficient matrices of these common latent factors. We propose a new unsupervised learning method, called the common and distinctive pattern analysis (CDPA), which appropriately defines the two types of data patterns by further incorporating the common and distinctive patterns of the coefficient matrices. A consistent estimation approach is developed for high-dimensional settings, and shows reasonably good finite-sample performance in simulations. Our simulation studies and real data analysis corroborate that the proposed CDPA can provide better characterization of common and distinctive patterns and thereby benefit data mining.

stat.ML↗

FedLGA: Towards System-Heterogeneity of Federated Learning via Local Gradient Approximation

Federated Learning (FL) is a decentralized machine learning architecture, which leverages a large number of remote devices to learn a joint model with distributed training data. However, the system-heterogeneity is one major challenge in a FL network to achieve robust distributed learning performance, which comes from two aspects: i) device-heterogeneity due to the diverse computational capacity among devices; ii) data-heterogeneity due to the non-identically distributed data across the network. Prior studies addressing the heterogeneous FL issue, e.g., FedProx, lack formalization and it remains an open problem. This work first formalizes the system-heterogeneous FL problem and proposes a new algorithm, called FedLGA, to address this problem by bridging the divergence of local model updates via gradient approximation. To achieve this, FedLGA provides an alternated Hessian estimation method, which only requires extra linear complexity on the aggregator. Theoretically, we show that with a device-heterogeneous ratio $ρ$, FedLGA achieves convergence rates on non-i.i.d. distributed FL training data for the non-convex optimization problems with $\mathcal{O} \left( \frac{(1+ρ)}{\sqrt{ENT}} + \frac{1}{T} \right)$ and $\mathcal{O} \left( \frac{(1+ρ)\sqrt{E}}{\sqrt{TK}} + \frac{1}{T} \right)$ for full and partial device participation respectively, where $E$ is the number of local learning epoch, $T$ is the number of total communication round, $N$ is the total device number and $K$ is the number of selected device in one communication round under partially participation scheme. The results of comprehensive experiments on multiple datasets show that FedLGA outperforms current FL methods against the system-heterogeneity.

cs.LG↗

LoMar: A Local Defense Against Poisoning Attack on Federated Learning

Federated learning (FL) provides a high efficient decentralized machine learning framework, where the training data remains distributed at remote clients in a network. Though FL enables a privacy-preserving mobile edge computing framework using IoT devices, recent studies have shown that this approach is susceptible to poisoning attacks from the side of remote clients. To address the poisoning attacks on FL, we provide a \textit{two-phase} defense algorithm called {Lo}cal {Ma}licious Facto{r} (LoMar). In phase I, LoMar scores model updates from each remote client by measuring the relative distribution over their neighbors using a kernel density estimation method. In phase II, an optimal threshold is approximated to distinguish malicious and clean updates from a statistical perspective. Comprehensive experiments on four real-world datasets have been conducted, and the experimental results show that our defense strategy can effectively protect the FL system. {Specifically, the defense performance on Amazon dataset under a label-flipping attack indicates that, compared with FG+Krum, LoMar increases the target label testing accuracy from $96.0\%$ to $98.8\%$, and the overall averaged testing accuracy from $90.1\%$ to $97.0\%$.

cs.LG↗

Context-Aware Online Client Selection for Hierarchical Federated Learning

Federated Learning (FL) has been considered as an appealing framework to tackle data privacy issues of mobile devices compared to conventional Machine Learning (ML). Using Edge Servers (ESs) as intermediaries to perform model aggregation in proximity can reduce the transmission overhead, and it enables great potentials in low-latency FL, where the hierarchical architecture of FL (HFL) has been attracted more attention. Designing a proper client selection policy can significantly improve training performance, and it has been extensively used in FL studies. However, to the best of our knowledge, there are no studies focusing on HFL. In addition, client selection for HFL faces more challenges than conventional FL, e.g., the time-varying connection of client-ES pairs and the limited budget of the Network Operator (NO). In this paper, we investigate a client selection problem for HFL, where the NO learns the number of successful participating clients to improve the training performance (i.e., select as many clients in each round) as well as under the limited budget on each ES. An online policy, called Context-aware Online Client Selection (COCS), is developed based on Contextual Combinatorial Multi-Armed Bandit (CC-MAB). COCS observes the side-information (context) of local computing and transmission of client-ES pairs and makes client selection decisions to maximize NO's utility given a limited budget. Theoretically, COCS achieves a sublinear regret compared to an Oracle policy on both strongly convex and non-convex HFL. Simulation results also support the efficiency of the proposed COCS policy on real-world datasets.

cs.LG↗

Topological charge-entropy scaling in kagome Chern magnet TbMn$_6$Sn$_6$

In ordinary materials, electrons conduct both electricity and heat, where their charge-entropy relations observe the Mott formula and the Wiedemann-Franz law. In topological quantum materials, the transverse motion of relativistic electrons can be strongly affected by the quantum field arising around the topological fermions, where a simple model description of their charge-entropy relations remains elusive. Here we report the topological charge-entropy scaling in the kagome Chern magnet TbMn$_6$Sn$_6$, featuring pristine Mn kagome lattices with strong out-of-plane magnetization. Through both electric and thermoelectric transports, we observe quantum oscillations with a nontrivial Berry phase, a large Fermi velocity and two-dimensionality, supporting the existence of Dirac fermions in the magnetic kagome lattice. This quantum magnet further exhibits large anomalous Hall, anomalous Nernst, and anomalous thermal Hall effects, all of which persist to above room temperature. Remarkably, we show that the charge-entropy scaling relations of these anomalous transverse transports can be ubiquitously described by the Berry curvature field effects in a Chern-gapped Dirac model. Our work points to a model kagome Chern magnet for the proof-of-principle elaboration of the topological charge-entropy scaling.

cond-mat.str-el↗

Field-induced quantum spin disordered state in spin-1/2 honeycomb magnet Na2Co2TeO6

Spin-orbit coupled honeycomb magnets with the Kitaev interaction have received a lot of attention due to their potential of hosting exotic quantum states including quantum spin liquids. Thus far, the most studied Kitaev systems are 4d/5d-based honeycomb magnets. Recent theoretical studies predicted that 3d-based honeycomb magnets, including Na2Co2TeO6 (NCTO), could also be a potential Kitaev system. Here, we have used a combination of heat capacity, magnetization, electron spin resonance measurements alongside inelastic neutron scattering (INS) to study NCTO's quantum magnetism, and we have found a field-induced spin disordered state in an applied magnetic field range of 7.5 T < B (vertical to b-axis) < 10.5 T. The INS spectra were also simulated to tentatively extract the exchange interactions. As a 3d-magnet with a field-induced disordered state on an effective spin-1/2 honeycomb lattice, NCTO expands the Kitaev model to 3d compounds, promoting further interests on the spin-orbital effect in quantum magnets.

cond-mat.str-el↗

How to Test the Randomness from the Wireless Channel for Security?

We revisit the traditional framework of wireless secret key generation, where two parties leverage the wireless channel randomness to establish a secret key. The essence in the framework is to quantify channel randomness into bit sequences for key generation. Conducting randomness tests on such bit sequences has been a common practice to provide the confidence to validate whether they are random. Interestingly, despite different settings in the tests, existing studies interpret the results the same: passing tests means that the bit sequences are indeed random. In this paper, we investigate how to properly test the wireless channel randomness to ensure enough security strength and key generation efficiency. In particular, we define an adversary model that leverages the imperfect randomness of the wireless channel to search the generated key, and create a guideline to set up randomness testing and privacy amplification to eliminate security loss and achieve efficient key generation rate. We use theoretical analysis and comprehensive experiments to reveal that common practice misuses randomness testing and privacy amplification: (i) no security insurance of key strength, (ii) low efficiency of key generation rate. After revision by our guideline, security loss can be eliminated and key generation rate can be increased significantly.

cs.CR↗

Anomalous Hall effect in distorted kagome magnets (Nd, Sm)Mn$_6$Sn$_6$

We report magnetic and electrical properties for single crystals of NdMn$_6$Sn$_6$ and SmMn$_6$Sn$_6$. They crystallize into a structure which has distorted, Mn-based kagome lattices, compared to the pristine kagome lattices in heavy-rare-earth-bearing RMn$_6$Sn$_6$ compounds. They are hightemperature ferromagnets of which the R moment is parallel with the Mn moment. We observed a large intrinsic anomalous Hall effect (AHE) that is comparable to the ferrimagnetic, heavy-R siblings in a wide range of temperature. We conclude that their intrinsic AHE is stemming from the Mn-based kagome lattice, just as in the heavy RMn$_6$Sn$_6$.

cond-mat.str-el↗

Rare earth engineering in RMn$_6$Sn$_6$ topological kagome magnets

Exploration of the topological quantum materials with electron correlation is at the frontier of physics, as the strong interaction may give rise to new topological phases and transitions. Here we report that a family of kagome magnets RMn$_6$Sn$_6$ manifest the quantum transport properties analogical to those in the quantum-limit Chern magnet TbMn$_6$Sn$_6$. The topological transport in the family, including quantum oscillations with nontrivial Berry phase and large anomalous Hall effect arising from Berry curvature field, points to the existence of massive Dirac fermions. Our observation demonstrates a close relationship between rare-earth magnetism and topological electron structure, indicating the rare-earth elements can effectively engineer the Chern quantum phase in kagome magnets.

cond-mat.mtrl-sci↗

Stragglers Are Not Disaster: A Hybrid Federated Learning Algorithm with Delayed Gradients

Federated learning (FL) is a new machine learning framework which trains a joint model across a large amount of decentralized computing devices. Existing methods, e.g., Federated Averaging (FedAvg), are able to provide an optimization guarantee by synchronously training the joint model, but usually suffer from stragglers, i.e., IoT devices with low computing power or communication bandwidth, especially on heterogeneous optimization problems. To mitigate the influence of stragglers, this paper presents a novel FL algorithm, namely Hybrid Federated Learning (HFL), to achieve a learning balance in efficiency and effectiveness. It consists of two major components: synchronous kernel and asynchronous updater. Unlike traditional synchronous FL methods, our HFL introduces the asynchronous updater which actively pulls unsynchronized and delayed local weights from stragglers. An adaptive approximation method, Adaptive Delayed-SGD (AD-SGD), is proposed to merge the delayed local updates into the joint model. The theoretical analysis of HFL shows that the convergence rate of the proposed algorithm is $\mathcal{O}(\frac{1}{t+τ})$ for both convex and non-convex optimization problems.

cs.LG↗

Magnetoelectric effect arising from a field-induced pseudo Jahn-Teller distortion in a rare earth magnet

Magnetoelectric materials are attractive for several applications, including actuators, switches, and magnetic field sensors. Typical mechanisms for achieving a strong magnetoelectric coupling are rooted in transition metal magnetism. In sharp contrast, here we identify CsEr(MoO4)2 as a magnetoelectric material without magnetic transition metal ions, thus ensuring that the Er ions play a key role in achieving this interesting property. Our detailed study includes measurements of the structural, magnetic, and electric properties of this material. Bulk characterization and neutron powder diffraction show no evidence for structural phase transitions down to 0.3 K and therefore CsEr(MoO4)2 maintains the room temperature P2/c space group over a wide temperature range without external magnetic field. These same measurements also identify collinear antiferromagnetic ordering of the Er3+ moments below TN = 0.87 K. Complementary dielectric constant and pyroelectric current measurements reveal that a ferroelectric phase (P ~ 0.5 nC/cm2) emerges when applying a modest external magnetic field, which indicates that this material has a strong magnetoelectric coupling. We argue that the magnetoelectric coupling in this system arises from a pseudo Jahn-Teller distortion induced by the magnetic field.

cond-mat.mtrl-sci↗

Quantum oscillations in the non-centrosymmetric superconductor and topological nodal-line semimetal PbTaSe$_2$

We observed quantum oscillations in thermoelectric and magnetic torque signals in non-centrosymmetric superconductor PbTaSe$_2$. One oscillatory frequency stems from the orbits formed by magnetic breakdown, while others are from two-dimensional-like Fermi surfaces near the topological nodal rings. Our comprehensive understanding of the Fermi surface topology of PbTaSe$_2$, including nailing down the Fermi level and detecting the Berry phases near the nodal rings, is crucial for searching plausible topological superconductivity in its bulk and surface states.

cond-mat.supr-con↗

Topological semimetal state and field-induced Fermi surface reconstruction in antiferromagnetic monopnictide NdSb

We report the experimental realization of Dirac semimetal state in NdSb, a material with antiferromagnetic ground state. The occurrence of topological semimetal state has been well supported by our band structure calculations and the experimental observation of chiral anomaly induced negative magnetoresistance. A field-induced Fermi surface reconstruction is observed, in response to the change of spin polarization. The observation of topological semimetal state in a magnetic material provides an opportunity to investigate the magneto-topological phenomena.

cond-mat.mtrl-sci↗

Single Crystal Growth, Transport, and Electronic Band Structure of YCoGa$_5$

Single crystal of YCoGa5 has been grown via Ga self-flux. In this paper, we report the single crystal growth, crystallographic parameters, resistivity, heat capacity, and band structure results of YCoGa5. YCoGa5 accommodates the HoCoGa5 type structure (space group P4/mmm (No. 123), Z = 1, a = 4.2131(6) A, c = 6.7929(13) A, which is isostructural to the extensively studied heavy fermion superconductor system CeMIn5 (M = Co, Rh, Ir) and the unconventional superconductor PuCoGa5 with Tc = 18.5 K. No superconductivity is observed down to 1.75 K. Band structure calculation results show that its band at the Fermi level is mainly composed of Co-3d and Ga-4p electrons states, which explains its similarity of physical properties to YbCoGa5 and LuCoGa5.

cond-mat.supr-con↗

The effect of Al doping on the structure and magnetism in cobaltite CaBaCo4O7

We report the effects of Al-doping on the structure and magnetic properties in CaBa(Co$_{1-x}$Al$_{x}$)$_4$O$_7$ (0$\leq$x$\leq$0.25). The system exhibits a structural transition from an orthorhombic symmetry to a hexagonal symmetry when the Al content exceeds $x =$ 0.1. The Curie temperature and the value of the magnetization decrease with increasing Al doping level, indicating that the ferrimagnetic ground state is gradually suppressed. The ground state eventually transits into a spin-glass state for $x >$ 0.1. Moreover, the short-range magnetic correlations, which occur at high temperatures in CaBaCo$_4$O$_7$, are found to be gradually suppressed with increasing Al content and eventually disappear for $x =$ 0.25. By comparing our results with other Co-site doping cases, we suggest that the lattice and the spin degrees of freedom are relatively decoupled in CaBaCo$_4$O$_7$.

cond-mat.mtrl-sci↗

Spin-phonon coupling probed by infrared transmission spectroscopy in the double perovskite Ba$_2$YMoO$_6$

In this work, we investigate the local structural distortion of the double perovskite Ba$_2$YMoO$_6$ by means of infrared transmission spectroscopy. At 300 K, three bands are observed at $\sim$ 255.1 cm$^{-1}$, $\sim$ 343.4 cm$^{-1}$, and $\sim$ 561.5 cm$^{-1}$, which are related to the motion between the cation Ba$^{2+}$ and the anion YMO$_6^{-2}$, the Y-O stretching motion and the stretching vibration of the MoO$_6$ octahedron, respectively. These modes continue to harden upon cooling owing to the shrink of the lattice constant. When the temperature decreases to $T \leq$ 130 K around which the spin singlet dimer begins to form, an additional phonon mode appears at $\sim$ 611 cm$^{-1}$, suggesting the occurrence of local distortion of MoO$_6$ octahedra. With further decrease of the temperature, its intensity enhances and its peak position keeps unchanged. These results indicate that the formation of the spin singlet dimers is accompanied with the occurrence of the local structure distortion of MoO$_6$ octahedra, providing evidence for the strong spin-phonon coupling in the double perovskite Ba$_2$YMoO$_6$.

cond-mat.str-el↗

The effect of disorder on quantum phase transition in the double layered ruthenates (Sr1-xCax)3Ru2O7

(Sr1-xCax)3Ru2O7 is characterized by complex magnetic states, spanning from a long-range antiferromagnetically ordered state over an unusual heavy-mass nearly ferromagnetic (NFM) state to an itinerant metamagnetic (IMM) state. The NFM state, which occurs in the 0.4 > x > 0.08 composition range, freezes into a cluster-spin-glass (CSG) phase at low temperatures [Z. Qu et al., Phys. Rev. B 78, 180407(R) (2008)]. In this article, we present the scaling analyses of magnetization and the specific heat for (Sr1-xCax)3Ru2O7 in the 0.4 > x > 0.08 composition range. We find that in a temperature region immediately above the spin freezing temperature T$_f$, the isothermal magnetization M(H) and the temperature dependence of electronic specific heat C_e(T) exhibit anomalous power-law singularities; both quantities are controlled by a single exponent. The temperature dependence of magnetization M(T) also displays a power-law behavior, but its exponent differs remarkably from that derived from M(H) and C_e(T). Our analyses further reveal that the magnetization data M(H,T) obey a phenomenological scaling law of M(H,T) \propto H^αf(H/T^δ) in a temperature region between the spin freezing temperature T_f and the scaling temperature T_scaling. T_scaling systematically decreases with the decease of Ca content. This scaling law breaks down near the critical concentration x = 0.1 where a CSG-to-IMM phase transition occurs. We discussed these behaviors in term of the effect of disorder on the quantum phase transition.

cond-mat.str-el↗

Magnetic properties of the ferrimagnetic cobaltite CaBaCo4O7

The magnetic properties of the ferrimagnetic cobaltite CaBaCo$_4$O$_7$ are systematically investigated. We find that the susceptibility exhibits a downward deviation below $\sim$ 360 K, suggesting the occurrence of short range magnetic correlations at temperature well above $T_C$. The effective moment is determined to be 4.5 $μ_B$/f.u, which is consistent with that expected for the Co$^{2+}$/Co$^{3+}$ high spin species. Using a criterion given by Banerjee [Phys. Lett. \textbf{12}, 16 (1964)], we demonstrate that the paramagnetic to ferrimagnetic transition in CaBaCo$_4$O$_7$ has a first order character.

cond-mat.str-el↗