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Zhendong Zhu

Publications and source records attributed to Zhendong Zhu.

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A universal framework for nonlinear frequency combs under electro-optic modulation

Nonlinear frequency combs, including electro-optic and Kerr combs, have become central platforms for chip-scale frequency synthesis. Recent breakthroughs in strong-coupling electro-optic modulation further expanded their accessible nonlinear dynamics, unlocking new phenomena and functionalities, but the underlying foundation remains largely unexplored. Here we establish a universal theoretical and experimental framework for nonlinear combs under arbitrary electro-optic modulation by introducing a general evolution equation (GEE) that transcends the mean-field Lugiato-Lefever equation. The GEE reduces to a discrete-time Integration Hamiltonian that provides a frequency-domain formalism unifying strong-coupling electro-optic modulation with photonic synthetic dimensions. Together with a band-wave correspondence linking modulation waveforms to synthetic band structures, the formalism enables programmable spectral control. We further show compatibility between Kerr nonlinearity and strong-coupling electro-optic modulation, highlighting their cooperative dynamics. Our work provides a foundational model for strong-coupling electro-optics in nonlinear combs, opening a route toward chip-integrated, microwave-programmable comb sources for metrology, spectroscopy, and emerging photonic technologies.

physics.optics

Fano-resonance boosted cascaded field enhancement in a plasmonic nanoparticle-in-cavity nanoantenna array and its SERS application

Cascaded optical field enhancement (CFE) can be realized in some specially designed multiscale plasmonic nanostructures, where the generation of extremely strong field at nanoscale volume is crucial for many applications, for example, surface enhanced Raman spectroscopy (SERS). Here, we propose a strategy of realizing a high-quality plasmonic nanoparticle-in-cavity (PIC) nanoantenna array, where strong coupling between a nanoparticle dark mode with a high order nanocavity bright mode can produce Fano resonance at a target wavelength. The Fano resonance can effectively boost the CFE in the PIC, with a field enhancement factor up to 5X10^2. A cost-effective and reliable nanofabrication method is developed with room temperature nanoimprinting lithography to manufacture high-quality PIC arrays. This technique guarantees the generation of only one gold nanoparticle at the bottom of each nanocavity, which is crucial for the generation of the expected CFE. As a demonstration of the performance and application of the PIC array, it is used as active SERS substrate for detecting 4-aminothiophenol molecules. The SERS enhancement factor up to 2X10^7 is obtained experimentally, verifying the field enhancement and potential of this device.

physics.optics