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Zhenlin Wang

Publications and source records attributed to Zhenlin Wang.

At least 37 records · Page 2Linked to original sources

Best Arm Identification with Safety Constraints

The best arm identification problem in the multi-armed bandit setting is an excellent model of many real-world decision-making problems, yet it fails to capture the fact that in the real-world, safety constraints often must be met while learning. In this work we study the question of best-arm identification in safety-critical settings, where the goal of the agent is to find the best safe option out of many, while exploring in a way that guarantees certain, initially unknown safety constraints are met. We first analyze this problem in the setting where the reward and safety constraint takes a linear structure, and show nearly matching upper and lower bounds. We then analyze a much more general version of the problem where we only assume the reward and safety constraint can be modeled by monotonic functions, and propose an algorithm in this setting which is guaranteed to learn safely. We conclude with experimental results demonstrating the effectiveness of our approaches in scenarios such as safely identifying the best drug out of many in order to treat an illness.

cs.LG↗

System inference via field inversion for the spatio-temporal progression of infectious diseases: Studies of COVID-19 in Michigan and Mexico

We present an approach to studying and predicting the spatio-temporal progression of infectious diseases. We treat the problem by adopting a partial differential equation (PDE) version of the Susceptible, Infected, Recovered, Deceased (SIRD) compartmental model of epidemiology, which is achieved by replacing compartmental populations by their densities. Building on our recent work (Computational Mechanics, 66, 1177, 2020), we replace our earlier use of global polynomial basis functions with those having local support, as epitomized in the finite element method, for the spatial representation of the SIRD parameters. The time dependence is treated by inferring constant parameters over time intervals that coincide with the time step in semi-discrete numerical implementations. In combination, this amounts to a scheme of field inversion of the SIRD parameters over each time step. Applied to data over ten months of 2020 for the pandemic in the US state of Michigan and to all of Mexico, our system inference via field inversion infers spatio-temporally varying PDE SIRD parameters that replicate the progression of the pandemic with high accuracy. It also produces accurate predictions, when compared against data, for a three week period into 2021. Of note is the insight that is suggested on the spatio-temporal variation of infection, recovery and death rates, as well as patterns of the population's mobility revealed by diffusivities of the compartments.

physics.bio-ph↗

Temperature-sensitive spatial distribution of defects in PdSe2 flakes

Defect engineering plays an important role in tailoring the electronic transport properties of van der Waals materials. However, it is usually achieved through tuning the type and concentration of defects, rather than dynamically reconfiguring their spatial distribution. Here, we report temperature-sensitive spatial redistribution of defects in PdSe2 thin flakes through scanning tunneling microscopy (STM). We observe that the spatial distribution of Se vacancies in PdSe2 flakes exhibits a strong anisotropic characteristic at 80 K, and that this orientation-dependent feature is weakened when temperature is raised. Moreover, we carry out transport measurements on PdSe2 thin flakes and show that the anisotropic features of carrier mobility and phase coherent length are also sensitive to temperature. Combining with theoretical analysis, we conclude that temperature-driven defect spatial redistribution could interpret the temperature-sensitive electrical transport behaviors in PdSe2 thin flakes. Our work highlights that engineering spatial distribution of defects in the van der Waals materials, which has been overlooked before, may open up a new avenue to tailor the physical properties of materials and explore new device functionalities.

cond-mat.mes-hall↗

GRAPHSPY: Fused Program Semantic-Level Embedding via Graph Neural Networks for Dead Store Detection

Production software oftentimes suffers from the issue of performance inefficiencies caused by inappropriate use of data structures, programming abstractions, and conservative compiler optimizations. It is desirable to avoid unnecessary memory operations. However, existing works often use a whole-program fine-grained monitoring method with incredibly high overhead. To this end, we propose a learning-aided approach to identify unnecessary memory operations intelligently with low overhead. By applying several prevalent graph neural network models to extract program semantics with respect to program structure, execution order and dynamic states, we present a novel, hybrid program embedding approach so that to derive unnecessary memory operations through the embedding. We train our model with tens of thousands of samples acquired from a set of real-world benchmarks. Results show that our model achieves 90% of accuracy and incurs only around a half of time overhead of the state-of-art tool.

cs.LG↗

System inference for the spatio-temporal evolution of infectious diseases: Michigan in the time of COVID-19

We extend the classical SIR model of infectious disease spread to account for time dependence in the parameters, which also include diffusivities. The temporal dependence accounts for the changing characteristics of testing, quarantine and treatment protocols, while diffusivity incorporates a mobile population. This model has been applied to data on the evolution of the COVID-19 pandemic in the US state of Michigan. For system inference, we use recent advances; specifically our framework for Variational System Identification (Wang et al., Comp. Meth. App. Mech. Eng., 356, 44-74, 2019; arXiv:2001.04816 [cs.CE]) as well as Bayesian machine learning methods.

q-bio.PE↗

Gate-tunable van der Waals heterostructure for reconfigurable neural network vision sensor

Early processing of visual information takes place in the human retina. Mimicking neurobiological structures and functionalities of the retina provide a promising pathway to achieving vision sensor with highly efficient image processing. Here, we demonstrate a prototype vision sensor that operates via the gate-tunable positive and negative photoresponses of the van der Waals (vdW) vertical heterostructures. The sensor emulates not only the neurobiological functionalities of bipolar cells and photoreceptors but also the unique synaptic connectivity between bipolar cells and photoreceptors. By tuning gate voltage for each pixel, we achieve reconfigurable vision sensor for simultaneously image sensing and processing. Furthermore, our prototype vision sensor itself can be trained to classify the input images, via updating the gate voltages applied individually to each pixel in the sensor. Our work indicates that vdW vertical heterostructures offer a promising platform for the development of neural network vision sensor.

cond-mat.mtrl-sci↗

Investigation of plasmonic evolution of atomically size-selected Au clusters by electron energy loss spectrum--from solid state to molecular scale

Versatile quantum modes emerge for plasmon describing the collective oscillations of free electrons in metallic nanoparticles when the particle sizes are greatly reduced. Rather than traditional nanoscale study, the understanding of quantum plasmon desires extremal atomic control of the nanoparticles, calling for size dependent plasmon measurement over a series of nanoparticles with atomically adjustable atom number over several orders of magnitude. Here we report the N dependent plasmonic evolution of atomically size selected gold particles with N= 100 70000 using electron energy loss (EEL) spectroscopy in a scanning transmission electron microscope. The EEL mapping assigns a feature at 2.7 eV as the bulk plasmon and another at 2.4 eV as surface plasmon, which evolution reveals three regimes. When N decreases from 70000 to 887, the bulk plasmon stays unchanged while the surface plasmon exhibits a slight red shift from 2.4 to 2.3 eV. It can be understood by the dominance of classical plasmon physics and electron boundary scattering induced retardation. When N further decreases from 887 to 300, the bulk plasmon disappears totally and the surface plasmon shows a steady blueshift, which indicates that the quantum confinement emerges and modifies the intraband transition. When N 100 300, the plasmon is split to three fine features, which is attributed to superimposed single electron transitions between the quantized molecular like energy level by the time dependent density functional theory calculations. The surface plasmon's excitation ratio has a scaling law with an exponential dependence on N ( N^0.669), essentially the square of the radius. A unified evolution picture from the classical to quantum, molecular plasmon is thus demonstrated.

physics.atm-clus↗

A Perspective on Regression and Bayesian Approaches for System Identification of Pattern Formation Dynamics

We present two approaches to system identification, i.e. the identification of partial differential equations (PDEs) from measurement data. The first is a regression-based Variational System Identification procedure that is advantageous in not requiring repeated forward model solves and has good scalability to large number of differential operators. However it has strict data type requirements needing the ability to directly represent the operators through the available data. The second is a Bayesian inference framework highly valuable for providing uncertainty quantification, and flexible for accommodating sparse and noisy data that may also be indirect quantities of interest. However, it also requires repeated forward solutions of the PDE models which is expensive and hinders scalability. We provide illustrations of results on a model problem for pattern formation dynamics, and discuss merits of the presented methods.

physics.comp-ph↗

Higher-order Quantum Spin Hall Effect of Light

Band topology and related spin (or pseudo-spin) physics of photons provide us with a new dimension for manipulating light, which is potentially useful for information communication and data storage. Especially, the quantum spin Hall effect of light, where electromagnetic waves propagate along surfaces of samples with strong spin-momentum locking, paves the way for achieving topologically protected photonic spin transport. Recently, the conventional bulk-edge correspondence of the band topology has been extended to higher-order cases that enables the explorations of topological states with codimensions larger than 1 such as hinge and corner states. Here, for the first time, we demonstrate a higherorder quantum spin Hall effect of light by utilizing an all-dielectric C6v-symmetric photonic crystal. We observe corner states with opposite pseudospin polarizations at different corners owing to nontrivial higher-order topology and finite spin-spin coupling. By applying the spin-polarized excitation sources, we can selectively excite the corner states at different spatial positions through spin-momentum-locked decaying edge states, resembling the quantum spin Hall effect in a higher-order manner. Our work which breaks the barriers between the spin photonics and higher-order topology opens the frontiers for studying lower-dimensional spinful classical surface waves and supports explorations in robust communications.

cond-mat.mtrl-sci↗

Variational system identification of the partial differential equations governing pattern-forming physics: Inference under varying fidelity and noise

We present a contribution to the field of system identification of partial differential equations (PDEs), with emphasis on discerning between competing mathematical models of pattern-forming physics. The motivation comes from developmental biology, where pattern formation is central to the development of any multicellular organism, and from materials physics, where phase transitions similarly lead to microstructure. In both these fields there is a collection of nonlinear, parabolic PDEs that, over suitable parameter intervals and regimes of physics, can resolve the patterns or microstructures with comparable fidelity. This observation frames the question of which PDE best describes the data at hand. This question is particularly compelling because identification of the closest representation to the true PDE, while constrained by the functional spaces considered relative to the data at hand, immediately delivers insights to the physics underlying the systems. While building on recent work that uses stepwise regression, we present advances that leverage the variational framework and statistical tests. We also address the influences of variable fidelity and noise in the data.

physics.comp-ph↗

Generation of optical frequency comb in a chi-2 sheet micro optical parametric oscillator via cavity phase matching

Chi-3 micro resonators have enabled compact and portable frequency comb generation, but require sophisticated dispersion control. Here we demonstrate an alternative approach using a chi-2 sheet cavity, where the dispersion requirement is relaxed by cavity phase matching. 21.2 THz broadband comb generation is achieved with uniform line spacing of 133.0 GHz, despite a relatively large dispersion of 275.4 fs^2/mm around 1064nm. With 22.6 % high slope efficiency and 14.9 kW peak power handling, this chi-2 comb can be further stabilized for navigation, telecommunication, astronomy, and spectroscopy applications.

physics.optics↗

Experimental identification of critical condition for drastically enhancing thermoelectric power factor of two-dimensional layered materials

Nano-structuring is an extremely promising path to high performance thermoelectrics. Favorable improvements in thermal conductivity are attainable in many material systems, and theoretical work points to large improvements in electronic properties. However, realization of the electronic benefits in practical materials has been elusive experimentally. A key challenge is that experimental identification of the quantum confinement length, below which the thermoelectric power factor is significantly enhanced, remains elusive due to lack of simultaneous control of size and carrier density. Here we investigate gate tunable and temperature-dependent thermoelectric transport in $γ$ phase indium selenide ($γ$ InSe, n type semiconductor) samples with thickness varying from 7 to 29 nm. This allows us to properly map out dimension and doping space. Combining theoretical and experimental studies, we reveal that the sharper pre-edge of the conduction-band density of states arising from quantum confinement gives rise to an enhancement of the Seebeck coefficient and the power factor in the thinner InSe samples. Most importantly, we experimentally identify the role of the competition between quantum confinement length and thermal de Broglie wavelength in the enhancement of power factor. Our results provide an important and general experimental guideline for optimizing the power factor and improving the thermoelectric performance of two-dimensional layered semiconductors.

cond-mat.mes-hall↗

Optical Lattices with Higher-order Exceptional Points by Non-Hermitian Coupling

Exceptional points (EPs) are degeneracies in open wave systems with coalescence of at least two energy levels and their corresponding eigenstates. In higher dimensions, more complex EP physics not found in two-state systems is observed. We consider the emergence and interaction of multiple EPs in a four coupled optical waveguides system by non-Hermitian coupling showing a unique EP formation pattern in a phase diagram. In addition, absolute phase rigidities are computed to show the mixing of the different states in definite parameter regimes. Our results could be potentially important for developing further understanding of EP physics in higher dimensions via generalized paradigm of nonHermitian coupling for a new generation of parity-time (PT) devices.

physics.optics↗

Low-Temperature Eutectic Synthesis of PtTe2 with Weak Antilocalization and Controlled Layer Thinning

Metallic transition metal dichalcogenides (TMDs) have exhibited various exotic physical properties and hold the promise of novel optoelectronic and topological devices applications. However, the synthesis of metallic TMDs is based on gas-phase methods and requires high temperature condition. As an alternative to the gas-phase synthetic approach, lower temperature eutectic liquid-phase synthesis presents a very promising approach with the potential for larger-scale and controllable growth of high-quality thin metallic TMDs single crystals. Herein, we report the first realization of low-temperature eutectic liquid-phase synthesis of type-II Dirac semimetal PtTe2 single crystals with thickness ranging from 2 to 200 nm. The electrical measurement of synthesized PtTe2 reveals a record-high conductivity of as high as 3.3*106 S/m at room temperature. Besides, we experimentally identify the weak antilocalization behavior in the type-II Dirac semimetal PtTe2 for the first time. Furthermore, we develop a simple and general strategy to obtain atomically-thin PtTe2 crystal by thinning as-synthesized bulk samples, which can still retain highly crystalline and exhibits excellent electric conductivity. Our results of controllable and scalable low-temperature eutectic liquid-phase synthesis and layer-by-layer thinning of high-quality thin PtTe2 single crystals offer a simple and general approach for obtaining different thickness metallic TMDs with high-melting point transition metal.

cond-mat.mtrl-sci↗

A multi-physics battery model with particle scale resolution of porosity evolution driven by intercalation strain and electrolyte flow

We present a coupled continuum formulation for the electrostatic, chemical, thermal, mechanical and fluid physics in battery materials. Our treatment is at the particle scale, at which the active particles held together by carbon-binders, the porous separator, current collectors and the perfusing electrolyte are explicitly modeled. Starting with the description common to the field, in terms of reaction-transport partial differential equations for ions, variants of the classical Poisson equation for electrostatics, and the heat equation, we introduce solid-fluid interaction to the problem. Our main contribution is to model the electrolyte as an incompressible fluid driven by elastic, thermal and lithium intercalation strains in the active material. Our treatment is in the finite strain setting, and uses the Arbitrary Lagrangian-Eulerian (ALE) framework to account for mechanical coupling of the solid and fluid. We present a detailed computational study of the influence of solid-fluid interaction and magnitude of intercalation strain upon porosity evolution, ion distribution and electrostatic potential fields in the cell.

physics.comp-ph↗

Analog Circuit Applications based on Ambipolar Graphene/MoTe2 Vertical Transistors

The current integrated circuit (IC) technology based on conventional MOS-FET (metal-oxide-semiconductor field-effect transistor) is approaching the limit of miniaturization with increasing demand on energy. Several analog circuit applications based on graphene FETs have been demonstrated with less components comparing to the conventional technology. However, low on/off current ratio caused by the semimetal nature of graphene has severely hindered its practical applications. Here we report a graphene/MoTe2 van der Waals (vdW) vertical transistor with V-shaped ambipolar field effect transfer characteristics to overcome this challenge. Investigations on temperature dependence of transport properties reveal that gate tunable asymmetric barriers of the devices are account for the ambipolar behaviors. Furthermore, to demonstrate the analog circuit applications of such vdW vertical transistors, we successfully realized output polarity controllable (OPC) amplifier and frequency doubler. These results enable vdW heterojunction based electronic devices to open up new possibilities for wide perspective in telecommunication field.

cond-mat.mes-hall↗

Optimal double resonant condition in metallic core-shell nanocavity for third harmonic generation

As the rapid development of nonlinear optics, the enhancement of optical third harmonic generation becomes a pop research realm in the fields of physics, chemistry, biology, materials science, information science and other fields. In this letter, theoretical analysis on double resonance situation in metallic core-shell nanostructure is performed in order to optimize the efficiency of third harmonic generation. As plenty of cavity modes ranging from visible area to near infrared can be excited efficiently in core-shell nanospheres, kinds of double resonant conditions can be formed by matching two different multipolar cavity modes. Numerical simulations show that the third harmonic generation (THG) intensity in the far field can be enhanced remarkably when the THG signal couples well with the high order cavity mode. More importantly, THG efficiency is optimum from the cavity on double resonant conditions coupling two modes with the same order. The THG intensity differs up to 3 magnitudes on this condition. Subsequent theoretical analysis indicates that changing third-order nonlinear susceptibility of the metal shell while keeping that of the core fixed has almost no effect on THG efficiency. This finding about optimal double resonance has an appreciable effect on optimizing THG in spherical cavity structures.

physics.optics↗

Tunable hyperbolic metamaterial cavity towards few exciton strong coupling

We theoretically investigate coupling interaction between molecule excitons and whispering gallery modes (WGMs) that approaches the limit of single exciton strong coupling in hyperbolic metamaterial (HMM) cavity, composed of a dielectric core wrapped by several stacks of alternative layers of metal and dielectric. We demonstrate that associated with the excitation of the whispering gallery mode, the electric fields with resonance wavelengths that are much larger than the cavity size can be highly localized within a dielectric layer, leading to extremely small mode volumes. By using temporal coupled mode theory to model the interaction in the proposed WGMs-exciton system, we are able to demonstrate that the coupling between molecular excitons and hyperbolic cavity WGMs can reach the strong coupling regime. Furthermore, we also prove that changing both the thickness of inner core and outermost layer can lead to invariant resonance frequency while the threshold number of coupled excitons to fulfill the criteria for strong coupling remains ~ 4 in various sets of tunable HMM cavities.

physics.optics↗