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Zhenzhong Shi

Publications and source records attributed to Zhenzhong Shi.

18 recordsLinked to original sources
arXiv2025

The Future of the Correlated Electron Problem

A central problem in modern condensed matter physics is the understanding of materials with strong electron correlations. Despite extensive work, the essential physics of many of these systems is not understood and there is very little ability to make predictions in this class of materials. In this manuscript we share our personal views on the major open problems in the field of correlated electron systems. We discuss some possible routes to make progress in this rich and fascinating field. This manuscript is the result of the vigorous discussions and deliberations that took place at Johns Hopkins University during a three-day workshop January 27, 28, and 29, 2020 that brought together six senior scientists and 46 more junior scientists. Our hope, is that the topics we have presented will provide inspiration for others working in this field and motivation for the idea that significant progress can be made on very hard problems if we focus our collective energies.

cond-mat.str-el↗
arXiv2022

Beyond Single Tetrahedron Physics of Breathing Pyrochlore Compound Ba3Yb2Zn5O11

Recently a new class of quantum magnets, the so-called breathing pyrochlore spin systems, have attracted much attention due to their potential to host exotic emergent phenomena. Here, we present magnetometry, heat capacity, thermal conductivity, Muon-spin relaxation, and polarized inelastic neutron scattering measurements performed on high-quality single-crystal samples of breathing pyrochlore compound Ba3Yb2Zn5O11. We interpret these results using a simplified toy model and provide a new insight into the low-energy physics of this system beyond the single-tetrahedron physics proposed previously.

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arXiv2021

Realization of Quantum Dipoles in Triangular Lattice Crystal Ba3Yb(BO3)3

We investigate the thermodynamic properties of the ytterbium-based triangular lattice compound Ba3Yb(BO3)3. The results demonstrate the absence of any long-range ordering down to 56 mK. Analysis of the magnetization, susceptibility and specific heat measurements suggests that Ba3Yb(BO3)3 may realize a S = 1/2 quantum dipole lattice, in which the dominant interaction is the long range dipole-dipole coupling on the geometrically frustrated triangular lattice, and exchange interactions are subdominant or negligible.

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arXiv2021

Towards understanding the magnetic properties of the breathing pyrochlore compound Ba3Yb2Zn5O11: A single crystal study

Ba3Yb2Zn5O11 is unique among breathing pyrochlore compounds for being in the nearly decoupled limit where inter-tetrahedron interactions are weak, hosting isolated clusters or "molecular magnet" like tetrahedra of magnetic ytterbium (Yb3+) ions. In this work, we present the first study carried out on single-crystal samples of the breathing pyrochlore Ba3Yb2Zn5O11, using a variety of magnetometry and neutron scattering techniques along with theoretical modeling. We employ inelastic neutron scattering to investigate the magnetic dynamics as a function of applied field (with respect to both magnitude and direction) down to a temperature of 70 mK, where inelastic scattering reveals dispersionless bands of excitations as found in earlier powder sample studies, in good agreement with a single-tetrahedron model. However, diffuse neutron scattering at zero field and dc-susceptibility at finite field exhibit features suggesting the presence of excitations at low-energy that are not captured by the single tetrahedron model. Analysis of the local structure down to 2 K via pair distribution function analysis finds no evidence of structural disorder. We conclude that effects beyond the single tetrahedron model are important in describing the low-energy, low temperature physics of Ba3Yb2Zn5O11, but their nature remains undetermined.

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arXiv2021

Magnetic field reveals vanishing Hall response in the normal state of stripe-ordered cuprates

The origin of the weak insulating behavior of the resistivity, i.e. $ρ_{xx}\propto\ln(1/T)$, revealed when magnetic fields ($H$) suppress superconductivity in underdoped cuprates has been a longtime mystery. Surprisingly, the high-field behavior of the resistivity observed recently in charge- and spin-stripe-ordered La-214 cuprates suggests a metallic, as opposed to insulating, high-field normal state. Here we report the vanishing of the Hall coefficient in this field-revealed normal state for all $T<(2-6)T_{\mathrm{c}}^{0}$, where $T_{\mathrm{c}}^{0}$ is the zero-field superconducting transition temperature. Our measurements demonstrate that this is a robust fundamental property of the normal state of cuprates with intertwined orders, exhibited in the previously unexplored regime of $T$ and $H$. The behavior of the high-field Hall coefficient is fundamentally different from that in other cuprates such as YBa$_2$Cu$_3$O$_{6+x}$ and YBa$_2$Cu$_4$O$_{8}$, and may imply an approximate particle-hole symmetry that is unique to stripe-ordered cuprates. Our results highlight the important role of the competing orders in determining the normal state of cuprates.

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arXiv2021

Phase diagram of the Shastry-Sutherland Compound SrCu2(BO3)2 under extreme combined conditions of field and pressure

Motivated by the intriguing properties of the Shastry-Sutherland compound SrCu2(BO3)2 under pressure, with a still debated intermediate plaquette phase appearing at around 20 kbar and a possible deconfined critical point at higher pressure upon entering the antiferromagnetic phase, we have investigated its high-field properties in this pressure range using tunnel diode oscillator (TDO) measurements. The two main new phases revealed by these measurements are fully consistent with those identified by infinite Projected Entangled Pair states (iPEPS) calculations of the Shastry-Sutherland model, a 1/5 plateau and a 10 x 2 supersolid. Remarkably, these phases are descendants of the full-plaquette phase, the prominent candidate for the intermediate phase of SrCu2(BO3)2. The emerging picture for SrCu2(BO3)2 is shown to be that of a system dominated by a tendency to an orthorhombic distortion at intermediate pressure, an important constraint on any realistic description of the transition into the antiferromagnetic phase.

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arXiv2021

Phase Diagram of YbZnGaO4 in Applied Magnetic Field

Recently, Yb-based triangular lattice antiferromagnets have garnered significant interest as possible quantum spin liquid candidates. One example is YbMgGaO4, which showed many promising spin liquid features, but also possesses a high degree of disorder owing to site-mixing between the non-magnetic cations. To further elucidate the role of chemical disorder and to explore the phase diagram of these materials in applied field, we present neutron scattering and sensitive magnetometry measurements of the closely related compound, YbZnGaO4. Our results suggest a difference in magnetic anisotropy between the two compounds, and we use key observations of the magnetic phase crossover to motivate an exploration of the field- and exchange parameter-dependent phase diagram, providing an expanded view of the available magnetic states in applied field. This enriched map of the phase space serves as a basis to restrict the values of parameters describing the magnetic Hamiltonian with broad application to recently discovered related materials.

cond-mat.str-el↗
arXiv2020

Incommensurate two-dimensional checkerboard charge density wave in the low dimensional superconductor Ta4Pd3Te16

We report the observation of a two-dimensional (2D) checkerboard charge density wave (CDW) in the low-dimensional superconductor Ta4Pd3Te16. By determining its CDW properties across the temperature-pressure (T-P) phase diagram and comparing with prototypical CDW materials, we conclude that Ta4Pd3Te16 features: a) an incommensurate CDW with a mixed character of dimensions (Q1D considering its needle-like shape along the b-axis, Q2D as the CDW has checkerboard wavevectors, and 3D because of CDW projections along all three axes); and b) one of the weakest CDWs compared to its superconductivity (SC), i.e. enhanced SC with respect to CDW, suggesting an interesting interplay of the two orders.

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arXiv2020

Constraining the Parameter Space of a Quantum Spin Liquid Candidate in Applied Field with Iterative Optimization

The quantum spin liquid (QSL) state is an exotic state of matter featuring a high degree of entanglement and lack of long-range magnetic order in the zero-temperature limit. The triangular antiferromagnet YbMgGaO4 is a candidate QSL host, and precise determination of the Hamiltonian parameters is critical to understanding the nature of the possible ground states. However, the presence of chemical disorder has made directly measuring these parameters challenging. Here we report neutron scattering and magnetic susceptibility measurements covering a broad range of applied magnetic field at low temperature. Our data shows a field-induced crossover in YbMgGaO4, which we reproduce with complementary classical Monte Carlo and Density Matrix Renormalization Group simulations. Neutron scattering data above and below the crossover reveal a shift in scattering intensity from M to K points and, collectively, our measurements provide essential characteristics of the phase crossover that we employ to strictly constrain proposed magnetic Hamiltonian parameters despite the chemical disorder. Constrained exchange parameters further suggest the material's proximity to the QSL state in the clean limit. More broadly, our approach demonstrates a means of pursuing QSL candidates where Hamiltonian parameters might otherwise be obscured by disorder.

cond-mat.str-el↗
arXiv2020

Unveiling the phase diagram of a striped cuprate at high magnetic fields: Hidden order of Cooper pairs

The interplay of charge orders with superconductivity in underdoped cuprates at high magnetic fields ($H$) is an open question, and even the value of the upper critical field ($H_{c2}$), a measure of the strength of superconductivity, has been the subject of a long-term debate. We combined three complementary transport techniques on underdoped La$_{1.8-x}$Eu$_{0.2}$Sr$_{x}$CuO$_{4}$ with a "striped" charge order and a low $H=0$ transition temperature $T_{c}^{0}$, to establish the $T-H$ phase diagram and reveal the ground states in CuO$_2$ planes: a superconductor, a wide regime of superconducting phase fluctuations (i.e. a vortex liquid), and a high-field normal state. The relatively high $H_{c2}$ is consistent with the opening of a superconducting gap above $T_{c}^{0}$, but only at $T\sim (2$-$3)T_{c}^{0}$, an order of magnitude below the pseudogap temperature. Within the vortex liquid, an unanticipated, insulatinglike region, but with strong superconducting correlations, begins to emerge already at $T\lesssim T_{c}^{0}$. The results suggest that the presence of stripes plays a crucial role in the freezing of Cooper pairs in this novel state. Our findings provide a fresh perspective on the pairing strength in underdoped cuprates, and introduce a new avenue for exploring the interplay of various orders.

cond-mat.supr-con↗
arXiv2020

Signatures of a pair density wave at high magnetic fields in cuprates with charge and spin orders

In underdoped cuprates, the interplay of the pseudogap, superconductivity, and charge and spin ordering can give rise to exotic quantum states, including the pair density wave (PDW), in which the superconducting (SC) order parameter is oscillatory in space. However, the evidence for a PDW state remains inconclusive and its broader relevance to cuprate physics is an open question. To test the interlayer frustration, the crucial component of the PDW picture, we performed transport measurements on La$_{1.7}$Eu$_{0.2}$Sr$_{0.1}$CuO$_{4}$ and La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_{4}$, cuprates with "striped" spin and charge orders, in perpendicular magnetic fields ($H_\perp$), and also with an additional field applied parallel to CuO$_2$ layers ($H_\parallel$). We detected several phenomena predicted to arise from the existence of a PDW, including an enhancement of interlayer SC phase coherence with increasing $H_\parallel$. Our findings are consistent with the presence of local, PDW pairing correlations that compete with the uniform SC order at $T_{c}^{0}< T<(2-6) T_{c}^{0}$, where $T_{c}^{0}$ is the $H=0$ SC transition temperature, and become dominant at intermediate $H_\perp$ as $T\rightarrow 0$. These data also provide much-needed transport signatures of the PDW in the regime where superconductivity is destroyed by quantum phase fluctuations.

cond-mat.supr-con↗
arXiv2019

Vortex phase diagram and the normal state of cuprates with charge and spin orders

The phase diagram of underdoped cuprates in a magnetic field ($H$) is the key ingredient in understanding the anomalous normal state of these high-temperature superconductors. However, the upper critical field ($H_{c2}$) or the extent of superconducting phase with vortices, a type of topological excitations, and the role of charge orders that are present at high $H$, remain under debate. We address these questions by studying stripe-ordered La-214, i.e. cuprates in which charge orders are most pronounced and zero-field transition temperatures $T_{c}^{0}$ are lowest; the latter opens a much larger energy scale window to explore the vortex phases compared to previous studies. By combining linear and nonlinear transport techniques sensitive to vortex matter, we determine the $T$-$H$ phase diagram, directly detect $H_{c2}$, and reveal novel properties of the high-field ground state. Our results demonstrate that, while the vortex phase diagram of underdoped cuprates is not very sensitive to the details of the charge orders, quantum fluctuations and disorder play a key role as $T\rightarrow 0$. The presence of stripes, on the other hand, seems to alter the nature of the anomalous normal state, such that the high-field ground state is a metal, as opposed to an insulator.

cond-mat.supr-con↗
arXiv2018

Emergent Bound States and Impurity Pairs in Chemically Doped Shastry-Sutherland System

The search for novel unconventional superconductors is a central topic of modern condensed matter physics. Similar to other Mott insulators, Shastry-Sutherland (SSL) systems are predicted to become superconducting when chemically doped. This makes SrCu2(BO3)2, an experimental realization of SSL model, a suitable candidate and understanding of the doping effects in it very important. Here we report doping-induced emergent states in Mg-doped SrCu2(BO3)2, which remain stable up to high magnetic fields. Using four complementary magnetometry techniques and theoretical simulations, a rich impurity-induced phenomenology at high fields is discovered. The results demonstrate a rare example in which even a small doping concentration interacts strongly with both triplets and bound states of triplets, and thus plays a significant role in the magnetization process even at high magnetic fields. Moreover, our findings of the emergence of the very stable impurity pairs provide insights into the anticipated unconventional superconductivity in SrCu2(BO3)2 and related materials.

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arXiv2016

Current-voltage characteristics and vortex dynamics in highly underdoped La$_{2-x}$Sr$_{x}$CuO$_{4}$

The temperature dependence of the nonlinear current-voltage ($I$-$V$) characteristics in highly underdoped La$_{2-x}$Sr$_{x}$CuO$_{4}$ ($x=0.07$ and 0.08) thick films has been studied in both zero and perpendicular magnetic fields $H$. Power-law behavior of $V(I)$ is found for both $H=0$ and $H \neq 0$. The critical current $I_{c}$ was extracted, and its temperature and magnetic field dependences were studied in detail. The Berezinskii-Kosterlitz-Thouless physics dominates the nonlinear $I$-$V$ near the superconducting transition at $H=0$, and it continues to contribute up to a characteristic temperature $T_x(H)$. Nonlinear $I$-$V$ persists up to an even higher temperature $T_{h}(H)$ due to the depinning of vortices.

cond-mat.supr-con↗
arXiv2016

Effective 2D thickness for the Berezinskii-Kosterlitz-Thouless-like transition in a highly underdoped La$_{2-x}$Sr$_x$CuO$_4$

The nature of the superconducting transition in highly underdoped thick films of La$_{2-x}$Sr$_x$CuO$_4$ ($x=0.07$ and 0.08) has been investigated using the in-plane transport measurements. The contribution of superconducting fluctuations to the conductivity in zero magnetic field, or paraconductivity, was determined from the magnetoresistance measured in fields applied perpendicular to the CuO$_2$ planes. Both the temperature dependence of the paraconductivity above the transition and the nonlinear current-voltage ($I-V$) characteristics measured across it, exhibit the main signatures of the Berezinskii-Kosterlitz-Thouless (BKT) transition. The quantitative comparison of the superfluid stiffness, extracted from the $I-V$ data, with the renormalization-group results for the BKT theory, reveals a large value of the vortex-core energy. This finding is confirmed by the analysis of the paraconductivity obtained using different methods. The results strongly suggest that the characteristic energy scale controlling the BKT behavior in this layered system corresponds to the superfluid stiffness of a few layers.

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arXiv2015

Proliferation of metallic domains caused by inhomogeneous heating near the electrically-driven transition in VO$_2$ nanobeams

We discuss the mechanisms behind the electrically driven insulator-metal transition in single crystalline VO$_2$ nanobeams. Our DC and AC transport measurements and the versatile harmonic analysis method employed show that non-uniform Joule heating causes phase inhomogeneities to develop within the nanobeam and is responsible for driving the transition in VO$_{2}$. A Poole-Frenkel like purely electric field induced transition is found to be absent and the role of percolation near and away from the electrically driven transition in VO$_{2}$ is also identified. The results and the harmonic analysis can be generalized to many strongly correlated materials that exhibit electrically driven transitions.

cond-mat.str-el↗
arXiv2014

Non-monotonic resistance noise in the charge density wave pinned state in single nanoribbons of CDW conductor NbSe$_{3}$

Electrical transport and broadband resistance noise measurements in an ultra low frequency window (30 mHz - 8 Hz) are carried out in single nanoribbon devices of charge density wave (CDW) conductor NbSe$_{3}$. In the temperature and electric field range where the CDW is expected to be completed pinned by residual impurities, a hitherto unseen non-monotonic behavior in the noise magnitude vs. electric field is observed. This behavior can be attributed to the proliferation of thermally activated phase slip events and this idea is supported by the observation of a smeared activated behavior described by the Dutta-Horn relation. Certain features of the temperature dependence of the noise magnitude do not follow an activated behavior pointing to a complex origin of the fluctuations in a CDW system.

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