arXiv subjects

Zheru Qiu

Publications and source records attributed to Zheru Qiu.

18 recordsLinked to original sources

arXiv2026

A fully integrated dispersion-managed femtosecond mode-locked laser

Femtosecond lasers underpin applications ranging from material processing to corneal surgery, while their regular pulse trains form optical frequency combs that have revolutionized timekeeping, spectroscopy, and metrology. On-chip optical frequency combs, such as Kerr microcombs, have enabled high-repetition-rate applications in optical communications and microwave photonics. However, integrated chip-scale sources operating at low repetition rates (100 MHz to 1 GHz), crucial for high peak intensities, remain elusive, as existing devices typically operate well beyond 10 GHz. Here, we demonstrate a self-starting, photonic integrated mode-locked laser based on a dispersion-managed architecture that accesses this regime. The laser combines erbium-implanted silicon nitride gain waveguides, integrated chirped Bragg gratings, and a semiconductor saturable absorber mirror to generate optical pulses with repetition rates from 0.5 to 1.2 GHz, pulse durations as short as 300 fs, and mode-locking thresholds down to 27.3 mW. The output forms a passively stable optical frequency comb with a comb-line drift below 1% of the repetition rate, surpassing the stability of commercial fiber lasers by two orders of magnitude. Leveraging this ultra-low threshold, we achieve complete hybrid integration by co-packaging the laser with a telecom-grade 980-nm III-V pump diode chip inside a compact photonic module. The resulting electrical-in/optical-out module delivers turnkey, stable mode-locked pulses, providing a compact, low-power, and vibration-insensitive foundry-compatible platform for field-deployable optical metrology and precision sensing.

physics.optics↗

arXiv2025

High-pulse-energy integrated mode-locked lasers based on a Mamyshev oscillator

Ultrafast lasers have unlocked numerous advances across science and technology: they enable corneal surgery, reveal chemical reaction dynamics, and underpin optical atomic clocks. Over the past decades, extensive efforts have been devoted to developing photonic integrated circuit-based mode-locked lasers that are compact, scalable, and compatible with further on-chip functionalities. Yet, existing implementations fall short of pulse energies required for their subsequent uses in nonlinear applications. In this work, we demonstrate the first mode-locked laser that overcomes this limitation in low-loss erbium-doped silicon nitride photonic integrated circuits. The laser is based on the Mamyshev oscillator architecture, which employs alternating spectral filtering and self-phase modulation for mode-locking. It delivers a 176 MHz stream of pulses with nanojoule energy, comparable to fiber lasers and surpassing previous photonic integrated sources by more than two orders of magnitude. The output pulses exhibit excellent coherence, can be linearly compressed to 147 fs and directly drive a 1.5-octave-spanning supercontinuum in an integrated waveguide. Our work establishes a new generation of high-pulse-energy photonic integrated mode-locked lasers and paves the way for their widespread adoption.

physics.optics↗

arXiv2025

Copper-impurity-free photonic integrated circuits enable deterministic soliton microcombs

Chip-scale optical frequency combs based on microresonators (microcombs) enable GHz-THz repetition rates, broad bandwidth, compactness, and compatibility with wafer-scale manufacturing. Silicon nitride photonic integrated circuits have become a leading platform due to their low loss, broad transparency, lithographic dispersion control, and commercial 200-mm-wafer foundry access. They have enabled system-level applications in optical communications, LiDAR, frequency synthesis, low-noise microwave generation, and convolutional processing. However, real-world deployment is hindered by the challenge of deterministic soliton microcomb generation, primarily due to thermal instabilities. Although techniques like pulsed pumping, fast scanning, and auxiliary lasers help mitigate these effects, they often add complexity or reduce soliton stability. In this work, we overcome thermal limitations and demonstrate deterministic soliton generation in silicon nitride photonic circuits. We trace the thermal effects to copper impurities within waveguides, originating from residual contaminants in CMOS-grade silicon wafers that are gettered into silicon nitride during fabrication. By developing effective copper removal techniques, we significantly reduce thermal instabilities. This enables soliton generation with arbitrary or slow laser scanning, removing a key barrier to microcomb deployment. Our approach is compatible with front-end-of-line foundry processing, paving the way for broader adoption of soliton microcomb technologies.

physics.optics↗

arXiv2025

Full C- and L-band tunable erbium-doped integrated lasers via scalable manufacturing

Erbium (Er) ions are the gain medium of choice for fiber-based amplifiers and lasers, offering a long excited-state lifetime, slow gain relaxation, low amplification nonlinearity and noise, and temperature stability compared to semiconductor-based platforms. Recent advances in ultra-low-loss silicon nitride (Si$_3$N$_4$) photonic integrated circuits, combined with ion implantation, have enabled the realization of high-power on-chip Er amplifiers and lasers with performance comparable to fiber-based counterparts, supporting compact photonic systems. Yet, these results are limited by the high (2 MeV) implantation beam energy required for tightly confined Si$_3$N$_4$ waveguides (700 nm height), preventing volume manufacturing of Er-doped photonic integrated circuits. Here, we overcome these limitations and demonstrate the first fully wafer-scale, foundry-compatible Er-doped photonic integrated circuit-based tunable lasers. Using 200 nm-thick Si$_3$N$_4$ waveguides, we reduce the ion beam energy requirement to below 500 keV, enabling efficient wafer-scale implantation with an industrial 300 mm ion implanter. We demonstrate a laser wavelength tuning range of 91 nm, covering nearly the entire optical C- and L-bands, with fiber-coupled output power reaching 36 mW and an intrinsic linewidth of 95 Hz. The temperature-insensitive properties of erbium ions allowed stable laser operation up to 125$^{\circ}$C and lasing with less than 15 MHz drift for over 6 hours at room temperature using a remote fiber pump. The fully scalable, low-cost fabrication of Er-doped waveguide lasers opens the door for widespread adoption in coherent communications, LiDAR, microwave photonics, optical frequency synthesis, and free-space communications.

physics.optics↗

arXiv2025

Terabit-class coherent communications enabled by an integrated photonics erbium doped amplifier

Coherent technologies have revolutionized optical communications, driving the capacity per fiber to multi-terabit per second (Tb/s) in combination with wavelength division multiplexing (WDM). With an ever-increasing deployment density of coherent systems, the demand for highly integrated WDM coherent transceivers has been rising. While tremendous progress has been made on silicon photonics compatible high-speed modulation and photodetection on chip, a solution for monolithically integrable amplifier with high gain and output power remains a challenge. Recently, an erbium doped waveguide amplifier based on ultra-low loss silicon nitride waveguides has demonstrated gain and output power levels potentially suitable for Terabit class coherent communications. Here, we demonstrate a WDM coherent system enabled by this integrated photonic amplification solution. The system uses the waveguide amplifier as a booster amplifier of 16 WDM signals each carrying a net data rate of 1.6 Tb/s, achieving 25.6-Tb/s net capacity over 81-km fiber transmission. Our results highlight a fully integrated solution for highly parallel coherent transceivers including amplification, that has the potential to transform future optical communications.

physics.optics↗

arXiv2024

Electrons herald non-classical light

Free electrons are a widespread and universal source of electromagnetic fields. The past decades witnessed ever-growing control over many aspects of electron-generated radiation, from the incoherent emission produced by X-ray tubes to the exceptional brilliance of free-electron lasers. Reduced to the elementary process of quantized energy exchange between individual electrons and the electromagnetic field, electron beams may facilitate future sources of tunable quantum light. However, the quantum features of such radiation are tied to the correlation of the particles, calling for the joint electronic and photonic state to be explored for further applications. Here, we demonstrate the coherent parametric generation of non-classical states of light by free electrons. We show that the quantized electron energy loss heralds the number of photons generated in a dielectric waveguide. In Hanbury-Brown-Twiss measurements, an electron-heralded single-photon state is revealed via antibunching intensity correlations, while two-quantum energy losses of individual electrons yield pronounced two-photon coincidences. The approach facilitates the tailored preparation of higher-number Fock and other optical quantum states based on controlled interactions with free-electron beams.

quant-ph↗

arXiv2024

Ultrafast tunable photonic integrated Pockels extended-DBR laser

Frequency-agile lasers that can simultaneously feature low noise characteristics as well as fast mode hop-free frequency tuning are keystone components for applications ranging from frequency modulated continuous wave (FMCW) LiDAR, to coherent optical communication and gas sensing. The hybrid integration of III-V gain media with low-loss photonic integrated circuits (PICs) has recently enabled integrated lasers with faster tuning and lower phase noise than the best legacy systems, including fiber lasers. In addition, lithium niobate on insulator (LNOI) PICs have enabled to exploit the Pockels effect to demonstrate self-injection locked hybrid lasers with tuning rates reaching peta-hertz per second. However, Pockels-tunable laser archetypes relying on high-Q optical microresonators have thus far only achieved limited output powers, are difficult to operate and stabilize due to the dynamics of self-injection locking, and require many analog control parameters. Here, we overcome this challenge by leveraging an extended distributed Bragg reflector (E-DBR) architecture to demonstrate a simple and turn-key operable frequency-agile Pockels laser that can be controlled with single analog operation and modulation inputs. Our laser supports a continuous mode hop-free tuning range of over 10 GHz with good linearity and flat actuation bandwidth up to 10 MHz, while achieving over 15 mW in-fiber output power at 1545 nm and kHz-level intrinsic linewidth, a combination unmet by legacy bulk lasers. This hybrid laser design combines an inexpensive reflective semiconductor optical amplifier (RSOA) with an electro-optic DBR PIC manufactured at wafer-scale on a LNOI platform. We showcase the performance and flexibility of this laser in proof-of-concept coherent optical ranging (FMCW LiDAR) demonstration, achieving a 4 cm distance resolution and in a hydrogen cyanide spectroscopy experiment.

physics.optics↗

arXiv2024

Foundry compatible, efficient wafer-scale manufacturing of ultra-low loss, high-density Si$_3$N$_4$ photonic integrated circuits

Silicon nitride (Si$_3$N$_4$) photonic integrated circuits (PICs) have shown low linear loss, negligible nonlinear loss, and high power handling over traditional silicon photonics. To achieve high-density photonic integration and high effective nonlinearity through tight optical confinement, thick stoichiometric Si$_3$N$_4$ films are indispensable. However, when using low-pressure chemical vapor deposition (LPCVD) to achieve high optical material transparency, Si$_3$N$_4$ films exhibit large tensile stress on the order of GPa. Methods for crack prevention are therefore essential. The photonic Damascene process has addressed this issue, attaining record low loss Si$_3$N$_4$ PICs, but it lacks control of the waveguide height. Conversely, precise waveguide dimension and ultra-low loss have been achieved with subtractive processing, but this method is not compatible with mass production due to the use of electron beam lithography. To date, an outstanding challenge is to attain both lithographic precision and ultra-low loss in high confinement Si$_3$N$_4$ PICs that are compatible with large-scale foundry manufacturing. Here, we present a single-step deposited, DUV-based subtractive method for producing wafer-scale ultra-low loss Si$_3$N$_4$ PICs that harmonize these necessities. By employing deep etching of densely distributed, interconnected trenches into the substrate, we effectively mitigate the tensile stress in the Si$_3$N$_4$ layer, enabling direct deposition of thick films without cracking and substantially prolonged storage duration. Lastly, we identify ultraviolet (UV) radiation-induced damage that can be remedied through rapid thermal annealing. Collectively, we develop ultra-low loss Si$_3$N$_4$ microresonators and 0.5 m-long spiral waveguides with losses down to 1.4 dB/m at 1550 nm with high production yield.

physics.optics↗

arXiv2024

Hydrogen-free low-temperature silica for next generation integrated photonics

The advances in novel low-loss "on insulator" integrated photonics platforms beyond silicon, such as thin-film LiNbO3, LiTaO3, GaP and BaTiO3 have demonstrated major potential across a wide range of applications, due to their unique electro-optical or nonlinear optical properties. This has heralded novel devices, ranging from low-voltage and high-speed modulators to parametric amplifiers. For such photonic integrated circuits, a low-loss SiO2 cladding layer is a key element, serving as a passivation layer for the waveguides and enabling efficient fiber-to-chip coupling. However, numerous novel ferroelectric or III-V "on insulator" platforms have low tolerances for process temperature. This prohibits using high-temperature anneals to remove hydrogen, a common impurity that is inherent to ordinary chemical vapor deposited SiO2 and causes significant optical loss in the near infrared. Here, we satisfy the dichotomy of a low-loss wafer scale manufactured SiO2 cladding and low processing temperature. Inspired by the manufacturing of optical fibers, we introduce a hydrogen-free, low-loss SiO2 cladding that is deposited at low temperatures (300 degrees Celsius) by using SiCl4 and O2 as precursors in inductively coupled plasma-enhanced chemical vapor deposition (ICPCVD). By replacing hydrogenous silicon precursors (e.g. SiH4) with SiCl4, the deposited film is inherently free from residual hydrogen. The process temperature is compatible with the "on insulator" platforms and CMOS electronic integrated circuits. We demonstrate a wide low-loss window that covers all telecommunication bands from 1260 nm to 1625 nm. We achieve a < 2.5 dB/m waveguide loss at 1550 nm, comparable with 1200 degree Celsius annealed films. Our SiCl4 process provides a key future cladding for all recently emerged "on-insulator" photonics platforms, that is low cost, scalable in manufacturing, and directly foundry compatible.

physics.optics↗

arXiv2024

Large-scale photonic chip based pulse interleaver for low-noise microwave generation

Microwaves generated by optical techniques have demonstrated unprecedentedly low noise and hold significance in various applications such as communication, radar, instrumentation, and metrology. To date, the purest microwave signals are generated using optical frequency division with femtosecond mode-locked lasers. However, many femtosecond laser combs have a radio frequency (RF) repetition rate in the hundreds of megahertz range, necessitating methods to translate the generated low-noise RF signal to the microwave domain. Benchtop pulse interleavers can multiply the pulse repetition rate, avoid saturation of photodetectors, and facilitate the generation of high-power low-noise microwave signals, which have to date only been demonstrated using optical fibers or free space optics. Here, we introduce a large-scale photonic integrated circuit-based interleaver, offering size reduction and enhanced stability. The all-on-chip interleaver attains a 64-fold multiplication of the repetition rate, directly translated from 216 MHz to 14 GHz in microwave Ku-Band. By overcoming photodetector saturation, the generated microwave power was improved by 36 dB, with a phase noise floor reduced by more than 10 folds to -160 dBc/Hz on the 14 GHz carrier. The device is based on a low-loss and high-density photonic integrated circuit fabricated by the photonic Damascene process. Six cascaded stages of Mach-Zehnder interferometers with optical delay lines up to 33 centimeters long are fully integrated into a compact footprint of 8.5 mmx1.7 mm. The lithographically defined precision of the optical waveguide path length enables the scaling up of the interleaved frequency to millimeter-wave bands, which is challenging the fiber-based counterparts. This interleaver has the potential to reduce the cost and footprint of mode-locked-laser-based microwave generation, allowing for field deployment.

physics.optics↗

arXiv2023

Free-electron interaction with nonlinear optical states in microresonators

The short de Broglie wavelength and strong interaction empower free electrons to probe scattering and excitations in materials and resolve the structure of biomolecules. Recent advances in using nanophotonic structures to mediate bilinear electron-photon interaction have brought novel optical manipulation schemes to electron beams, enabling high space-time-energy resolution electron microscopy, quantum-coherent optical modulation, attosecond metrology and pulse generation, transverse electron wavefront shaping, dielectric laser acceleration, and electron-photon pair generation. However, photonic nanostructures also exhibit nonlinearities, which have to date not been exploited for electron-photon interactions. Here, we report the interaction of electrons with spontaneously generated Kerr nonlinear optical states inside a continuous-wave driven photonic chip-based microresonator. Optical parametric processes give rise to spatiotemporal pattern formation, or dissipative structures, corresponding to coherent or incoherent optical frequency combs. By coupling such microcombs in situ to electron beams, we demonstrate that different dissipative structures induce distinct fingerprints in the electron spectra and Ramsey-type interference patterns. In particular, using spontaneously formed femtosecond temporal solitons, we achieve ultrafast temporal gating of the electron beam without the necessity of a pulsed laser source or a pulsed electron source. Our work elucidates the interaction of free electrons with a variety of nonlinear dissipative states, demonstrates the ability to access solitons inside an electron microscope, and extends the use of microcombs to unexplored territories, with ramifications in novel ultrafast electron microscopy, light-matter interactions driven by on-chip temporal solitons, and ultra-high spatiotemporal resolution sampling of nonlinear optical dynamics and devices.

physics.optics↗

arXiv2023

Hertz-linewidth and frequency-agile photonic integrated extended-DBR lasers

Recent advances in the development of ultra-low loss silicon nitride (Si3N4)-based photonic integrated circuits have allowed integrated lasers to achieve a coherence exceeding those of fiber lasers and enabled unprecedentedly fast (Megahertz bandwidth) tuning using monolithically integrated piezoelectrical actuators. While this marks the first time that fiber laser coherence is achieved using photonic integrated circuits, in conjunction with frequency agility that exceeds those of legacy bulk lasers, the approach is presently compounded by the high cost of manufacturing DFB, as required for self-injection locking, as well as the precise control over the laser current and temperature to sustain a low noise locked operation. Reflective semiconductor optical amplifiers (RSOA) provide a cost-effective alternative solution but have not yet achieved similar performance in coherence or frequency agility, as required for frequency modulated continuous wave (FMCW) LiDAR, laser locking in frequency metrology or wavelength modulation spectroscopy for gas sensing. Here, we overcome this challenge and demonstrate an RSOA-based and frequency agile integrated laser tuned with high speed, good linearity, high optical output power, and turn-key operability while maintaining a small footprint. This is achieved using a tunable extended distributed Bragg reflector (E-DBR) in an ultra-low loss 200 nm thin Si3N4 platform with monolithically integrated piezoelectric actuators. We co-integrate the DBR with a compact ultra-low loss spiral resonator to further reduce the intrinsic optical linewidth of the laser to the Hertz level -- on par with the noise of a fiber laser -- via self-injection locking.

physics.optics↗

arXiv2023

Photonic-electronic integrated circuit-based coherent LiDAR engine

Microelectronic integration is a key enabler for the ubiquitous deployment of devices in large volumes ranging from MEMS and imaging sensors to consumer electronics. Such integration has also been achieved in photonics, where compact optical transceivers for data centers employ co-integrated photonic and electronic components. Chip-scale integration is of particular interest to coherent laser ranging i.e. frequency modulated continuous wave (FMCW LiDAR), a perception technology that benefits from instantaneous velocity and distance detection, eye-safe operation, long-range and immunity to interference. Full wafer-scale integration of this technology has been compounded by the stringent requirements on the lasers, requiring high optical coherence, low chirp nonlinearity and requiring optical amplifiers. Here, we overcome this challenge and demonstrate a photonic-electronic integrated circuit-based coherent LiDAR engine, that combined all functionalities using fully foundry-compatible wafer scale manufacturing. It is comprised of a micro-electronic based high voltage arbitrary waveform generator, a hybrid photonic circuit based tunable Vernier laser with piezoelectric actuators, and an erbium-doped waveguide optical amplifier - all realized in a wafer scale manufacturing compatible process that comprises III-V semiconductors, SiN silicon nitride photonic integrated circuits as well as 130nm SiGe BiCMOS technology. The source is a turnkey, linearization-free, and can serve as a 'drop-in' solution in any FMCW LiDAR, that can be seamlessly integrated with an existing focal plane and optical phased array LiDAR approaches, constituting a missing step towards a fully chip-scale integrated LiDAR system.

physics.app-ph↗

arXiv2023

A fully hybrid integrated Erbium-based laser

Erbium-doped fiber lasers exhibit high coherence and low noise as required for applications in fiber optic sensing, gyroscopes, LiDAR, and optical frequency metrology. Endowing Erbium-based gain in photonic integrated circuits can provide a basis for miniaturizing low-noise fiber lasers to chip-scale form factor, and enable large-volume applications. Yet, while major progress has been made in the last decade on integrated lasers based on silicon photonics with III-V gain media, the integration of Erbium lasers on chip has been compounded by large laser linewidth. Recent advances in photonic integrated circuit-based high-power Erbium-doped amplifiers, make a new class of rare-earth-ion-based lasers possible. Here, we demonstrate a fully integrated chip-scale Erbium laser that achieves high power, narrow linewidth, frequency agility, and the integration of a III-V pump laser. The laser circuit is based on an Erbium-implanted ultralow-loss silicon nitride Si$_3$N$4$ photonic integrated circuit. This device achieves single-mode lasing with a free-running intrinsic linewidth of 50 Hz, a relative intensity noise of $<$-150 dBc/Hz at $>$10 MHz offset, and output power up to 17 mW, approaching the performance of fiber lasers and state-of-the-art semiconductor extended cavity lasers. An intra-cavity microring-based Vernier filter enables wavelength tunability of $>$ 40 nm within the C- and L-bands while attaining side mode suppression ratio (SMSR) of $>$ 70 dB, surpassing legacy fiber lasers in tuning and SMRS performance. This new class of low-noise, tuneable Erbium waveguide laser could find applications in LiDAR, microwave photonics, optical frequency synthesis, and free-space communications. Our approach is extendable to other wavelengths, and more broadly, constitutes a novel way to photonic integrated circuit-based rare-earth-ion-doped lasers.

physics.optics↗

arXiv2022

A photonic integrated circuit based erbium-doped amplifier

Erbium-doped fiber amplifiers have revolutionized long-haul optical communications and laser technology. Erbium ions could equally provide a basis for efficient optical amplification in photonic integrated circuits. However, this approach has thus far remained impractical due to insufficient output power. Here, we demonstrate a photonic integrated circuit based erbium amplifier reaching 145 mW output power and more than 30 dB small-signal gain -- on par with commercial fiber amplifiers and beyond state-of-the-art III-V heterogeneously integrated semiconductor amplifiers. We achieve this by applying ion implantation to recently emerged ultralow-loss Si3N4 photonic integrated circuits with meter-scale-length waveguides. We utilize the device to increase by 100-fold the output power of soliton microcombs, required for low-noise photonic microwave generation or as a source for wavelength-division multiplexed optical communications. Endowing Si3N4 photonic integrated circuits with gain enables the miniaturization of a wide range of fiber-based devices such as high-pulse-energy femtosecond mode-locked lasers.

physics.optics↗

arXiv2021

Compact, spatial-mode-interaction-free, ultralow-loss, nonlinear photonic integrated circuits

Nonlinear photonics based on integrated circuits has enabled applications such as parametric amplifiers, soliton frequency combs, supercontinua, and non-reciprocal devices. Ultralow optical loss and the capability for dispersion engineering are essential, which necessitate the use of multi-mode waveguides. Despite that rich interaction among different spatial waveguide eigenmodes can give rise to novel nonlinear phenomena, spatial mode interaction is typically undesired as it increases optical loss, perturbs local dispersion profile, and impedes soliton formation. Adiabatic bends, such as Euler bends whose curvature varies linearly with their path length, have been favoured to suppress spatial mode interaction. Adiabatic bends can essentially connect any two waveguide segments with adiabatic mode conversion, thus efficiently avoid mode mixing due to mode mismatch. However, previous works lack quantitative measurement data and analysis to fairly evaluate the adiabaticity, and are not based on photonic integrated circuits with tight optical confinement and optical losses of few dB/m. Here, we adapt, optimize, and implement Euler bends to build compact racetrack microresonators based on ultralow-loss, multi-mode, silicon nitride photonic integrated circuits. The racetrack microresonators feature a small footprint of only 0.21 mm^2 for 19.8 GHz FSR. We quantitatively investigate the suppression of spatial mode interaction in the racetrack microresonators with Euler bends. We show that the optical loss rate (15.5 MHz) is preserved, on par with the mode interaction strength (25 MHz). This results in an unperturbed microresonator dispersion profile. We further demonstrate single soliton of 19.8 GHz repetition rate. The optimized Euler bends and racetrack microresonators can be key building blocks for integrated nonlinear photonic systems, programmable processors and photonic quantum computing.

physics.optics↗

arXiv2020

Herriott-cavity-assisted all-optical atomic vector magnetometer

We report an all-optical atomic vector magnetometer using dual Bell-Bloom optical pumping beams in a Rb vapor cell. This vector magnetometer consists of two orthogonal optical pumping beams, with amplitude modulations at $^{85}$Rb and $^{87}$Rb Larmor frequencies respectively. We simultaneously detect atomic signals excited by these two pumping beams using a single probe beam in the third direction, and extract the field orientation information using the phase delays between the modulated atomic signals and the driving beams. By adding a Herriott cavity inside the vapor cell, we improve the magnetometer sensitivity. We study the performance of this vector magnetometer in a magnetic field ranging from 100~mG to 500~mG, and demonstrate a field angle sensitivity better than 10~$μ$rad/Hz$^{1/2}$ above 10~Hz.

physics.atom-ph↗

arXiv2019

Interactions between non-resonant rf fields and atoms with strong spin-exchange collisions

We study the interactions between oscillating non-resonant rf fields and atoms with strong spin-exchange collisions in the presence of a weak dc magnetic field. We find that the atomic Larmor precession frequency shows a new functional form to the rf field parameters when the spin-exchange collision rate is tuned. In the weak rf field amplitude regime, a strong modification of atomic Larmor frequency appears when the spin-exchange rate is comparable to the rf field frequency. This new effect has been neglected before due to its narrow observation window. We compare the experimental results with density matrix calculations, and explain the data by an underdamped oscillator model. When the rf field amplitude is large, there is a minimum atomic gyromagnetic ratio point due to the rf photon dressing, and we find that strong spin-exchange interactions modify the position of such a point.

physics.atom-ph↗