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Zheyuan Xie

Publications and source records attributed to Zheyuan Xie.

4 recordsLinked to original sources

Observation of flat-bottom U-shaped energy gap in high-Tc nickelate (La,Pr)3Ni2O7 thin films

The discovery of high transition temperature (high-Tc) superconductivity in Ruddlesden-Popper (R-P) bilayer nickelates under high pressure has stimulated extensive work to understand the underlying mechanism and search for superconductors with higher Tc. The recent realization of superconductivity in R-P bilayer nickelate thin films with onset Tc above 40 K at ambient-pressure enables the use of a wide array of powerful experimental tools to investigate the unconventional high-Tc superconductivity in bilayer nickelates. Here, using ultra-low temperature scanning tunneling microscopy/spectroscopy (STM/S) and electrical transport study, we report the first successful observation of an energy-symmetric, flat-bottom U-shaped gap with zero residual density of states around the Fermi level in the high-Tc nickelate (La,Pr)3Ni2O7 thin film grown on SrLaAlO4 substrate. Before and after STM/S studies, transport measurements on the same sample reveal consistent superconducting behaviors showing zero resistance, with an onset Tc above 40 K and zero resistance Tc above 20 K. The tunneling spectra exhibit highly unconventional temperature evolution, characterized by a rapid filling of the U-shaped energy gap to a V-shaped gap as the temperature increases. Furthermore, the U-shaped energy gap is reduced under a c-axis magnetic field of 14 T. The energy-symmetric U-shaped gap, taken together with its dependence on magnetic field and temperature, is consistent with the behavior of a superconducting gap, suggesting a nodeless gap function at ultra-low temperatures. Our findings shed new lights on the nature of high-Tc superconductivity and provide an encouraging and thought-provoking hint for a local superconductivity with Tc above liquid nitrogen boiling temperature in nickelate superconductors at ambient or zero pressure.

cond-mat.supr-con

Time-reversal symmetry breaking superconductivity with electronic glass in nickelate (La, Pr, Sm)3Ni2O7 films

The discovery of Ruddlesden-Popper (R-P) nickelate superconductors under high pressure heralds a new chapter of high-transition temperature (high-Tc) superconductivity. Recently, ambient-pressure superconductivity is achieved in R-P bilayer nickelate thin films through epitaxial compressive strain, unlocking the potential for understanding the nature of the unconventional superconductivity. Here, through electrical transport study, we report the discovery of time-reversal symmetry (TRS) breaking superconductivity with electronic glass in bilayer nickelate (La, Pr, Sm)3Ni2O7 films. It emerges in the lower-temperature regime of superconducting transition to the zero-resistance state, and is captured by three remarkable characteristics: 1. Unconventional magnetoresistance hysteresis, the direct evidence of TRS breaking, which is robust under different magnetic field orientations and differs fundamentally from trapped vortices or long-range-ordered magnetism. Successive oxygen reductions simultaneously weaken both the superconductivity and hysteresis, revealing their mutual connections to selective electronic orbitals. 2. Magnetic field history-dependence and zero-field non-reciprocity in the current-voltage responses, further substantiating the intrinsic and spontaneous TRS breaking. 3. Logarithmically slow resistance relaxations upon the removal of magnetic field, the hallmarks of glassy dynamics. Distinguished by the striking magnetic field history- and time-dependent properties, our findings uncover an unprecedented superconducting state in the nickelate superconductors, providing phenomenological and conceptual advances for future research on high-Tc superconductivity.

cond-mat.supr-con

Emergent quantum phenomena via phase-coherence engineering in infinite-layer nickelate superconductors

Dimensionality of a physical system, conventionally an invariant geometric characteristic, fundamentally governs the universality class of phase transitions and the landscape of emergent collective phenomena. In low-dimensional or layered high-temperature superconductors, the macroscopic phase coherence of superconducting orders is typically confined in two dimensions, underscoring the critical role of phase fluctuations in determining the overall phase diagrams. Here, we strategically enhance the phase fluctuations by fabricating periodically arranged nano-holes in the infinite-layer nickelate superconducting films, effectively constructing Josephson junction arrays. In the nano-patterned films, the weakening of macroscopic phase coherence drives a two-stage superconducting transition towards an anomalous metallic ground state with saturated resistance. The emergence of charge-2e quantum oscillations manifests the coherence across the array, while an anomalous zero-field magnetoresistance peak signifies the extreme quantum phase fluctuations persisting to ultralow temperatures. Remarkably, with quantum fluctuations enhanced synergistically by nano-patterning and magnetic fields, an anomalous reversal of superconducting anisotropy is observed in Nd-nickelates, where in-plane critical fields fall below out-of-plane values. The evolution of anisotropy may unmask an internal exchange-Zeeman field coupled to the collective electronic states. Our results unveil how superconductivity evolves in response to phase fluctuations, establishing nano-patterning as a powerful paradigm to uncover hidden intertwined orders in strongly correlated systems.

cond-mat.supr-con

Rotational symmetry breaking in superconducting nickelate Nd0.8Sr0.2NiO2 films

The infinite-layer nickelates, isostructural to the high-Tc superconductor cuprates, have risen as a promising platform to host unconventional superconductivity and stimulated growing interests in the condensed matter community. Despite numerous researches, the superconducting pairing symmetry of the nickelate superconductors, the fundamental characteristic of a superconducting state, is still under debate. Moreover, the strong electronic correlation in the nickelates may give rise to a rich phase diagram, where the underlying interplay between the superconductivity and other emerging quantum states with broken symmetry is awaiting exploration. Here, we study the angular dependence of the transport properties on the infinite-layer nickelate Nd0.8Sr0.2NiO2 superconducting films with Corbino-disk configuration. The azimuthal angular dependence of the magnetoresistance (R(ϕ)) manifests the rotational symmetry breaking from isotropy to four-fold (C4) anisotropy with increasing magnetic field, revealing a symmetry breaking phase transition. Approaching the low temperature and large magnetic field regime, an additional two-fold (C2) symmetric component in the R(ϕ) curves and an anomalous upturn of the temperature-dependent critical field are observed simultaneously, suggesting the emergence of an exotic electronic phase. Our work uncovers the evolution of the quantum states with different rotational symmetries and provides deep insight into the global phase diagram of the nickelate superconductors.

cond-mat.supr-con