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Zhi-Feng Liu

Publications and source records attributed to Zhi-Feng Liu.

13 recordsLinked to original sources

Topological Tunneling Magnetoresistance Driven by Type-II Weyl-Like States in the Room-Temperature Half-Metal Mn2PC Monolayer

We predict the tetragonal Mn2PC monolayer to be a room-temperature ferromagnetic half-metal with a Curie temperature of 554 K. The spin-up channel hosts type-II Weyl-like crossings at the Fermi level with highly anisotropic band dispersion, whereas the spin-down channel is a wide-gap semiconductor. Topological edge states obtained from tight-binding calculations confirm the non-trivial bulk topology. Spin-orbit coupling opens a small gap of 11.2 meV at the Weyl-like crossings, generating pronounced Berry curvature and a sizable anomalous Hall conductivity near the Fermi level. Based on these properties, we propose topological tunneling magnetoresistance in a Mn2PC-based magnetic tunnel junction: the parallel configuration conducts through fully spin-polarized Weyl-like carriers, while the antiparallel configuration is suppressed by the half-metallic gap, yielding a giant magnetoresistance ratio. The concurrent anomalous Hall effect in the conducting state provides an experimentally accessible signature of the topological carriers. These results identify the Mn2PC monolayer as a promising platform for room-temperature topological spintronic devices.

cond-mat.other

Enhancing Oxygen Reduction Reaction on Pt-Based Electrocatalysts through Surface Decoration for Improved OH Reduction Equilibrium and Reduced H2O Adsorption

Electrochemical energy and substance conversion devices involve complex electrode processes, characterized by multiple charge transfer steps, competing pathways, and various intermediates. Such complexity makes it challenging to enhance electrocatalytic activity. The prevailing strategy typically focuses on optimizing the geometric and electronic structures of the electrocatalysts to align the adsorption energies of reaction intermediates with the peak of the activity Volcano curve. In this study, we demonstrate that surface decoration can effectively shape the micro reaction environment for the model system of oxygen reduction reaction (ORR) on Pt electrodes. By applying a partial hydrophobic I* adlayer on the Pt surface, we can shift the equilibrium of OH* reduction and weaken H2O* adsorption, which significantly enhances ORR kinetics. With in situ scan tunneling microscopy (STM) and theoretical calculations, our study reveals the formation of isolated Pt2 surface units situated in a hydrophobic valley surrounded by adsorbed iodine atoms. This minimalist Pt2 active unit exhibits significantly greater activity for ORR compared to an extended Pt surface. This strategy could pave the way for developing highly efficient catalysts with potential applications in fuel cell technology and metal air batteries and extension to other electrochemical conversion reactions such as ammonia synthesis and CO2 reduction.

physics.chem-ph

A three-body form factor at sub-leading power in the high-energy limit: planar contributions

We consider two-loop planar contributions to a three-body form factor at the next-to-leading power in the high-energy limit, where the masses of external particles are much smaller than their energies. The calculation is performed by exploiting the differential equations of the expansion coefficients, both for facilitating the linear relations among them, and for deriving their analytic expressions. The result is written in terms of generalized polylogarithms involving a few simple symbol letters. Our method can be readily applied to the calculation of non-planar contributions as well. The result provides crucial information for establishing sub-leading factorization theorems for massive scattering amplitudes in the high-energy limit.

hep-ph

Heralded High-Dimensional Photon-Photon Quantum Gate

High-dimensional encoding of quantum information holds the potential to greatly increase the computational power of existing devices by enlarging the accessible state space for fixed register size and by reducing the number of required entangling gates. However, qudit-based quantum computation remains far less developed than conventional qubit-based approaches, in particular for photons, which represent natural multi-level information carriers that play a crucial role in the development of quantum networks. A major obstacle for realizing quantum gates between two individual photons is the restriction of direct interaction between photons in linear media. In particular, essential logic components for quantum operations such as native qudit-qudit entangling gates are still missing for optical quantum information processing. Here we address this challenge by presenting a protocol for realizing an entangling gate -- the controlled phase-flip (CPF) gate -- for two photonic qudits in arbitrary dimension. We experimentally demonstrate this protocol by realizing a four-dimensional qudit-qudit CPF gate, whose decomposition would require at least 13 two-qubit entangling gates. Our photonic qudits are encoded in orbital angular momentum (OAM) and we have developed a new active high-precision phase-locking technology to construct a high-dimensional OAM beam splitter that increases the stability of the CPF gate, resulting in a process fidelity within a range of $ [0.64 \pm 0.01, 0.82 \pm 0.01]$. Our experiment represents a significant advance for high-dimensional optical quantum information processing and has the potential for wider applications beyond optical system.

quant-ph

Reclassifying Feynman integrals as special functions

Although Feynman integrals in general cannot be expressed as well-studied special functions, they can be calculated systematically and efficiently using the \texttt{AMFlow} method in combination with differential equations in the kinematic space. Therefore, it is constructive to define Feynman integrals as a new class of special functions (or transcedental numbers if there is no kinematic variable). Several crucial avenues for further exploration in this direction are outlined.

hep-ph

Numerical strategy on the grid orientation effect in the simulation for two-phase flow in porous media by using the adaptive artificial viscosity method

It is a challenge to numerically solve nonlinear partial differential equations whose solution involves discontinuity. In the context of numerical simulators for multi-phase flow in porous media, there exists a long-standing issue known as Grid Orientation Effect (GOE), wherein different numerical solutions can be obtained when considering grids with different orientations under certain unfavorable conditions. Our perspective is that GOE arises due to numerical instability near displacement fronts, where spurious oscillations accompanied by sharp fronts, if not adequately suppressed, lead to GOE. To reduce or even eliminate GOE, we propose augmenting adaptive artificial viscosity when solving the saturation equation. It has been demonstrated that appropriate artificial viscosity can effectively reduce or even eliminate GOE. The proposed numerical method can be easily applied in practical engineering problems.

math.NA

Manipulating spatial structure of high-order quantum coherence with entangled photons

High-order quantum coherence reveals the statistical correlation of quantum particles. Manipulation of quantum coherence of light in temporal domain enables to produce single-photon source, which has become one of the most important quantum resources. High-order quantum coherence in spatial domain plays a crucial role in a variety of applications, such as quantum imaging, holography and microscopy. However, the active control of high-order spatial quantum coherence remains a challenging task. Here we predict theoretically and demonstrate experimentally the first active manipulation of high-order spatial quantum coherence by mapping the entanglement of spatially structured photons. Our results not only enable to inject new strength into current applications, but also provide new possibilities towards more wide applications of high-order quantum coherence.

quant-ph

Automatic computation of Feynman integrals containing linear propagators via auxiliary mass flow

We proposed a recipe to systematically calculate Feynman integrals containing linear propagators using the auxiliary mass flow method. The key of the recipe is to introduce a quadratic term for each linear propagator and then using differential equations to get rid of their effects. As an application, we calculated all master integrals of vacuum integrals containing a gauge link up to four loops, and we checked the results by nontrivial dimensional recurrence relations.

hep-ph

Hong-Ou-Mandel Interference between Two Hyper-Entangled Photons Enables Observation of Symmetric and Anti-Symmetric Particle Exchange Phases

Two-photon Hong-Ou-Mandel (HOM) interference is a fundamental quantum effect with no classical counterpart. The exiting researches on two-photon interference were mainly limited in one degree of freedom (DoF), hence it is still a challenge to realize the quantum interference in multiple DoFs. Here we demonstrate the HOM interference between two hyper-entangled photons in two DoFs of polarization and orbital angular momentum (OAM) for all the sixteen hyper-entangled Bell states. We observe hyper-entangled two-photon interference with bunching effect for ten symmetric states (nine Boson-Boson states, one Fermion-Fermion state) and anti-bunching effect for six anti-symmetric states (three Boson-Fermion states, three Fermion-Boson states). More interestingly, expanding the Hilbert space by introducing an extra DoF for two photons enables to transfer the unmeasurable external phase in the initial DoF to a measurable internal phase in the expanded two DoFs. We directly measured the symmetric exchange phases being $0.012 \pm 0.002$, $0.025 \pm 0.002$ and $0.027 \pm 0.002$ in radian for the three Boson states in OAM and the anti-symmetric exchange phase being $0.991 π\pm 0.002$ in radian for the other Fermion state, as theoretical predictions. Our work may not only pave the way for more wide applications of quantum interference, but also develop new technologies by expanding Hilbert space in more DoFs.

quant-ph

Determining Feynman integrals with only input from linear algebra

We find that all Feynman integrals (FIs), having any number of loops, can be completely determined once linear relations between FIs are provided. Therefore, FIs computation is conceptually changed to a linear algebraic problem. Examples up to 5 loops are given to verify this observation. As a byproduct, we get a powerful method to calculate perturbative corrections in quantum field theory.

hep-ph

Nonlinear manipulation of orbital angular momentum spectra with second- and third- harmonic generation in a quasi-periodically poled crystal

Optical orbital angular momentum (OAM), as an important degree of freedom of light, has been attracted extensive attention, due to its intrinsic feature of natural discrete infinite dimension. Manipulation of OAM spectra is crucial for many impressive applications from classical to quantum realms, in particular, nonlinear manipulation of OAM spectra. Here we realized the nonlinear manipulation of OAM spectra by using the simultaneous second- and third-harmonic generation in a single nonlinear crystal of quasi-periodically poled potassium titanyl phosphate, for fundamental waves with a variety of OAM spectra, especially for customized OAM spectra of the second and third harmonics. The experimental results confirmed the theoretical predictions. Our approach not only provides a novel way to manipulate OAM spectra at new shorter wavelengths that are hard to be directly generated, but also may find new applications towards multiplexing in classical optics and high-dimensional information processing in quantum optics.

physics.optics

A new explanation to the cold nuclear matter effects in heavy ion collisions

The J/Psi cross section ratios of p-A/p-p under different collision energy is calculated with cold nuclear matter effects redefined in this paper. The advantage of these new definitions is that all cold nuclear matter effects have clear physical origins.The radios are compared with the corresponding experiment data and that calculated with classic nuclear effects. The ratios calculated with new definitions can reproduce almost all existing J/Psi measurements in p-A collisions more accuratly than that calculated with classic nuclear effects. Hence, this paper presents a new approach to explain cold nuclear effects in the hardproduction of quarkonium.

hep-ph

Sealing off a carbon nanotube with a self-assembled aqueous valve for the storage of hydrogen in GPa pressure

The end section of a carbon nanotube, cut by acid treatment, contains hydrophillic oxygen groups. Water molecules can self-assemble around these groups to seal off a carbon nanotube and form an "aqueous valve". Molecular dynamics simulations on single-wall (12,12) and (15,15) tubes with dangling carboxyl groups show that the formation of aqueous valves can be achieved both in the absence of and in the presence of high pressure hydrogen. Furthermore, significant diffusion barriers through aqueous valves are identified. It indicates that such valves could hold hydrogen inside the tube with GPa pressure. Releasing hydrogen is easily achieved by melting the "aqueous valve". Such a design provides a recyclable and non- destructive way to store hydrogen in GPa pressure. Under the storage conditions dictated by sealing off the container in liquid water, the hydrogen density inside the container is higher than that for solid hydrogen, which promises excellent weight storage efficiency.

cond-mat.mes-hall