arXiv subjects

Zhi-Han Zhu

Publications and source records attributed to Zhi-Han Zhu.

At least 19 recordsLinked to original sources

arXiv2025

Structured Harmonic Generation via Geometric Phase Enabled Pump Shaping

Nonlinear optics is crucial for shaping the spatial structure of shortwave light and its interactions with matter, but achieving this through simple harmonic generation with a single pump is challenging. This study demonstrates nonlinear spin-orbit conversion using spin-dependent pump shaping via geometric phase, allowing the direct creation of desired structured harmonic waves from a Gaussian pump beam. By using the liquid-crystal flat optical elements fabricated with photoalignment, we experimentally produce higher-order cylindrically vectorial modes in second harmonic fields. We examine the vectorial spatial wavefunctions, their propagation invariance, and nonlinear spin-orbit conversion. Our results provide an efficient method for full structuring nonlinear light in broader harmonic systems, with significant applications in laser micromachining and high-energy physics.

physics.optics↗

arXiv2025

All-optical convolution utilizing processing in memory based on a cold atomic ensemble

Processing in memory (PIM) has received significant attention due to its high efficiency, low latency, and parallelism. In optical computation, coherent memory is a crucial infrastructure for PIM frameworks. This study presents an all-optical convolution experiment conducted within computational storage based on a cold atomic ensemble. By exploiting the light-atom phase transfer facilitated by the electromagnetically induced transparency, we demonstrated spiral phase contrast processing of photon images in memory, resulting in the edge enhancement of retrieved images recorded using time-correlated photon imaging. In particular, adopting state-of-the-art atomic techniques provides a coherent memory lifetime exceeding 320 us for PIM operations. Our results highlight the significant potential of cold atomic ensembles as computational storage for developing all-optical PIM systems.

physics.app-ph↗

arXiv2024

Talbot-like pattern evolution in complex structured light from unitary transformation

Astigmatic unitary transformations allow for the adiabatic connections of all feasible states of paraxial Gaussian beams on the same modal sphere, i.e., Hermite-Laguerre-Gaussian (HLG) modes. Here, we present a comprehensive investigation into the unitary modal evolution of complex structured Gaussian beams, comprised by HLG modes from disparate modal spheres, via astigmatic transformation. The non-synchronized higher-order geometric phases in cyclic transformations originates a Talbot-effect-like modal evolution in the superposition state of these HLG modes, resulting in pattern variations and revivals in transformations with specific geodesic loops. Using Ince-Gaussian modes as an illustrative example, we systematically analyze and experimentally corroborate the beamforming mechanism behind the pattern evolution. Our results outline a generic modal conversion theory of structured Gaussian beams via astigmatic unitary transformation, offering a new approach for shaping spatial modal structure. These findings may inspire a wide variety of applications based on structured light.

physics.optics↗

arXiv2023

Structured Light Modal Interface via Liquid-Crystal Planar Optics

Recent advances in planar optics with geometric-phase superstructures have brought a new paradigm in the control of structured light and, in particular, has substantially enhanced the capabilities of generating and detecting orbital angular momentum (OAM) states of light and associated spatial modes. However, the structured modal interface that can reciprocally link OAM states via adiabatic control and access-associated higher-order geometric phase remains absent in planar optics. In this work, we propose and experimentally demonstrate a planar optical astigmatic retarder fabricated with liquid-crystal (LC) geometric phase. The LC superstructure was designed with the principle of fractional Fourier transformation and is capable of reciprocal conversion between all possible OAM states on the same modal sphere. Such a planar device paves the way towards an easily deployed modal interface of paraxial OAM states, unlocks the resource of higher-order geometric phase, and has promising applications in high-dimensional classical/quantum information.

physics.optics↗

arXiv2023

Single-shot, full characterization of the spatial wavefunction of light fields via Stokes tomography

Since the diffraction behavior of a light field is fully determined by its spatial wavefunction, i.e., its spatial complex amplitude (SCA), full characterization of spatial wavefunction, plays a vital role in modern optics from both the fundamental and applied aspects. In this work, we present a novel complex-amplitude profiler based on spatial Stokes tomography with the capability to fully determine the SCA of a light field in a single shot with high precision and resolution. The SCA slice observed at any propagation plane provides complete information about the light field, thus allowing us to further retrieve the complete beam structure in 3 dimensions space, as well as the exact modal constitution in terms of spatial degrees of freedom. The principle demonstrated here provides an important advancement for the full characterization of light beams with a broad spectrum of potential applications in various areas of optics, especially for the growing field of structured light.

physics.optics↗

arXiv2023

Toward arbitrary spin-orbit flat optics via structured geometric phase gratings

Reciprocal spin-orbit coupling (SOC) via geometric phase with flat optics provides a promising platform for shaping and controlling paraxial structured light. Current devices, from the pioneering q-plates to the recent J-plates, provide only spin-dependent wavefront modulation without amplitude control. However, achieving control over all the spatial dimensions of paraxial SOC states requires spin-dependent control of corresponding complex amplitude, which remains challenging for flat optics. Here, to address this issue, we present a new type of flat-optics elements termed structured geometric phase gratings that is capable of conjugated complex-amplitude control for orthogonal input circular polarizations. By using a microstructured liquid crystal photoalignment technique, we engineered a series of flat-optics elements and experimentally showed their excellent precision in arbitrary SOC control. This principle unlocks the full-field control of paraxial structured light via flat optics, providing a promising way to develop an information exchange and processing units for general photonic SOC states, as well as extra-/intracavity mode convertors for high-precision laser beam shaping.

physics.optics↗

arXiv2022

Observation of Anomalous Orbital Angular Momentum Conservation in Parametric Nonlinearity

Orbital angular momentum (OAM) conservation plays an important role in shaping and controlling structured light with nonlinear optics. The OAM of a beam originating from three-wave mixing should be the sum or difference of the other two inputs because no light-matter OAM exchange occurs in parametric nonlinear interactions. Here, we report anomalous OAM conservation during parametric upconversion, in which a Hermite-Gauss mode signal interacts with a specially engineered pump capable of astigmatic transformation in a crystal, resulting in Laguerre-Gaussian mode sum-frequency generation (SFG). The anomaly here refers to the fact that the pump and signal carry no net OAM, while their SFG does. We show that the lost OAM with the opposite sign that maintains OAM conservation in the system is hidden in the residual pump. This unexpected OAM selection rule improves our understanding of OAM conservation in parametric nonlinear systems and may inspire new ideas for controlling OAM states via nonlinear optics, especially in quantum applications.

physics.optics↗

arXiv2022

Real-time superresolution interferometric measurement enabled by structured nonlinear optics

Optical interferometers are pillars of modern precision metrology, but their resolution is limited by the wavelength of the light source, which cannot be infinitely reduced. Magically, this limitation can be circumvented by using an entangled multiphoton source because interference produced by an N-photon amplitude features a reduced de Broglie wavelength λ/N. However, the extremely low efficiency in multiphoton state generation and coincidence counts actually negates the potential of using multiphoton states in practical measurements. Here, we demonstrate a novel interferometric technique based on structured nonlinear optics, i.e., parametric upconversion of a structured beam, capable of superresolution measurement in real time. The main principle relies in that the orbital angular momentum (OAM) state and associated intramodal phase within the structured beam are both continuously multiplied in cascading upconversion to mimic the superresolved phase evolution of a multiphoton amplitude. Owing to the use of bright sensing beams and OAM mode projection, up to a 12-photon de Broglie wavelength with almost perfect visibility is observed in real time and, importantly, by using only a low-cost detector. Our results open the door to real-time superresolution interferometric metrology and provide a promising way toward multiphoton superiority in practical applications.

physics.optics↗

arXiv2022

Highly sensitive measurement of a megahertz rf electric field with a Rydberg-atom sensor

Rydberg atoms have great potential in electric field measurement and have an advantage with a large frequency bandwidth from the kHz to the THz scale. However, the sensitivity for measuring a weak MHz electric field signal is limited by the spectroscopic resolution, because the weak electric field induces only a small perturbation of the population and energy level shift of the Rydberg atoms. Here, we report highly sensitive measurement of a weak MHz electric field using electromagnetically induced transparency with Rydberg atoms in a thermal atomic system. Using the heterodyne method on a 30-MHz electric field, we successfully measure the minimum electric field strength to be \textcolor{black}{37.3 $\mathrm{μV/cm}$} with a sensitivity up to $-65$ dBm/Hz and a linear dynamic range over 65 dB. Additionally, we measure an amplitude-modulated signal and demodulate the signal with a fidelity over 98\%. This work extends the sensitivity of atomic sensors for measuring MHz electric fields, which advances atomic electric field-sensing technology.

physics.atom-ph↗

arXiv2022

Directly determining orbital angular momentum of ultrashort Laguerre-Gauss pulses via autocorrelation measurement

Autocorrelation measurement based on second-harmonic generation (SHG), the best-known technique for measuring the temporal duration of ultrashort pulses, could date back to the birth of ultrafast lasers. Here, we propose and experimentally demonstrate that such well-established technique can also be used to measure the orbital angular momentum of ultrashort Laguerre-Gauss (LG) pulses. By analysing the far-field pattern of the SHG signal, the full spatial structure of ultrashort LG pulses, including both azimuthal and radial indices, are unambiguously determined. Our results provide an important advancement for the well-established autocorrelation technique by extending it to reach its full potential in laser characterization, especially for structured ultrashort pulses.

physics.optics↗

arXiv2022

Frequency conversion of abruptly autofocusing waves

Abruptly autofocusing waves and associated ring-Airy (RA) beams are attracting increasing interest owing to their fascinating properties such as their ability of abruptly autofocusing to small F-number. Optical frequency conversion via nonlinear interactions can further expand their applications to new area, yet are rarely studied. In this work, we report the frequency conversion of RA beams via sum-frequency generation using perfect flattop and common Gauss beams as the pump beams. The nonlinear transformation of the spatial complex amplitude of the signal and associated influences on autofocusing behavior, under different conditions of interaction location (i.e., original, autofocusing, and Fourier planes) and pump structure, were systematically studied and experimentally investigated. This proof-of principle demonstration provides a general guideline to build the frequency interface for abruptly autofocusing waves and a reference for relevant studies involving nonlinear transformation of abruptly autofocusing waves.

physics.optics↗

arXiv2022

Propagation-invariant high-dimensional orbital angular momentum states

Photonic states encoded in spatial modes of paraxial light fields provide a promising platform for high-dimensional quantum information protocols and related studies, where several pioneering theoretical and experimental demonstrations have paved the path for future technologies. Crucially, critical issues encountered in free-space propagation still represent a major challenge. This is the case of asynchronous diffraction between spatial modes with different modal orders, which experience variations in their transverse structure upon free-space propagation. Here we address this issue by proposing an encoding method based on the use of Laguerre-Gaussian (LG) modes of the same modal order N to define a N + 1 dimensional space. Noteworthy, such modes endowed with orbital angular momentum (OAM) experience the same propagation aberrations featuring an identical Gouy phase and wavefront curvature. We demonstrate our proposal experimentally by using time-correlated-single-photon imaging combined with a digital propagation technique. Importantly, our technique allows to eliminate, without the use of imaging systems, all issues related to asynchronous diffraction, providing an accessible way to generate propagation-invariant OAM qudits for quantum optical protocols.

physics.optics↗

arXiv2021

Conformal frequency conversion for arbitrary vectorial structured light

Vectorial structured light with spatially varying amplitude, phase, and polarization is reshaping many areas of modern optics, including nonlinear optics, as diverse parametric processes can be used to explore interactions between such complex vector fields, extending the frontiers of optics to new physical phenomena. However, the most basic nonlinear application, i.e., frequency conversion, still remains challenging for vectorial structured light since parametric processes are polarization dependent, leading to a change in the spatial topological structure of signals. In this work, to break this fundamental limit, we propose a novel conformal frequency conversion scheme that allows to maintain the full spatial structure of vectorial structured light in the conversion; and systematically examine its spatial polarization independence based on non-degenerate sum-frequency generation with type-0 phase matching. This proof-of-principle demonstration paves the way for a wide range of applications requiring conformal frequency conversion, and, particularly, to implement frequency interfaces with multimodal communication channels, high-dimensional quantum states, and polarization-resolved upconversion imaging.

physics.optics↗

arXiv2021

Gouy-phase-mediated propagation variations and revivals of transverse structure in vectorially structured light

Exploring the physics and potential applications of vectorially structured light with propagation-invariant transverse structures has benefited many areas of modern optics and photonics. In this paper, we investigate the non-eigen vector modes of paraxial light fields, focusing on the propagation variations and revivals of their transverse structures, including both spatial and polarization structures. We show that the physical mechanism behind the variations and revivals of their transverse structure is linked to the evolution of the intramodal phases between the constituting spatial modes. Such evolution originates from fractional Gouy phases, or rather, Geometric-phase difference between spatial modes with different orders under a same unitary transformation. This underlying principle, provides a general guideline for shaping vectorially structured light with custom propagation-evolution properties, and may also inspire a wide variety of new applications based on structured light.

physics.optics↗

arXiv2021

Heralded generation of vectorially structured photons with high purity

Engineering vector spatial modes of photons is an important approach for manipulating high-dimension photonic states in various quantum optical experiments. In this work, we demonstrate generation of heralded single photons with well-defined vector spatial modes by using a self-locking polarizing interferometer comprising a spatial light modulator. Specifically, it is shown that, by carefully tailoring and compensating spatial and temporal amplitudes of manipulated photons, one can exactly convert ultrafast single photons into desired spin-orbit states with extremely high purity. This compact and robust device provides a versatile way for not only generation, but also manipulation and characterization of arbitrary photonic spin-orbit states.

physics.optics↗

arXiv2020

Experimental demonstration of Cavity-Free Optical Isolators and Optical Circulators

Cavity-free optical nonreciprocity components, which have an inherent strong asymmetric interaction between the forward- and backward-propagation direction of the probe field, are key to produce such as optical isolators and circulators. According to the proposal presented by Xia et al., [Phys. Rev. Lett. 121, 203602 (2018)], we experimentally build a device that uses cross-Kerr nonlinearity to achieve a cavity-free optical isolator and circulator. Its nonreciprocal behavior arises from the thermal motion of N-type configuration atoms, which induces a strong chiral cross-Kerr nonlinear response for the weak probe beam. We obtain a two-port optical isolator for up to 20 dB of isolation ratio in a specially designed Sagnac interferometer. The distinct propagation directions of the weak probe field determine its cross-phase shift and transmission, by which we demonstrate the accessibility of a four-port optical circulator.

quant-ph↗

arXiv2020

Radial modal transitions of Laguerre-Gauss modes during parametric upconversion: towards the full-field selection rule of spatial modes

Optical orbital angular momentum transformation and corresponding azimuthal-mode selection rules have been studied exhaustively for various nonlinear optical interactions. However, nonlinear transformation of radial mode has not been systematically studied since the pioneering work [Phys. Rev. A 56, 4193, 1997]. In this paper, we theoretically study and experimentally verify the radial modal transitions of Laguerre-Gauss (LG) modes in parametric upconversion. Specifically, we provide a general solution that describes the sum-frequency generation (SFG) field excited by two arbitrary LG modes. Based on the solution, one can predict the full spatial complex amplitude of SFG fields upon propagation precisely and readily obtain the associated full-field selection rule including both azimuthal and radial modes. This work provides a theoretical basis for quantum and nonlinear optical research involving parametric upconversion of complex structured light, and paves the way for future work on full-field transformation of spatial modes in other nonlinear interactions.

physics.optics↗

arXiv2020

Spatial polarization independent parametric upconversion of vectorially structured light

Spatial polarization independent (SPI) parametric conversion is the basis of many optical applications, such as SPI frequency interface for communication channels carried by vector modes and upconversion detection for polarization-resolved imaging. However, realizing such conversion remains a challenge. In this proof-of-principle work, we demonstrated SPI parametric upconversion using a polarization Sagnac nonlinear interferometer based on type-II second-harmonic generation (SHG). Our results show that the vector (including both polarization and intensity) profile and associated SOC state of the vector signal beam could be transferred to the SHG beam with a high fidelity. The principle lays a foundation of SPI frequency interface for quantum/classical channels based on vector modes and also paves the way for upconversion detection of polarization-resolved imaging in Mid-/far-infrared region.

physics.optics↗