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Zhi-Ming Yu

Publications and source records attributed to Zhi-Ming Yu.

At least 19 recordsLinked to original sources

Magnetic-Field Selection of Magnetic Order in Altermagnets and Noncollinear Antiferromagnets

Conventional field selection of magnetic order relies on the Zeeman coupling, which, however, vanishes in magnets without net magnetization, a rapidly growing class including altermagnets (AMs), noncollinear antiferromagnets (nc-AFMs), and PT-symmetric antiferromagnets (PT-AFMs). Here we show that the quantity that fundamentally couples a magnet to a uniform magnetic field is not the magnetization, but the binary order parameter eta that labels the two time-reversal-related minima of the Landau free energy. We develop a Landau theory of order selection based on eta under the constraints of magnetic point-group (MPG) symmetry, in which eta couples to odd-degree polynomials in the magnetic field. Within this framework, the linear term is the ferromagnetic Zeeman coupling, while higher-order couplings with leading degree n = 3, 5, 7, and 9 naturally appear in AMs and nc-AFMs. In contrast, combined PT symmetry forbids any such coupling. Consequently, it is the order-(n-1) magnetic susceptibility, rather than the net magnetization, that serves as the primary experimental observable for identifying the magnetic order of AMs and nc-AFMs. For all 122 MPGs, we classify the leading coupling degree and the corresponding polynomial forms. We demonstrate our framework in two representative materials: the AM MnF2 and the nc-AFM MnTe2. We further construct a symmetry-allowed spin model for an AM system to reveal the microscopic origin of the higher-order coupling and establish the coupling coefficient explicitly in terms of the spin-model parameters. Our work unifies the description of magnetic-order selection across magnets with and without net magnetization, offers a microscopic origin for this counterintuitive physics, and provides fingerprints for distinguishing intrinsic field selection from extrinsic switching.

cond-mat.mtrl-sci

N\'eel-order-dependent transverse transport in noncoplanar antiferromagnet $\text{MnTe}_{2}$

Antiferromagnets hold appealing potential in next-generation spintronic devices with higher frequency and scalability, thanks to their alternating spin orientations that cancel out net magnetization. However, the lack of a nonzero magnetization makes the detection of the magnetic configuration of antiferromagnet difficult, hampering the applications of antiferromagnets. Here, we report a new transverse transport effect in noncoplanar antiferromagnet $\text{MnTe}_{2}$. This effect is antisymmetric in both magnetic field and N\'eel order, but symmetric in its two indices. It can be understood in terms of the contribution induced by both magnetic field and geometric quantities, as confirmed by our theoretical calculations. Our discovery of a new N\'eel-order-dependent transverse transport effect provides opportunities to the advancing antiferromagnetic spintronics.

cond-mat.mtrl-sci

Quantized Spin Hall Effect in Three-Dimensional Nodal-Ring Semimetal: Geometric Scaling and Symmetry-Engineered Spin Response

The anomalous Hall conductivity in magnetic Weyl semimetals scales linearly with the momentum separation between Weyl nodes, establishing a geometric paradigm for three-dimensional Hall responses. Here we discover an analogous phenomenon in the spin Hall effect: a quantized spin Hall conductivity (SHC) in nodal-ring semimetals that scales linearly with the nodal-ring radius $R$. From an ideal model with a single nodal ring, we derive analytically that the SHC inside the spin-orbit-coupled gap obeys $\sigma_{\alpha \beta}^{S, 3D}=\sigma_0^{S,2D} \cdot (\pi R/2 \pi)$, where $\sigma_0^{S,2D}=(e^2/h) \cdot (\hbar/2 e)$ is the two-dimensional quantum spin Hall conductance. Crucially, the symmetry of the spin-orbit coupling acts as an independent switch: Rashba coupling generates purely conventional SHC components, while Weyl coupling additionally activates unconventional ones, providing separate control over response magnitude and tensor symmetry. We validate this principle in yttrium nitride, where strain tunes $R$ and symmetry breaking toggles between response types. Our work establishes a new paradigm for engineering quantized geometric responses in three dimensions, opening pathways to tailored spin-orbit functionalities.

cond-mat.mtrl-sci

Fractional Spin Ferroelectric and Sliding Spin Current in Magnetic Sliding Ferroelectrics

We investigate the fractional spin ferroelectric (FSFE) in magnetic sliding ferroelectrics (SFEs), where ferroelectric switching is characterized not only by the reversal of the out-of-plane electric polarization but also by a variation of fractional in-plane spin electronic polarization. We show that interlayer sliding in FSFEs can naturally lead to a symmetry-protected pure spin current, termed the sliding spin current here. The underlying mechanism is that, during switching, the contributions of valence electrons and ions to the in-plane charge transfer cancel each other, whereas the in-plane spin transfer, which stems solely from valence electrons, persists, leading to a pure spin current. We demonstrate our ideas in various material candidates, including $H$-stacked bilayer CrI$_3$, whose few-layer form has been experimentally confirmed to be a magnetic SFE, and $R$-stacked bilayers $2H$-V$X_2$ ($X=$ S, Se, Te), which have been experimentally synthesised. For a typical switching time of about $1$ ns, the estimated spin-current densities for bilayer CrI$_3$ and V$X_2$ reach $10^9 (\hbar/2e)\mathrm{A/m^2}$ and $10^8 (\hbar/2e)\mathrm{A/m^2}$, respectively. This means that by applying a periodic out-of-plane electric field, a significant alternating spin current can be generated in magnetic SFEs. Thus, our findings propose a compelling new mechanism for the all-electrical generation of pure spin current, and predict concrete realistic materials for experimental verification.

cond-mat.mtrl-sci

Unconventional Scaling of Electric Hall Effect in Magnetic Weyl Semimetals

Electric Hall Effect (EHE), a unique phenomenon in two-dimensional (2D) magnetic systems, refers to the generation of Hall current by an out-of-plane electric field $\Ez$. Here, we demonstrate that for 2D magnetic Weyl semimetals that host doubly degenerate nodal points, the EHE features multiple unconventional scaling laws. At zero temperature, the EHE exhibits a topological $E_F^{-1}$ Fermi-energy scaling. Remarkably, the prefactor of the scaling is determined by the global topological charge of the point without any dependence on the local parameters of the system, leading to a universal and significant enhancement of Hall response in any species of Weyl points as the Fermi energy approaches the Weyl point. This significant response enables a weak electric field to be directly converted into a measurable Hall signal. Surprisingly, this enhanced Hall response is not diminished by temperature, but evolves into an unconventional logarithmically corrected scaling at finite temperature $\sigma_{xy}\propto\Ez\ln(1/|\Ez|)$ for weak $\Ez$, still yielding a divergent electric-field susceptibility. Thus, our work not only unveils intriguing scaling laws resulting from the interaction between magnetism and topology, but also suggests a novel scaling-enhanced and temperature-robust mechanism that may enable weak electric-field sensing through a practical and all-electric route.

cond-mat.mes-hall

Generalized Space Groups from Internal Configuration Spaces

We develop a unified construction of generalized space groups for crystals with unconventional internal degrees of freedom. Starting from the full group $G_P$ of allowed internal transformations and the stabilizer $P$ of a reference object, we determine the pointwise and setwise symmetries, $J$ and $K$, of the allowed configuration set. Goursat's lemma then couples the internal quotient $K/J$ to a spatial quotient. The framework includes ordinary, magnetic, spin, and color space groups as special cases. As an example, we consider a dodecahedral object with $P=I\simeq A_5$, for which we obtain the nontrivial pair $T\triangleleft O$ with $O/T\simeq\mathbb Z_2$. The resulting generalized space group hosts a point node with topological charge $|C|=12$.

cond-mat.mtrl-sci

Ridge-Spin-Layer Coupling and Emergent Ridgetronics in 2D Altermagnets

Extending valleytronics from discrete points to continuous lines in momentum space transforms dispersionless bands into a controllable degree of freedom. Here we introduce ridge--spin--layer coupling (RSLC) in two-dimensional (2D) altermagnets, where a one-dimensional continuous line of dispersionless electronic states (a ridge) in momentum space locks to both spin polarization and atomic sublayer. This ridge-induced quenching of kinetic energy mimics flat-band physics, yet crucially, RSLC grants external control, allowing for layer-selective switching of ridge orientation in reciprocal space, spin-filtered transport in real space, and a distinct electric Hall response. Guided by collinear spin layer group symmetry, we identify three 2D candidate materials, namely Mg$_2$Mo$_2$(PO$_5$)$_2$, Ca(FeP)$_2$, and Mg$_2$V$_2$(SO$_5$)$_2$, each featuring a crossed-ridge structure with two ridges, one per spin channel and sublayer. Our work establishes ridgetronics as a controllable platform for direction-discriminating currents, bridging dispersionless bands with multifunctional device operation.

cond-mat.mtrl-sci

Rotation topological states: theory and material realization

The conventional characterization of topological materials relies on topological invariants calculated from the entire set of occupied bands. However, when a system possesses rotational symmetry, the occupied Hilbert space can be decomposed into multiple subspaces labeled by distinct rotation eigenvalues. We show that this decomposition reveals hidden topological states characterized by a novel $\mathbb{Z}_2^n$ topological invariant, where $n$ is the number of subspaces, while the conventional $\mathbb{Z}_2$ invariant may fail to detect the topology hidden in the rotation subspaces. Remarkably, time-reversal symmetry pairs conjugate rotation eigenvalues and guarantees that the two subspaces have the same $\mathbb{Z}_2$ invariants, making the topology always hidden from the conventional global invariant. We formulate the theory of rotation-subspace topology and demonstrate its material realization in bulk CsCl. Using first-principles calculations and symmetry analysis, we show that bulk CsCl, which is diagnosed as topologically trivial by the conventional approach, features a nontrivial $\mathbb{Z}_2^3$ invariant along the $\Gamma$-R path and a nontrivial $\mathbb{Z}_2^4$ invariant along the $\Gamma$-Z and M-R paths, leading to double Weyl points on the (111) and (001) surfaces, respectively. The subspace $\mathbb{Z}_2^n$ invariant proposed here serves as a necessary refinement for symmetry-protected topological phases and will facilitate the identification of a large class of topological states overlooked by existing diagnostics.

cond-mat.mtrl-sci

Topological Interstitial-Electron Conductor

Electron transport in solids arises primarily from two mechanisms: freely moving bulk electrons in metals, and gapless boundary states in topological insulators. Here, we report a new mechanism discovered in electrides. The topological interstitial-electron conductors (TIECs) proposed here are insulating electrides, but host interstitial electrons (IEs) distributed within crystal voids that traverse the entire unit cell. Without being tightly bound to real ions, the IEs generally experience low periodic potential barrier along the void channels. As a consequence, by applying a weak electric field sufficient to overcome the IE barriers but far below the system's dielectric breakdown threshold, one can expect that the TIECs would generate a persistent current contributed by the IEs and propagating along the void channels. We identify a family of realistic altermagnetic electrides, $A_5X_3$ ($A$ = Ca, Sr, Ba, Yb; $X$ = As, Sb), as TIECs. Remarkably, for $A_5X_3$ materials, the periodic potential barrier of the IEs along the void channels are ultralow, ranging from 13.43 to 67.96 meV per formula unit. This renders our proposal readily accessible to experimental verification. We further demonstrate that when the IEs of $A_5X_3$ undergo periodic motion along the channels, topological surface states will emerge at the boundary perpendicular to the channel direction, and continuously move across the bulk band gap. This pumping-like behaviour not only corroborates the topological nature of TIECs, but also rationalizes the finite-electric-field induced electronic transport within the band theory. Our findings expand the classification of electronic conductors, uncover unexplored transport properties of electrides, and establish a new material platform for low-power electronic devices.

cond-mat.mtrl-sci

Spin layer groups and their corepresentations

Spin layer groups are the crystallographic symmetry groups with a periodic plane, and their symmetry operations are inherited from three-dimensional (3D) spin space groups. However, the direct application of 3D symmetry groups to two-dimensional systems is often inadequate due to anisotropic axes and dimensional reduction. In this work, we systematically classify inequivalent spin layer groups and analytically derive their irreducible corepresentations. This classification establishes a foundational framework for investigating symmetry-protected properties and novel quantum states in low-dimensional magnetic materials.

cond-mat.mtrl-sci

Equivariant Space Group and Hamiltonian for Collinear Magnetic Systems

Condensed matter physics increasingly focuses on exploiting the magnetic order parameter orientation n as a tuning knob for properties of collinear magnetic materials, but a general method for constructing effective Hamiltonians with explicit n-dependence has been lacking. Here, we develop a symmetry-based framework, built on the equivariant space group, for constructing such Hamiltonians, termed equivariant magnetic Hamiltonians (EMHs). The resulting EMH lives in a higher-dimensional k-n space and exhibits unconventional symmetry actions and topological features. Using a 1D ferromagnetic chain and a 3D antiferromagnet as examples, we demonstrate that explicit n-dependence in EMHs enables the study of magnetic-dynamics-driven topological pumping, including even-integer charge pumping and a second-Chern-number-induced quantized pumping of surface anomalous Hall conductivity. Beyond model systems, we incorporate the framework into first-principles calculations to construct ab-initio EMHs that accurately capture the n-dependent band structures of real materials. The approach can also be generalized to non-collinear magnetic systems. Our work establishes a general framework for constructing EMHs and for exploring the rich physics arising from magnetic anisotropy and magnetic dynamics.

cond-mat.mtrl-sci

Pressure-Induced Superconducting-like Transition in the $\it d$-wave Altermagnet Candidate CsV$_2$Se$_2$O

Altermagnetism generates exchange-type spin splitting without net magnetization and, in its $\it d$-wave form, resembles the angular symmetry of unconventional $\it d$-wave superconductivity. Whether this correspondence bears directly on superconducting instabilities in real correlated materials remains open. Here we study the quasi-two-dimensional vanadium oxychalcogenide CsV$_2$Se$_2$O (CVSO), a square-net $\it d$-wave altermagnet candidate, through combined experimental and theoretical investigation of its lattice structure, electronic structure and transport properties. At ambient pressure, CVSO is a weakly insulating parent state with a density-wave-like anomaly near 100 K, and its bulk properties are most consistent with a G-type compensated antiferromagnetic background. Under compression, the density-wave-like feature is suppressed, the magnetoresistance evolves from predominantly negative to positive, and a superconducting-like resistive downturn emerges below about 3 K. This low-temperature anomaly is reproducible across samples and pressure media, and is suppressed by magnetic field. Room-temperature X-ray diffraction reveals no symmetry lowering, whereas does show a pronounced compressibility anomaly over the same pressure range. CVSO thus reveals a pressure-tuned phase diagram in which a reconstructed weakly insulating parent state gives way to strange-metal-like transport and superconducting-like behavior, echoing broader phenomenology associated with unconventional superconductors, including cuprates and nickelates.

cond-mat.supr-con

Interstitial-Electron Altermagnetism in Two Dimensions

Altermagnetism has so far been associated with compensated magnetic moments carried by atoms. Here we introduce Stoner instability induced interstitial-electron altermagnetism, a distinct mechanism in which altermagnetic order is carried instead by interstitial anionic electrons in electrides. We show that, owing to the quasi-nucleus-free nature of interstitial electrons, the Stoner instability in electrides hosting two interstitial electrons can naturally stabilize an altermagnetic state rather than the conventional ferromagnetic one. This mechanism leads to a practical design principle for two-dimensional materials, from which we identify monolayers Zr2N and Ti2N as representative candidates. The strong sensitivity of interstitial electrons to cavity size enables efficient strain control of the altermagnetic order and a pronounced piezo-altermagnetic effect. Moreover, we investigate the evolution of the magnetism in Zr2N under ultrafast laser excitation, which exhibits dynamics distinct from those in all previously reported magnetic materials where magnetism is carried by real atoms. Our work not only offers a novel pathway to realize altermagnetism but also reveals an efficient non-magnetic route for its control.

cond-mat.str-el

Manipulating Anomalous Transport via Crystal Symmetry in 2D Altermagnets

Anomalous transports, including the anomalous Hall effect (AHE) and anomalous Nernst effect (ANE), are typical manifestations of time-reversal-symmetry-breaking responses in materials. In general, the two Hall states with opposite Hall conductivities can be regarded as time-reversal pairs coupled to magnetic order, and switching between them relies on reversing the magnetization via an external magnetic field or electric current. Here, we introduce a approach for manipulating anomalous transport through crystal symmetry engineering in two-dimensional (2D) altermagnetic systems. Based on symmetry analysis, we demonstrate that 2D altermagnets (AM) with out-of-plane N\'eel vectors will not host any anomalous Hall transport. Remarkably, breaking the symmetry connecting the two magnetic sublattices, an anomalous Hall response can emerge immediately, and the signs of the anomalous Hall and anomalous Nernst conductivities can be flexibly controlled by the symmetry-breaking term, thereby realizing tunable sign-reversible anomalous transport. Furthermore, the feasibility of the theoretical scheme is further verified by explicit lattice-model construction. Using first-principles calculations, we investigate the realization of crystal symmetry-controlled anomalous transport in a 2D AM material Cr$_{2}$O$_{2}$. The results indicate that Cr$_{2}$O$_{2}$ with out-of-plane N\'eel vectors can sequentially exhibit the AHE and quantum anomalous Hall effect (QAHE) under continuous uniaxial strain. Interestingly, the sign reversal between these two effects can be achieved by simply rotating the strain direction by C$_{4z}$ symmetry. The corresponding ANE and its sign reversal are also revealed. Our findings provide a new strategy to manipulate anomalous transport, and should have significant potential applications.

cond-mat.mes-hall

Nonvolatile Electrical Control of Spin via Sliding Fractional Quantum Multiferroics

We propose a fractionally quantized polarization induced by interlayer sliding in bilayer altermagnets, unveiling a previously unrecognized multiferroic phase termed sliding fractional quantum multiferroicity (SFQM). This unconventional magnetic phase uniquely integrates sliding ferroelectricity with fractional quantum ferroelectricity, enabling highly efficient switching and nonvolatile electrical control of spin.~Unlike conventional multiferroics, SFQM simultaneously exhibits lattice-scale atomic displacements, ultralow switching barriers, and spin splitting, giving rise to a large fractionally quantized polarization and strong magnetoelectric coupling. Through symmetry analysis and first-principles calculations, we identify bilayer altermagnet Ca(CoN)$_2$ and its family materials as promising candidates hosting SFQM. In contrast to gate-controlled schemes, the spin-layer coupling in SFQM is intrinsically induced by spontaneous electrical and layer polarization, requiring no sustained gate field and exhibiting nonvolatile character. This mechanism enables nonvolatile electrical control of spin through biaxial sliding, where displacements along the \textit{x}- and \textit{y}-axes generate opposite polarization directions in the layer-dependent electrical polarization. Furthermore, SFQM exhibits a fully switchable anomalous Hall effect and a pronounced magneto-optical response, which can be utilized for its detection and distinction. These findings highlight the promising role of sliding-mediated couplings among unconventional magnetism, fractional quantum ferroelectricity, and stacking order in realizing electrically controllable two-dimensional multiferroics.

cond-mat.mtrl-sci

Anomalous shift in scattering from topological nodal-ring semimetals

An electron beam may experience an anomalous spatial shift during an interface scattering process. Here, we investigate this phenomenon for reflection from mirror-symmetry-protected nodal-ring semimetals, which are characterized by an integer topological charge $\chi_h$. We show that the shift is generally enhanced by the presence of nodal rings, and the ring's geometry can be inferred from the profile of shift vectors in the interface momentum plane. Importantly, the anomalous shift encodes the topological information of the ring, where the circulation of the shift vector field $\kappa_s$ over a semicircle is governed by the topological charge, with a simple relationship: $\kappa_s=-2\pi \chi_h$. Furthermore, we demonstrate that the shift and its circulation reflect distinct features of topological phase transitions of the charged rings. This study uncovers a novel physical signature of topological nodal rings and positions anomalous scattering shifts as a powerful tool for probing topological band structures.

cond-mat.mtrl-sci

Electric-Field Control of Terahertz Response via Spin-Corner-Layer Coupling in Altermagnetic Bilayers

Electric field control of electron charge and spin degrees of freedom is fundamental to modern semiconductor and spintronic devices. Yet controlling electromagnetic waves with an electric field, particularly in the terahertz (THz) band, remains a challenge. Here, we propose a spin-corner-layer coupling (SCLC) mechanism in second-order topological altermagnetic bilayers. By using an electric field to influence electrons between different layers, the SCLC mechanism enables simultaneous control over corner and spin degrees of freedom, thereby allowing electric-field tuning of the absorption, emission intensity, and even polarization of THz waves. Taking bilayer NiZrI$_6$ nanodisks as a prototype, we demonstrate that an ultralow electrostatic field can switch both the spin and the layer polarizations of corner states. This dual switching modulates transition dipole moments and oscillator strengths between different corner states, thereby enabling the manipulation of THz waves. This study establishes a mechanism for the electric-field control of spin and THz waves through SCLC, yielding important implications for the advancement of THz spintronics.

cond-mat.mtrl-sci

Type-II Antiferroelectricity

Antiferroelectricity (AFE) is a fundamental concept in physics and materials science. Conventional AFEs have the picture of alternating local electric dipoles defined in real space. Here, we discover a new class of AFEs, termed type-II AFEs, which possess opposite polarizations defined in momentum space across a pair of symmetry decoupled subspaces. Unlike conventional AFEs, the order parameter of type-II AFEs is rigorously formulated through Berry-phase theory and can be quantitatively extracted from the electronic band structure. Focusing on a subclass of type-II AFEs that preserve spin-rotation symmetry, we establish the relevant symmetry constraints and identify all compatible spin point groups. Remarkably, we find that type-II AFE order intrinsically coexists with antiferromagnetism, revealing a robust form of magnetoelectric coupling. We construct an altermagnetic model and identify several concrete antiferromagnetic/altermagnetic materials, such as FeS, Cr2O3, MgMnO3, monolayer MoICl2 and bilayer CrI3, that exhibit this novel ordering. Furthermore, we uncover unique physical phenomena associated with type-II spin-AFE systems, including spin current generation upon AFE switching and localized spin polarization at boundaries and domain walls. Our findings reveal a previously hidden class of quantum materials with intertwined ferroic orders, offering exciting opportunities for both fundamental exploration and technological applications.

cond-mat.mtrl-sci