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Zhibin Shao

Publications and source records attributed to Zhibin Shao.

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Nonmagnetic ground state of marcasite FeTe$_{2}$: The competition between crystal field splitting and on-site Coulomb repulsion

The magnetic ground states in crystalline systems are significant for both fundamental condensed matter physics and practical materials engineering. Marcasite FeTe$_{2}$, characterized as a small-gap semiconductor, exhibits anomalous magnetic behaviors in low-temperature experiments. In this study, first-principles density functional theory calculations combined with scanning tunneling microscopy/spectroscopy are employed to investigate the magnetic ground state of marcasite FeTe$_{2}$. It is revealed that the competition between crystal field splitting and on-site Coulomb repulsion plays the key role in the formation of localized magnetic moments in FeTe$_{2}$. The ground state of FeTe$_{2}$ bulk is confirmed to be nonmagnetic, while the magnetic responses of FeTe$_{2}$ observed at low temperature are suggested to be related to the magnetic Fe atoms on the crystal surfaces. Our work proposes a straightforward competing mechanism for determining ground-state magnetism of various localized-moment crystalline systems.

cond-mat.str-el

Discrete scale invariance of the quasi-bound states at atomic vacancies in a topological material

Recently, log-periodic quantum oscillations have been detected in topological materials zirconium pentatelluride (ZrTe5) and hafnium pentatelluride (HfTe5), displaying intriguing discrete scale invariance (DSI) characteristic. In condensed materials, the DSI is considered to be related to the quasi-bound states formed by massless Dirac fermions with strong Coulomb attraction, offering a feasible platform to study the long-pursued atomic-collapse phenomenon. Here, we demonstrate that a variety of atomic vacancies in the topological material HfTe5 can host the geometric quasi-bound states with DSI feature, resembling the artificial supercritical atom collapse. The density of states of these quasi-bound states are enhanced and the quasi-bound states are spatially distributed in the "orbitals" surrounding the vacancy sites, which are detected and visualized by low-temperature scanning tunneling microscope/spectroscopy (STM/S). By applying the perpendicular magnetic fields, the quasi-bound states at lower energies become wider and eventually invisible, meanwhile the energies of quasi-bound states move gradually towards the Fermi energy (EF). These features are consistent with the theoretical prediction of a magnetic-field-induced transition from supercritical to subcritical states. The direct observation of geometric quasi-bound states sheds light on the deep understanding of the DSI in quantum materials.

cond-mat.mtrl-sci

Surface Superconductivity in the type II Weyl Semimetal TaIrTe4

The search for unconventional superconductivity in Weyl semimetal materials is currently an exciting pursuit, since such superconducting phases could potentially be topologically nontrivial and host exotic Majorana modes. The layered material TaIrTe4 is a newly predicted time-reversal invariant type II Weyl semimetal with minimum number of Weyl points. Here, we report the discovery of surface superconductivity in Weyl semimetal TaIrTe4. Our scanning tunneling microscopy/spectroscopy (STM/S) visualizes Fermi arc surface states of TaIrTe4 that are consistent with the previous angle-resolved photoemission spectroscopy (ARPES) results. By a systematic study based on STS at ultralow temperature, we observe uniform superconducting gaps on the sample surface. The superconductivity is further confirmed by electrical transport measurements at ultralow temperature, with an onset transition temperature (Tc) up to 1.54 K being observed. The normalized upper critical field h*(T/Tc) behavior and the stability of the superconductivity against the ferromagnet indicate that the discovered superconductivity is unconventional with the p-wave pairing. The systematic STS, thickness and angular dependent transport measurements reveal that the detected superconductivity is quasi-one-dimensional (quasi-1D) and occurs in the surface states. The discovery of the surface superconductivity in TaIrTe4 provides a new novel platform to explore topological superconductivity and Majorana modes.

cond-mat.supr-con

Eightfold Fermionic Excitation in a Charge Density Wave Compound

Unconventional quasiparticle excitations in condensed matter systems have become one of the most important research frontiers. Beyond two- and fourfold degenerate Weyl and Dirac fermions, three-, six- and eightfold symmetry protected degeneracies have been predicted however remain challenging to realize in solid state materials. Here, charge density wave compound TaTe4 is proposed to hold eightfold fermionic excitation and Dirac point in energy bands. High quality TaTe4 single crystals are prepared, where the charge density wave is revealed by directly imaging the atomic structure and a pseudogap of about 45 meV on the surface. Shubnikov de-Haas oscillations of TaTe4 are consistent with band structure calculation. Scanning tunneling microscopy reveals atomic step edge states on the surface of TaTe4. This work uncovers that charge density wave is able to induce new topological phases and sheds new light on the novel excitations in condensed matter materials.

cond-mat.mtrl-sci

Scanning tunneling microscopic evidence of interface enhanced high-Tc superconductivity in Pb islands grown on SrTiO3

The discovery of the interface enhanced superconductivity in the single layer film of FeSe epitaxially grown on SrTiO3 substrates has triggered a flurry of activity in the field of superconductivity. It raised the hope to find more conventional high-Tc superconductors which are purely driven by the electron-phonon interaction at ambient pressure. Here we report the experimental evidence from the measurement of scanning tunneling spectroscopy for the interface enhanced high-Tc superconductivity in the Pb thin film islands grown on SrTiO3 substrates. The superconducting energy gap of the Pb film is found to depend on both the thickness and the volume of the islands. The largest superconducting energy gap is found to be about 10 meV, which is 7 times larger than that in the bulk Pb. The corresponding superconducting transition temperature, estimated by fitting the temperature dependence of the gap values using the BCS formula, is found to be 47 K, again 7 times higher than that of the bulk Pb.

cond-mat.supr-con