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Zhibin Su

Publications and source records attributed to Zhibin Su.

3 recordsLinked to original sources

Discovery of d-orbital order in Tb2CoAl4Ge2

Orbital order describes a quantum state where occupied orbitals line up in a periodic pattern. While orbital physics plays a fundamental and universal role in strongly correlated electron systems, the existence and particularly the band structure fingerprint of orbital order remain a long-standing mystery. Here, we report the discovery of rare earth 5d-orbital order developed by the surface states of intermetallic compound Tb2CoAl4Ge2. Angle-resolved photoemission spectroscopy reveals characteristic nematic features like Fermi surface deformation and band split. These experimental observations can be described by a ferro-orbital order term in the mean-field Hamiltonian. The structural and magnetic origin of such order is excluded by systematic high-resolution neutron powder diffraction and scanning tunnelling microscopy measurements. Our results provide strong evidence for a pure surface orbital order scenario avoiding complications from structural distortion as in colossal magnetoresistance manganites, magnetic order as in iron-based superconductors, and charge transfer p-orbital order in cuprates.

cond-mat.str-el

Dimensionality-Dependent Exciton Dispersion in a Single-Band Mott Insulator

Excitonic band structure is critical for investigating exciton dynamics. Theoretically, quantum effects from exchange scattering between electron-hole pairs significantly modulate exciton dispersion. Here, we report the direct observation of dimensionality-dependent exciton dispersion in a single-band Mott insulator Nb3Cl8 through high-resolution electron energy loss spectroscopy. In the high-temperature phase, the exciton in Nb3Cl8 hosts an exceptionally large binding energy, and exhibits clear quasi-two-dimensional massless linear dispersion. In contrast, in the low-temperature phase, the exciton splits into two bands, both displaying three-dimensional parabolic dispersion. These dramatic changes in the exciton dispersion stem from the dimensional mutation driven by a substantial enhancement of interlayer coupling across the phase transition. This Letter provides a clear and typical example of how exciton behavior evolves with dimensionality.

cond-mat.str-el

Observation of Topological Nodal-Ring Phonons in Monolayer Hexagonal Boron Nitride

Topological physics has evolved from its initial focus on fermionic systems to the exploration of bosonic systems, particularly phononic excitations in crystalline materials. Two-dimensional (2D) topological phonons emerge as promising candidates for future technological applications. Currently, experimental verification of 2D topological phonons has remained exclusively limited to graphene, a constraint that hinders their applications in phononic devices. Here, we report experimental evidence of topological phonons in monolayer hexagonal boron nitride using advanced high-resolution electron energy loss spectroscopy. Our high-precision measurements explicitly demonstrate two topological nodal rings in monolayer hexagonal boron nitride, protected by mirror symmetry, expanding the paradigm of 2D topological phonons beyond graphene. This research not only deepens fundamental understanding of 2D topological phonons, but also establishes a phononic device platform based on wide-bandgap insulators, crucial for advancements in electronics and photonics applications.

cond-mat.mtrl-sci